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Simone Herberger
Heiko Ulmer
AppliedSensor GmbH, Reutlingen,
Germany
Research Article
Indoor Air Quality Monitoring Improving AirQuality Perception
Energy-efficient ventilation strategies relating to good indoor air quality (IAQ) are a
major task for building performance according to the requirements set by the energy
performance of buildings directive (EPBD) in 2010. Applying demand-controlled venti-
lation (DCV) in buildings, using sensors for IAQ control that enables variable airflow
rates adapted to the actual indoor load conditions is one possibility to fulfill the
requirements of adequate IAQ while reducing the energy consumption at the same
time. CO2 concentrations above outdoors are generally used as an indicator for occu-
pancy generated indoor air pollution and corresponding ventilation rates. The objec-
tive of this study is focused on a micromachined metal oxide semiconductor gas sensor
module developed for IAQ control, based on volatile organic compound (VOC) detec-
tion. The sensor output was correlated with measured CO2 concentrations and quan-
tified VOCs in 15 field scenarios. Energy demand and IAQ, applying the sensor module
for DCV in an office, were compared to natural and time-scheduled ventilation in
the office. The study accentuates the need for DCV and proves the functionality of the
sensor module for IAQ control at adequate comfort levels. Compared to time-scheduled
ventilation, 15% heating energy and 70% power consumption were saved with DCV.
Keywords: Demand-controlled ventilation; Metal oxide semiconductor gas sensor;Microelectromechanical-system; Volatile organic compound
Received: July 15, 2010; revised: July 28, 2011; accepted: December 9, 2011
DOI: 10.1002/clen.201000286
1 Introduction
More than 40% of primary energy in Europe and the US is consumed
in buildings, whereof ventilation accounts for 10% [1]. In order to
promote energy-efficient buildings and reduce CO2 emission, the
European Parliament adopted the energy performance of buildings
directive (EPBD) in 2010 and the EU Member States were requested to
set up minimum requirements on the energy performance of new
and renovated buildings [2, 3]. More strict regulations on the air
tightness of buildings led to an increased role of ventilation com-
pared to other elements of the heat balance of a building. However,
sufficient ventilation in today’s airtight buildings is necessary to
remove or reduce indoor generated pollutants and humidity to
acceptable health and comfort levels and to maintain building
integrity.
Ventilation rates <0.5 air changes/h are considered as health risk
in residential buildings [4]. Not only health problems (e.g., asthma or
allergies) but also comfort complaints and a loss in productivity are
attributed to bad indoor air quality (IAQ) due to inadequate venti-
lation [5, 6]. Field experiments showed that measures to improve IAQ
are cost-effective, considering potential benefits of reduced sick
leave, reduced medical costs, and better performance at work gained
at improved IAQ [7]. However, the optimum ventilation rates with
respect to health and comfort aspects are still under discussion and
up till now only few guidelines on IAQ exist in the EU [8, 9].
Energy-efficient ventilation strategies providing adequate IAQ
became a major task for building performance in the recent past
[1]. Applying demand-controlled ventilation (DCV) in buildings, using
sensors for IAQ control that enables variable airflow rates adapted to
the actual load conditions in buildings, is one possibility to fulfill the
requirements of adequate IAQ while reducing the energy consump-
tion at the same time [1, 10]. State-of-the-art is to operate heating,
ventilation, and air conditioning (HVAC) systems on the basis of fixed
duty cycles (time-scheduled) or to apply ventilation on demand based
on CO2 concentrations above outdoors, used as an indicator for IAQ
related to humans and their bio-effluents [11, 12]. CO2 quantification
is thereby mainly realized by optical absorption techniques (non-
dispersive IR (NDIR) sensors) [11, 12]. Ventilation standards and guide-
lines supporting the EPBD, e.g., EN 15251 [13] and CR 1752 [14] as well
as American ASHRAE Standard 62.1-2 (2007) [15] specify ventilation
rates for different IAQ categories commonly based on CO2 concen-
trations above outdoors that can be related to the percentage of
people dissatisfied with the IAQ [14]. Building material emissions
are considered as a constant background level, requiring a minimum
basic ventilation rate and are not decisive for DCV [13].
Even though high CO2 levels were correlated with comfort com-
plaints and a loss in productivity [16], the odorless CO2 does not
Correspondence: S. Herberger, AppliedSensor GmbH, Gerhard-Kindler-Str. 8, D-72770 Reutlingen, GermanyE-mail: [email protected]
Abbreviations: AQL, air quality level; DCV, demand-controlledventilation; EPBD, energy performance of buildings directive; IAQ,indoor air quality; MEMS, microelectromechanical system; MOS, metaloxide semiconductor; NDIR, non-dispersive IR; PCB, printed circuitboard; PT-GC/MS, purge and trap GC/MS; VOC, volatile organic compound
Clean – Soil, Air, Water 2012, 00 (0), 1–8 1
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affect the perception of IAQ directly. DCV based on volatile organic
compound (VOC) detection goes beyond this approach. As metabolic
products, VOCs are present in the human breath and bio-effluents
but also in cooking odors, outdoor pollutants, cleaning supplies, etc.
Ethanol, acetone, isoprene, limonene, decanal, nonanal, a-pinene,
and eucalyptol are statistically confirmed to correlate with occu-
pancy and human activities and therefore rather contribute to the
IAQ perception than CO2 [17, 18].
Metal oxide semiconductor (MOS) gas sensors are suitable sensors
for the detection of VOCs. In the recent past, our work was focused on
the development of a microelectromechanical system (MEMS) MOS
gas sensor module for IAQ monitoring [19]. Implementation of an
empirical algorithm for the prediction of indoor CO2 concentrations
based on the VOC sum concentration as detected by the MOS
gas sensor allows signal-adherence to established ventilation stand-
ards using CO2 as indicator for DCV.
The objective of this study focuses on the reliability of the devel-
oped MOS gas sensor module for IAQ monitoring in different real-life
scenarios (differing in location, number of people, fluctuation
degree, conditioning rates, etc.) and the energy saving potential
applying the sensor module for DCV in an office. Correlations of
the MOS gas sensor output with measured CO2 concentrations and
quantified VOCs were investigated for seven field scenarios where
people are considered to be the main pollution source (meeting
rooms, office, and schools) as well as for eight field scenarios where
human activities are dominating (e.g., kitchens), as listed in Tab. 1.
Energy demand and IAQ for natural, time-scheduled and DCV in the
office were compared.
2 Experimental
2.1 Sensor module
The sensor module used in this study is shown in Fig. 1. The sensing
elements developed for the detection of VOCs are MEMS palladium
doped SnO2 thick film sensors, highly sensitive to ethanol and
acetone [19]. The sensor components are glued directly on the
printed circuit board (PCB) with integrated electronics and housed
in a plastic case covered with a membrane for gas exchange.
2.2 Evaluation algorithm
The predicted CO2 concentration, in the range from 450 to
2000 ppm, is used in this study to evaluate the sensor output. The
empirical evaluation algorithm is transferred to the microcontroller
on the PCB. The raw signal of the MOS gas sensor, the resistance R (V),
Table 1. List of field scenarios
Fieldscenario
Topic Vroom
(m3)Period
(h)Attendees Sampling/sensor
positionsRemarks
1 Meeting 40 1.5 Eight grown-ups, mixedage, and sex
Corner of theroom on table
One window tilted,coffee, and cake
2 Meeting 29 0.5 Six to nine grown-ups,mixed age, and sex
Corner of theroom on table
Coffee and cake
3 Meeting 240 3 Thirty-two grown-ups,mixed age, and sex
Corner of theroom on table
Temporarily open door
4 Meeting 473 2 Seventy grown-ups, mixedage, and sex
Corner of theroom on table
Windows tilted
5 Office 24 2.5 One to three grown-ups,mixed age, and sex
Next to entranceon table
Door open
6 Office 71 4.5 One to five grown-ups,mixed age, and sex
Corner of theroom on table
–
7 School 100 1.5 Thirty-nine teenagers, onegrown-up, mixed sex
Corner of theroom on table
–
8 Gym 1719 4.5 Seventeen to 21 kids andgrown-ups, mixed sex
Corner of gym ontable
–
9 Restroom 31 5 Ten at all, men, mixed age On table inrestroom area
Vestibule next torestroom area,
connecting door open10 Restroom 31 2.5 Ten at all, men, mixed age Vestibule next to
restroom area ontable
Ventilation on,vestibule next torestroom area,
connecting door open11 Restroom 22 2.5 Fourteen at all, women,
mixed ageVestibule next torestroom area on
table
Vestibule next torestroom area,
connecting door open12 Kitchen 54 3 One to seven grown-ups,
mixed age, and sexNext to door
frame kitchen/lunch area
Kitchen and lunch areaseparated
13 Kitchen 72 2 Ten to 20 grown-ups,mixed age, and sex
Sensor aboveexhaust hood,
sampling next tocooker
Tilted windows
14 Kitchen 77 4.5 Two to eleven grown-ups,mixed age, and sex
Middle of theroom on table
Door to connectingroom open
15 Cafeteria 240 1.5 One to five grown-ups,mixed age, and sex
Next to cookingactivities
Two windows tilted
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that is changed due to chemical catalytic reactions of the gas atmos-
phere with the thick film sensor surface, is transformed into con-
ductivity G (mS) followed by the calculation of a new corrected sensor
baseline. The predicted sensor signal in CO2 equivalent units (ppm) is
calculated based on a certain CO2 outdoor concentration in the
range from 350 to 450 ppm indicating good IAQ, i.e., a ventilated
state of the room as well as based on empirical factors. The predicted
sensor signal can be linked to specific air quality levels
(AQLs) according to definite threshold limits for indoor CO2 pollu-
tion. A detailed flow chart explaining data processing can be found
in [19].
2.3 Complementary analytics and
reference sensors
2.3.1 Purge and trap GC/MS
Purge and trap GC/MS (PT-GC/MS) and GC-olfactometry (GC-O) serves
to elucidate the efficiency of monitoring the IAQ with the MOS gas
sensor module in accordance with quantifiable VOCs and odorous
compounds during the field scenarios.
Air sampling has been carried out sequentially (every 20 or 30 min)
during the field scenarios, starting with the room in an empty,
ventilated state for definition of the background VOC profile in
the room (blank value). The blank value includes the sum of all
quantified VOCs released by building materials and furniture.
Sampling, identification, and quantification of VOCs were per-
formed according to the harmonized European standard DIN ISO
16000-6:2004 [20]. Compounds sampled by TENAX-TA1 with lower
retention times than hexane were also included in this study (very
volatile organic compounds, VVOCs). In order to determine VOC
profiles significant for occupancy and human activities, VOCs quan-
tified by the first air sample (blank value attributed to building
material and furniture emissions), were subtracted from VOCs quan-
tified by successive air samples. Identification of odorous compounds
was performed by GC-O. Intensity of the odorous compounds has
been rated by a 3-level intensity scale (weak, significant, and strong).
Detailed information on sampling parameters and instrumentation
can be taken from [18, 21].
2.3.2 Reference sensors
Temperature and relative humidity (r.h.) during the field scenarios
have been monitored using an EL-USB-2 rh/temp data logger manu-
factured by Lascar Electronics Ltd. (www.lascarelectronics.com) [22].
The AMUN 716-USB one channel NDIR CO2 sensor purchased from
Theben (www.theben.de) served to quantify the CO2 concentration
during the field scenarios to evaluate the effectiveness and reliability
of the implemented empirical algorithm for CO2 prediction.
2.4 Field scenarios
In Tab. 1, the field scenarios are listed. Field scenarios #1–7 are
attributed to occupancy, differing in number of attendees, location,
ventilation rate, etc. PT-GC/MS was used for VOC quantification. Field
scenarios #8–15 deal with typical human activities where the IAQ is
mainly affected by odorous compounds. Odorous compounds have
been identified by GC-O. In Fig. 2, an experimental setup comprising
all instrumentation is shown exemplarily. In [18], detailed infor-
mation on sensor position, course of events, etc., can be found.
2.5 Energy demand and IAQ in an office controlled
with the MOS gas sensor module
The energy saving potential and IAQ conditions applying the devel-
oped MOS gas sensor module for DCV was investigated in a 80-m3 test
office located in the ‘‘Versuchsgebaude fur energetische und raum-
klimatische Untersuchungen’’ (VERU) at the Fraunhofer-Institute for
Building Physics in Holzkirchen, Germany, in comparison to natural
and time-scheduled ventilation. The building is equipped with a
computer controlled centralized supply and exhaust air ventilation
system. No temperature or humidity control of the supply air has
been adjusted for the case study. The 0–5 V analog output of the
developed MOS gas sensor module has been connected to the venti-
lation system of the building for DCV. Ventilation rate for time-
scheduled ventilation has been set according to the requirements of
EN 15251 [13]. Four manually operated windows (each 1.5 m2) located
Figure 1. Sensor module – PCB equipped with MEMS MOS gas sensorand plastic housing.
Figure 2. Experimental setup – restroom.
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at the east facade of the building served for natural ventilation of the
office. Details on the ventilation strategies can be found in Tab. 2.
Each ventilation strategy was carried out for 1 wk, reiterating (test
period Dec 2009–April 2010). One to two people for 8 h/day and
5 days/wk, one weekly 1 h meeting with six to eight people and
one artificial event on Friday afternoon (evaporation of 5 mL ethanol
in a Petri dish) represented the normal pollution load in the office.
Attendees had to keep logbook on occupancy and special events,
e.g., window opening. Sensor data, ventilation system parameters
and energy consumption in the office have been logged during the
whole test period. CO2 concentrations have been measured for
comparison.
3 Results and discussion
3.1 VOC versus CO2 approach – occupancy
related field scenarios
Reliable correlations of predicted and measured CO2 concentrations
were obtained for the occupancy related field scenarios.
Quantification of VOCs showed that the best signal accordance is
reached when ethanol and/or acetone concentrations are dominat-
ing isoprene concentration in the course of the respective field
scenario.
In Fig. 3, one representative result as obtained for the occupancy
related field scenarios shows the nice correlation of the sensor
output with measured CO2 concentration in accordance with quan-
tified acetone, ethanol, and isoprene. Significant activities during
the field scenario #4 (see Tab. 1) are plotted in the lower graph.
Large deviations of predicted and measured CO2 concentrations
for the occupancy related field scenarios were found for field
scenario no. 6 in an office (see Fig. 4 and Tab. 1). PT-GC/MS analysis
pointed out isoprene to be the dominating quantified VOC. In the
course of this field scenario ethanol did not increase steadily but
resulted in a steady state concentration as indicated by the GC/MS
results. The MOS gas sensor that is the most sensitive to ethanol
therefore shows a lower predicted CO2 concentration compared to
the measured CO2 concentration.
Slight deviations of measured and predicted CO2 concentrations
detected during the occupancy related field scenarios can be inter-
preted by the metabolic VOC profile differing depending on age,
health, and gender of the test people. In the mornings, human
VOC emission seems to be lower than corresponding CO2 pro-
duction, whereas in the afternoon, metabolic VOC production
seems to be higher resulting in even slightly over-predicted CO2
concentrations.
The concentration course of quantified VOCs (ethanol, acetone,
isoprene, limonene, decanal, nonanal, a-pinene, and eucalyptol),
considered to be significant for occupancy, as well as the estimated
VOC sum content have been found to correlate with the MOS gas
sensor output and CO2 concentration characteristics for all occu-
pancy related field tests.
Table 2. Ventilation strategies
Ventilation strategy Description
Natural ventilation Window opening is up to people working in the office. According to occupancy logbook, peopleventilated the office once or twice a day by manually opening one of the four windows for around5 min
Time-scheduled constantventilation
Ventilation according to EN 15251 (assuming required IAQ level II in the office, low pollutingmaterials, and two attendees), 125 m3/h for working hours (Monday to Friday 8 a.m. to 6 p.m.), 6 m3/hotherwise (5% of the total ventilation rate)
Demand-controlled ventilation,MOS gas sensor module
MOS gas sensor output 0–5 V corresponding to 450–2000 ppm CO2 equivalents serves to triggerventilation rate in linear scale from 6 to 125 m3/h
Figure 3. Field scenario #4, meeting room.Seventy grown-ups, differing in age and sex,some with coffee cups, Vroom¼473 m3, win-dows tilted, a total of six air samples, first airsample in empty, ventilated room. Correlationof predicted MOS gas sensor signal with themeasured CO2 concentration (lower graph)and the concentration course of ethanol, ace-tone, isoprene, and sum VOC content (uppergraph).
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3.2 VOC versus CO2 approach – activity related
field scenarios
In Fig. 5, one representative result as obtained for activity related
field scenarios is presented by means of a cooking event (field
scenario #13, see Tab. 1). Occupancy is dominated by activities
and VOCs and odorous compounds that affect perceived air quality
are produced in great quantities. The correlation of the predicted
sensor signal and the concentration course of ethanol, acetone, and
isoprene can be taken from Fig. 5. Concentration course of ethanol
and acetone is in accordance with the intensity course of odorous
compounds (sulfur organic compounds, acids, ketones, roasting
flavors, etc.), determined by GC-O, and indicates times during
the field scenario when unique activities took place and quantifiable
VOCs and odorous compounds have been produced (see Fig. 6). The
NDIR reference sensor used for CO2 quantification however does not
detect odorous events and the measured CO2 concentration can be
only linked to the occupancy in the kitchen.
For activity related field scenarios, isoprene, a-pinene, nonanal,
and decanal have been found to correlate with occupancy and there-
fore the CO2 concentration characteristics whereas ethanol and
acetone attributed to unique activities in accordance with the inten-
sity course of odorous compounds correlate with the MOS gas sensor
signal.
The value of IAQ control with sensors became obvious by the field
scenarios. A big advantage compared to offline analytical methods is
the fast response and real-time capability of the MOS gas sensor
module for IAQ monitoring. The sensor module offers the function-
ality to detect in real-time unique VOC activities related to cooking
activities (see Fig. 5), cleaning processes, etc., in the background of
the predicted CO2 concentration and therefore provides additional
information on the IAQ than sole CO2 quantification. Faster response
times for the MOS gas sensor module than for the NDIR sensor were
detected.
Indoor air quality control with sensors may prevent human adap-
tion to indoor air pollution. However, VOC emissions from building
Figure 4. Field scenario #6, office. One to fivegrown-ups, differing in age and sex, some withcoffee cups, Vroom¼ 71 m3, a total of ten air sam-ples, first air sample in empty, ventilated room.Correlation of predicted MOS gas sensor signalwith the measured CO2 concentration (lowergraph) and the concentration course of ethanol,acetone, isoprene, and sum VOC content (uppergraph).
Figure 5. Field scenario #13, kitchen. Ten to20 grown-ups, differing in age and sex,Vroom¼72 m3, a total of six air samples, first airsample in empty, ventilated room. MOS gas sen-sor signal and measured CO2 concentration(lower graph). Correlation of MOS gas sensorsignal with the concentration course of ethanol,acetone, and isoprene as well as sum VOC con-tent (upper graph).
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materials and furniture that accumulate over time cannot be
detected by the MOS gas sensor module due to their slow steady
rise characteristics in indoor air.
Contrary to the occupancy related events, sum VOC content of the
activity related events is not in accordance with the concentration
course of the quantified VOCs. Sum VOC course seems to correlate
with occupancy, isoprene, a-pinene, nonanal, and decanal as well as
the CO2 concentration course whereas the MOS gas sensor signal is in
accordance with the intensity course of odorous compounds indi-
cating unique activities and therefore better correlates to the air
quality perception.
3.3 Implementation of the MOS gas sensor module
for DCV in an office
In Fig. 7, the predicted CO2 concentration from the detected VOC
level in the office is shown exemplarily for 1 wk within the test
period in comparison to the measured CO2 concentration. The pre-
dicted and measured CO2 concentrations are almost consistent and
with both sensing technologies, human presence in the office at
daytime can be clearly distinguished by their absence at nighttime.
Unique VOC events can be additionally detected by the MOS gas
sensor module.
Demand-controlled ventilation, using the MOS gas sensor module
for IAQ control and trigger for the supply air rate in linear scale
(from 6 to 125 m3/h) in comparison to time-scheduled ventilation
(125 m3/h for 10 h/day, 6 m3/h otherwise) is shown in the right hand
graph of Fig. 7. Occupancy times of the office are also plotted in the
right hand graph for the demonstrated DCV week. Compared to
time-scheduled ventilation, 60% less supply air rate was delivered
to the office for DCV for the whole test period. For time-scheduled
ventilation, air flow rates, and time schedules have to be adjusted in
the run-up to the operation, depending on the average grade of
occupancy or activity in the room. However, an overlap between
occupancy of the room and operation time of the ventilation system
is not always guaranteed as indicated by the right hand graph of
Fig. 7. In general, as indicated by the IAQ sensors, there is still a
pollution load in the room after the attendees have already left the
Figure 6. Concentration course of quantifiedVOCs and sum VOC content as well as intensitycourse of odorous compounds for field scenario#13.
Figure 7. Left hand side: One week sensor data in the office. The predicted and measured CO2 concentrations are almost consistent but VOC relatedactivities can only be detected by the MOS gas sensor module. Right hand side: Supply air rate (m3/h) using the MOS gas sensor signal for DCV, comparedto time-scheduled ventilation and occupancy of the office.
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office that still requires higher ventilation rates than the reduced
ventilation rate (6 m3/h) adjusted by the time-scheduled system.
Sensor based IAQ control ensures that fresh air is supplied to the
room whenever necessary, reducing energy consumption compared
to time-scheduled ventilation (see Fig. 7). DCV strategy clearly out-
matched the time-scheduled ventilation when looking at time-
resolved results in cases where the room occupancy did not match
the design occupancy of two people.
The overall energy consumption in the office was calculated based
on the individual measured power consuming parameters, such as
lighting, office equipment, heating energy, and fan. For each venti-
lation strategy (see Tab. 2), an average determination of the
measured power consuming parameters was conducted for a period
of 3 wk that resulted in an overall energy consumption for the
individual ventilation strategies as shown in the left hand graph
of Fig. 8. Lighting energy and power consumption of the office
equipment was considered independent of the respective ventilation
strategy. The average heating energy consumption is lowest for
natural ventilation. However, the achieved IAQ is rather poor. CO2
concentrations up to 1300 ppm for normal load condition corre-
sponding to IAQ level III, according to EN 15251, were obtained
for natural ventilation (Fig. 8, right hand graph) and can be
explained by human adaption that prevents bad air quality percep-
tion and people to ventilate the office. According to the occupancy
logbook, the office was only ventilated once or twice per day. DCV
saved �15% heating energy and resulted in �70% less power con-
sumption of the fan compared to time-scheduled ventilation. The
IAQ (IAQ level II according to EN 15251) was in overall not as good as
for time-controlled ventilation (lowest indoor CO2 concentrations,
IAQ level I according to EN15251) but still at an acceptable level (see
Fig. 8, right hand side). Moreover, there is still space for improve-
ments of the DCV strategy, e.g., adaptation of the linear scale used to
control the airflow in this study.
4 Concluding remarks
The field scenarios showed that the developed sensor module is well
applicable for real-time IAQ control in locations, where human
activities and therefore VOCs are dominating (kitchens, restrooms,
etc.) as well as in locations where occupancy and therefore CO2 is
dominating (offices, schools, etc.). The approach of the developed
MOS gas sensor module goes beyond CO2 quantification and offers
better correlation to IAQ perception by VOC detection. The combi-
nation of the developed MOS gas sensor element that is highly
sensitive to ethanol and acetone and the implementation of an
empirical algorithm for CO2 prediction based on a sum VOC detec-
tion allows a reliable correlation of predicted and measured CO2
concentrations and additional detection of point source VOCs,
emitted by cleaning agents, chemical, etc., in the background of
the predicted CO2 concentration.
This study also accentuates the need for DCV regarding actual load
conditions using sensor technologies and shows the energy saving
potential of the developed MOS gas sensor module. DCV prevents
human adaption compared to natural ventilation and reduces the
energy if compared to time-scheduled ventilation. Nevertheless, VOC
emissions from building materials and furniture that accumulate
over time are not detected by the developed sensor module due to
their slow steady rise characteristics in indoor air and a basic venti-
lation rate has therefore to be adjusted for unoccupied rooms. In
order to overcome the lack of selectivity and sensitivity of the
developed sensor module for individual indoor gases, pattern recog-
nition is currently under investigation.
Acknowledgments
A. Burdack-Freitag, R. Rampf, and F. Mayer from the Fraunhofer-
Institut fur Bauphysik (IBP), Valley/Oberlaindern, Germany, are
gratefully acknowledged for their support.
The authors have declared no conflict of interest.
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Clean – Soil, Air, Water 2012, 00 (0), 1–8 Indoor Air Quality Monitoring 7
� 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim www.clean-journal.com
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