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Challenges for Enhancing Fukushima Environmental Resilience Kaname MIYAHARA, Kimiaki SAITO Fukushima Environmental Safety Center Japan Atomic Energy Agency (JAEA) IAEA Technical Meeting on Remediation Techniques and Strategies in Post-Accident Situations 13-17 June 2016, IAEA Headquarters, Vienna, Austria 1

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Page 1: Challenges for Enhancing Fukushima Environmental Resilience · Remedial Management Options (i) external doses from surfaces contaminated by ... Other measures relevant for individual

Challenges for Enhancing

Fukushima Environmental Resilience

Kaname MIYAHARA, Kimiaki SAITO Fukushima Environmental Safety Center

Japan Atomic Energy Agency (JAEA)IAEA Technical Meeting on Remediation Techniques and Strategies in

Post-Accident Situations

13-17 June 2016, IAEA Headquarters, Vienna, Austria

1

Page 2: Challenges for Enhancing Fukushima Environmental Resilience · Remedial Management Options (i) external doses from surfaces contaminated by ... Other measures relevant for individual

Fukushima Regional Contamination� Initially concern focused on short-

lived iodine and other isotopes in

addition to radiocesium

� evacuation and restriction of

consumption of some foodstuffs

� After decay of short-lived isotopes,

now dominated by 134Cs/137Cs which

is the focus for off-site clean-up

actions

� Cs tends to bind strongly to soil

surface, especially clay

� Exposure doses of inhabitants are

mainly from external exposures,

generally not high, and have

continually reduced by decay of Cs,

washoff / soil mixing2

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Protective Actions

Designation of evacuation areas was

completed just after the accident

(Apr. 22, 2011)Specific Spots

Recommended for

Evacuation

3

Rapidly expanded

(3-km, 10-km, 20-km

radius by Mar. 12)20km

Evacuation Order Areas

� Regulatory limits for

contaminated food and

water based on

�<5 mSv/y (March 20, 2011)

�<1 mSv/y (April 1, 2012)

Category Limit (Bq/kg)

Drinking water 10

Milk 50

General Foods 100

Infant Foods 50

Food and water restrictions

Switched from

distance to a

threshold

radiation dose of

20 mSv/y on Apr.

22

Page 4: Challenges for Enhancing Fukushima Environmental Resilience · Remedial Management Options (i) external doses from surfaces contaminated by ... Other measures relevant for individual

Remedial Management Options

(i) external doses from surfaces contaminated by

deposited radionuclides;

� Currently, the dominant pathway of public

exposure

(ii) ingestion doses from the consumption of

contaminated foodstuffs and drinking water;

�Strict Food Restrictions; Government

restrictions put into place after the Fukushima

Daiichi accident kept most contaminated

foodstuffs off of the market (IAEA, 2011)

(iii) inhalation doses from resuspended material

� This route of exposure is of less significance and

not considered further (UNSCEAR, 2013)

� Decontamination (cleanup)*

� Restrictions on access to highly

contaminated areas (such as the

outer 20 m borders of forests

adjacent to settlements )

� Other measures relevant for

individual lifestyle (e.g. commute

route change) based on the

personal dose data and

understanding Cs behaviors in the

environment

* Dilution methods for soils such as plowing are

included

To reduce external doses

4

Management options are designed to

reduce:

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Decontamination Pilot Project (DPP) by JAEA� JAEA was chosen by the Government to conduct

decontamination pilot projects (DPP) at 16 model sites in

11 municipalities, including evacuation order areas (Sept.

2011~June 2012)

� Main challenges to implement full-scale decontamination

were lack of both real-world examples and also

experience for planning and implementing

decontamination technology appropriate to Japanese

boundary conditions

� Therefore, the decontamination pilot projects played a

key role to support drafting of guidelines and manuals

that can be used by the national government and local

municipalities to optimize regional remediation work

� Check the availability and efficacy of proven and new

techniques

� Investigate cost, work period, workforce, waste

generated, and radiation exposure of workers

� Establish waste management including volume

reduction of wastes and treatment of the secondary

waste

� Secure workers’ safety under radiation protection

� Establish optimal radiation monitoring

� Record the public communication* An examination conducted by a committee appointed by JAEA

Date City

Fukushima

City

Kusano area

Iitate

Village

Planned evacuation area

Soma CityDose rate

classification

Less than 5mSv/y

Kawamata

Town

Nihonmatsu City

Sakashita area

Tsushima area

Katsurao Municipal Office

and surrounding area

Katsurao Village

Tamura City

Miharu

Town

Koriyama

City

Ono Town

Minami Soma City

Restricted Area

Kanabusa Elementary School

and surrounding area

Gongendo areaNamie Town

Futaba Town

Jikenjo area

Kawauchi

Village

Okuma Town

Tomioka Daini Junior High SchoolTomioka Town

Fukushima

Dai-ichi

Yonomori Park

Kamishigeoka area

Naraha Town

Minami Industrial Complex

Hirono Town

Futaba Town has advised us that they would not join the Decontamination

Model Project as a target area.

Kainosaka area

Restricted Area

DeliberateEvacuation Area

Decontamination Pilot Project implementation areas

Ottozawa area

Chuo-dai/Nawashirogae areaIwaki City

Base of “Patrol Team for

the Entire Iitate Village”

Okuma Municipal

Office and

surrounding area

Target Municipalities

5

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Recommended Clean-up Technologies

◎:highly effective, ○:effective, △:moderately effective, ▲:limited effect

Land use classification Comprehensive evaluation

Forest

◎Removal of leaf litter and humus layers (on flat ground and slopes), 〇Removal of leaf litter, humus

layers and topsoil (on flat ground), ▲Trunk washing, 〇Branch trimming in the lower part (evergreen

tree)

Farmland

◎Machine that strips off surface of soils, 〇Backhoe (stripping off depth of 5 cm of the soil),

◎Reversal tillage (by tractor and plough), 〇Ploughing to replace surface soil with subsoil (by

backhoe)

Residential

area

Roof ▲High pressure water, 〇Brushing, 〇Wiping, ▲Apply a remover

Gutter �High pressure water, 〇Wiping

Wall 〇Brushing

Topsoil 〇Removal of topsoil

Rubble 〇Washing of the rubble, 〇Removal of the rubble

Turf 〇Removal of the Turf

Garden tree ▲Clipping a garden tree

Interlocking block �High pressure water

Large

structure

Concrete and Mortar surface�Sanding machine with the dust-collection (Plane which scrapes concrete), 〇Ultrahigh pressure

water (Over 150MPa), 〇High pressure water (10-20MPa), 〇Iron shot blasting

Roof

floor

Concrete surface 〇High pressure water (including brushing)

Waterproof coating surface 〇High pressure water (including brushing)

Downpipe 〇High pressure water(Maximum 50MPa)

Playing field〇Strips off surface of soils (Large mower+Sweeper), 〇Strips off surface of soils (Road planers), 〇

Strips off surface of soils(Motor grader), 〇Ploughing to replace surface soil with subsoil

Swimming pool 〇High pressure water

Turf 〇Turf stripper

Paved road

▲Road cleaners + Riding style road sweepers, �High pressure water (About 15MPa)+Brushing, �Car

of a functional recovery drainage pavement, 〇Ultrahigh pressure water (120~240MPa),○Iron shot

blasting, ○TS Road planers

6http://dx.doi.org/10.11484/jaea-review-2014-051

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Accident Recovery�The Act on Special Measures Concerning the

Handling of Radioactive Pollution (August

2011)

� Special decontamination areas; the Restricted Area + the

Deliberate Evacuation Area

�Further subdivided into three areas (August 2013)

• Area 1: <20 mSv “ready to be lifted”

• Area 2: 20-50 mSv ordered to remain evacuated

• Area 3: >50 mSv not expected to drop below 20 mSv/y

within 5 years

� Intensive contamination survey areas; all other

contaminated areas (1 mSv/y ~20 mSv)

�Decontamination of these areas involves the

cleaning of structures and removal of

contaminated soil

�Removed soil and other contaminated wastes

are being stored at remediation locations or at

temporary sites

�Contaminated soil and waste are to be

gathered and placed into interim storage

facilities until transferred to a long-term

disposal site outside of the Fukushima area

Principles set by ICRP

Emergency exposure situation

Existing exposure situation

Long-term objectives

Additional dose to be

1 mSv/y

100 mSv/y

20 mSv/y

1 mSv/y

Aiming at 20 mSv/y or

less

7

The national government

implements

decontamination work

Special decontamination areas

Municipalities

implement

decontamination work

funded by the

government

Intensive contamination

survey areas

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Waste Management Challenges

� Clean-up efforts are generating

huge volumes of contaminated

soil and waste, which must be

managed in a safe and cost-

effective manner, wherever

possible implementing waste

volume reduction

� Future reuse of soil for

construction purposes is an

important option, if constraints

in terms of allowable organic

and clay content can be

managed

Below

8kBq/kg

Over

8kBq/kg

below

100kBq/kg

Over

100kBq/kgIncinerated

ash over

100kBq/kg

Waste in

countermeasure

area over

100kBq/kg

5

10

0

10.06Mm3

10.35Mm3

0.01Mm3

1.55Mm3

0.02Mm3

Contaminated soil and wastes

Vo

lum

e (

Mm

3)

Contaminated soil

and wastes

Incinerated ash

16~22 Mm3

current estimation

Wet particle-size

separation

Chemical

treatment

Heat treatment

8

Soils & wastes

Cs removed or

reduced materials Reuse

Volume Reduction

Cs accumulated

materialsFinal disposal

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9

Current Status避難指示区域

(2011年11月25日)

Lifted on April

1, 2014

Lifted on

Oct. 1, 2014

Lifted on

Sept. 5, 2015

Various situations exist

* Exposure dose reduced to the evacuation standard of 20 mSv

y-1 or less

not expected to drop below 20 mSv/y within 5 years

ordered to remain evacuated

ready to be lifted

� Areas where people regain ordinary daily life

� Areas where the evacuation order was lifted*

� Areas where the evacuation order will be

lifted no later than March 2017

� Areas where the prospects for lifting the

evacuation orders are not in sight

Evacuation order areas

(2015/9/5)

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10

How to Enhance Fukushima Environmental Resilience

�Address the needs for better scientific and

technological capabilities to assess, predict, and

minimize the impact of radiological

contamination

�Enhance the understanding of radiation and

associated risks in the public

Kai Vetter, 2015

The concept of Resilience;

The ability to recover from or more successfully adapt to adverse events

Page 11: Challenges for Enhancing Fukushima Environmental Resilience · Remedial Management Options (i) external doses from surfaces contaminated by ... Other measures relevant for individual

Regional scale distribution Deposition of

Radiocaesium [Bq/m2]

River/Floodplain

Dam

11

Individual external

doses in living areas

Development of a Technical Basis

for Enhancing Fukushima Environmental Resilience

Transport and accumulation

in a river basin

Forest

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12

Evolution of Air Dose Rate Distribution

Dose rate maps derived from car-

borne surveys

� Analysis of repeated survey results clarified the trends in air dose rate reduction for different

conditions due to radioactive decay, decontamination and natural weathering processes

Elapsed me since June 2011

Avera

ge a

ir d

ose r

ate

 (r

ela

tive)

0 400 800 1200 1600

1.0

0.1

2

5

Physical decay &

Forest

Flat fields

Roads

(car survey)

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� An empirical approach was employed to predict the dose rate distribution based on statistical

analyses of large-scale environmental monitoring data accumulates since the accident

� The time-dependent decrease of air dose rate in any specific setting can be approximated by a

combination of two exponential functions, representing “fast” and “slow” reduction rates

� Analysis linked to geostatistical data shows that the air dose rate reduction clearly depends on land

use

Elapsed time after the accident(y)

5 years after 30 years after

13

Air

do

se r

ate

(re

lati

ve)

0.1 1 3 5 10 15 300.005

0.01

0.1

1

3Evacuated zone(20-50 µSv/y)except forests

Air dose rate(µSv h-1)

Air dose rate(µSv h-1)

0.2

1

10

50

1

10

50

0.2

Development of a Predictive Model

by an Empirical Approach

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14

Empirical Prediction of Air Dose Rate Distribution

air dose rate

(μSv/h)

air dose rate

(μSv/h)

Corresponding to the

evacuation standard of 20

µSv y-1*

*based on the assumption that people spend 8

hours a day outdoors and 16 hours a day indoors,

for the latter considering a dose reduction factor of

0.4

3.8 3.8

After 5 y After 30 y

� Area more than 3.8 µSv/h will decrease in 30 years after to as much as 5% of such area

in 5 years after the accident.

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Regional scale distribution Deposition of

Radiocaesium [Bq/m2]

River/Floodplain

Dam

15

Individual external

doses in living areas

Transport and accumulation

in a river basin

Forest

Development of a Technical Basis

for Enhancing Fukushima Environmental Resilience

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16

Natural Processes Causing Mobilazation of Radiocaesium

Transport /

accumulation in

a river system

Transport

by ocean

currents

transport from

tree crowns to litter

removal of

runoff

removal of

litter/soil by

runoff

Normal flow conditions During heavy rainfall

Cs tends to bind strongly to surface soil, especially clay

Soil loss by runoff

Deposition of Cs-loaded

suspended particles

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17

Cs Transport in the Forest

0

5

10

15

20

25

30

2013

/4/1

2013

/5/2

1

2013

/7/1

0

2013

/8/2

9

2013

/10/

18

2013

/12/

7

2014

/1/2

6

2014

/3/1

7

2014

/5/6

2014

/6/2

5

2014

/8/1

4

2014

/10/

3

放射

性セ

シウ

ム濃

度(B

q/L)

2013-2014年度

KA-1 Cs-134

Cs-137

Evolution of Cs concentration in stemflow (Bq/L)

Evolution of cumulative Cs due to transport

from tree crowns to forest floor

Throughfall Stemflow

Fallen leavesFY 2014

Fallenleaves

Stemflow

Throughfall

Cu

mu

lati

ve

am

ou

nt

of

13

7C

s (k

Bq

/m2)

Elapsed time after the accident(d)

0

60

120

180

100 500 1000 1300 0

10

20

30C

s co

nce

ntr

ati

on

(B

q/L

)

Mature Japanese cedar

137Cs 134Cs

Japanese cedar forest in Kawauchi village

� Currently, most of Cs deposited on tree

crowns has transported to forest floor

(Onda et al., 2016)

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A: Erosion rate of surface

soil

4.9

kg/3months

B: 137Cs concentration

in eroded soil64 kBq/kg

C: 137Cs transport rate by

erosion[A×B×4 / 54,000 m2]

0.023

kBq/m2/y

Cs Transport from Forest Areas by Runoff

A: Erosion rate of surface soi 0.012 kg/m2/y

B: 137Cs concentration in

eroded soil16 kBq/kg

C: 137Cs transport rate by

erosion (A×B)0.19 kBq/m2/y

D: 137Cs deposition in surface

soil770 kBq/m2

Ratio of annual 137Cs loss to 137Cs deposition in surface

soil (C/D)

0.03%/y

Measurement of accumulated 137Cs in

stream sediments in Kawauchi Village

(2014/6/27~ 2014/9/30)

Measurement at a monitoring plot in

Kawauchi village

(2013/11/19 ~2014/10/20)

A monitoring plot to

measure erosion rates of

surface soil137Cs transport rate by

erosion1.2 kBq/m2/y

Ratio of annual 137Cs loss to 137Cs deposition in surface

soil

0.15%/y

(FY 2013)

18

137Cs transport rates by surface-soil erosion

A sampling point of stream sediments

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19

1.2 0.7 1.5 3.6

18.5

32.9

0.4

5.8

22.0

0

10

20

30

40

50

60

2 (0.6) 11 (1.4) 16 (1.8)

土砂

濃度

(mg

/L)

流量(m3/s) (水位 (m))

>60 um

3-60 um

0.45-3 um

Flow rate (m3/s)

(Water level (m))

13

7C

s co

nce

ntr

ati

on

water flow 2 m3/s 16 m3/s

Dissolved 137Cs (A) 0.3 Bq/L 0.3 Bq/L

Particulate-bound 137Cs (B)

0.1 Bq/L 2.2 Bq/L

(A)+(B) 0.6 Bq/L 3.3 Bq/L

Normal flow High river flow

Co

nce

ntr

ati

on

of

susp

en

de

d s

ub

sta

nce

s (m

g/L

)Cs Transport by River Flow

(dissolved/particulate-bound Cs)

Ukedo riv.

Takase riv.

Ogaki dam

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0

20

40

60

80

0 200 400 600 800 1,000

De

pth

(cm

Activity conc. (kBq/kg)St.2

134Cs

137Cs

134+137Cs

0

20

40

60

80

0 200 400 600 800 1,000

De

pth

(cm

Activity conc. (kBq/kg)St.5

134Cs

137Cs

134+137Cs

0

20

40

60

80

0 500 1,000 1,500 2,000

De

pth

(cm

Activity conc.(kBq/kg)St.7

134Cs

137Cs

134+137Cs

Simulation of Sediment inflow

due to a flood event

(Deposition of sand, silt, and clay

120 hr after the event) Observed Cs concentration in the

sediment of dam lake

20

Sand

Silt

Clay

Cs Accumulation in the Sediment of Dam Lake

Water levelElevation: 140 m(Current water level)

Elevation: 170 m*

Ratio of silt outflow 4.5% 1.6%

Ratio of clay outflow 54% 34%

Ratio of 137Cs outflow 9.0% 3.5%

Ratio of silt-bound 137Cs 40% 18%

Ratio of clay-bound 137Cs 60% 82%

More than 90% of inflow sediment and 137Cs deposited in

the reservoir during and after heavy rainfall events

*Operational water level before the accidents

Measured

Simulated

Concentration of 137Cs in Flow

at the exit of the reservoir

Co

nce

ntr

ati

on

of

13

7C

s (B

q/L

)

Ogaki dam

St.2

St.5

St.7

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Overview of 137Cs Flux from Each Catchment of

Ukedo River Basin

Total flux

to the

ocean

1 TBq/y

Ogaki-dam outflow

0.07 TBq/y

Ukedo riv.

Takase riv.

3 km

More than 90% of radiocaesium flowing into the Ogaki

dam lake was sedimented in the lake

Annual transport rate of 137Cs of the forest topsoil is

around 0.1%

21Inventory Discharge

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Recovery of the Coastal Marine Environment

Fisheries Agency of Japan (2015)

22

0

0.2

0.4

0.6

0.8

1

0

500

1000

1500

2000

2500

3000

グラフ タイトル

系列1 系列2 系列3

500

1000

1500

2000

2500

3000

0

20

40

60

80

100

0Oct.-Dec.

Jul.-Sep. Jan.-Mar. Oct.-Dec. Apr.-Jun.

Jul.-Sep. Jan.-Mar. Oct.-Dec. Apr.-Jun.

Jul.-Sep. Jan.-Mar. Apr.-Jun.

Excess ratio %Number of samples

>100Bq/kg

<100Bq/kg

Excess ratio

Jul.-Sep.

2012 20142011 2013

Oct.-Dec. Jan.-Mar.

Apr.-Jun. Jul.-Sep.

Oct.-Dec. Jan.-Feb.

Apr.-Jun.

2015 2016

**Otosaka and Kobayashi (2013) + Updated

Statistics on fish samples

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Regional scale distribution Deposition of

Radiocaesium [Bq/m2]

River/Floodplain

Dam

23

Individual external

doses in living areas

Transport and accumulation

in a river basin

Forest

Development of a Technical Basis

for Enhancing Fukushima Environmental Resilience

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24

• Currently applied simple method

results in larger uncertainties.

• D(p) and t(p) are not realistically

considered in estimate.

Individual doses estimated from air dose rates

�Amount of time spent indoors or

outdoors depending on occupation

�Variations in working places

depending on the type and location

of work

�Distribution of Cs deposition

on the surface (ground,

pavement etc.)

�Weathering effects

Outdoors (Location-specific

external exposure)

Difference of lifestyleIndoors

D(p) varies according to locationt(p) varies according to individual

pavement ground

E = Σ c•D(p)•t(p)

E : total effective dose

C : conversion coefficient from air dose to effective dose

D(p) : air dose rate at location p

t(p) : residence time at location p

�Dose reduction factor

depending on house

type and surrounding

conditions

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25

Measurement of air dose rates according to

the individual’s daily route

� Communicate with evacuees who wish to return to their homes

Detailed data

acquisition by interview

to know how much time

will be spent along

individual’s daily route

after evacuees return to

their homes

Man-borne survey

Realistic estimates of Individual doses

経路/場所ID 地点(部屋) 移動手段 開始時刻 終了時刻

1 自宅(寝室) 0:00 5:30

2 自宅(リビング) 5:30 8:00

3 徒歩 8:00 8:05

4 裏山 8:05 11:55

3 徒歩 11:55 12:00

2 自宅(リビング) 12:00 13:00

5 徒歩 13:00 13:05

6 畑 13:05 13:50

7 徒歩 13:50 14:00

8 畑 14:00 14:50

7 徒歩 14:50 15:00

2 自宅(リビング) 15:00 16:00

9 車 16:00 16:10

10 銭湯 16:10 17:50

9 車 17:50 18:00

2 自宅 18:00 0:00

Interview to evacuees

Realistic estimates of individual doses according to individual’s daily route

IndoorField 1

Field 2

Estimated external cumulative radiation doses

Air

do

se r

ate

Sv

/h)

Time Walking on roadsHill

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Knowledge and experience gained for Enhancing

Fukushima Environmental Resilience

26

�Cleanup Navihttp://c-navi.jaea.go.jp/en/The Cleanup-navi Communication Platform provides an overview of regional contamination due to the accident and approaches to

remediation. It also includes background information on the nature of ionising radiation and its health effects to allow the user to make informed judgements as to the value of the remediation actions that are being undertaken.

�DPP reports http://fukushima.jaea.go.jp/english/outline/20150327.htmlPart 1 summarises the Decontamination Pilot Project, providing the background required to put this work in context for

an international audience. In Part 2, the subsequent application of output from this project to regional remediation is discussed, along with a status update on such work (including radioactivity monitoring), an overview of JAEA’s associated R&D and international input to / review of regional environmental decontamination in Fukushima.

� Lessons learned report http://fukushima.jaea.go.jp/english/outline/20150327.htmlThis report provides a concise overview of knowledge and experience gained from the activities for environmental

remediation after the Fukushima Daiichi accident. It is specifically tailored for international use, to establish or refine the technical basis for strategic, off-site response to nuclear incidents.

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Thank you for your attention