30
Opto-Electronics & Materials L Opto-Electronics & Materials L aboratory aboratory Li-Jen Chou ( 周周周 ) 周周周周周周周周 周周周 周周周 周周周周周周周周周 :、、 Investigations on low-dimensional nano structures: synthesis, characterization, applications and fundamental mechanism s Department of Materials Science and Eng ineering National Tsing Hua University, Hsinchu, Taiwan

Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Embed Size (px)

Citation preview

Page 1: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Li-Jen Chou ( 周立人 )

低維奈米結構研究:合成、鑑定、應用與基本成長機制

( Investigations on low-dimensional nanostructures: synthesis, characterization, applications and f

undamental mechanisms )

Department of Materials Science and EngineeringNational Tsing Hua University, Hsinchu, Taiwan

Page 2: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Team Members

– 各教師成長不同奈米結構材料

– 陳力俊 : 超高真空穿透式電子顯微鏡觀測– 果尚志 : 多重尺度及階層式的組裝及量測– 呂世源 : 表面功能化處理– 周立人 : 場發射穿透式電子顯微鏡觀測– 徐文光 : 機械性質量測– 嚴大任 : 電子束微影與微光學量測

Page 3: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

96年執行情形

Publication 陳力俊、果尚志、呂世源 周立人、徐文光、嚴大任s: Impact No. (No. Papers)PI 1: ~10 (3), ~8 (2), ~6 (1), ~4 (7)PI 2: ~ 4 (13)PI 3: ~ 6 (1), ~5(1), ~4 (2)PI 4: ~10 (2), ~8 (2), ~6 (2), ~4 (2)PI 5: ~ 4 (4)Nano Lett. (~10), Adv. Mater. (~8), Small (~6), Che

m. Mater. (~5), J. Mater. Chem. Appl. Phys. Lett. (~4)

Page 4: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

97年執行情形

Publications: Impact No. (No. Papers)PI 1: ~ 26 (1), ~ 10 (3), ~8 (3), ~4 (2) , > 3.5 (2)PI 2: ~ >7 (2), >5 (2), > 3.5 (7)PI 3: ~ >8 (1), >6 (1), ~5(2), ~4 (2), > 3.5 (3)PI 4: ~ 10 (3), ~4 (2) , ~ 3.5 (1) PI 5: ~ 4 (1), ~ 3.5 (4) PI 6: ~ 8 (1) , ~ 4 (1) Science (~26), Nano Lett. (~10), Adv. Mater. (~8), S

mall (~6), Chem. Mater. (~5), J. Mater. Chem. (~4), Appl. Phys. Lett. (~3.5)

Page 5: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Prof. Z.L. Wang (Gatech, USA)

Profs. K.N. Tu, Y. Hwang (UCLA, USA)

Prof. D. Shindo (Tohoku Univ. Japan)

Prof. S. Isoda (Kyoto Univ. Japan) Profs. M. Aono, Y. Bando, (NIMS, Japan)

國際合作、校外合作、產學合作

Page 6: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Observation of Atomic Diffusion at Twin-modified Grain Boundaries in Copper

Page 7: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

K.C. Chen et al. Science, 321, 1066 (2008).

Page 8: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Page 9: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and
Page 10: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Page 11: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

PSSA Back Cover, May, 2008

Page 12: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

J. Mater. Chem. Invited

Highlight Paper

Page 13: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Y.C. Lin et al. Nano Lett. 8, 913 ( 2008)

Page 14: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

“In-situ TEM observation of repeating events of nucleation in epitaxial growth of nano CoSi2 in nanowires o

f Si,”

Nano Letters 8, 2194 (2008).

Page 15: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

0.0 0.5 1.0 1.5 2.0 2.5 3.0

0

10

20

30

40

50

60

F (

nN)

|L-L0|

(g)(b) (c)

(d) (e) (f)

(a)

0.0 0.3 0.6 0.9 1.2 1.5

0

3

6

9

12

Stre

ss (

MP

a)

Strain (%)

G

L0 L(h)

(µm)

Pcr

3µm

R

L d

Adv. Mater. 20 , 3919 (2008)

”Elastic Properties and Buckling of Silicon Nanowires,”

Page 16: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Formation and Characterization of NixInAs/InAsNanowire Heterostructures

Nano Letters, Vol. 8, No. 12, p 4528 - 4533, (2008).

Page 17: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Nano Letters, Vol. 8, No. 10, p 3288 - 3292, (2008).

Coaxial Metal-Oxide-Semiconductor (MOS)

Au/Ga2O3/GaN for Nitride Based Logic Nano

devices

Page 18: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Coaxial Metal-Oxide-Semiconductor (MOS) Au/Ga2O3/GaN Nanowires

Nano Letters, Vol. 8, No. 10, p 3081 - 3085, (2008).

Page 19: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Tunable Plasmonic Response from Alkanethiolate-Stabilized Gold Nanoparticle Superlattices: Evidence of Near-Field Coupling

J. Am. Chem. Soc. (Communication) 2008, 130, 824−826

自組裝金奈米粒子超晶格 ( 晶格常數可調 ) 群體耦合式電漿光學響應 ( 近場耦合 )

Page 20: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Comparison of Ni-Si and Co-Si systems

Y.C. Chou et al. Nano Lett. 9 (in press, 2009)

Page 21: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

M.P. Lu et al. “Piezoelectric Nanogenerator using p-type ZnO Nanowire Arrays,” Nano Lett. 9, 1223 (2009)

Page 22: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Figure 7.4 (a-c) A sequence of TEM images of the Au-Ga2O3 core-shell nanowires transform into Au-peapodded Ga2O3 nanowires heated at 1000 in the in-situ TEM.℃

In-situ Observation of Complex NanowiresResults and Discussion

Page 23: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Nano-Photonic Switch

Surface Plasmon Resonance (SPR )of Metal Nanoparticles

Nano Letters, Vol. 8, No. 10, p 3288 - 3292, (2008).

Page 24: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

In our case, an electric potential hologram was acquired by the electron holography under the illumination of the green and red lasers.

Procedures

Green Light

Turn on Turn on

Red Light

Experimental Procedures

Page 25: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Figure (a) and (b) are the electron hologram and reconstructed phase imageunder the illumination of 532 nm laser. The phase shift is mostly due to the mean field potential.

(a) (a)(a) (b)

dzzyxcvV

),,(])/(11[

22

Page 26: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

The phase shift image (right figure) due to the LSPR effect (under green light) is deduced.

We assume that these bright spots is due to the excited state of the electrons.

High ElectricPotential Area

Page 27: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

The phase shift due to the excited electrons is not obvious under the illumination of red light,which is consistent with the LSPR theory.

Page 28: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Prelim. Results

Page 29: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

In-situ TEM FE Measurements

Page 30: Opto-Electronics & Materials Laboratory Li-Jen Chou ( ) Investigations on low-dimensional nanostructures: synthesis, characterization, applications and

Opto-Electronics & Materials LaboratoryOpto-Electronics & Materials Laboratory

Thanks For Your Attention