Characterization of LWR Spent Fuel MCC-Approved Testing ... · The first lot of spent fuel, ATM-101, for use as an ATM has been obtained after discharge from the H. B. Robinson pressurized

-I(~~~

I I

PNL-3109Original lssue

UN7TO

McMaterials Characterization Center

Characterization of LWRSpent Fuel MCC-ApprovedTesting Material-ATM-101

June 1984

Prepared for the U.S. Department of Energyunder Contract DE-AC06-76RLO 1830

Pacific Northwest Laboratory-Operated for the U.S. Department of Energyby Battelle Memorial Institute

IC

rimusP30. Baltelle

X-I'd-

/

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PNL-5109Original Issue

UC-70

CHARACTERIZATION OF LWR SPENT FUELMCC-APPROVED TESTING MATERIAL - ATM-101

J. 0. Barner

June 1984

Prepared forthe U.S. Department of Energyunder Contract DE-AC06-76RL0 1830

Pacific Northwest LaboratoryRichland, Washington 99352

NOTICE

This report is intended to be a "living document" with additional charac-

terization data being included in subsequent revisions as the data becomes

available. This planned recurrent publication will permit the maximum usage of

the characterization data by the users of Spent Fuel ATM-101.

I

ABSTRACT

The characterization data, obtained to date, for Materials Characterization

Center (MCC) Approved Testing Material (ATM)-101, spent fuel from H. B. Robinson,

Unit 2, Assembly BO-5, are described. ATM-101 consists of 27 equal-length seg-

ments from nine fuel rods. Characterizations provided for ATM-101 include,

1) reactor, assembly, and fuel rod descriptions, 2) Assembly BO-5 irradiation

history, 3) a description of unusual incidents that occurred to the rods,

4) fission gas release measurements, 5) results of ceramography/metallography

examinations, 6) fuel burnup measurement results and correlations, 7) results

of gamma scanning, 8) calculated values of the radionuclide inventory, and

9) results of a radionuclide chemical overcheck. Calculations for and measure-

ment of radial distributions of selected radionuclides are planned. A descrip-

tion of pertinent results from other studies on sibling rods from Assembly BO-5

is also included. The distribution of ATM-lOl to date is described along with

characterization results on specially processed material.

It is intended that this report be revised and updated as additional char-

acterization data become available.

V

SUMMARY

This report describes the characterization plan, methods, and results for

light water reactor (LWR) Materials Characterization Center (MCC) spent fuel

Approved Testing Material (ATM)-101. ATM-101 s spent fuel from the H. B.

Robinson, Unit 2, Assembly B-5, a moderate-burnup, pressurized water reactor

(PWR) fuel that released very small quantities of fission products and fission

gas from the fuel during commercial operation.

The characterization plan for the ATM-101 is described in Section 3.0 and

includes discussions/sampling for 1) fuel rod, assembly and reactor descriptions,

2) irradiation and decay histories, 3) unusual incident description, 4) fission

gas release, 5) transverse and longitudinal ceramography/metallography, 6) burnup

distribution, 7) gross and spectral axial gamma scanning, 8) calculations of

the axial radionuclide distribution, and 9) chemical overchecks of the axial

radionuclide distributions. Calculation of the radial radionuclide distribu-

tions and measurement of radial radionuclide distributions are also planned.

Characterization data that are available to date for items 1 through 9are

presented in this original version of the characterization report. In addi-

tion, descriptions of the preparation and characterization of some special

ATM-101 materials are discussed. Additional data for all categories of the

characterization data will be published in subsequent versions of this report.

vii

CONTENTS

1.0 INTROCTI .............. 2 1.1

3.0 CHARACTERIZATION PLAN FOR ATM-11.................................... 31

4.0 CHARACTERIZATION OF ATM-101 ... 4.1

4.1 REACTOR, ASSEMBLY AND FUEL ROD DESCRIPTIONS .................... 4.1

4.2 ASSEMBLY BO-5 IRRADIATION HISTORY ............. 4.3

4.3 DESCRIPTION OF UNUSUAL INCIDENTS ............. 4.5

4.4 FISSION GAS RELEASE MEASUREMENTS .............................. 4.6

4.5 CERAMOGRAPHIC/METALLOGRAPHIC EXAMINATIONS ...................... 4.6

4.6 FUEL BURNUP MEASUREMENTS ....................................... 4.28

4.7 GAMMA SCANNING RESULTS .......... 4.37

4.8 RADIONUCLIDE INVENTORY CALCULATION ........... 4.40

4.9 RADIONUCLIDE CHEMICAL OVERCHECK ............. 4.43

4.10 PERTINENT RESULTS FROM SIBLING RODS ........................... 4.44

4.10.1 Nondestructive Examination Results ..................... 4.44

4.10.2 Destructive Examination Results ........................ 4.46

5.0 DISTRIBUTION OF ATM-101 SPENT FUEL .............. . . s..... 5.1

5.1 CRUSHED MATERIAL FOR BWIP - SEGMENT N-9C ..................... 5.1

5.2 MATERIAL FOR NNWSI - SEGMENT C-5C ... ............. 5.7

5.3 MATERIAL FOR CSFMPO - SEGMENT N-9B ... .. .......... 5.7

ACKNOWLEDGMENTS ...... 1

10319aix

REFERENCES..................... ............. R.1

APPENDIX A - POWER HISTORY FOR ASSEMBLY BO-5 ............................. A.1

APPENDIX B - SECTIONING DIAGRAMS ........................................ B.1

APPENDIX C - DETAILS OF GAS ANALYSES............................. ........ C.

APPENDIX D - GAMMA SCAN RESULTS ..................................... .... D.1

APPENDIX E - RESULTS OF RADIONUCLIDE INVENTORY CALCULATIONS.............. E.1

APPENDIX F - RADIOISOTOPES DETERMINED DURING BURNUP ANALYSES............. F.1

x

FIGURES

4.1 Core Arrangement of H. B. Robinson Unit 2-Reactor .................. 4.2

4.2 Layout of H. B. Robinson Assembly BO-5 ............................. 4.3

4.3 Power History for Assembly BO-5 .................................... 4.4

4.4 Transverse Photomacrograph of Sample N-9C-C, High PowerRegion............................... .................................... 4.10

4.5 Longitudinal Photomacrograph of Sample N-9C-F, High PowerRegion............................... .................................... 4.11

4.6 Transverse Photomacrograph of Sample N-9C-I, Grid Spacer Areain High Power Region............................................... 4.12

4.7 Longitudinal Photomacrograph of Sample N-9C-K, Grid Spacer Areaof High Power Region .............................................. 4.13

4.8 As-Polished Transverse Sample N-9C-C............................... 4.16

4.9 As-Polished Longitudinal Sample N-9C-F ............................. 4.18

4.10 As-Polished Transverse Sample N-9C-I............................... 4.20

4.11 As-Polished Longitudinal Sample N-9C-K............................. 4.22

4.12 Noble Metal Fission Product Agglomeration in Samples from(a) Central High-Power Region of Rod N-9, and (b) GridSpacer Region at 12% Lower Power ................................... 4.24

4.13 Ion-Etched Transverse Sample N-9C-C................................ 4.26

4.14 True Grain Size of Fuel as a Function of Radius for FourSamples from N-9C ................. 0............................ 00 4.28

4.15 Examples of Outer Surface Oxide on ATM-101 Rods .................... 4.30

4.16 Examples of Inner Surface Oxide from Rod N-9C ...................... 4.31

4.17 Hydride Orientation in Rod N-9C Cladding ........................... 4.32

4.18 Correlation Between Burnup Analyses and 137Cs Gamma Counting ....... 4.33

4.19 Composite of Gross Gamma Scans for Rod N-9 ......................... 4.38

4.20 Composite of 137Cs Gamma Scans for Rod N-9 ......................... 4.39

4.21 137Cs Gamma Scan of Rod C5C with Narrow Slit and Small Steps....... 4.42

xi

4.22 Oxide Thickness Variations Along Zircaloy Fuel Rod fromH. B. Robinson Unit 2................... ......... ........... 4.48

5.1 Comparison of Fission Product Concentration in BWIP Materialwith Three Particle Sizes.......................................... 5.5

xii

TABLES

3.1 Characterization Plan and Sampling Matrix for ATM-101 .............. 3.3

4.1 As-Fabricated Fuel Rod Characteristics for ATM-101 ................. 4.4

4.2 Gas Pressure, Gas Composition, and Rod Void Volume for Rodsfrom ATM-101 ...... .......... ................... ..... s.. 4.7

4.3 Isotopic Gas Analyses for ATM-101 Rods .............................. 4.8

4.4 Fission Gas Release Results for ATM-101 Rods ....................... 4.9

4.5 Summary of Estimate of Fragment Areas per Unit Length ofFuel Rod ......... ............. ...... ...... .......... 4.15

4.6. Results of Fuel Grain Size Measurements ............................ 4.25

4.7 Outer and Inner Oxide Thickness in ATM-101 Rods .................... 4.29

4.8. Burnup Results for ATM-101 Samples .................. e.....e.e... 4.34

4.9 Rod-Average Burnup in ATM-101 Fuel Rods ....... ..geeeeeg. eg.... 4.36

4.10 Regions of Apparent In-Reactor Densification and Fuel Settling ..... 4.41

4.11 Comparison of Chemical Overchick Results to ORIGEN-CalculatedRadionuclide Inventory ................................. 4.45

4.12 Comparison of Fission Gas Data from Nine ATM-101 Rods toData from 28 Sibling Rods from Assembly BO-5 ....................... 4.47

4.13 Strength and Elongation Values for Cladding fromAssembly BO-5 Sibling Rods ............ 4.48

5.1 Description of Initial Run on BWIP Material ....................... 5.2

5.2 Description of BWIP Material .... 5.2

5.3 BWIP Crushed Fuel Distribution .................................... 5.3

5.4 ICP Results on Crushed BWIP Material ........................... 5.4

5.5 Results from X-ray Diffraction Analyses of BWIP Crushed Material... 5.6

xiii

1.0 CONCLUSIONS

As a result of the characterization completed to date, the following con-

clusions are made:

1. ATM-101 s a moderate-burnup, low-releasing (fission products

in-reactor), originally solid-pellet, U02 fuel material that falls

Into the class of typical" spent fuel that may be deposited n a

repository (Barner, 1984).

2. The premise appears to be confirmed that a correlation between

limited burnup sampling and axial gamma-scanning distribution data

for 137Cs can be used to predict the burnup and, therefore, the

radionuclide inventory (source term) in sibling, low-releasing

ATM-101 material.

1.1

2.0 INTRODUCTION

The Materials Characterization Center (MCC) has the responsibility to pro-

vide spent fuel Approved Testing Materials (ATMs) for use in the investigation

of nuclear waste disposal forms. The first lot of spent fuel, ATM-101, for use

as an ATM has been obtained after discharge from the H. B. Robinson pressurized

water reactor. This material is a moderate burnup fuel, approximately

30 MWd/kgM, that had only minor fission gas release from the U02 during opera-

tion. This report describes the initial characterization results for ATM-101.

These results are expected to be beneficial to experimenters that will utilize

the material for ascertaining the release behavior of the entrained radionu-

clides. The characterization plan (Section 3.0) was developed based upon the

general MCC plan for characterization of spent fuel ATMs described by Barner

(1984). The results of the characterization are presented in Section 4.0.

Because not all the ATM-101 fuel rods have been sampled for characterization,

and because of budgetary/schedule considerations, the characterization results

that are presented in this original document are incomplete. Section 5.0

describes the distribution of ATM-101 specimens as of the date of publication

of this report. Additional characterization results and ATM distributions are

anticipated in the near future, and will be described in future issues of this

report.

ATM-101 consists of 27 fuel rod segments of approximately equal length

from nine H. B. Robinson, Unit 2, fuel rods from Assembly BO-5. The cutting of

the fuel rods into segments was required to transport them expeditiously from

the Test Area North (TAN) hot cell at the Idaho Nuclear Engineering Laboratory

(INEL) to the PNL hot cells at Hanford. The exposure of the segments to air

was minimized by sealing the segments with plastic caps during transport and by

subsequent storage of individual segments in a limited-volume, air-atmosphere,

sealed tube after arrival at PNL.

2.1

....3.0 CHARACTERIZATION PLAN FOR ATM-lOl

The logic for and an example of a generic characterization plan for MCC

spent fuel ATMs was described by Barner (1984). The actual plan for charac-

terizatiorT of ATM-101 is based on this generic plan and consists of measure-

ments or descriptions in the following areas:

o Descriptions of the fuel rods, the assembly of rods,-and the reactor

(Section 4.1).

* A description of the irradiation and decay histories of the fuel

assembly (Section 4.2).

P A description of unusual incidents to the fuel assembly'subsequent

to discharge from'the reactor (Section 4.3).

o Measurement of the fission gas release from each fuel rod

(Section 4.4).

o Light microscope examination of transverse and longitudinal samples'to ascertain the degree of fuel cracking, fuel microstructure

characteristics, and cladding oxidation (Section 4.5).

o Measurement of the fuel burnup distribution (Section 4.6).

o Measurement of the axial distribution of the gross gamma activity

and the activities of individual radionuclides in the fuel rods

(Section 4.7).

a Calculation of the radionuclide inventory in the fuel as a function

of burnup and the decay period (Section 4.8).

A Chemical determination of the inventory of several radionuclides tospot-check the calculated radionuclide inventory (Section 4.9).

• Calculation of the radial distribution of the radionuclide inventory

in the fuel as a function of burnup and the decay period.

• Measurement of radial distribution of the radionuclides within thefuel as an overcheck of the calculation of the radial distributions.

3.1

The last two characterization items have not yet been conducted. Results for

these items will be published as they become available.

The detailed characterization plan and sampling matrix for the nine fuel

rods that comprise ATM-101 are listed in Table 3.1. Fuel rod N-9 was used to

obtain several ceramography/metallography, burnup, and chemical samples. The

locations of these groups of samples were selected to cover the wide range in

burnup levels present in any of the fuel rods. The selected burnup analyses

and the gamma scan results from each individual rod can be combined to assign

the burnup and a resultant radionuclide inventory for any ATM specimen that

will be provided from the lot of fuel rods.

In addition to the characterizations planned for the ATM-101 material,

special characterizations were conducted on some processed specimens distri-

buted to experimenters. The results from these special characterizations are

described in the appropriate subsection of Section 5.0 of this report that

describes the distribution of ATM-101 specimens, e.g., results from the special

examination of crushed ATM-101 material for the Basalt Waste Isolation Project(BWIP) are described in Section 5.1.

Five to ten percent of the ATM-101 spent fuel will be retained by the MCC

as archive material for future use.

3.2

c C C c C C IC C ~~C C

TABLE 3.1. Characterization Plan and Sampling Matrix for ATM-1O1(a)

Fuel Historical

Rod Records(b)

C-5

D-10G-9G-13

J-12!A L-8

WA N-4

N-9N-12

xxxxxxxxx

FissionGas

Releasa(c)

x

xxXxxXxx

Ceramography-Metalloqraphy

Transverse Longitudinal urnup

Analytical

Gamma Inventory Spot-check

Scan (d) Calculation Inventory(°)

I

I

15

I X-x

-x

-x

-x

-x

-x

5 X-x

xxxxxxxxx

5

Radial

Distribution

Calculation

x

x

x

x

x

x

x

x

x

Analytical

Spot-checkRadial

DistrIbution

5 1

(a) X denotes description/measurement will be made.- denotes measurement will not be mde.numerical value Indicates number of samples from the Individual fuel rod.

(b) Includes descriptions of fuel, Irradiation history and any unusual Incidents.(c) Includes gas composition, gas pressure and volume.

(d) Includes gross, 137Cs, 134Cs and 15 4Eu axial gamma scans.

(e) Includes analyses for 235U, 249pu 237Np, 99Tc, 137 and 14C.

4.0 CHARACTERIZATION OF ATM-101

This section describes the characterization results obtained to date for

ATM-101. Historical information is described in Sections 4.1, 4.2, and 4.3,

fission gas release 'results in Section 4.4, ceramography/metallography results

in Section 4.5, burnup results in Section 4.6, gamma scanning results in Sec-

tion 4.7, calculated radionuclide inventories in Section 4.8, and results of

the radionuclide chemical overchecks in Section 4.9. The bulk of the histori-

cal information was taken from the summary provided by Einziger and Fish

(1982). Other pertinent information for rods from Assembly BO-5, taken from

this reference, are described in Section 4.10.

Locations of individual samples from sectioned ATM-101 rods are given in

Appendix B.

4.1 REACTOR, ASSEMBLY AND FUEL ROD DESCRIPTIONS

The ATM-101 fuel was irradiated in the H. B. Robinson, Unit 2, reactor,

which is a three-loop, 665 MWe (2192 MWt),-pressurized water reactor (PWR)

located in Hartsville, S. C. and is operated by Carolina Power and Light Com-

pany. The core consists of 157 fuel assemblies of the 15 x 15 design that were

designed and fabricated by Westinghouse Company. The core has three enrichment

zones (Figure 4.1). The ATM-101 fuel was originally 2.55 wt% enriched in 235U

Each assembly contains 204 fuel rods, 20 control rods, and one possible in-core

instrumentation tube as shown in Figure 4.2. The rod separation is maintained

along the length of the assembly by seven grids, five ofwhlch.are wholly

within the fueled length. The ATM-101 fuel was rradiated in Assembly BO-5

during the first two operating cycles of the H. B. Robinson, Unit 2, the first

cycle in position F9 and the second cycle in position M (Figure 4.1).

Each fuel rod in the assembly consisted of a column of dished cylindrical

urania fuel pellets stacked within a sealed Zircaloy-4 cladding tube. The fuel

rods were pressurized with helium during fabrication. Although the initial

pressurization level is proprietary, gas analysis after irradiation indicates

the original pressurization level was approximately 1.8 MPa (260 psia). It was

4.1

.2

45

6

a ~~~~~~~10

1213

1415

Core Arrangement - H.B. Robinson Reactor

Showing Location of Assembly B0-5During First 01) and Second (2) Cycles

ElRegion 1 (Enrichment 1.85%) 53 AssembliesLFj Region 2 (Enrichment 2.55%) 52 Assemblies

Region 3 (Enrichment 3.10%) 52 Assemblies

FIGURE 4.1. Core Arrangement of H. B. Robinson Unit 2 Reactor

also reported that there were indication s that the rods might have been pres-

surized without completely purging the internal air. However, review of the

published data and the gas analyses reported n Section 4.4 for ATM4-101 indi-

cates the nitrogen content of the gas is only 1 of that that would be expected

for an originally air-filled rod. As-built characteristics of the fuel rodsare given in Table 4.1. The location of the.ATM-101 fuel rods in Assembly BO-5are shown in Figure 4.2.

4.2

P

N CO C T C ScM CL C T I C1 I IK IC C

J

H C C C

G

F C C

E IC_ C

D C 0c C c I I C ICB

A

1 2 3 4 5 6 7 8 9 10 11 12 13 14 15

= Control Rod

[21=Instrument Tube

l) =ATM-101 Fuel Rod

FIGURE 4.2. Layout of H. B. Robinson Assembly BO-5

4.2 ASSEMBLY BO-5 IRRADIATION HISTORY

The Assembly BO-5 irradiation commenced with the initial operation of.

H. B. Robinson, Unit 2, reactor n March 1971. The Assembly BO-5 irradiation

was completed after two reactor cycles and the assembly discharged on May 6,

1974. The rradiation accumulated a total of 799 effective full power days

(EFPD). The power history is illustrated in Figure 4.3 and tabulated in Appen-

dix A.- The peak linear heat generation rate (LHGR), of 32.7 kW/m (10.0 kW/ft),

occurred n December 1971 shortly after the irradiation began. At the end of

the rradiation, the LHGR had dropped to 21.2 kW/m (6.5 kW/ft). The estimated

peak-pellet and assembly-average burnups were 31.36 and 28.03 MWd/kgM,

respectively.

4.3

TABLE 4.1. As-Fabricated Fuel Rod Characteristics for ATM-101

Cladding 0.D., mm 10.70

Claddi ng I. D., mm 9.46Cladding wall thickness, mm 0.62

Dilametral gap, mm 0.165

Cl adding material Zi rcal oy-4

Fuel rod length, m 3.86

Fuel pellet material Sintered U02

Pellet type Solid, dished

Fuel density, g/cm2 (X T.D.) 10.08 (92)235 U enrichment, wt% 2.55

Pellet diameter, mm 9.30

Pellet length, mm 15.2

Fuel stack height, m 3.65

Plenum length, mm 173.5

End cap length, mm 17.5

40 . _

Peak Pellet 10

E

20 _i

:3: Assembly Average _

10 Cycle 1 _ Cycle 2

0 100 200 300 400 500 600 700 800Effective Full Power Days

FIGURE 4.3. Power History for Assembly 80-5

4.4

4.3 DESCRIPTION OF UNUSUAL INCIDENTS

During the transport of Assembly BO-5 from the reactor to the TAN hot cell

and the'subsequent'unloading of the transport cask,-a series of-events took

place that caused the temperature of portions of the assembly to exceed the

boiling point of water. During initial transport of the assembly in a hori-

zontal position from the H. B. Robinson, Unit 2, site to the TAN hot cell, a

portion of the assembly was uncovered for about one week. This happened

because an air space was permitted in the cask in order to allow for thermal

expansion of the cooling water. When the cask arrived at the hot cell, it was

placed in a vertical attitude where the assembly was also partially uncovered

for about six hours. After removal of the assembly from the cask, it was held

vertically in the air for approximately two hours before it was placed in a

storage pool.' When it was placed n the pool, large amounts of steam formed.

Later the assembly was held in a horizontal position for seven hours during rod

removal, but no steam formed when the assembly was placed back in the pool.

Calculations indicate that cladding temperatures could have been as high as

466°C during the vertical hold in air and 343°C during the horizontal shipment.

However, microhardness measurements made on the cladding did not reveal any

significant recovery of irradiation-induced hardening, indicating that the,

cladding temperature was less than 350°C during the handling in the vertical

attitude and less than 3000C during the horizontal holding period. Further,

subsequent temperature measurements made to estimate the fuel temperatures in

the horizontal and vertical attitudes indicated that the cladding surface tem-

perature was less than 1500C for both cases. It was, therefore, concluded that

none of the assembly temperature excursions was 'long enough or high enough to

significantly change the condition of the fuel rods in Assembly BO-5.

During repacking of the fuel segments in the PNL hot cells, segment G-9C,

was damaged by bending while sealed in its storage tube. This segment has been

set aside and will only be used as a source of ATM material if the nondamaged

portions can be removed from the storage tube in a manner that assures that the

material is adequate for any intended use.

4.;5

4.4 FISSION GAS RELEASE MEASUREMENTS

Fission gas release measurements were previously made on thirteen fuel

rods from Assembly BO-5 (Einziger and Fish, 1982). For the ATM-101 rods the

measured internal rod void volume, total volume of gas recovered, internal rod

pressure, and gas analyses are listed in Table 4.2. Table 4.3 provides theIndividual isotopic analyses for the fission gases. Table 4.4 lists the items

used in the fission gas release calculation and the fission gas release value

for each rod. The average fission gas release from the thirteen sibling rods

was 0.21% with a standard deviation of 0.05%. Results for the nine rods com-

prising ATM-101 are apparently similar (Table 4.4). The generated fission gas

was calculated using a value of 31.0 cm3 of generated fission gas per MWd at

standard temperature and pressure and the rod average burnup for each rod. The

procedures for gas sampling, void volume measurement, gas analysis and methods

of determining uncertainties are described in Appendix C.

The rod-average burnup values were taken from Section 4.6 of this report.

For the case where the gamma scanning has not been completed as of the issuance

of this report, burnup for the rod in question was assumed to be the same asfor rod N-9 and the preliminary fission gas release value for the rod is shown

in brackets in Table 4.4.

4.5 CERAMOGRAPHIC/METALLOGRAPHIC EXAMINATIONS

Ceramography was conducted on fuel samples, primarily from fuel rod N-9,

in order to determine the degree of pellet fragmentation and changes in micro-

structure/porosity. The cladding from the same samples was examined to char-

acterize the outer and inner surface oxidation and the hydride orientation.

Both transverse and longitudinal cross-sections were sectioned from positions

adjacent to burnup/chemistry samples. (See sectioning diagrams in Appendix B).

Photomacrographs of the transverse and longitudinal sections from segments

N-9C are shown in Figures 4.4, 4.5, 4.6, and 4.7, respectively. The N-9C-C/F

pair of samples is typical of the high-burnup/high-power region of the fuel,

while the -9C-IK pair of samples is typical of material from the grid spacer

region of the high-burnup/high power portion of the rod, i.e., the power in the

4.6

S_.

(( C ( C~~~ r c C 0 ~ ~~~ I

TABLE 4.2. Gas Pressure, Gas Composition, and Rod Void Volume for Rods from ATM-101

Measured

Rod Void Volume,No. em

C-5 23.9±1.1

D-10 22.5±1 el1

G-9 22.2±1.0

G-13 20.0±0.9

J-12 22.8±1.1

L-8 22.1_1.0

Total Recovered

Gas at STP. m

362+8.7

369±8.9

373±8.9

357±8.6

368±8.8

364±8.7

368+8.8

Pressureat O'C,

We me Xe Kr Ar 2Co N°

2 2i

1.54 98.3 - 0.89 0.10 0.61 (0.01 0.01 0.06±0.07 ±0.2 ±0.015 +0.044 ±0.01 -- - to.004

1.66 98.2 1.03 0.12 0.61 0.02 <0.01 0.05+0.08 t0.2 ±0.08 ±0.004 ±0.01. ±0.008 - ±0.004

1.70 98.9 0.72 0.08 0.30 cO.01 <0.01 0.04_0.08 ±0.2 ±0.012 t0.003 +0.005 - - _0.004

<0.01

<0.01

<0.01

<0.01

Orginics

<0.01

0.02

<0.01

1.81 97.9 0.98 0.11±0.08 ±0.2 ±0.017 ±0.004

0.91 0.02±0.016 t0.008

<0.01 0.05- ±0.004

<0.02

1.63 98.7 0.88 0.10 0.25 <0.01 <0.01±0.08 +0.2 ±0.015 *0.004 ±0.005 --

1.67 96.7 1.42 0.16 0.76 0.03 <0.01±0.08 0.02 ±0.024 ±0.006 t0.013 *0.008 -

0.05±0.004

<0.01

0.74 0.120.13 _0.004

N-4 20.1±0.9

1.85 98.7 0.74t0.09 ±0.2 ±0.013

0.08 0.33 0.02*0.003 +0.006 ±0.008

<0.01 0.08 <0.01-- ±0.004 -

N-9 1 9, 7 (a) 371 1.9(a) 98.3 0.89 0.10 0.63 <0.01 <0.01 0.08 0.018.9 -- ±0.2 ±0.015 ±.004 ±0.01 -- - ±0.005 _-.006

N-12 1 2 5 (b) 365 2 ,9 6 (b) 98.5 0.85 0.09 0.40 <0.01 <0.01 0.15 0.03±8.8 - ±0.2 +0.015 ±0.003 ±0.01 - - *0.004 _0.005

(a) Result may be slightly low due to Incipient valve failure that was discovered during sampling the next fuel rod;however, result Is within two standard deviations of results for first seven rods listed.

(b) Result in error due to faulty valve.

0.02

0.02

(0.01

<0.01

TABLE 4.3. Isotopic Gas Analyses for ATM-101 Rods

Rod No. i~u lXenon, % Krpton, No . 128 1JU LJL LJZ 14

C-5 <0.1 0.1 8.3 20.6 28.6-- ±0.05 ±0.3 0.4 0.5

150

42.4±0.7

12.0±0.5

31.7 3.8 52.4±1.2 ±0.7 ±1.9

Xe-KrRatio

8.9

D-10 <0.1 0.1 8.3 20.5-- ±0.005 ±0.13 0.4

G-9 <0.1 0.1 8.4 20.5-- ±0.06 ±0.03 ±0.4

28.4 42.7±0.5 0.7

28.2 42.8±0.5 0.7

12.1±0.6

31.9 3.7 52.5±1.2 ±0.6 1.9

8.6

9.012.1 31.9 3.5 52.4±0.8 ±1.2 ±0.5 ±1.9

G-13 <0.1 0.1 8.2-- t0.04 +0.3

J-12 <0.1 0.1 8.1-- ±0.05 ±0.3

L-8 <0.1 0.1 7.7-- +0.03 ±0.3

20.4 28.4 42.8+0.4 0.5 ±0.7

11.9+0.7

31.9 3.8 52.4+1.2 ±0.5 +1.9

20.6±0.4

28.5t0.5

42.6±.07

42.8±0.7

11.6 32.1 3.6 52.7±0.4 ±1.2 ±0.5 ±1.9

11.5 32.5 3.6 52.4±0.4 ±1.2 ±0.5 ±1.9

8.9

8.8

8.920.9 28.5±0.4 0.5

N-4 <0.1 0.2 8.3 20.7-- ±0.08 ±0.3 ±0.4

N-9 <0.1 0.1 8.0 20.8-- ±0.05 ±0.3 ±0.4

28.3 42.5t0.5 ±0.7

28.2 42.8±0.5 ±0.7

12.2 31.8 3.7 52.3t0.9 t1.2 ±0.9 ±1.9

12.0 32.2 4.1 51.8t0.7 ±1.2 ±0.7 ±1.9

9.3

8.9

N-12 <0.1 0.1 8.5 20.5 28.2-- ±0.05 ±0.03 ±0.04 ±0.5

42.6±0.7

12.2 31.5 3.9 52.3±0.8 ±1.1 ±0.8 ±1.9

9.4

latter pair was about

regions is fragmented

12% lower than the former pair. The fuel from both

both transversely (longitudinal sections) and radially

(transverse sections). In order to estimate the degree of fragmentation for

use in dissolution/leaching experiments on similar fuel specimens the following

logic was applied.

* First, the sum of the lengths of the major radially oriented, longi-

tudinal cracks was estimated from the transverse photomacrograph in

units of equivalent radii. The assumption was made that all these

cracks were parallel to the centerline of the fuel rod. An estimate

of the area per unit length of fuel rod of longitudinal crack was

made by multiplying the sum of the crack lengths by the fuel pellet

radius (4.65 mm), by two for the two new facing surfaces, and by a

4.8

TABLE 4.4. Fission Gas Release Results for ATM-101 Rods

Rod No.

C-5

D-10

G-9

G-13

J-12

L-8

N-4

N-9

W-12

Sibling Rods

TotalRecoveredGas at3

STP,. cm

362

I369

373

357

368

364

368

371

365

Xe + Kr,

0.99

1.15

0.80

1.09

0.99

1.58

0182

0.99

0.94

Volume ofXe + Krat SP,

cm3.584.24

2.983.89

3.645.753.023.673.43

Rod-Average

Burnuo fMWd/kgM

28.2

[Z8.4]

<28.4]

t28.4]

[28.4)

30.0

[28.4)

28.4

29.4

EstimatedFis

Produged,,,cm

1906

[19193£19191£1919]

[1919]

2027

[1919]

1919

1987

FissionGas'aj

Released,

0.19

[0.22]

£0.163

[0.203

[0.19]

0.28

[0.16]

0.19

0.17

0.21

(a) Values shown in brackets are preliminary pending. 137Cs-iamda-'scan results.For nonscanned rods the burnup is assumed to be the same as N-9.

(b) Calculated from fuel dimensions and density listed in Table 2, and assuminga fuel ume reduction of lX for dishes, metal t6 oxide ratio of 0.88, and31.0 cm11fission gas per Wd.

unit length of one millimeter. This method tends to overestimate

the fragment surface-area by assuming the cracks run the total

length of a pellet, where in fact most do not. However, it tends to

underestimate the area by ignoring small cracks and the fact that

cracks that are not parallel to the centerline will have a larger'

area than estimated.

* Second, the areas of the transverse cracks were estimated by count-

ing the primarily radial (crack 'is near- nomal to tladding')tran's-!verse crcs69telnitudinal photo-macrograph 1or cecks~ta

tended to intercept the cljaddingsur'face at'an ange between 'i45 -

and 80 a value -of oMhe-hal-f a, transverse crack wa's assigned because--

of the`p'ossibty fthat its 'equValent bad beencounted nntthetransverse photomacrograph. Cracks intercepting the cladding at'---,

I .A16W

f~

S.,~~~~~~~~~~~~~~~~~~~I

*~~ II *rn'

I IN '000- rl_� '-I

FIGURE 44. Transverse Photomacrograph of Sample N-9C-CHigh Power Region

angles of less than 450 were gnored. The area per unit length of

the transverse cracks was estimated by equating the sum of the

cracks to equivalent diameters, calculating the number of equivalent

cross-sections in the sample, multiplying by two for the two new

surfaces, and dividing by the length of the samplps.

* Third, the area/per unit length of the new surfaces generated during

commercial operation can be estimated by summing the estimates of

the area of the longitudinal and transverse crack areas as described

above.

* Fourth, the area per unit length of the original pellet was deter-

mined by summing the cylindrical and end surfaces and dividing by

15.2 mm (the original length of the pellets).

* Finally, the total fragment surface area per unit length can beobtained by summing the totals for-the new surfaces and the originalsurfaces. - -

4.10

.4

*t. �..

",' .**

i-A-~~~~~~-

.FIGUEA.5.Lonttudnal hotomacrograph of SmleI-9High Power Regin

IK' I..

4.'1

�

I�r

L

4. 11

'Si

I~ mm /

FIGURE 4.6. Transverse Photomacrograph of Sample N-9C-IGrid Spacer Area in High Power Region

'-.1

4.12

FIGURE 4.7. Longitudinal Photo-macrograph of Simple,?4-9C-K :Grid Spacer Area of High PowerRegion -

U -�., N

9*

e�

'. �..i *a $

.*.-.

* 'I

* . It � � -�

-�

\�'1n�<i.

�f7�%.1 V. -'� -I � �.

.*- ; .* *

.. *. .4 . .

.

- - - -. �'.j 4.

4A3 ",--.

The estimates of the surface areas per unit length for the N-9C-I/K and

N-9C-C/F pairs are listed in Table 4.5. At this stage of characterization of

ATM-lOl, it is considered fortuitous that the newly generated surface areas

correlate with the burnup/power levels in the samples. More samples arerequired in order to provide a statistical basis for such a correlation.

Examples of the porosity distribution in the N-9C-C, N-9C-F, N-9C-I, and

N-9C-K samples are illustrated in Figures 4.8, 4.9, 4.10, and 4.11, respec-tively, as a function of fuel radius. The larger pores evident in most of the

photomacrographs are typical of the porosity caused by using a pore-former dur-

ing fabrication of the fuel. The significant amount of relatively small poro-

sity near the edges of the pellets that was observed in most of the pellets is

apparently a combination of original porosity (relatively rounded porosity) and

grain pullout during sample preparation (angular porosity). lntergranular fis-

sion-gas-generated porosity is evident near the centerline of the fuel in the

N-9C-C/F pair of samples, but was absent in the H-9C-I/K pair. These observa-

tions indicate that the power was just sufficient to cause diffusion of xenon

and krypton out of the grains to the grain boundaries in the N-9C-C/F pair and

was not high enough to cause gas diffusion in the N-9C-I/K pair that operatedat a power level approximately 12% lower than the former pair. There was also

more evidence of noble metal fission product agglomeration (Figure 4.12) in the

higher powered region, samples N-9C-C/F, than in the slightly lower power

region, samples N-9C-1/K.

The ceramographic sections were etched using argon ions in a cathode

vacuum etcher to determine the grain structure and grain size. An example of

the etched structure is shown in Figure 4.13. There was a general increase in

the size of the grains from the outer edge of the fuel pellet to the centerline

for both the N-9C-C/F and N-9C-I/K sample pairs (Table 4.6 and Figure 4.14).

The grain size increase was greater in the higher-powered -9C-C/F pair than in

the slightly lower-powered N-9C-1/K pair.

Oxide thickness measurements were made on the as-polished samples. The

results of these measurements on the inner and outer surfaces of the claddingfor samples N-9C-F and N-9C-K are listed in Table 4.7. There is a trend for an

increase in the thickness of the outer, uniformly thick, oxide layer with

-4.14

C ( C C C C C C, C r C

TABLE 4.5. Summary of Estimate of Fragment Areas per Unit Length of Fuel Rod

-. Major Longitudinal Major Transverse Length of __ _

4N

a l

Section 'Cracks, Cross-Sections, uI Longitudinal Longiltudina

-Nbo_. ' Equivalent Radii Number Section. mm Cracks(C)

Exaeninations In progress

_ N-'5C-C :- a , - 84:N-9C-F 6.25 28 -

N9C-I 8 -- 74,N9C-K , 7.50 29

' 'N-9-E .'.J

N- U0 '' Examinatlons In progress

N-96-T ,K-g9-R '

-a) Oetermined by counting'major crack equivalent radlli.(b) Determined bycounting major radlal transverse cracks plus cracks of <451

ohe-half a major radial transverse crack.(c) Area'- (number equivalent radlI) (4.65 mm radius) (2 aides) (1 mm length).

(d) Akea (number-',equivalent'cross-sectlons), (7) (*.05 2mm2 radius) (22 sides) -

'f(rea 'cv1nrical surface) + :ariea.ends) 38 mm(6) Area'- 15,2 'm pellet length mm

I

Area. mm2 /mmTransverse Total OriginalCracks(d) Cracks Surf aceee)

-

30

35

114

109

38

38 - 147

, .."

TotalFragments

, 152

to tube wall belng equivalent

(length of speclmen)-

(length of specimen)'

to '

$ b~~~~~~~~J

* ~ ~ .'' 1.,.~~~~s** il

49.

PA~ ~~~~ .%.~*'*~

- *~~~ entelin

-

99

<.9I

� -'

I S.

S *

* , b

'

S.

a-a e.

SQO O

*1 .4>

L4zj40 urna

b) 1/3 Radius

FIGURE 4.8. As-Polished Transverse Sample N-9C-C(Neg. Nos. N-4700 through N-4704)

4.16

ru :: j : i9s- ^

by '. 0 7..=

Ad - 3 -; ; .; --r In ,;s~~~'a

v

�-

* . 4

* a

U.ft . .1

A - -

S

* B. U* d

I ..

S

I

_P

'.L---- J .

40pm

c) 2/3 Radius

A.. - ~ ~ * .. .*

4%

0. ,.' ~~~ ... * B. C sa g~% . *'."

- . # - . * , . I - .

. b~~~~~~~~~~4' ~ ~ ~ 1

* qt' LJ. * a.,. -~V.

~~ ' ~ ~ ~ ~ ~ * * 0p

-.. d) geI

-. F IGURE:-48 4 Co-td)

4.17

P*. Pt --- 4--4 0 .. . 0** . .. 0*~~~ ~

.4 . '0 * 0 ~~~~ ~~~ ~~~~~~~~~~~~~~~~~~~~. 0

*. ..' .. S.. ..... *0 4 * ..~~~~~~~~~~~~~~~~~~~~~41- * . .4 k~*

. .* 4 .. .~~~~~~ .. *. b~~~S

P. ~ ~ ~ ~ ~ ~ *f 4.4 4 * .b.?..~~~ ~~~~~~~ P1,

* * 0*.'** * 0 -~~~~~~JP P

POP.4* a * 0*~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .0~~~~~~~~O

S * .44 40#

V .. * .*a Centerline

-~ * . . * 5

; ~~* l *; ; S -

E* X i* . **H

: e *e- * . ;:

4 ~ ~~~ , .9. ', ', .

S ~ ~ ~ ~ *9 ' , '-. ;. ,

'_* - 0 - 0 ; .'H ,

,¢_-'"'*''. '-'-s*12-' s '

-. ~ (Ng Nos N-78 thog .7

4.18~~0 4

.9., I.

1.60I~~~~~~~~~~~~~~~~~C

* 4 .4

9 . I C

.* - 9-

I

a 4 O .m

c) 2/3 Radius

-d. Edge

FIGURE 4;9. Contd)

-z -+ -z e -;4 * --'

. A I ':

; .1. .I : ..

9

s *

*~ -

i

e

I

I.

4

F ~ ~~f

0+**a; HAv:

: F "' '

f

'A *

U0.

9

a) Centerline

- el__ - - I

" I X Sa

9

0 1I . - I

.

I *. -. 6p

S.

*'.;

* F

. :p4Opm

'-.d

I . P. *.0

.9 a

* 0S

'p. 9*9b) 1/3-Radius

FIGURE 4.10. As-Polished Transverse Sample -9C-I(Neg. Nos. N-4706 through N-4709)

4.20

.. 4,

: * ' f I': . <:

i:'

w r w4.- - -

* . . 9 :-' .

* . ,.

* ~~~- .9~ ,.- ..

: 9 .I : . * ,. t ' * *~~*

t

* - ,.

9 . .9.. .

* VW

,* 4Opm) * . . .

T, . ..

. _1 1

_I ;

. IV

i. -0.,

*- V .

_ V

~~ L ' .~~~

tj,:

v

c) 2/3 Radius

4~ ~ *s$

*" * g' 5

'i) Edge

', fIGUtRE4.1O. .Contd).

4.21

4

* 4'9 S-'5

-Fw � � ., -. -�

I � �

B �

4.9

-

4. -

9 -I

4 I

I *

4 4 4#mn

a) Centerline

S

0

Olu%P

,*4, .I .0 - . - .

9 -~~~~~~

I .. . .

., x,>V . a

a. t

* , ' !~~,

B -

I~~~~~., *4

* ' v

90 ., .*.' B

P . i_ *,4-, I .4.f.Pm,

b) 1/3 Radius

FIGURE 4.11. As-Polished. Longitudinal Sample N-9C-K(Neg. Nos. N-4679 through N-4682)

4.22

t

(

*

1�

S

1

a

4.. ¶sS �

l''* �4'<� .4 . a4

* . 4

,t� let V. a a*.1

'C..

- 'I; 0

: * .

I .

..I

I

a. .

: . I <

t f a.' . . . - ,E ' .'' s ;'-, t., '

- 4 .; ' , F a ;* S > .

. . ~ *

I

.

.

. .

.

' -.:. 5

* 4

* ; -q '

i'' .* *

[0g

-, -

. I I

. 4. ' L

--- - - c) 2/3 Rad~us

,9 _ , '. ' - * . ... .. -- a ... . , - - ' ,* -

V, _ * * . -, ; . .V p. * .. *; _

4-~~~~~~ ~ ~~~~~ w%"* ' ' . ! ?

'4:_i_ -- -- a

, L I *,I

d) Edge

FIGURE 4.11: . (Contd)

4.23

a -'T��' S.. a

S - d

* U'a - *

p * . 4 4I 4A

aA ** *A� V

-� *'a -V -

I *

* 4-I -. a'

U�- *.s A

� I

4 t*' S A*S A'a.

lI�D. 4

a,a

I #.

S

I

x 4ft

I

A.

- a) Sample N-9C-C (eg. No. N-7404)

e i. w

* x I

..... . . .

-. t:

.

. . . * , . . .

.. . .

+

. . w..

.

.

t .! ._,

b - t

I

I

P I_0p

l0oum

b) Sample N-9C-I (Neg. No. N-4710)

Noble Metal Fission Product Agglomeration (light-coloredspots) n Samples from a).Central High-Power Region ofRod N-9, and (b) Grid Spacer Region at 12X Lower Power

FIGURE 4.12.

4.24

TABLE 4.6. Results of Fuel Grain Size Measurements(8)

Grai.n Sze at Fractional Radius) m :-

Section Centerline -1/3 Radius 2/3 Radius _ Edge _

No. 1tiii

N-9C-C

W-9C-F

N-9C-I

N-9C-K

N-9B-C'

N-9B-E

N-9B-0

N-9B-M

tercept True

5.8 9.1

6.5 10.2-

5.0 7.8

5.8 9.0

intercept-- 5.1

6.1

4.9

5.0.

* True8.0

9.6

7.7

7.8

- ntercet True- Intercept

3.9 6.2.- 5 '3.9

-5.1 8.0 -;- --

True

6.1

5.9

5.93.9

3.9

6.1 . 3.8

6.1 - 3.8

Examinations in progress

N-9B-T

n-9B-R

C-5C-B

C-5C-F

(a) Intercept' grainsike determined by I11ne ntercept method from ASTM E 112.

'True' grain sze equals-the 'intercept' grain size multiplied by 1.57.

14~~~~~~~~~~~~~~~~.

4.05

vS

a) Centerline

b) 1/3 Radius

FIGURE 4.13. Ion-Etched(Neg. Nos.

Transverse Sample N-9C-CN-4757 through -4760)

4.26

c) 2/3 Radius

~~~~A,

40p

d) Edge

' FIGURE 4.13. (Contd)

4.27

12

10

U) N-9C-l

4

0 0.25 0.50 0.75 1.00Center Une Fractional Radius Edge

FIGURE 4.14. True Grain Size of Fuel as a Function of Radiusfor Four Samples from N-9C

increasing elevation in the assembly, as would be expected for PWR fuel. The

outer oxide was layered and tended to be cracked in a direction parallel to the

surface of the cladding (Figure 4.15). The inner oxide layer aried signifi-

cantly in thickness (Figure 4.16); in some places it was not observed. In some

cases the inner oxide appeared to be spalling away from the zircaloy cladding.

The cladding was etched with B-etch" (45X glycerine, 45X nitric acid, and

1O hydrofluoric acid) in order to check the hydride orientation. Examples of

the hydride orientation is shown in Figure 4.17. The hydrides are primarily

oriented as platelet-type stringers in the longitudinal-tangential direction.

4.6 FUEL BURNUP MEASUREMENTS

Burnup analyses were completed on five samples from rod -9 at positions

representative of five burnup levels. An additional random burnup sample was

4.28

C C C ( C' C r C C C C

0

TABtE4.7. .Outer

Approx a te. 'Axia 'Lo cation, -.

Sset on cm ( n)' from 'ppNo., 'Bottom 6*'F'ual Stack Typical

N-9C-K i 198" (78)" . : 15.2 (0.60) +1.

N-9C-' ; 2288.) 19.8 (0.78) ±2.

N-9B-k '05'o(41. )

N-9B:M4 '- . ';25 ('t.8)' .I;___________ J. , 'z ;Examinations In

N-BQ -- 12 (4.R8v.

--Ct 'X >'217 {85) " :

a.) TjpIcaM where pre4ent.-

L..l

and Inner Oxide Thickness in ATM-lOl Rods.;

Oxide Thicknessi.mmfln) x IOuter Laver #,InCu LUY

,roximteRanne.0 (0.04)

.0 (0.08)

__. __ -. roxilmte-Comments ' Typical Range

Uniform thickness, 9.7 (0.38) ±9.7 (0.38)layered, often :cracked '

CommentsVaries signifl-cantly In thick-ness, solid oxide

Uniform thickness, 4.4 0.17)(a) +2.5layered -4.4

(0.10) LocalIzed,(0.17) spalling

progress

J * 9

. 'i

a) Sample N-9C-K Neg. No. N-5006)

a I

I . I , .

I I

.i

b) Saple N-9C-F (Neg. No. N-4995)

Examoles of Outer Surface Oxide-onFIGURE 4.15. ATM-101 Rods

40'30

. 1 .~ I - .11 '' - . l- o- I ,- e e I .; M ,;i

N-9C-K (Neg. No. N-5012.: .- -a) Sampl e

I- "i -1I ,:' .Z -

. ~~~~~~~~~~~~

b) Sample N-9C-F (Neg. No. N-5001)

FIGURE 4.16. Examples -f Inner Surface Oxide from Rod N-9C

-.. -

4.31

- -

a) Transverse Sample -9C-C(1SOX) (Neg. No. N-5015)

b) Longitudinal Saiiple N-((Neg. No. 14-50031) X-F~~~-

5Opm7

FIGURE 4.17. Hydride Orientation in Rod N-9C Cladding

4.32

taken from rod C-5. The burnup samples were taken in order to correlate with

137Cs gamma scan results to predict the burnup and radionuclide content of any

particular specimen of ATM-101 that might be provided to a repository experi-

menter. The burnup analyses were performed by Hanford Engineering Development

Laboratory CHEDL) according to ASTM Standard E 321. The results are listed in

Table 4.8. The results of the burnup analyses are compared to the 137Cs counts

taken during 300 s (Section 4.7), at the location of the burnup sample, in Fig-

ure 4.18. BurnUp values based upon 137Cs are also listed in Table 4.8. The

good correlations between 137Cs and burnup, and the burnup values based upon

148Nd and 137Cs, indicate that the 137Cs has not migrated axially to any

significant degree, and therefore, burnup values determined by ntercomparison

of '37Cs gamma activities between rods is valid for ATM-101.

120

. § 100

8) 80

c:. , 'C

c 60 -

40~ ~~~~~~'

0

~ 0

U . 9 /

r 20 _ -'9

0 10 20 l 30

Burnup, MWd/kgM

FIGURE 4.18. Correlation Between Burnup Analyses and 137Cs Gamma Counting

4.33

WALE 4.8. Burnup Results for ATM-101 Samples(a)

SpecimenNo.

N-9C-D

14Burnup(148Nd basis)

At. MWd/kgM3s32eC 1 366 C)

Burnup (137Cs fbasis)Wd/8gM

31.8

Sample Location

Typical peak burnup ncenter segment ofrod N-9.

N-9C-J 2.98(c) 28.47(c) 27.9 Burnup in grid spacerlocation of rod N-9.

N-9B-D Typical peak burnup inbottom segment ofrod N-9.

N-9B-N

N-9B-S

Representative ofapprof[rately 75% ofpeak 1 1Cs activity inbottom segment ofrod N-9.

Analyses in progress

Representative ofapproj~Tately 50 ofpeak Cs activity inbottom segment ofrod N-9.

Typical of peak burnupin rod C-5.

C-5C-D

(a) See sectioning diagrams in Appendix B for sample locations with respectto gamma activity.

(b) Calculation based upon 37Cs half-life of 30.174 yr and effective fissionyield of 6.138S.

(c) Results listed for specimens N-9C-D and N-9CW are the average twoanalyses. Ranges were 0.07 at (0.70 MWd/kgM) for N-9C-D and 0.02at X (0.15 MWd/kgM) for N-9C-J. *'0

4.34

This burnup-137Cs activity correlation is

Ai-. U~i B.U.N-jNN9D D

N-90

(1)

where B.U.1 = the burnup for the portion of the rod in question, MWd/kgM

B.U.N-9D the average of the two analyses for the burnup sample N-9C-D

31.7 MWd/kgM

A = the average 137Cs activity for the portion of the rod ini~~~~~~~~~~~~~~~~~~~~~~~~~~~~

question, counts per 300 s

AN-9D = the average 13 Cs activity for the burnup sample N-9C-D = 112,496counts per 300 s

This burnup value can be used in conjunction with the radionuclide inventory

calculations in Section 4.8 to determine the radioisotope inventory for a par-

ticular portion of specimen that might be used by an experimenter.

In order to determine the average burnup in a particular fuel rod that is

required for the fission gas release calculation (Section 4.4), a modification

of Equation 1 ws used. Normalizing factors for determining the rod-average

burnup in rod N-9 nd the relationship between rods were used, i.e.,

AN-9 AiCU=B B.UN-9D - - (2)

N-9D N-9Cwhere FJJ1 = rod-average burnup for the rod in question, MWd/kgM

B.U.N-9D = the average of the two analyses for the burnup sample N-9C-D

31.7 MWd/kgM

AN-g = the average 137Cs activity for the entire rod -9 = 100,926

counts per 300 sA ~~~~~~~137Csatvt o o unpsmlN-9D = the average * Cs activity for for burnup sample N-9C-D = 112,496

counts in 300 s

A4-C = the average 137Cs activity along the length of the center segment

of the rod in question, counts per 300 s.

= the average 37Cs activity along the length of the center segmento 9Cof rod N-9 = 110,259 counts n 300 s

4.35

or,

w:T. 1 = 2.58 x 10 4 n c) (3)

The results of this calculation for the nine rods in ATM-101 are tabulated in

Table 49. For those rods for which the center segment has not as yet been

gamma scanned, AC has been assumed to be the same as for segment -9C and the

rod-average burnup value is shown as preliminary in brackets.

It s noted that the AN to ratio (0.897) is very close to the peak

to assembly-average burnup ratio (0.894) previously reported (Einziger and

Fish, 1982). It is also noteworthy that the burnup and 137Cs counts for sampleN-9C-D, in the typical peak burnup region, and sample N-9C-J, in grid spacer

region, agree within 0.2X, .e, 31.16 MWd/kgM and 112,496 counts vs.

28.47 MWd/kgM and 101,348 counts, respectively.

TABLE 4.9. Rod-Average Burnup in ATM-101 Fuel Rods

RodNo.

C-5

0-10

G-9

G-13

J-12

L-8

N-4

N-9

N-12

Centr?7Segment- Average Cs ActiviAt c' Counts per 300 s)

109,416*

*

116,341*

110,256

113,833

Rod-AverageBurnu

~a)MWd/kgMza

28.2

[28.4]

[28.4]

[28.4]

[28.4]

30.0

[28.4]

28.4

* 29.4

(a) * Value assumed to be equal to that for N-9pending gamma scan result. Preliminary burnupvalue in [].

4.36

4.7 GAMMA SCANNING RESULTS

Each fuel rod segment was gamma scanned axially in the HEDL hot cells

using germanium-drifted gamma-ray detector. In most cases, the same counting

geometry, counting equipment, analyzing equipment, and data storage equipment

were used for each measurement. Because of changes in an electronic package

and a resulting change in calibration, it was necessary to determine a normali-

zation factor for some'of the gross gamma scans by counting segment N9T with

both electronic packages.

Initial spectral counting of the high activity regions of the fuel showed

only one large peak corresponding to the 662.5 Kev 137Cs gamma ray. Several

other very small peaks were observed. Of these the 605.5 and 796.8 Kev peaks

for '34Cs and the 724.1 and 1275.0 Kev peaks for 154Eu were adjudged to have

sufficient activity to record. An additional peak at 98.6 Key, possibly 241Am,

was also recorded. Of the axial gamma distributions that were recorded, the

gross (total activity), the 137Cs (606.5 Kev), the 134Cs (605.5 Kev) and the54Eu (1275.0 Kev) data had adequate counting statistics to be published. The

individual plots, for each fuel rod segment that has been scanned to date are

shown in Appendix D. Composites of the individual scans for the bottom, cen-

ter, and top segments of rod N-9 for the gross and '37Cs scans are shown for

illustration in Figures 4.19 and 4.20. Of note is, that even using a rela-

tively wide slit width of 2.5 mm (0.100 in.) and steps of 2.5 mm (0.100 in.),

the pellet-pellet interfaces and associated dishing are easily distinguished as

sharp dips in the gamma activity on an approximate pellet-length pitch of

15 mm, even in the central higher-power regions of the fuel rods. The axial

locations of the grid spacers in the BO-5 assembly are also easily distin-

guished as a general activity decrease of approximately 10X over severalcentimeters in length.

Several segments exhibit nonsymmetric, relatively random decreases in the

axial gamma activity distribution, indicating the presence of localized regionswhere there is a decrease in the effective density of the fuel. For those

localized regions where the activity changed drastically in the first few cen-

timeters of fuel from the end of the segment that was sectioned prior to

shipping to PL, the activity loss can be attributed to fuel fallout during

4.37

DISTANCE FROM BOTTOM. In40 60 so to0 20 120 140

a

in0

Cs0Cn0L

-

2

C0

V

.-5:Ir-

7

6

5

4

3

2

1

co

00 50 t0 150 200 250 300

DISTANCE FROM BOTTOM. cm

Composite of Gross Gamma Scans for Rod N-9

- 350 400

FIGURE 4.19.

C ( (. ( ( C ( C ( ~~~~ f

C C

14

I 12

. 0:, O

0 To

L4-

Ii

0= 6

a:4

;< 2

0

c ( C C C ( Cc ( c ( C

20I DISTANCE FROM BOTTOM. In40 60 so 100

* Z4ED

0 50 100 150DISTANCE

200 ' 250 300

FROM BOTTOM. cm350 400

FIGURE 4.20. Composite of Cs Gamma Scans for Rod N-9

handling and/or shipping. Where activity decreases occur away from a sectioned

end of a segment, the region of low activity is assumed to be due to a small

amount of in-reactor densification and minor rearrangement or settling of the

fuel stack during commercial operation. These regions of low activity due to

in-reactor densification are tabulated in Table 4.10.

A portion of the center segment of rod C-5 was gamma scanned with a narrow

slit, .e., 0.25 mm (0.010 in.), in an effort to determine if any significant

137Cs migration had occurred during operation. This slit width probably

approximates the sum of the dish depth in adjacent pellets, although the

as-built geometry of the dishes has not been published. Axial steps of 0.25 mm

(0.010 in.) and a counting time of 1000 s for each step were used. The results

of the scan over approximately four pellets is shown in Figure 4.21. Whereas

the nterpellet activity dropped approximately 4 with the wider 2.5 m slit,

the dips in activity with the narrow 0.25 mm slit were about 30X. The latter

approximates the decrease in activity that would be expected from the missing

fuel associated with typical dishes. Therefore, it is concluded that no signi-

ficant axial or radial migration of 137Cs occurred during the commercial'opera-

tion and that the 137Cs activity is appropriate for use in normalizing burnups

between rods (see Section 4.6).

4.8 RADIONUCLIDE INVENTORY CALCULATION

The radionuclide inventory in the ATM-101 spent fuel was calculated using

the ORIGEN-2 code (Croff, 1980) for functions of burnup level (power level) and

decay time. These inventory calculations were performed to permit estimation

of the source term for any particular portion of ATM-101 that might be used in

an experiment. Calculations were made for burnup levels from 10 to 35 Wd/kgt4

in 5 MWd/kgM increments with decay times of 10, 12, 14, and 16 years, i.e., the

period over which ATM-101 is expected to be used in radionuclide release

experiments. The ORIGEN-2 results provide inventories of both the actinides

and fission products in units of both grams per gram original uranium and

curies per gram of original uranium. Appendix E provides tables of the inven-

tories at the six burnup levels and the four decay times for individual

4.40

TABLE 4.10. Regions of Apparent In-Reactor Densification and Fuel Setting(a)

RodSegment

No.

C-5-B-C-T

D-10-B-C-T

G-9-B-C-T

G-13-B-C-T

J-12-B-C-T

Regions of Apparent Densificatlon, and Settling,Distance from Bottom of Fuel n Segment, cm (in.)

11.7 to 29.2 (5.4 to 11.5)

0 to 11.4 (Oto 4.5)L-8-B

-C-T

N-4-B-C-T

N-9-B

-C*-T

N-12-B-C-T

80.8 to 85.6 (31.8 to 33.7), 89.7 to93.5 (35.3 to 36.8)None0 to 7.1 ( to 2.8), 61.5 to 65.0 (24.2 to25.6), 78.2 to 83.8 (30.8 to 33.0), 102.9 to105.7 (40.5 to 41.6)

None

(a) Blank spaces indicate examinations not currentlyscheduled. ;

4.41

DISTANCE16

FROM BOTTOM, in17I5

4 I I I

c5c Cs

I - - -

co

x

0a

0

M

WV

0.r.

cto

u

3.5

3

2.5

2

1.5

1

0.5

0 I I I I I b38 39 40

DISTANCE41 42FROM BOTTOM.

43

cm44 45

FIGURE 4.21. 137Cs Gamma Scan of Rod C5C with Narrow Slit and Small Steps

C ( ( ( ( ( ( ( 4? (,~~~~

isotopes and the elements, as well as listings of the sources of neutrons. A

concentration cutoff of 10 units was used to reduce the listings to a

manageable level.

An estimate of the amount of an isotope or element of interest in a par-

ticular specimen sample can be determined from a knowledge of the fuel burnup

(Section 4.6), weight of the specimen sample, and linear interpolations between

1) the burnup levels that bracket the actual burnup, and 2) the decay periods

that bracket the decay time of interest. For example, if the one is interested

in the curies of 233U in a 10 sample of U02 at a burnup of 28.0 MWd/kgM in

November 1987, the inventory is found as follows:

* The tables that bracket the burnup levels for actinides in units of

Ci/gUl are determined, i.e., Tables E.4.c (25 MWd/kgM) and E.5.c

(30 MWd/kgM).

* The inventories per gram uranium of 233U after a decay period of

13 1/2 years are determined by linear interpolation between the 12

and 14 year data columns for both burnup levels, i.e., 1.540 x 10-11

CI/gU at 25 MWd/kgM and 1.874 x 10-11 CI/gU at 30 MWd/kgM.

* The inventory per gram uranium of 233U at the specific burnup of

28.0 MWd/kgM is determined by linear interpolation between the

burnup values, i.e., 1.740 x 10-11 Ci/gU.

* Finally, the total 23 3 U inventory for the specimen is determined,i.e., (1.740 x 10-11 Ci/gU) (10 g) (0.881) = 1.533 x 10-1 Ci.

Note that the inventories are listed in units per gram of uranium. Therefore,

if the weight of the specimen sample is in units per gram of oxide, the listed

values need to be multiplied by 0.881.

4.9 RADIONUCLIDE CHEMICAL OVERCHECK

A few isotopes from the ORIGIN-calculated inventories listed in Sec-

tion 4.8 were compared with chemically determined inventories. The isotopes

that were planned for chemical determination for this overcheck were 235239pu, 237Np, 99Tc, and 137Cs. The 235U and 239Pu were determined as part of

the burnup analyses using ASTM Standard procedure E 321. Analyses for 237Np

4.43

are currently still in progress. The 9 Tc was determined using a combination-Ion-exchange and solvent-extraction separation procedure and beta counting oncalibrated thin-window gas flow proportional counters. The 137Cs analyses weremade using ASTM Standard Procedure E 692. Analyses for these Isotopes havebeen completed for two of the five samples from five burnup levels in rod N-9.

The analytical results are compared to the ORIGEN-calculated inventoriesin Table 4.11. Values of other radioisotopes routinely determined as part ofthe burnup analyses are also tabulated in Appendix F. The analytical resultsare within ±10' of the calculated results, indicating that the ORIGEN-calcu-lated results can be used for estimates of the radionuclide inventory inATM-101 specimens for radionuclide release studies.

In addition, because the original nitrogen content (the source of 4C) ofthe fuel was unknown, the 14C content of a fuel sample and a nondecrudded clad-ding sample were determined, and are listed in Table 4.11. The 14C was deter-mined by a total combustion technique in an induction furnace at 13000C. Thereleased gases were passed over a catalyst for conversion of any CO to C02, andthen trapped in a basic solution for counting in solution by liquidscintillation.

4.10 PERTINENT RESULTS FROM SIBLING RODS

Several nondestructive examinations and destructive examinations have beenperformed on sibling rods from Assembly BO-5. The results of these examina-tions are discussed below and were primarily taken from the summary of Einzigerand Fish, 1982.

4.10.1 Nondestructive Examination Results

Visual examinations were performed for defects and crud deposits oneighteen fuel rods from Assembly BO-5 in the Battelle Columbus Laboratory (BCL)hot cells. Below approximately the 320 cm (130 in.) level only light axial

scratches were observed during the assembly dismantling process. The crud inthis region was very light and almost unnoticeable. Above the 320 cm levelthere was a relatively heavy crud deposit on all the rods.

4.44

(s c c ( C

:~~~~~~~~~

TABLE 4.11. Comparison of Chemical Overcheck Results to ORIGEN-Calculated Radionuclide Inventory

RadlouWclide Intw,-35U *n filct) Ow& (OeXid) Z37u i l CSe. Cl/I exIdo 1 Ic l/ (ide)

Smple bursu. la) ncicMA, ancts)oimb AR1ytca AnltA A-nalytIn(I 1 calW" naxibctiacya.aNow piWditoqM I~~~)oIub) ~ nltc 0RGIua WTE Anaytial 01KGEN TFAayia l~gb)~7g AAI)-fjy N-9C4 31.6 4.86 0.99 4.20 x 103 4.47 ' 0.940 - 713x i

20 1 .09 03

11-9c- 28.47 g.z x r3

S.s6 a 1w-3

i.Oio 4.51 x 1034.41 103 .1.030 6.27 a 1ig2 6.27 a 10-2 1.00 . a 0-4

9.96 a 10-S 2J99

11.9114

1.99414sb* 11911-54. b

7 1OCS 31.6 - - - - - - -- - - - 3 I

N-9C Cladding SA - - - - - - - - - 4. 100

7.) Fran analytical beN analysis. Table F.. ib) Frae Rl;EIs runs, pendix E. Valves re from a linear lerpotation batw* nearest burnu levels. xItPlied by 0O. to

corect t basis of original xide weght. and a tn year dcay period.

Diameter measurements were also performed in the BCL hot cells on eighteen

rods from Assembly BO-5. A spiral profilometer was used to make the measure-

ments. The amount of creepdown.o6er the central two-thirds of the length of

the rods was apparently about 0.7 percent, i.e., 0.076 mm (0.003 in.), based

upon the preirradiation diameter. No evidence of ridging at pellet-pellet

interfaces was observed. The position of maximum ovality in the cladding of

the rods was routinely in the upper 10X of the fueled length.

Gamma scanning results were also carried out on several rods at BCL, ANL,

and LANL. The results were similar to those obtained for the ATM-101 rods

(Section 4.7) except that fuel stack heights were determined for the nonsec-

tioned sibling rods. The stack heights in eighteen rods measured at BCL was

very uniform in length, 365.5 1.0 cm (143.5 0.4 n.). On the average the

stacks contained 6 3 large pellet-pellet gaps. Pellet-pellet interfaces were

easily discerned when the counting geometry and statistics permitted

resolution.

Eddy-current examinations were conducted by BCL on eighteen rods from

Assembly BO-5. Cladding defect indications were found on only four rods.

Indications in two of these rods correlated with large pellet-pellet gaps. The

eddy-current indications in the other two rods did not correlate with any known

feature, and may be actual defects. The signal from one rod, P-4, indicated a

very long-length defect, e.g., about 7.6 cm, and apparently the source of the

signal was a longitudinal defect on the inner surface of the cladding. This

type of signal is not typical of more common defects, e.g., pits, holes,

hydride cracks, and pellet-cladding interaction type cracks, and may represent

an as-fabricated tubing defect that was not detected.

4.10.2 Destructive Examination Results

Gas analyses were performed on the fill gas from 28 sibling rods from

Assembly BO-5. The results from the rods are compared to the data from ATM-101

rods in Table 4.12. The results from the two data sets compare very favorably.

Metallographic examination of the cladding from two sibling rods was per-

formed by EG&G-Idaho. Hydride precipitation was primarily circumferentially

oriented. The thickness of exterior and interior oxide formation was measured

4.46

'4

TABLE 4.12. Comparison of Fission Gas Data from Nine ATM-101 Rodsto Data from 28 Sibling Rods from Assembly BO-5(including standard deviations)

Void Gas Volume, Gas Fission Gas

Volume, cm3 cm3 STP Pressure, MPa Release,

Sibling rods 24.7 1.5 370 10 1.52 0.10 0.21 t0.05ATM-101 rods(a) 21.9 1.3 366 5 1.69 t0.10 0.20(b)

(a) Computed from acceptable data from Table 4.2.(b) Sufficient burnup data not available to compute actual average and

standard deviation

along the length of the fuel rods. The data are depicted in Figure 4.22, along

with the external oxide thickness determined for two samples from rod N-9. The

exterior oxide thickness increases with height along the rod, as expected due

to increasing coolant temperature up the rod. The results for rod N-9 tend to

be slightly lower than results for similar rods. No evidence of nodular

oxidation/corrosion was observed.

Cladding microhardness measurements were made at BCL during the effort to

estimate the assembly temperatures during the handling incident (Section 4.3).

The Knoop hardness with a one kilogram load was measured at five axial loca-

tions on six rods with indentions both parallel to and perpendicular to the

radius of the cladding. No significant differences in hardness were observed

either between rods, at the different levels, or in the two directions. The

average microhardness was 250.

Tensile specimens from the cladding of several rods were also tested at

BCL over the temperature range from 27 to 371°C. Strength and elongation

values are listed in Table 4.13.

Ceramographic examination of the fuel was reported by EG&G-Idaho and ANL.

Transverse ceramography indicated formation of from four to thirteen fragments

with the cracks oriented primarily radially. There was some indication of

grain growth in the fuel, from 4 to 7m diameter at the centerline of speci-

mens taken near the midplane of the rod. This result compares favorably with

4.47

mm0.0150.025 0.020 0.010 0.005

160

140

C0

0E04-

0to

E0

U.0UC

a

1201

1001

801

0 Rod 0-14 External Oxide0Rod K-4 External Oxide

- VRod N-9 External Oxide (ATM-101)ARod K-4 Internal Oxide

I I I _ ~ I I I I _.

�.o

0

1400

_ 300

1 200 cm

601

401 100

201

nt on1.1 1.0 0.9 0.8 0.7 0.6 0.5 0.4 0.3 0.2 0.1 0.0

Oxide Thickness, inx 10

FIGURE 4.22. Oxide Thickness Variations Along Zircaloy Fuel Rod fromH. B. Robinson Unit 2

TABLE 4.13. Strength and Elongation Values for Claddingfrom Assembly BO-5 Sibling Rods a

Temperature,°C *30

27

93

204

316

371

Strength, MPa (ksi)(b) Elongationultimate

974 (141)

907 (132)

799 (116)

685 (100)

659 (96)

0.2 Offset815 (118)

750 (109)

659 (96)

578 (84)

528 (77)

Uni form

3.37

3.73

4.01

2.59

3.63

T Total6.01

6.57

6.74

6.29

1 2 . 6 (c)

(a) Average of three measurements at strain rate of0.005/min to yield and 0.025/lin to fractyre.

(b) Based on tube area of 0.19 cm' (0.029 in. ).(c) Based on only two measurements,

'la

4.48

la

the "intercept" grain sizes determined for rod N-9 (Table 4.6). The presence

of large pores indicated that the fuel had been fabricated using a pore-former.

Both PNL and LANL conducted radial microprobe measurements on fuel from

Assembly BO-5. The distributions of plutonium and ruthenium peaked near the

outer edge of the pellet, while technetium, barium, cesium, zirconium, iodine,

tellerium, and cerium distributions were essentially constant across the

radius. Details for these measurements are discussed in Einziger and Fish,1982.

4.49

5.0 DISTRIBUTION OF ATM-101 SPENT FUEL

Several segments of ATM-101 have been sectioned and distributed to experi-

menters. This section describes pertinent information relating to these dis-

tributed materials. Sectioning diagrams for the segments are provided in

Appendix B.

5.1 CRUSHED MATERIAL FOR BWIP - SEGMENT -9C

The Basalt Waste Isolation Project (BWIP) requested 250 g of ATM-101. The

material was requested'to be crushed to the -60 to.+250 mesh size range, with

material in the -60 to +115 mesh range being preferred. ATM-101 fuel rod seg-

ment N-9C was used to produce this material, along with several MCC characteri-

zation samples. The sectioning diagram for segment N-9C is shown in

Figure B.3.

Material for the crushed BIP fuel was taken from Sections A, G and N.

The material from Sections A and G was first ground and sieved and then the

location of the N-0 cut was determined to provide sufficient material for the

lot. Each cut for MCC samples was made using an Isomet low-speed saw equipped

with a Buehler low concentration diamond wafering blade. The cuts were made

dry, i.e., no lubricant was used. No loss of fuel fragments from the ends of

any of the samples or BWIP material was observed during this sectioning proce-

dure. Sections A and G were cut into approximately 5 cm-long (2 in.) lengths

using a tubing cutter. The fuel in each rod piece was removed from the clad-

ding by striking the cladding with an impactor. The collected fuel was weighed

and placed in a Torsien Model-MG-2 power-grinder. The power-grinder was

equipped with corundum mortar and pestle. The fuel was ground for approxi-

mately five seconds and then sieved through a 60 mesh screen. The +60 mesh

material was returned to the grinder. This sequence was repeated approximately40 times until all the material from Sections A and G passed through the60 mesh screen. After further screening, the quantity of material in thevarious particle size ranges was determined (Table 5.1).

5.1

TABLE 5.1. Description of Initial Run on BWIP Material

Particle Size Weight, g Weight,

(Initial fuel) 287.7 100.0

-60 +115 155.7 54.1-115 +250 61.6 21.4

-250 63.8 22.2

Not recovered 6.6 2.3

Section N was processed in the same manner as Sections A and G. It

required approximately 25 grindings/screenings to reduce the material to less

than the 60 mesh size. Loss of material during processing Section N was not

recorded. The crushed fuel from Sections A, G, and N was combined and mixed by

repeating the screening operation. The quantities of material in the various

particle size ranges for the entire lot are listed n Table 5.2.

The three sizes fractions were separated nto samples/specimens as listed

in Table 5.3.

The crushed BWIP material was also subjected to analyses by inductively-

coupled plasma (ICP) spectrometry and x-ray diffraction in order to ascertain

if there were any significant differences in composition between the three

particle size ranges.

For the ICP analyses, the materials were fused in KOH in a nickel crucible

at red heat and then dissolved in distilled water. A drop of acid was added to

the solution to prevent precipitation. Because the presence of uranium inter-

fered with the individual elemental analyses, a set of matrix-matched standard

uranium solutions was prepared, analyses completed at the appropriate elemental

TABLE 5.2. Description of BWIP Material

Weight inParticle Size Weight, g Weight, -60 to +250 Range,

-60 +115 mesh 221.8 55.2 0.72

-115 +250 mesh 88.2 21.9 0.28

-250 mesh 91.9 22.9 -

Total 401.9 100.0 100.0

5.2

TABLE 5.3. BWIP Crushed Fuel Distribution

* Sample/SpecimfnIdentification aATM-101, RIATM-101, R2ATM-l01 R3

N-9C, R1,222SN-9C, R2, 222SN-9C, R3, 222S

N-9C, RI, MCCN-9C, R2, MCCW-9C, R3, MCC

N29C, RIN-9C, R2N-9C, R3

N-9C, RiN-9C, R2N-9C, R3

N9C, RiN9C, R2N9C, R3

Weight, g Distribution/Location -

166.3 BWIP product'shipped to HEDL - 325 Bldg.32.335.1

30.4 BWIP product stored in D-cell - 324 Bldg..30.3 . for later transfer to Rockwell-222S Bldg.30.9

14.9 MCC archive material, stored in D-cell -15.2 324 Bldg.15.6

1.9 Shipped to HEDL - 327 Bldg. for optical2.2 microscopy -2.0

3.23.02.9

5.15.25.4

Shipped to HEDL/PNL-325 Bldg. for chemicalanalysis

Spare material stored in D-cell - 324 Bldg.

(a) R = -60 to +115 mesh material.R2'= -115 to +250 mesh material.R3 = -250 mesh material.

signals, and'a uranium data fit was produced, using a linear regression

analysis, in order to provide a curve for subtraction'of the uranium backgroundfrom the individual elemental results. The regression coefficient was suffici-

ent'for all the standard elements analyzed by ICP except Ba, Ca, Mg, Na, and

Zn. The results of the ICP analyses are listed in Table 5.4 and the results

for the fission'product elements are shown graphically in Figure 5.1. Ones

initial reaction'to the data is that there might be a tendency for lower con-

centration of the fission products in the smaller sized particles, e.g., theconcentration of Ce, Rh, Te, Ru, La and Nd appear to decrease with particlesize. However, these are the elements for which the largest corrections are

required for uranium interference (greater than one-half the total signal) and,

5.3

TABLE 5.4. ICP Results on Crushed BWIP Material(a)

Concentration,ug/_ of fuel(c)Element(b)

Al

B

Ca

Fe

La

Mn

Mo

Nd

Rh

Ru

Si

Sr

Te

Zr

-

-6U 115 mesn -110 * dou esn -45u mesn

220

806

200

980

260

2500

2780

730

1680

530

260

2330

700 (460)

- (403)

170 (185)

900 (940)

230 (245)

2400 (2450)

2200 (2490)

- (365)

1430 (1555)

510 (520)

80 (170)

2130 (2230)

_ - (-)

_ 190 (95)

350 - (175)

280 32 (156)

980 890 (935)

350 320 (335)

2500 2450 (2475)

2900 1660 (2280)

790 - (395)

1580 1260 (1420)

520 520 (520)

2280 2230 (2255)

1320 690 (1005)

_ _ (-)

_- (-)

170 170 (170)

950 880 (915)

210 220 (215)

2480 2380 (2430)

1920 1950 (1935)

1320 1320 (1320)

2650 2120 (2385)

530 510 (520)

2420 2250 (2335)

(a)Fuel fused in KOH in a nickel crucible.(b) Cr, Dy, Li, and T not detected. Regression fit for

adequate to determine Ba, Ca, Mg, Na and Zn.(c) Values shown are derived from two solutions prepared

1000X dilution; average in parentheses.

interference of U not

at 2000X dilution, and

'-S

therefore, are subject to the largest variability in result. For those ele-

ments with the lowest required correction for uranium interference, i.e., Mo,

Sr, and Zr, there are no significant differences between the three particle

sizes. There is not sufficient information to absolutely conclude that there

was no significant segregation of the radionuclides during preparation of the

material; however, given the relatively moderate operating temperature of the

fuel and minor amount of fission product migration observed in the fuel mate-

rial, it is likely that most radionuclides are in solid solution in the U02 and

it is probable that there was no significant segregation during preparation.

The source of the Al and S in the smallest sized particle fraction was

probably the grinding material used n the automated mortar and pestal. The

5.4

S.

Ce Rh Te

600

400

. 200

n'

LOv9-

0co0

0LO

n--

U)

+OI 0

- I

fL . .

U . .

*' 1600. j

c 1200

'' 8004-.24.-

c 4008C. o0. 0

Sr

_ 0

W_ +I + La

I W ..

I . . I

-no

3000 -

2000 LO

0U)

OrnN

IDI9-

Mo Zr

M l0ILOC.,'1000 -

0 - -. '- l _ _

FIGURE 5.1. Comparison of Fission Product Concentration in7; - BWIP Material with Three Particle Sizes

source of the iron was probably the cutoff saw blade, because the iron concen-

tration is nearly constant in all the particle sizes. No source of the boronis offered.

The x-ray diffraction analyses were performed using the as-crushed mate-

rials. These particles were mounted in a 5/8 in. diameter, 3/64 in. deep spe-cimen holder. A 0.00025 in. thick Mylar film was used to retain the powder and

prevent contamination. The 260-2e Mylar peak was used as an internal standard.Diffraction scans were made in 0.029 steps with one second counting times. The

5.5

only phase observed in the three particle sizes was -urania (Table 5.5). The

two larger particle sizes showed identical lattice parameters, while in the

smallest sized material the parameters were slightly smaller. The latter is

generally considered to indicate a higher oxygen content, which is consistent

with a small amount of room-temperature surface oxidation of the high-surface-

area smallest particles. A possible explanation for the variation in relative

peak intensities is that the particles are too large to prevent nonrandom

orientation of the particles.

TABLE 5.5. Results from X-ray Diffraction Analyses of BW1P Crushed Material

SampleIdentification hkl 2e d A , dAa) a, A

-60 +115 mesh 111 28.22 3.160 90 5.470200 32.73 2.734 64 5.468220 46.95 1.934 100 5.469311 55.70 1.649 90 5.468222 58.45 1.578 4 5.465 5.468 .002 A

-115 +250 mesh 111 28.19 3.163 100 5.478200 32.70 2.736 36 5.472220 46.97 1.933 82 5.467311 55.74 1.648 79 5.465222 58.44 1.578 14 5.466400 68.62 1.367 6 5.466 5.469 i .005 A

-250 mesh 111 28.30 3.151 73 5.457200 32.83 2.726 70 5.451220 47.07 1.929 88 5.456311 55.85 1.645 100 5.455222 58.57 1.575 37 5.455400 68.73 1.365 29 5.458 5.455 /002 A

(a) Relative intensities for U02 are: 111, 100; 200, 48; 220, 49; 311, 47;222, 13; and 400, 9. (JPDS card 5-0555).

5.6

5.2 MATERIAL FOR NWSI - SEGMENT C-5C

The Nevada Nuclear Waste Site Investigation (Tuff Program) requested a

segment of ATM-101 for studies at HEDL of the effects of potential cladding

breaches on the release of radionuclides. ATM-101 fuel rod segment C-5C was

provided to HEDL for these tests. A MCC transverse ceramography/metallography

sample and MCC burnup sample were to be sectioned from the segment for charac-

terization purposes. HEDL also planned to section a longitudinal ceramography/

metallography specimen from the segment and will provide the examination

results for inclusion n Section 4.5 of later versions of this report. The

preliminary sectioning diagram for segment C-5C is shown in Figure B.1.

5.3 MATERIAL FOR CSFMPO - SEGMENT N-9B

The Commercial Spent Fuel Management Program Office (CSFMPO) requested one

of several segments of ATM-101 that they expect to need in the next two years.

Because they desired a variation in the degree of pellet fragmentation and

resultant fuel surface area for fuel oxidation studies, an end segment, N-9B,

was provided for these tests. Several MCC burnup, chemistry, and ceramography/

metallography samples were also planned to be sectioned from the rod segment to

complete the characterization of fuel rod N-9. These samples will be sectioned

using the same procedures described in Section 5.1 for the BWIP material. The

preliminary sectioning diagram for segment N-9B is shown in Figure B.2.

5.7

ACKNOWLEDGMENTS

The characterization of ATM-101 s the result of the efforts of several

organizations and many people. The author would like to express his thanks to

the following people for their efforts in characterizing this material:

• EG&G - Idaho- James A. Cook; gas sampling, rod segmenting, and shipping

* Exxon Nuclear - Idaho

- Richard A. Rankin; gas analysis

o Hanford Engineering Development Laboratory

- Norris H. Johnson and Mabry E. McMahan; gamma scanning

- William Y. Matsumoto and John J. McCown; chemical analysis, and 148Nd

and 137Cs burnup calculations

- Raymond D. Bell, Delbert J. DesChane, and Jon 14. Lott; ceramography-

metallography

e Pacific Northwest Laboratory

- Randy E. Thornhill and Cheryl A. Knox; sectioning, sampling, and storage

- Urban P. Jenquin; ORIGEN calculations

- George B. Mellinger; shipping and BWIP material characterization

- Nancy J. Wildung; data reduction

- J. Leland Daniel and John E. Mendel; program direction and management

This report summarizes work conducted for the U.S. Department of Energy by

Pacific Northwest Laboratory under Contract DO-AC06-76RLO-1830.

Ack.1

REFERENCES

Annual Book of ASTM Standards. .1980. Part 11. ASTM E112 Standard Methodsfor Estimating the Average Grain Size of Metals. pp. 186-Z2O.

Annual Book-of ASTM Standards. 1983. Section 12, Vol. 12.02. ASTME 692,Standard Test Method for Cesium -137 in Irradiated Nuclear Fuels by High-Resolution Gamma-Ray Spectral Analysis. p. 98.

ibid. ASTM E 321 Standard Test Method for Atom Percent Fission in Uranium andPlutonRum Fuel Neodymium -148 Method). p. 140.

Barner, J.O. 1984. "LWR Spent Fuel Approved Testing Materials for Radio-nuclide Release Studies." Pacific Northwest Laboratory, PNL-4686.

Croff, A. G. 1980. "ORIGEN-2A Revised and Updated Version of the Oak RidgeIsotope Generation and Depletion Code." Oak Ridge National Laboratory,ORNL-5621.

Einziger, R. E. and R. L. Fish. 1982. "Characterization of LWR Spent FuelRods Used in the NRC Low-Temperature Whole Rod and Crud Performance Test."Hanford Engineering Development Laboratory, NUREG/CR-2871 (HEDL-TME 82-27).

R.1

APPENDIX A

POWER HISTORY FOR ASSEMBLY BO-5

APPENDIX A

POWER HISTORY FOR ASSEMBLY BO-5

A month-by-month'summary of

H. B. Robinson Unit-2 reactor IsI

the power

listed In

history for

Table A.1.

Assembly BO-5 in the

I

A.1

TABLE A.1. Power History for Assembly BO-5

Date

October 1971November 1971December 1971January 1972February 1972March 1972April 1972May 1972June 1972July 1972August 1972September 1972October 1972November 1972December 1972January 1973February 1973March 1973

Cycl e I

Average

22.922.923.323.823.922.922.922.522.522.721.621.321.520.820.421.421.820.1

kW/mPeak

31.331.732.731.331.128.629.228.628.628.327.125.627.527.327.026.927.926.4

EFPD

95.7120.0149.9177.2205.3235.5265.2270.7289.5312.6341.2369.0398.6423.6443.9460.4475.7487.2

'So

.

Date

May 1973June 1973July 1973August 1973September 1973October 1973November 1973December 1973January 1974February 1974March 1974April 1974May 1974

Cycle IILHGR,

Average

17.816.918.318.417.917.317.517.617.717.617.617.517.5

Peak

22.921.524.624.423.122.721.922.222.222.121.921.921.2

EFPD

6.525.458.887.6

116.6145.2166.2192.6221.2247.8278.1307.2311.8

Total 799 EFPD

Average burnup - 28.0 MWd/kgMPeak burnup - 31.4 MWd/kgMRemoved May 6, 1974

A.2

APPENDIX B

SECTIONING DIAGRAMS

APPENDIX B

SECTIONING DIAGRAMS

Segments C-SC, N-9C, and N-9B of ATM-101 have been or are in the process

of being sectioned and distributed to experimenters. The material has been

distributed as listed below:

Segment No.

C-SC

: I ~ IN-9B

: v : N-9C X

FigureDestination No.

NNWSI B.1

CSFMPO B.2,

BWIP B.3

B.1

DISWANE FROM BOTTO InI 30 40

a

w2

bo

9

L.

S.fA-S-

9

d

7

6

5

4

3

2

I

wS~

00 20 40 60 so DO 120 140

DTAN FROM BOTTOM. cm160

Legend

A. NNWSI Nondefected SpecimenB. MCC Transverse Ceramography (upper surface)C. NNWSI Laser-Drilled SpecimenD. MCC Burnup SampleE. NHWSI Slit Specimen

F. NNWSIG. SpareH. NNWSII. Spare

Longitudinal CeramographyMaterialBare Fuel SpecimenMaterial and MCC Archive

FIGURE B.1. Preliminary Sectioning Diagram for Segment C-5C

( ( ( ( ( ( ( ( ( ((

C C C' ( C C C ( C

DISTANCE FROM BOTTOM. in

* - ' _ T 5 _ Te- *S 7o ~~T -0

6U Q P K J

: , 2040 60DITANC

Legend

A. CSFMPO Cladding Defect SpecimenB. CSFMPO Declad-SpecimenC. MCC Transverse Ceramography (upper surface)D. MCC Burnup SampleE. MCC Longitudinal CeramographyF. CSFMPO Declad SpecimenG. Spare MaterialH. CSFMPO Cladding Ring SpecimenI. CSFMPO Cladding Ring SpecimenJ. Spare MaterialK. CSFMPO Cladding Defect Specimen

0

so 10 120 U40

E FROM BOT`TOM, cmNO

L.M.N.0.p.Q.R.S.T.U.

MCC ArchiveMCC Longitudinal CeramographyMCC Burnup SampleMCC Transverse Ceramography (upper surface)CSFMPO Declad SpecimenCSFMPO Declad SpecimenMCC Longitudinal CeramographyMCC Burnup SampleMCC Transverse Ceramography (upper surface)Spare Material

FIGURE B.2. Preliminary Sectioning Diagram for Segment N-9B

DISTANCE FROM BOTOM. In20 30 40

S

laK

S.

0.

93

7

5

4

3

2

IW

00- 20 40 40

DsANCE F1

Legend

A. BWIP aterialB. MCC 1 C SampleC. MCC Transverse CeramographyD. MCC Burnup SampleE. MCC SEM SampleF. 14CC Longitudinal CeramograpiG. BWIP MaterialH. Spare Material

so 00 U20 MD 16tOM BOTTOM. cm

I. MCC Transverse Ceramography (lower surface)J. MCC Burnup SampleK. MCC Longitudinal CeramographyL. Spare MaterialN. MCC ArchiveN. BWIP Material0. Spare Material

(upper surface)

ny

FIGURE B.3. Final Sectioning Diagram for Segment N-9C

( C ( ( C. ( ( C ( ( (

APPENDIX C

DETAILS OF GAS ANALYSES

APPENDIX C

DETAILS OF GAS ANALYSES

This appendix s organized in the following manner: Part 1 deals with the

volume, internal pressure, and gas composition data for each fuel rod that was

analyzed; Part 2 discussed the methods and assumptions used in the calculation

of the random error for each of the individual data elements; Part 3 summarizes

the procedures used, including the apparatus, the actual gas collection and

measurement, and the void volume and internal pressure determination; and

Part 4 deals with instrument calibration records. Gas sampling was conducted

by EG&G-Idaho and chemical analyses were conducted by Exxon Nuclear, Idaho.

PART 1: SEPARATE DATA FOR EACH ROD

Gas volume and internal pressure data for each fuel rod are given in Sec-

tion 4.4 of the body of this report along with a value representing the random

error for each of the individual data elements. Details of the method used in

calculating each of the random errors are given in the Part 2 of this Appendix.

Note that for two of the rods N-12 and N-9, the void volume measurement appears

to be in error. This was due to a faulty valve. The volume percent composi-

tion for each of the gas samples taken from the separate fuel rods is also

listed in Section 4.4 of the body of the report, along with an associated ran-

dom error. For these data, a lower limit of detection of 0.01 vol% was estab-

lished, based upon instrument operating experience. For components which mea-

sured below this limit, no uncertainty was calculated. Organic components,

estimated to be primarily lighter molecules, were only approximated. Isotopic

compositions for both xenon-and krypton are also given in Section 4.4 of the

body of the report. Following is a synopsis of unusual events that occurred

with gas collection from each rod, given in the order that they were drilled.

Element Unusual Events

L-8 Rod was drilled without difficulty. Soon after gas collection

was made, mercury inadvertently entered the pumping system (a

C.1

design flaw in the gas collection apparatus). This necessi-

tated the removal and cleaning of parts of the pumping system.

After this point, the 10 nm remote head of the Baratron pres-

sure measurement device no longer functioned properly. At this

time, a particulate filter was added to the cell line to pre-

vent contamination of the gas collection equipment.

N-12 Several problems occurred with the drill fixture provided byEG&G Idaho Hot Cells South. It was necessary to remove thefixture and work on it. It was necessary to backfill the fuel

rod three times to get two void volume measurements to agree.

This was probably due to a leaking valve that was not dis-

covered until later.

N-9 No apparent difficulties; possibility of the data being v

affected slightly by an incipient value failure.

C-5 Discovered that the fixture valve was leaking. The backfillprocedure was changed to backfill to the cell line valve, so as

to eliminate the fixture valve from consideration. Drilling of

the fuel rod went well.

G-9 Time was lost in this drilling, due to room temperature rising

above 100°F. Otherwise drilling was uneventful.

J-12 The temperature problem continued, with no other apparent

difficulties.

D-10 On the first drill attempt, the drill broke. A new sample linehad to be installed because the fitting broke at the fixture.At this time, the faulty fixture valve was removed from thesystem. The fixture was removed to repair the drill andreturned to the cell. A leak was discovered in the fixture,and the fixture was again removed and repaired. After twodays, the fuel rod was drilled.

G-13 No apparent problems.

N-4 No apparent problems.

C.2

PART 2: CALCULATION OF UNCERTAINTY

Several different methods were used by Exxon Nuclear, Idaho, to estimate

uncertainty for the various types of data. An estimate of the random error

encountered with the-first type of data, i.e., volume and pressure data, was

based upon the assumption that the largest source of error in the measurement

is represented by variations in repeated calibrations of the gas collection

apparatus. The random error for this type of measurement was estimated by cal-

culating the relative standard deviation of several calibration measurements.

For the simpler pressure, volume, temperature relationships, such as measure-

ment of the gas volume within the fuel element, a factor of two times the rela-

tive standards deviation is sufficient. For the more complex measurements,

such as determination of the void volume, errors obtained in the different mea-

surement sequences were summed. Using this method, the estimated random error

associated with these measurements were:

Gas volumes t2.4%

Void volumes i4.7%

Internal pressure t4.7%

Note that this s only an estimate of the random error. Any systematic

errors due to the method of sample collection are not included. Other data

types are the volume percent of gases and isotopic composition data. There

were three different methods used to estimate the random errors associated with

these data elements. The first method (a) was based on the premise that the

gas mass spectrometer recording medium cannot be read accurately to better than

0.5 chart divisions. This type of method would be used when the peak height

was small enough that this is the dominant error associated with the calcula-

tion. The'second method (b) is used in calculation of krypton isotopic com-

position where the peaks were large enough to be read reasonably'well, but were

smaller than the standard calibration peak heights. It was assumed that this

error was included within the variation in the overall krypton to xenon ration.

The third method (c) used to estimate the random error was based on routine

calibration records for the period when the samples were analyzed. This method

C.3

was used for the components that were routinely checked during calibration and

for those whose percent composition was the range of the calibration values.

The estimated random error produced by method (a) varies with individual

peak height. Method (a) was used to estimate the error associated with the

following data: hydrogen (where applicable); nitrogen (except element 18);

oxygen, xenon i30; krypton 83; and krypton 85.

The estimated random error (twice the relative standard deviation) pro-

duced by method (b) was 3.65%. Method (b) was used to estimate the error in

the following data: krypton volume percent, xenon 131, krypton 84, and

krypton 86.

The estimated random error (twice the relative standard deviation) pro-

duced by method (c) varied according to component and percent composition.

This is summarized below:

N2 0.22% Range 40-100%

Ar 1.70% Range 0.5-10%

Method (c) was used to estimate the error in the following data: helium;

nitrogen in L8; argon; xenon volume percent; xenon 132, 134 and 136.

The organic volume percent data is an approximation, and no random error

is estimated for the data elements.

PART 3: SUMMARY OF OPERATING PROCEDURES

Both the detailed operating procedure and the equipment used in the col-

lection of gases from fuel were the responsibility of EG&G Idaho. The follow-

ing summary is provided as a brief description of the gas analysis and

collection procedure.

APPARATUS

The apparatus used to collect and measure the volume of gases contained in

the fuel rods consisted of two basic systems. The first system, located within

the EG&G hot cell, consisted of an air operated drill and vacuum-tight rod

fixture. The rest of the collection and measuring system was located outside

C.4

the hot cell and was connected to the fixture with metal tubing. The collec-

tion and measurement apparatus included a Baratron pressure measurement system

with two remote heads (ranges 0-10 mm and 0-1000 mm). Various expansion vol-

umes'were used, depending upon the volume of the gas collected. The volume of

the system was calibrated by introducing known amounts of gas into the system

and using the pressure, volume and temperature relationship to calculate the

system volumes. The volume of the tubing connecting the fixture to the system

and the volume of the fixture itself, were calculated using a similar

procedure.

GAS COLLECTION/MEASUREMENT

With the fuel rod clamped in the vacuum tight fixture, the system was

evacuated to the lowest pressure obtainable as indicated by the Baratron sys-

tem, usually less than 0.1 torr. The system was then isolated from the pumping

line to check for leaks as would be observed by a rise in pressure. No rise

should be observed before puncturing a fuel rod.

When the system was shown to be leak tight, the rod was drilled and the

gas was collected. When the system pressure stabilized, the final pressure was

recorded and the quantity of gas was derived from the pressure, temperature,

and system volume. The gas was then transferred to a gas bulb to await gas

mass spectrometry analysis (using the Teoppler pump). The gas analysis was

performed using a CEC-103 gas mass spectrometer. The use and calibration of

this instrument are detailed in the CEC-103 Operations and Methods Manual.

VOID VOLUME

The void volume of the fuel rod was obtained by backfilling the rod with a

known amount of gas, and measuring the volume of the system and the rod, then

subtracting the volume of the system, as determined earlier. The system used

for this work varied for different fuel rods due to a bad fixture valve, and

the need to change the cell line.

C.5

SECTION 4: CALIBRATION

The equipment used in this work was calibrated according to the standard

procedures described above. Calibration records that are applicable to this

work are found in CEC-103 Gas mass Spectrometer Log Book No. 7 and Remote Gas

Collection and Void Volume Log Book No. 2.

C.6

'-

APPENDIX D

GAMMA SCAN RESULTS

F IGURES

D.1

D.2

D.3

D.4

D.5

D.6

Gross Gamma

Gross Gamma

Gross. Gamma

Gross Gamma

Gross Gamma

Gross Gamma

Scan-Segment

Scan-Segment

Sc an-Segment

Scan-Segment

Scan-Segment

Scan-Segment

cSc.... . ..................................

.... ....................................

N9B................. ..... .... .............

.... ...... ... ............................

N 9T. ................. .....................

Ni 2C......................................

D.3

D.4

D.5

D.6

D.7

D.8

0.7 Spectral Gamma Scan

D.8

D.9

D.10

D.11

D.12

D.13

D.14

D.15

D.16

D.17

D 18

D.19

D .20

D.21

D.22

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Spectral

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Gamma

Scan

Scan

for 137Cs

for 137CS

for 137Cs

for 137CSScan

Scan for

Scan for137CS

Scan for 134Cs

Scan for 134Cs

Scan for 134Cs

Scan for 134Cs

Scan for 134Cs

Scan for 13 4Cs

Scan for 154Eu

Scan for 154Eu

Scan for 154Eu

Scan for 154Eu

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

- Segment

N 9Bo.o.o.o....o.o.o.oooo...

N9..ooooooo.ooo**e**eo.o***

Ni 2C...........ooo...o....

N 9Boo*..*o.. e .*ooeee.oo...

N9.*.o.oe**o.e**9o.**o**...

D.9

D .10

D.11

D 12

D.13

D .14

D.15

D.16

D. 17

D.18

D.19

D .20

D.21

D.22

D.23

D.24

D.23 Spectral Gamma Scan for 54Eu - Segment N12C ...... ................ D.25

D.1

C C C C ( C ( C (7 C Cr

DISTANCE FROM BOTTOM. In

a

0

to0

,

L

V)~ e

I-CL

I-V:

7

6

5

4

3

2

1

4

00 20 40 60

DISTANCE80 100

FROM BOTTOM.120

cm140 160

FIGURE D.1. Gross Gamma Scan-Segment C5C

DISTANCE ROM BOTTOM. in20 30 400 10 50 60a

0

xina4o

)c040

QL.

CLa-

0

I:Fu

7

6

5

4

3

2

1

I I , I

Lc GROSS

! | I I

II00 20 40 60

DISTANCEso too

FROM BOTTOM.120

cm

140 MO

FIGURE D.2. Gross Gamma Scan-Segment L8C

( ( ( ( ( ( ( (

( C C C (~~( r ( ( (


a

7

a.

C>

0'V

I-rn

6

5

4

3

2

1

0C"

00 20 40 -60 80

DISTANCE FROM100

BOTTOM,120

cm

140 160

FIGURE D.3. Gross Gamma Scan-Segment N9B

DISTANCE FROM BOTTOM. in20 30 40

. p0 t0 50 60

toa

x

40

0CL

CaU

1=FTi

7

6

5

4

3

2

1

N9C GROSS

I I ~ I

All~~~~~~~~~1

|I I I_ I I I I 0

0 20 40 60

DISTANCE80

FROMtoo 120

BOTTOM. cm140 160

FIGURE D.4. Gross Gamma Scan-Segment N9C

( C ( ~~~~~~~~~~~~~~~t ( C

Ct C' C C. C C C ~ ~~~ ~ ~ ~ ~~~~~~~ C( C

DISTANCE FROM BOTTOM In

a

0an0

:0COM

0

V

0

7

6

5

4

3

2

1

00 20 40 60

DISTANCEso 100

FROM BOTTOM.120

cm

140 160

FIGURE D.5. Gross Gamma Scan-Segment N9T


a

inax

0

L

C*

5:.~~0

F

U0

7

6

5

4

3

2

1

0

00 20 40 60

DISTANCEs0

FROM10

BOTTOM.120

cm

140 160

FIGURE D.6. Gross Gamma Scan-Segment N12C

c ( ( C ( ( ( ( ( ((~~~~ f

e c C C C C C Cc c C

DISTANCE FROM BOTTOM, In0 10 20 30 40 50 60

14

w

0

W.

ha-C

0

L

. _,-

U

I-

-

12

10

8

6

4

2

f=.o

00 20 j40 60 80 too

DISTANCE FROM BOTTOM. cm20 140 160

- FIGURE D.7. Spectral Gamma Scan for 137Cs'- Segment C5C

DISTANCE FROM BOTTOM In14

0

00

La-

CLo

0M

OmC

12

10

8

6

4

2

V

Q-

00 20 40 60 80 100 120

DISTANCE FROM BOTTOM. cmSpectral Gamma Scan for 137Cs - Segment L8C

140 160

FIGURE D.8.

(( ( ( C C C C C

C C C C C C C C' C C C( ( f C~ C

DISTANCE FROM BOTTOM. In20 X 30 40

14

qr0x

o

a

MU.

20*_0

t1-

-°

10

,.6I--

4

2'

00 20 40 60

DISTANCE80

FROM100 120

BOTTOM. cm140 160

FIGURE D.9. Spectral Gamma Scan for Cs - Segment N9B


14

1w0x

0M

Le

a-0

I-I-4

c_

>

12

10

8

6

4

2

M

00 20 40 60 80 100 120.

DISTANCE FROM BOTTOM. cm140 160

FIGURE D.10. Spectral Gamma Scan for 137Cs - Segment 9C

( (~~~ ( ( ( C C C

C' C' (. C C C ~~~~~~~~~~~~~~~~C c

DISTANCE FROM BOTTOM, In

'4

K

.0X,

4

C. 0

-.

V:

I--

12

10

8

6

4

2

0I-

00 20 40 60 80

DISTANCE FROM100

BOTTOM.120 140 160

cm

,FIGURE D.11. Spectral Gamma Scan for 137Cs - Segment N9T

DISTANCE FROM BOTTOM. n20 30 40

14

IV

aVox

(s0Lo

0CL

C

0u

12

10

a

6

4

2

offift*�"

0o

0

0 20 40 60

DISTANCE80 100

FROM BOTTOM.120

cm

140 160

FIGURE D.12. Spectral Gamma Scan for 137Cs - Segment N12C

C ( ( ( ( C ( ( ( I

e c C C ( C C C CC C C


14

0

00CS

5-

*, C

on

F

UC

12

10

a

6

4

2

00

Ln

00 20 40 60

DISTANCE80 100

FROM BOTTOM.120

cm

140 160

FIGURE D.13. Spectral Gamma Scan for 134Cs - Segment C5C

DISTANCE FROM BOTTOM in20 30 40

4

esa

4.,

x

a*a

L

0~0.

aI-

d

5U

12

10

a

6

4

2

0~

00 20 40 60

DISTANCE80

FROM100 120

BOTTOM. cmHO 160

FIGURE D.14. Spectral Gamma Scan for 134Cs- Segment L8C

( C ( ( ( C C C ciC

c c ( r C C C C ~~~~~~~~~C Cc C C

DISTANCE FROM20 . 30

BOTTOM. In

14

V%

x

0

CL

0I-

5:Vi=

12

10

0

B

6

4

2

0.0 20 40 60

DISTANCE80 100

FROM BOTTOM.120

cm

140 160

FIGURE'D.15. Spectral Gamma Scan for '34 Cs - Segment N9B

S

DISTANCE FROM BOTTOM In20 30 40

14

.0

.L

CL

0

i

12

10

S

6

4

2

0~

co

00 20 40 60

DISTANCEso 100 120


FIGURE D.16. Spectral Gamma Scan for 134Cs - Segment 9C

( ( ( ( C C C (

( C C C C C C C C (c r c~~

DISTANCE FROM BOTTOM. In0 - 10 20 30 40 - 50 60

'4

0U.-.

0t0

0V

I.-0FV

S

6

4

2

12

10

00 20 40 . 60 80

DISTANCE FROMtoo 120

BOTTOM. cm140 160

FIGURE D.17. Spectral Gamma Scan for 134Cs - Segment N9T

DISTANCE FROM BOTTOM. In20 30 400 10 50 60

14

K0

0

C-)

in

C0

d

I--

5;

FoV

12

10

8

6

4

2

0oCD

00 20 40 60 80 100

DISTANCE FROM BOTTOM.120

cm

140 160

FIGURE D.18. Spectral Gamma Scan for 134Cs - Segment N12C

( ( ( ( ( C (

c c c C ( Cc c C- c

DISTANCE FROM BOTTOM. In20 30 400 10 s0 60

14

C40

0

0

C

a

I-

1:

12

10

a

6

4

2

0)

00 20 40 60 80

DISTANCE FROM100 120

BOTTOM. cm140 160

FIGURE D.19. Spectral GammaScan for 154Eu - Segment C5C

DISTANCE20

FROM BOTTOM In30 400 t0 50 60

14

0x

o0

0

0A

C

0u

I-

I~-v

12

10

8

6

4

2

ID

r%)1

00 20 40 60 80 100 120

DISTANCE ROM BOTTOM. cm140 160

FIGURE D.20. Spectral Gamma Scan for '54Eu - Segment L8C

C L ( ( ( ( ( ( ( ( ( (< C

c c IC C C C

DISTANCE FROM BOTTOM, In20 30 400 10 ,o 60

14

12

0x

gto

C

060

t'4

< t,2

3%)(a)

0

0 20 40 60

DISTANCE80 100

FROM BOTTOM,120

cm140 160

FIGURE 0.21 . Spectral Gamma Scan for 154Eu - Segment N9B

DISTANCE FROM20 30

BOTTOM. in

14

5.X

,5 o1..

so.

CL-

Co 6

24

<2

0;

00 20 40 60

DISTANCE80 oo 120


FIGURE D.22. Spectral Gamma Scan for 54Eu - Segment 9T

L ( ( ( ( ( C ( (C (

~~~C C' C c r c r

DISTANCE FROM BOTTOM, in0 10 20 30 40 50 60

14

0x

C1(n

so

>

CL

-

F:V-

12

to

a

6

4

2

enC,'

00 20 40 60

DISTANCEso 100

FROM BOTTOM.120

cm

140 160

FIGURE D.23. Spectral Gamma Scan for 154Eu - Segment N12C

APPENDIX E

RESULTS OF RADIONUCLIDE INVENTORY CALCULATIONS

TABLES

E.1

E.2

E.3

E.4

E.5

E.6

Radionucilde

Radionuci de

Radionuci de

Radionuciide

Radionuciide

Radionuc i de

Inventories

Inventories

Inventories

Inventories

Inventories

Inventories

at 10 MWd/kgM

at 15 MWd/kgM

at 20 MWd/kgM

at 25 MWd/kgM

at 30 MWd/kgM

at 35 MWd/kgM

as a Function

as a Function

as a Function

as a Function

as a Function

as a Function

of Decay

of Decay

of Decay

of Decay

of Decay

of Decay

Time

Time

Time

Time

Time

Time

I

E.1

TABLE E.1.

Subtable

E.1.a

E.1.b

E.1.c

E.1.d

E.1.e

E.1.f

E.1.g

E.1.h

E.1.1

E.1.j

Radionuclide Inventories at 10 MWd/kgM as a Function of Decay Time

Species-Units

Actinides (Isotopic), g/gU E.5

Actinides (Elemental), g/gU E.6

Actinides (Isotopic), Ci/gU E.7

Actinides (Elemental), C/gU E.9

Fission Products (Isotopic), g/gU E.10

Fission Products (Elemental), g/gU E.14

Fission Products (Isotopic), C/gU E.15

Fission Products (Elemental), Ci/gU E.17

Neutron Source (Alpha-n), neutrons/sec-gU E.18

Neutron Source (Spontaneous fission), neutrons/sec-gU E.18

E.3

TABLE E.l.a. Actinides (Isotopic), g/gU, at 10 MWd/kgM

10 YEARS 12 YEARS 14 YEARS

HE 4 9.S05-008 1.151-007 1.321-007P8207 2.805-015 4.312-015 6.261-015P8208 4.694-012 6.261-012 7.890-012P9212 1.354-015 1.432-015 1.471-015RA224 -1.181-014 '1.249-014 1.283-014RA226 1.C48-015 1.562-015 2.213-015AC227 2.258-014 2.979-014 3.783-014TH228 2.295-012 2.421-012 2.487-012TH229 2.400-014 2.815-014;3.281-014TH230 - 2.550-011 3.287-011 4.108-011TH231, 6.'650-014 6.65C-014 6.650-014TH232 5.409-010 6.359-010 7.308-010TH234 1.404-011 1.4C4-011 1.404-011PA231 1.975-010 2.292-01C 2.609-010PA233 '3.C25-012 3.039-012 3.056-012U232 9.d61-011 9.759-011 9.746-011U233 4.S12-010 5.110-01C 5.712-010U234 1.247-006 1.398-006 1.547-006U235 1.636-002 1.636-002 1.636-002U236 1.631-003 1.631-003 1.631-003U237 5.958-012 5.411-012 4.914-012U238 9.668-001 9.668-001 9.668-001

NP236 S.C06-011 S.OC6-011 5.006-011NP237 8.S05-005 8.948-005 8.996-005NP238 2.440-014 2.418-014 2.396-014NP239 1.408-012 1.407-012 1.407-012PU236 7.523-012 4.626-012 2.845-012PU238 9.766-006 9.613-OC6 9.464-006PU239 3.684-003 3.683-003 3.683-003PU240 7.287-004 7.2t6-004 7.284-C04PU241 1.924-004 1.748-004 1.587-004PU242 2.52-005 2.952-005 2.952-005PU244 1.C75-010 1.075-01G 1.075-010AM241 1.275-004 1.447-004 1.602-004AK242K 1.302-007 1.29G-007 1.278-007AN242 1.557-012 1.543-012 1.529-012AK243 1.638-006 1.638-006 1.637-006CN242 3.150-010 3.125-01G 3.C97-010CM243 6.G81-009 5.792-009 5.517-009C1244 8.C23-008 7.432-008 6.884-008CK245 1.656-009 1.656-009 1.656-009CM246 5.281-011 5.279-011 5.277-011CN247 1.423-013 1.423-013 1.423-013CN248 1.994-015 1.994-015 1.994-015SF250 2.287-013 2.461-013 2.628-013SUNTOT 9.897-001 9.897-001 9.897-001

16 'YEARS

1.497-0078.699-0159.548-0121.485-0151.296-0143.016-0154.665-0142.511-0123.7.98-0145.011-0116.651-0148.258-0101.404-0112.926-0103.073-0129.667-0116.317-0101.693-0061.636-0021.632-0034.463-0129.668-0015.006-0119.049-OC52.374-0141.407-0121.749-0129.316-0063.683-0037.283-0041 .441-0042.952-0051.075-0101 .743-0041.266-0071.515-0121.637-0063.069-0105.255-0096.377-0081.656-0095.276-0111.423-0131.994-0152.790-0139.897-001

TOTAL 9.£97-001 .8S7-001 9.897-001 9.897-001

E.5

TALE E.1.b. Actinides (Elemental), /gU, at 10 MWd/kgM

IC YEARS 12 WEARS 14 YEARS 16 YEARS

HESFPsRAACTMPA

UNPPuANCmSUNTOT

TOTAL

9.905-008 1.151-OC72.287-013 2.461-0134.698-012 6.266-0121.289-014 1.409-0142.258-014 2.979-0145.829-010 6.853-01C2.CO5-010 2.322-OIC9.848-001 9.848-0018.505-005 8.948-0054.644-003 4.626-OC31.292-004 1.464-OC48.833-008 8.213-0089.0897-001 9.897-001

1.321-CO? 1.497-OC?2.628-013 2.790-0137.897-012 9.558-0121.510-014 1.604-0143.783-014 4.665-0147.885-010 8.926-0102.640-010 2.957-0109.848-001 9.848-0018.996-005 9.049-0054.609-003 4.594-0031.620-004 1.760-OC47.638-008 7.104-OC89.897-001 9.897-001

9.897-001 9.897-001 9.897-001 9.897-001

'S.

E.6

TABLE E.l.c. Actinides (Isotopic), C/gU, at 10 MWd/kgM

.10 YEARS 12 YEARS 14'YEARS 16 YEARS

TL207TL208TL209PB209PS210P8211PE212P8214812108121191212bI21381214P0210PC211'IP0212P0213P0214P0215P0216P0218Ait217RN219RN220RN222FR221FR223-RA223RA224RA225RA226RA228AC225AC227AC228TH227TH228TH229TH230TH231TH232TH234PA231PA233PA234MPA234U232U233U234U235U236U237

1.630-012 2.153-012 2.734-012 3.372-0126.?60-010 7.15C-01G 7.345-010 7.418-0101.103-016 1.294-016 1.S08-016 1.746-0165.108-015 5.99C-015 6.981-015 8.083-0151.300-016 1.993-016 2.991-016 4.362-0161.E34-012 2.159-012 2.742-012 3.382-0121.J82-009 1.99-009 2.044-CO9 2.064-OC91.C36-015 1.545-015 2.189-CI5 2.983-0151.!00-016 1.994-016 2.992-016 4.363-0161.34-012 2.159-012 2.742-012 3.382"0121.182-009 1.99C-009 2*044-CO9 2.064-OC95.108-015 5.99C-015 6.981-C15 8.083-0151.C36-015 1.545-015 2.189-015 2.983-0151.00-016 1.776-016 2.675-016 3.929-016

,4.576-015 6.045-015 7.678-C15 9.469-0151.206-009 1.275-009 1.310-009 1.323-OC94.998-015 5.861-015 6.831-C15 7.908-0151.036-015 1.544-01S 2.188-015 2.982-0151a.34-012'.2.159-012 2.742-C12 3.382-0121.J82-009 1.99C-OCS 2.C44-009 2.064-009

'1.C36-015 1.545-015 2.189-C15 2.983-0155.108-0155.99C-015 6.981-C15 8.083-0151.634-012 2.159-01212.742-C12 3.382-012i.882-009 1.99C-OCS 2044-009 2.064-OC91.C36-015 1.545-015 2.189-015 2.983-0155.108-015 5.99C-015 6.981-015 8.083-0152.255-014 2.9?5-014 3.778-014 4.659-0141.634-012 2.159-012 2.742-012 3.382-0121.J82-009 1.990-005'2.044-009 2.064-0095.108-015 5.990-015 6.981-015 8.083-0151.C36-015 1.545-015 2.189-015 2.983-0152.454-017 3.205-017 4.011-017 4.860-0175.108-015 S.990-015 6.981-015 8.083-0151.634-012 2.156-012 2.737-012 3.376-0122.454-017 3.2G5-017 4.011-017 4.861-0171.12-012 2.129-012 2.704-012 3.335-0121.881-009 1.985-009 2.039-009 2.059-0095.108-015 5.99G-015 6.981-015 8.083-0155.150-013 6.639-013 8.296-013 1.012-0123.537-008 3.537-001 3.537-008 3.537-008S.535-017 6.977-017 8.019-017 9.060-0173.252-007 3.252-007 3.252-007 3.252-0079.331-012 1.083-011 1.233-011 1.383-0116.280-008 6.310-008 6.344-008 6.381-0083.252-007 3.252-007 3.252-007 3.252-0074.227-010 4.227-010 4.227-010 4.227-0102.C69-009 2.090-009 2.087-009 2.070-0094.369-012 4.949-012 5.532-012 6.118-0127.798-009 8.741-009 9.668-009 1.058-0083.537-008 3.537-00e 3.537-008 3.537-0081.056-007 1.056-O07 1.056-007 1.056-0074.865-007 4.418-007 4.013-007 3.644-007

E.7

TABLE E.l.c. (Contd)

IC YEARS 12 YEARS 14 YEARS 16 YEARS

3.252-007 3.252-007 3.252-C07 3.252-007U238U240

NP235NP236NP237NP238NP239NP240PPU236PU238PU239PU240PU241PU242PU244AN241AP242AN242A 243CM242CM243CM24%CM24SCM246CF249CF230SUMTOT

1.505-015 1.9C5-0159.864-0136.598-0136.280-0086.327-0093.267-0071.905-0153.S99-0091.672-0042.291-0041.661-0041.583-0021.128-0071 .08-0154.376-0041.265-0061.259-0063.267-007I.C42-0063.140-0076.494-0062.845-0101 .23-0113.306-0175.148-0172.C84-002

2.747-0136.598-0136.31C-OCe6.27C-OCS3.266-0071 .9C5-0152.459-0091 .64-OC42. 291-OC41.661-OC41 .8C-0021.128-o?1.908-0154.96e-0041.254-0CC1.248-0063.266-0071.034-OCt2.991-0076.015-OC62.345-01C1.622-0113.294-0174.63C-017I.9CI-002

1.905-ClS7.650-0146.598-0136.344-0086.213-C093.266-0071.905-0151.512-0091.6 21-0042.290-0041.660-CO41.636-0021.128-0071.908-0155.501-0041.243-CO61.236-0063.266-0071.024-0062.849-0075.572-0062.844-0101.622-C113.2 81-0174.164-0171.748-C02

1.905-0152.130-0146.597-0136.381-008C.156-O93.265-0071.905-0159.299-0101.596-0042.290-0041.660-0041.486-0021.128-0071.908-0155.983-0041.231-0C61.225-0063.265-0071.015-0062.714-0075.161-0062.844-0101.621-0113.268-0173.746-0171.602-O2

V'0

TOTAL 2.C84-002 1.9C8-OC2 .748-002 1.602-002

E.8

TABLE E.1.d. Actinides (Elemental), CgU, at 10 MWd/kgM

IC-YEARS 12 YEARS 14 YEARS 16 YEARS

TLPe -

POATRNFR;RAACTNPA

U-NPPUAM'

CfSUMTOT

TOTAL

6.777-010 7.172-Q1C 7.372-010-1.83-009 1.992-009 2.047-C091.883-009 1.992-009 2.047-0093.C89-009 3.267-009 3.357-0095.108-015 5.99C-015 6.981-C151.E83-009 1.992-00; 2.047-C092.766-014 3.574-014 4.476-C141.83-009 1.992-009 2.047-CO91.639-012 2.162-012 2.744-Cl23.624-007 3.625-OC7 3.626-0073.E84-007 3.887-OC? 3.e90-CO79.625-007 9.188-OC? 8.792-CO?3.958-007 3.96C-007 3.962-CO72.C39-002 1.857-OC2 1.691-C024.405-004 4.996-OC4 5.530-0047.850-006 7.348-006 6.881-006-8.578-017 6.0Ce-017 7.505-0172.CS4-002 1.9C8-002 1.748-002

2.C84-002 1.9CI-002 1.748-002

7.451-0102.068-0092.068-OC93.391-OC98.083-0152.068-OC95.467-0142.068-0093.384-0123.626-0073.894-0078.43 2-OC73.965-0071.541-0026.011-0046.448-0067.060-0171 .602-OC2

1 .602-OC2

i I .I ;

E.9

TABLE E .. e . Fission Products (Isotopic), g/gU, at 10 MWd/kgM

1C YEARS 12 YEARS 14 YEARS 16 YEARS

H 3LX 6LI 7BE 9BE 1GC 14

ZN 66ZN 67GA 71GE 72GE 73GE 74AS 75GE 76SE 76SE 77SE 78SE 79BR 79SE 80KR bO3R 81KR 81SE 82KR 82KR 83KR 84KR 85RB 85KR 86SR 86RB 87SR 87SR 88Y 89

SR 90Y 90

ZR 90ZR 91ZR 92ZR 93NS 93NB 93ZR 94NB 94MO 95ZR 96MO 96MO 97MO 98TC 98TC 99

9.295-009. 8.3C8-OC99.462-011 9.662-0113.C83-012 3.083-0125.540-012 5.94C-0123.S62-011 3.962-0118.C01-012 7.999-0121.294-014 1.294-0145.426-016 5.426-0162.422-013 2.422-0136.411-009 6.411-OCS1.419-008 1.419-OCS2.S92-008 2.992-0086.455-008 6.455-0081.616-007 1.616-0075.753-010 5.753-01C3.427-007 3.427-OC?7.391-007 7.391-0071.E66-006 1.864-OCt2.268-010 2.647-O1C4.251-006 4.251-OC65.255-011 5.255-0117.187-006 7.1e7-OC63.C78-012 3.078-0121.106-005 1.1C6-OC51.177-007 1.177-0071.638-005 1.638-OC53.508-005 3.5C8-0054.226-006 3.713-00d3.685-005 3.736-0056.471-005 6.471-0054.453-008 4.453-0088.337-005 8.337-OC53.t56-010 3.856-01C1.198-004 1.198-0041.'72-004 1.572-OC41.450-004 1.382-0043.36-008 3.467-0084.524-005 5.198-OCS2.C04-004 2.0C4-OC42.129-004 2.129-0042.371-004 2.371-0043.427-010 4.487-01C8.789-010 9.878-01C2.364-004 2.364-0041.649-010 1.649-01C2.482-004 2.482-OC42.520-004 2.52C-0043.284-006 3.284-0062.456-004 2.456-0042.514-004 2.514-0046.152-010 6.152-0102.528-004 2.528-004

E.10

7.426-C099.6 62-0113.C83-01 25.940-C123.962-Cll7.997-C121.2 94-C145.426-C162.422-0136.411-0091.419-COS2.992-0086.455-0081.616-0075.753-C103.427-0C77.391-0071. 8 66-0063.C65-CIO4.251-C065.255-C117.187-C063.078-Cl21.106-0051.177-C071.638-0053.508-0053.263-0063.781-C056.471-0054.453-C088.337-0053.856-C101.198-0041.572-0041.318-0043.306-0085.841-0052.004-0042.1 29-0042.371-0045.652-C101.C86-0092.364-C041.649-C102.482-0042.520-0043.284-0062.456-C042.514-0046.1 52-0102.528-004

6.637-0099.662-0113.083-0125.940-0123.962-0117.995-0121.294-0145.426-0162.422-0136.411-OC91.419-0082. 992-0086.455-0081.616-0075.753-0103.427-OC77.391-0071 .866-O063.463-0104.251-0065.255-0117.187-0063.078-0121.106-0051.177-0071.638-0053.508-0052.867-0063.821-0056.471-0054.453-0088.337-OC53.856-0101.198-0041 .572-0041.257-OC43.152-OC86.454-0052.004-0042.129-0042.371-0046.913-0101.175-0092.364-0041.648-0102.482-OC42.520-OC43.284-0062.456-OC42.514-0046.152-0102.528-004

TABLE E.l.e. (Contd)


RU 99M 1 00RU1I00

RU102RH102RH103RU104P0104PD105RU106RH106PD106PD107AG1 07PD108'AG108FPCD1 08

.A6109C0109PolioAG110

CD110CD112

CD1I13

!N114

CD16.SNI 14INlISSNIISC0116SN 16SNI 17SNIISSNII 9SN119FSN120SN121Se121SN122TE122SN1 2356 23TEI 23SN1124TE1245125TE1 25TEt25FSN1 26

9.286-0092.108-0049.340-0062.351-0042.166-0049.491-0121.031-0041.361-0042.240-0059.528-0053.539-0083.327-0146.E69-0054.3 33-0055.102-0112.883-0051 .46-0132.654-0111.719-0054.105-0179.788-0062.436-0122.2 70-0065. S64-0063.*10-0061.198-0073.616-0082.521-0085.857-0069.795-O11

1.093-0E 1.258-0082.8Cs-004 2.EOs-0049.34C-006 9.340-0062.351-004 2.351-C042.166-OC4 2.166-0045.885-012 3.648-0121.631-004 1.631-C041.361-004 1.361-0042.24C-005 2.240-0059.528-005 9.528-0058.946-009 2.261-0098.4C9-015 2.125-0156.871-005 6.872-co54.333-oc5 4.333-0056.027-011 6.952-0112.883-OCS 2.883-0051.925-013 1.904-0132.654-011 2.654-0111.719-005 1.719-0051.614-017 5.419-C1S9.788-O06 9.788-0063.211-013 4.233-0142.27C-00d 2.270-C065.964-O06 5.964-0063.91C-006 3.910-0061.19t-OC? 1.198-Co73.288-O0E 2.990-0082.849-008E3.147-0085.857-006 5.e57-0069.795-011 9.795-C11

I .422-0C82.808-oC49.340-oc62.351-OC42.166-OC42.262-0121.631-0041.361-0042..240-0059.528-ocs5. 715-0105.372-0166.s72-OC54.333-OCs7. 876-0112.883-OCs1.884-0132. 654-0111 .719-OCs1.820-0189.788-0065.580-0152. 270-0065.964-0063.910-0061.198-0072.719-0083.417-0085.857-oC69 .795-o111 .540-0069.422-0082.411-0061.21 -62.453-0062.476-0062.458-0068.901-0162.514-0066.796-0102.570-0062.782-0065.412-0083.083-0213.119-0063. 590-0103. 775-0064.014-0087.292-0085. 260-0061.020-0097.694-006

1.540-006 1.54c-oc6 1.540-0069.422-008 9.422-008 9.422-0082.411-006 2.411-006 2.411-0061.218-006 1.21E-006 1.218-0062.453-006 2.453-00 .2.453-0062.476-006 2.476-OC6 2.476-0062.458-006 2.45e-oce 2.458-co64.384-013 5.551-014 7.029-0152.514-006 2.514-006 2.514-0067.386-010 7.184-OIC 6.987-0102.570-006 2.570-00i 2.570-0062.782-006 2.7e2-006 2.782-0065.412-008 t.412-00E 5.412-0083.943-016 7.822-018 1.552-0193.119-006 3.119-006 3.119-0063.590-010 3.590-010 3.590-0103.775-006 3.775-006 3.775-0064.C14-008 4.014-008 4.014-0083.273-007 1.984-007 1.203-0075.C02-006 5.133-006 5.212-0064.578-009 2.776-009 1.683-0097.94-006 7.694-006 7.694-006

E.11



S 8126S31 26PTE1 26IE1 27P

112?TE128XE1 281129

XE129TE130XEI 30XE131XE132BA1 32CS133X E1 34CS134SAl 34C S1 359A135XE1 363A136CS137BA137BA137P3A1 38LA138LAI 39CE140PR141CE142ND142N0143CE144PR144PR144N0144ND1145ND1 46P1 46SM46PM1147S14 47ND148S1I48S1449ND1SOSf150EU150S1151EU151S1 52

3.d55-0132. 7 79-0151.£77-0073. 389-0171. 51-0053.117-0052.5 59-0075.226-0055.201-0101.C19-0041.126-0061.409-0042.E44-0041 .56-0103.7 81-0044. 471-0044.520-0071.667-0051.863-0048.5 27-0095.998-0043. 5 03-0062.162-C048.5 30-0054.379-0113.954-0042.492-0093. 7 97-0043.753-0043.515-0043.509-0042.468-0063.116-0041.6 43-0086.S38-0133.468-0153. 5 33-0042.287-0041.950-0042.886-0109. 384-0105.584-0061.C29-0041.121-0042.924-0051.676-0065.C45-0057.341-0058.484-0147.234-0065.973-0074.402-005

3.655-0132.779-0151.678-OC?3.256-0191.551-OC53.117-OCS2.559-OC75.226-OC55.247-01C1 .019-0041.126-OCt1 .6C9-0042.844-OC41.856-01C3.781-OC44.471-0042.3C7-OC?1.689-OC51 .863-0048.639-0C95.998-OC43.5C3-OC62.733-OC49.82 3-0054.181-0113.954-0042.492-OC93.797-OC43.753-0043.515-OC43.5C9-0C42.468-0063.116-0042 .767-0091.168-0135. 841-0163.533-OC42. 287-0041 .95C-0042.243-01C9.622-01C3.292-0061.052-0041.121-0042.924-OC51.676-0065.04 5-0057. 341-0058.16 4-0147.124-0067.079-0074.4C2-005

3.655-0132.779-C151.679-0073.139-0211.5 51-0053.117-COS2.559-0075.226-0055.293-0101.G19-0041.126-C061.609-0042. 44-C041.856-C103.781-0044.471-0041.178-0071.700-CO51.863-0048.752-0095. 998-0043.503-0062.610-0041 .106-C043.993-0113.954-0042.492-0093.797-C043.7 53-0043.515-0043. 509-C042.468-0063.116-0044.661-CIO1.968-0149.8 38-0173.5 33-0042.287-0041.950-0041.743-0109.807-0101.9 41-006I.C66-0041.121-0042.9 24-0051.676-0065.045-0057.341-0057.855-0147.015-0068.168-0074.402-005

3.655-0132.779-0151.680-0072. 463-0231.551-0053.117-0052.559-OC75.226-0055.339-0101.01 9-0C41.126-0061.609-0042. 844-0041.856-0103.781-0044.471-0046.014-OC81.706-0051 .863-0048.864-OC95.998-0043. 503-0062.492-OC41. 224-0043.812-0113.954-0042.492-0093.797-0043.753-0043.515-0043.509-0042.468-OC63.116-0047. 850-0113. 314-0151.657-0173.533-0042.287-0041.950-0041.355-0109.951-0101.144-0061.074-0041.121-0042.924-0051.676-0065.045-0057.341-0057.559-0146.908-0069.240-0074.402-005

E.12


10 YEARS 12 YEARS 14 YEARS 16 YEARS

EU15260152EU1536D153IMl 54EU1546D154£U155GD15560156.G0157G0158T81596D1600Y160OY161DY162DY1o3DY164H0165H0166MER166ER167ER168TM169ER17CY0170TM171Y8171YB172SUTOT

TOTAL

2.394-008 2.162-OCE 1.952-008 1;763-0081.761-008 1.826-00e 1.884-0082.248-005 2.248-005 2.248-00SI.C80-013 1.333-014 1.645-C158.S02-006 e.9C2-0C6 8.902-C061.748-006 1.487-00e 1.266-0062.424-006 2.6E4-0Cd 2.906-0065.525-007. 4.4eC-oC7 3.387-C071.4E3-0061.988-0C6 2.097-C066.776-006 6.776-OC6 6.776-0063.452-008 3.452-OCE 3.452-0083.C09-006 3.0C9-OC6 3.009-0065.C24-007 5.024-OC7, 5.024-C072.446-007-2.446-OC7 2.446-0072.159-008.2.159-00e 2.1,59-C089.905-008 9.9C5-0OC 9.905-0087.196-008 7.196-OCe 7.196-0083.982-008 3.982-008 3.982-C088.E45-009 8.845-OC9 8.845-C091.t64-008 1.664-008 1.664-0086.274-011 6.267-011 6.260-C115.152-009 5.152-OCS 5.152-0091.C95-009 1.095-OCS 1.C9s-0099.718-010 9.718-01C 9.718-0102.558-012 2.558-012 2.558-C123.729-016 3.729-016 3.729-0162.536-013 2.536-013 2.536-0139.298-017 4.517-017 2.194-0175.542-015 -5.59C-015 5.613-0155.C19-017-5.01S-017 5.C19-C171.C33-002 1033-002 1.C33-C02

1.937-0082.248-O0S2.030-0168.902-006I.078-OC63.094-OC62. 561-OC72.1.79-0066.776-0063.452-OC83.009-OC65.024-0072.446-0072.159-0089.905-0087.196-OC83.982-OC88.845-OC91.664-OC86.253-0115.152-OC91.095-OC99.71e-OIC2.558-0123.729-0162.536-0131.066-0175.625-0155.019-0171.033-002

1.033-OC21.C33-002-1.033-OC2 1.033-C02

.

.~~ ~ ~~~~ . I

E.13

TABLE E.l.f. Fission Products (Elemental), g/gU, at 10 MWd/kgM


HLIBE

C-ZN-GAGEASSEeRKRRaSR

ZRNBMOTCRU.RHPDAG.CD.INSNSB -

TEI

XE-CSBALACEPRNDPMSMEUGDTBDYHOERTMYESUMTO1

9.295-009 .3C8-OC9 7.426-0099.S70-011 .97C-011 9.970-0114.556-011 4.556-011 4.556-011S.CO1-01Z'7.999-012 7.997-C121.348-014 1.348-014 1.348-0142.422-013-2.422-013 2.422-G132.121-007-2.121-OC? 2.121-CO?6.455-008 6.455-OCE 6.'455-C081.E26-005 1.826-005 1.826-0057.187-0067.187-006 7.187-0061.205-004 1.2CC-OC4 1.196-C041.202-004 1.2C7-OC4'1.212-C042.649-004 2.581-OC4 2.517-C041.572-004 1.572-OC4"1.572-0041.184-003 1.191-OC3 1.197-C031.'87-009'1.6C1-OCS 1.816-0091.C29-003 1.029-OC3 1.029-C032.528-004 2.52E-OC4 2.528-C045.571-0045.971-OC4 5.971-C041N.e1-004 1.631-004 1.631-0042.83-004 2.6e3-OC4'2.683-C041.719-005 1.719-005 1.719-0052.C57-005 2.056-005 2.C56-0051.5'65-00 1.569-O0 1.571-C062.546-005 2.54i-OC5 2.546-0056.C17-006 5.888-OCt 5.810-0061.384-004 1.385-004 1.386-0046.776-005 6.776-OC5 6.776-0051.494-003 1.494-OC3 1.494-0038.511-004 E.379-004 8.255-0045.CO9-004' 5.14C-004 5.265-C04

6.637-0099.970-0114.556-0117.995-0121.348-0142.422-0132.121-OC76.455-0081.826-0057.187-0061.192-OQ41.216-0C42.456-OC41.572-0041.203-0032.031-OC91.029-OC32.528-OC45.971-OC4I .631-OC42.683-OC41.719-0052.056-0051.574-0062.546-0055.763-0061.386-0046.776-0051.494-0038.136-0045.383-OQ43.797-O47.261-0043.515-0041.254-0031.144-0062.715-0042.475-0051.536-0055.024-0072.413-0071.670-0087.219-0092.558-0122.593-0131.033-002r

3.797-0047.262-0043. 515-0041.254-003S.585-0062.674-0042.544-0051.435-005S.C24-0072.413-0071.670-0087.219-0092.5 58-0122.592-013I.C33-002

3 .797-OC47.261-0043.515-OC41.254-0033.292-OC62.696-OC42.514-OC51.475-OCS5.024-OC?2.413-0071 .670-00e7. 219-0092. 558-0122.593-0131 .033-002

3.797-0047.261-0043.515-G041.254-C031.941-0062.708-0042.4 92-0051.508-0055.024-0072.413-0071.670-0087.219-0092.558-C122.593-0131 .C33-002

TOTAL I.C33-002 1.033-OC2 1.033-002 1.033-002

E. 14

TABLE E.1.g. Fission Products (Isotopic), C/gU, at 10 MWd/kgM


H 3BE 10C 14

SE 79K R 81KR 85R8 87SR 90Y 90

ZR 93NE 93PNE 94TC 98TC. 99RHI02RU106RH106PD107A6108AGIOV8AG109YCD109AGIIOAG11OPCD113 SN1 19PSN121SN123TEl23VSB125TE125PSN126SB126S8126FTE127TE127PI129

CS134CS135CS137BA137MCE142CE144PR144PR144VN0144PM146-SM146PM1147S4147EU150SMf151

8.574-005 8.021-OCS 7.169-COS6.857-013 8.857-013 8.857-0133.568-011 3.567-011 3.566-011t.301-007 1.3C1-OC7 1.301-0076.475-014 f.475-014 6.475-014-1.459-003 1.458-003 1.281-0037.298-012 7.2SE-012 7.298-0121.578-002 1.886-OC21.S79-002 1.887-OC25.561-007 5.961-OC72.485-007 2.793-0073.C90-011 3.09C-0115.347-013 5.347-0134.287-006 4.2e7-OCt1.148-008 7.115-OCS1.185-004 2.9S4-0051.185-004 2.9S4-OC52.229-008 2.229-OCE4.516-013 4.467-0135.C75-012 5.019-0121.241-013 4.1t8-0141.241-013 4.16E-0141.540-010 2.03C-0111.158-008 1.526-0097.E44-006 7.133-0061.564-009 2.487-01C4.369-008 4.249-OC03.242-012 6.432-0142.748-016 4.022-01E3.381-004 2.05C-0048.249-005 5.0C2-OC52.184-007 2.184-0073.C57-008 3.057-OCE2.184-007 2.184-0073.132-013 3.0C9-0153.198-013 3.072-0159.229-009 9.229-005.f50-004 2.987-0C42.146-007 2.146-OC72.491-002 2.378-0C22.356-002 2.25C-0028.423-012 8.423-0125.243-005 8.831-O65.244-005 8.831-0066.292-007 1.060-0074.181-016 4.181-0161.285-007 9.9e9-OCE3.284-014 3.367-0145.179-003 3.053-OC32.340-012 2.392-0125.619-012 5.4C7-0121.904-004 1.875-004

E.15

1 .799-0021 .799-Ca25.961-C73.C71-0073.090-0115.347-C134.287-CC64.411-0097.569-C067.569-0062.229-COS4.419-C134.9 65-0121.400-0141.4 00-0142.476-Cl22.C12-0106.486-G063.149-C114.133-CO1.276-C151.273-0191.243-C043.C32-0052.1 84-0073.057-0082.1 84-0072.901-0172.962-0179.229-0091.525-0042.146-0072.271-0022.148-0028.423-C121.487-0061.487-0061.785-0084.181-0167.764-0083.432-0141.800-0032.423-0125.203-0121.846-004

6.408-00 58.857-0133.56S-0111.300-OC76.475-0141.125-OC37.298-0121.715-0021.716-0025.961-OC73.322-OC?3.090-0115.347-0134.287-OC62.735-OC91.913-0061.913-0062.229-OC84.371-0134.911-0124.700-0154.70C-0153.527-0132.652-0115.898-OC63.988-0124.020-OC82. 535-017

.0007.532-OC51.838-0052.184-OC73.057-0082.184-0072.787-0192.325-0199.229-0097.784-OCS2.146-0072.169-0022.051-0028.4 23-0122. 505-0072.505-0073.006-0094.181-0166.034-0083.482-0141.061-0032.441-0125.006-0121.818-004

TABL EE.1.g. (Contd)

IC YEARS 12 YEARS 14 YEARS 16 YEARS w

EU152 4.141-006 3.74C-OCd 3.378-006 3.050-006GD153 3.809-010 4.TCI-011 5.802-012 7.161-013EU154 4.719-004 4.017-OC4 3.419-004 2.910-004EU155 2.757-004 2.084-004 1.576-004 1.192-004H0166P 1.126-010 1.125-O1C 1.124-010 1.123-010TP171 1.C13-013 4.92C-014 2.390-014 1.161-014 %SUITO 9.728-002 9.0C6-OC2 8.435-002 7.954-OC2

TOTAL 9.728-002 S.oC6-oC2 8.435-002 7.954-002

E.16

TABLE E.1.h. Fission Products (Elemental), C/gU, at 10 MWd/kgM

IC YEARS 12 YEARS 14 YEARS 16'YEARS

H 8.S74-005 E.021-OC5 7.169-C05 6.408-OCSBE 8.857-013 8.857-013 8.857-013 8.857-013C 3.568-011 3.567-011 3.566-011 3.565-011

SE 1.301-007 1.3G1-0C? 1.301-C07 1.300-OC?KR 1.659-003 1.458-003 1.281-C03 1.125-003RB 7.298-012 7.296-012 7.298-012 7.298-012SR 1.978-002 1.886-OC2 1.799-002 1.715-OC2

Y 1.S79-002 1.887-02 1.799-002 1.716-OC2ZR 5.S61-007 5.961-OC? 5.961-C07 5.961-OC7NB 2.466-007 2.794-007 3.C72-007-3.323-007TC 4.287-006 4.287-006 4.287-C06 4.287-006RU 1.185-004 2.994-OC5 7.569-CO6 1.913-OC6RH 1.185-004 2.995-005 7.573-.CO6 1.916-OC6PD 2.229-008 2.229-008 2.229-C08 2.229-008AG f.174-008 1.552-OCS 2.C93-C1O 3.222-011'CO 7.E44-006 7.133-OCd 6.486-C06 5.898-OC6SN 2.t40-007 2.611-OC7 2.597-CO7 2.586-OC7-SB 3.383-004 2.052-004 1.245-004 7.557-OCS;TE 8.249-005 S.OC2-OC5 3.C32-005 1.838-OC5I 9.229-009 9.229-OC9 9.229-009 9.229-OC9

CS 2.550-002 2.4C.-OC2 2.286-002 2.176-OC2BA 2.356-002 2.25C-OC2 2.148-C02 2.051-OC2CE 5.243-005 8.831-OC6 1.487-006 2.505-007PR 5.307-005 1.937-OC6 1.505-C06 2.535-007ND 4.181-016 4.181-016 4.181-C16 4.181-016PM 5.179-003 3.053-OC3 1.800-003 1.061-003SM 1.SG4-004 1.875-004 1.846-004 1.818-004EU 7.517-004 6.139-OC4 5.C29-004 4.132-00460 3.809-010 4.7C1-011 5.E02-012 7.161-013HO 1.126-010 1.125-01C 1.124-010 1.123-010TM 1.C13-013 4.920-014 2.390-014 1.161-014SUMTOT 9.728-002 9.OC6-OC2 8.435-002 7.954-002

TOTAL 9.728-002 9.OC6-002 8.435-002 7.954-002

E.17

TABLE E.1.i. Neutron Source (Alpha-n), Neutrons/sec-gU,at 10 MWd/kgM


PU238 1.591-001 1.566-001 1.542-001 1.518-00'PU239 1.f69-001 1.668-OC 1.668-001 1.668-OC'PU240 s 1.259-C01!1.258-OC1 1.258-CO 1.258-00'AM241 4.197-001 4.765-OCI 5.277-001 5.739-00'CM242 - 1.-399-003 1.3E-OC3 1.375-C03 1.363-00:CI244 7.410-003 6.864-OC! 6.358-C03 5.890-OC:

TABLE E.1.J. Neutron Source (Spontaneous fission),Neutrons/sec-gU, at 10 MWd/kgM


U238 - 1.227-C02 1.227-002 1.227-02 1.227-O0PU238 2.595-002 2.555-OC2 2.515-002 2.476-00PU240 6.635-001 6.634-O1 6.632-C01 6.631-00'PU242 4.S76-002 4.976-OC2 4.976-002 4.976-OC;CM242- ; 6.786-003 6.733-003 6.672-003 6.611-OCCM244 8.522-001 8.264-OCI 7.655-CO1 7.091-OC

1III33

221231

E.18

TABLE E.2.

Subtable

E.2.a

E.2.b

E.2.c

E.2.d

E.2.e

E.2.f

E.2.g

E.2.h

E.2.i

E.2.J


Species-Units



Actinides (Isotopic), C/gU E.23

Actinides (Elemental), C/gU E.25

Fissibn Products (Isotopic), g/gU E.26


Fission Products (Isotopic), Ci/gU E.31


Neutron Source (Alpha-n), Neutrons/sec-gU E.34

Neutron Source (Spontaneous fission), Neutrons/sec-gU E.34

E.19

TABLE E.2.a. Actinides (Isotopic), g/gU, at 15 MWd/kgM

IC YEARS 12-YEARS 14 YEARS' 16 YEARS

HE 4P8207P8208PB212RA224RA226AC227TH228TH229TH230TH231TH232T.H 234PA231PA233U232U233U234U235U236U237U238NP235NP236NP237NP238NP239PU236PU238PU239PU240PU241PU242PU244AM241AM242PAM242AM243CM242CM243CM244CM245CM246CM247CM248SF250SUMTOl

2.259-007 2.555-007 2.867-CO72.219-015 3.412-015 4.955-0151.C78-011 1.449-011 1.836-0113.200-015 3.399-015 3.500-C152.791-014 2.965-014 3.053-C141.893-015 2.917-015 4.250-C151.787-014 2.359-014 2.997-0145.424-012 5.747-012 5.919-C124.593-014 5.243-014 5.983-0144.S96-011 6.638-011 8.500-0115.292-G14 5.292-014 5.292-G147.274-010 1.546-OIC 9.819-0101.398-011 1.398-011 1.398-C111.566-010 1.818-01C 2.C71-CIO

F

I

5.275-012 5.3C2-012 5.332-C122.299-010 2.327-01C 2.326-C107.C26-010 E.07C-01C 9.120-t102.746-006 3.145-006 3.538-0061.'02-002 1.3C2-OC2 1.302-C022.186-003 2.166-003 2.186-0031.108-011 1.0G6-011 9.136-0129.629-001 9.629-001 9.629-0011.652-015 4.6CC-01 1.281-0161.C87-010 1.087-01C 1.087-0101.553-004 1.561-004 1.570-0046.C02-014 5.948-014 5.894-G147.334-012 7.332-012 7.331-0121.905-011 1.171-011 7.202-0122.588-005 2.548-005 2.508-CO54.336-003 4.336-OC3 4.336-0031.186-003 1.186-003 1.185-C033.577-004 3.249-004 2.951-0049.475-005 9.675-OC5 9.675-0059.C56-010 9.056-01C 9.C56-C102.380-004 2.7CO-004 2.989-0043.201-007 3.172-OC7 3.143-0073.129-012 3.795-012 3.760-0128.534-006 8.532-OC6 8.530-0067.749-010 7.686-010 7.617-0103.C53-008 2.9Ce-008 2.770-0086.818-007 6.316-007 5.851-0072.C06-008 2.00S-008 2.005-0081.COI-009 1.001-00 1.001-0094.124-012 4.124-012 4.124-C128.952-014 8.952-014 8.952-0149.617-013 1.047-012 1.128-0129.E45-001 9.845-001 9.845-C01

3.191-OC76.888-0152.231-0113.541-0153.089-0145 .930-0153.698-0145.987-0126.813-0141.058-0105. 292-0141.109-OC91.398-0112.323-01C5.366-0122.309-010I.018-093. 925-0061.302-0022.186-OC38.297-0129.629-0013.567-0171.087-0101.580-0045.840-0147.330-0124.429-0122.469-0054.335-OC31.185-0032.680-0049.675-OC59.056-0103.250-0043.115-0073.726-0128.529-0067.548-0102.639-0085.419-0072.005-0081.000-0094.124-0128.952-0141.203-0129.845-001

TOTAL 9.845-001 9.845-001 9.845-001 9.845-001

E .21

ThBLE E.2.b. Actinides (Elemental), g/gU, at 15 MWd/kgM


HESFP3RAACTNPA

UNPPUAMCMSUMTOT

2.259-0079.417-0131.C78-012.583-0141.787-0147. 569-0101.d19-0109.781-0011.553-0046. C02-0032.463-0047.3 42-0079.E45-001

2.555-OC71.047-0121.45C-0113.26C-0142.359-0149.4C8-01C1 .871-01C9.781-OC11.561-0045.969-OC32.789-OC46.825-OC79.845-O1

2.867-CO?1.128-0121.837-C113.482-C142.997-C141.C87-0092.124-0109.781-COI1.570-0045.938-C033.C78-C046. 3 46-0079.345-001

3.191-OCI1.203-0122.232-0113.687-0143.698-0141.235-0092.377-0109.781-OC1.580-0045.910-0033.338-0045.901-OC?9.345-OCI

TOTAL 9.E45-001 9.845-OCI 9.845-COI 9.845-001

'-S

E.22

TABLE E.2.c. Actinides (Isotopic), C/gU, at 15 MWd/kgM


TL207TL208'TL209P8209P821CP8211P921,2PE214BI210812118I21281213B1214P0210P0211P0212P0213P0214P0215P0216 -P0218AT217RN219RN220 ;RN222FR221FR223RA223RA224RA225RA226AC225AC227TH227tH228tH229TH230TH231TH232TH234PA231PA233PA234P,PA234U232U233U234U235U236U237U238U240

1.290-012 1.7C-012 2.167-0121.598-009 1.6S7-OC9 1.748-0092.111-016 2.41C-01 2.750-0169.774-015 1.116-014 1.273-0142.547-016 3.813-016 5.7.03-C161.293-012 1.71C-012 2.173-0124.447-009 4.724-OC9 4.865-C091.872-015 2.885-015 4.202-0152.548-016 3.815-016 5.705-C161.293-012 1.71C-012 2.173-0124.447-009 4.724-009.774-015 1.116-0141.E72-015 2.885-0152.548-016 3.411-0163.621-015 4.7E7-0152.849-009 3.027-0C99.563-015 1.092-0141.872-015 2.884-0151.293-012 1.71C-0124.447-009 4.724-0091.873-015 2.885-0159.774-015 1.116-0141.293-012 1.710-0124.447-009 4.724-0091.E73-015 2.865-0159.774-015 1.116-0141.784-014 2.356-0141.293-012 1.71C-0124.447-009 4.724-OCS9.774-015 1.116-0141.873-015 2.885-0159.774-015 1.116-0141.293-012 1.7C7-0121.275-012 1.686-0124.447-009 4.713-0099.774-015 1.116-0141.C09-012 1.34C-0122.814-008 2.815-OCE7.S&1-017 9.377-0173.238-007 3.238-0077.399-012 8.592-0121.C95-007 1.IC1-0073.238-007 3.238-0074.210-010 4.21C-QiC4.923-009 4.982-0096.£04-012 7.815-0121.716-008 1.966-0082.E14-008 2.815-0081.415-007 1.415-0079.C44-007 8.214-0073.238-007 3.238-0071.f05-014 1.6C5-014

4.865-0091.2 73-0144.202-0155.101-C16

.83-0 153.117-C091.246-C144.202-0152.173-0 124.865-0094.203-Cl 51.273-0142.173-C 124.E65-0094.203-C151.273-0142.993-0142.173-C124.865-0091.273-0144.203-0151.273-0142.169-0122.143-0124.8 53-0091.273-0141.716-0122.815-0081.077-0163.2 38-0079.785-0121.107-C073.238-0074.210-0104.981-0098.832-0122.211-0082.815-COB1.415-0077.460-0073.238-0071.605-014

2.673-0121.768-0093.132-0161.450-0148.375-0162.681-0124.922-0095.864-0158.379-0162.681-0124.922-0091.450-0145.864-0157.529-0167.506-0153.153-0091.419-0145.863-0152.681-0124.922-0095.865-0151.450-0142.681-0124.922-0095.865-0151.450-0143.693-0142.681-0124.922-0091.450-0145.865-0151.450-0142.676-0122.644-0124.909-OC91.450-0142.136-0122.815-0081.217-0163.238-0071.098-0111.114-0073.238-0074.210-0104.944-0099.855-0122 .453-0082.815-0081 .41 5-0076. 775-0073. 238-0071 605-014

E. 23

TABLE E.2.c. (Contd)


NP235NP236NP237NP23aNP239NP24OMPU236PU238PU239PU240PU241PU242PU243PU244AM241AM242PAM242AM243CM242CM243CM244CM245C 246CR247CR248BK249CF249Cf250CF252SUMTOT

2.318-012 6.456-0131.432-012 1.432-0121.C95-007 1.1C1-OC?1.556-008 1.542-0081.702-006 1.7C-UCd1.f05-014 1.6C5-0141.C12-008 6.226-0054.432-004 4.363-OC42.496-004 2.696-OC42.703-004 2.7G3-OC43.487-002 3.348-OC23.696-007 3.696-OC73.828-016 3.828-0161.407-014 1.6C7-0148.171-004 S.27C-OC43.112-006 3.084-OC63.C97-006 3.069-0Ct1.702-006 1.7C2-0Cd2.563-006 2.542-OCt1.577-006 1.5C2-00t5.519-005 5.112-OC53.445-009 3.444-0093.C76-010 3.076-01C3.828-016 3.828-0163.808-016 3.8C8-0162.745-016 5.641-0172.118-015 2.111-0154.340-015 3.9C4-0151.705-016 1.0C8-0163.f74-002 3.545-002

1 .798-C131.432-0121.107-0071 .528-C081.701-0061.605-0143.823-0094.2 95-0042.696-C042.702-0043.C41-0023.696-C073.828-0161.607-0141.C26-C033.056-0063.C41-C061.701-C062.519-C061.430-CO64.7 35-0053.444-0093.C75-C1O3.8 28-0163.807-0161.160-0172.102-0153.511-0155.961-Cl?3.247-002

5.006-0141.432-0121.114-0071.514-OC81.701-OC61 .605-0142.354-0094.228-OC42.696-OC42.702-0042.762-OC23.696-0073.828-0161.607-0141.116-0033.028-0063.013-0C61 .701-OC62.497-OC61 .363-OC64.386-OC53.443-OC93.074-0103.828-0163.8G7-0162. 375-0182.094-0153.158-0153. 525-0172.976-002

TOTAL 3.874-002 3.545-002 3.247-C02 2.976-002

'-

E.24

TABLE E.2.d. Actinides (Elemental), C/U, at 15 MWd/kgM


TLPe

POAT'RNFRRAAC

PAU'

NP:PUAMCMBKCFSUMTCT

TOTAL

1.599-009 1.6S9-009 1.750-0094.449-009 4.726-OC9 4.867-0094.449-009 4.726-009 4.867-0097.298-009 7.752-009 7.984-0099.774-015 1.116-014 1.273-C144.449-009 4.726-OC9 4.867-C092.762-014 3.471-014 4.266-014-4.449-009 4.726-OCS 4.867-0091.303-012 1.712-012 2.182-C123.564-007 3.567-007 3.569-C074.338-007 4.344-0C7 4.350-0071.420-006 1.34C-004 1.267-0061.227-006 1.827-0061.827-0063.785-002 3.446-002 3.138-0028.250-004 9.349-OC4 1.034-0035.S33-O0S 5.517-005 5.131-CO52.745-016 5.641-017 1.160-C176.657-015 t.143-015 5.701-0153.E74-002 3.545-OC2 3.247-002

3.274-002 3.545-OC2 3.247-002

I .771-OC94.924-0094.924-0098.07e-oC91.45C-0144.924-0095.143-0144.924-OC92.690-0123.569-0074.357-0071 .201-OC61. 827-OC62.858-O21 .124-OC34.773-0052.375-0185.316-0152.976-002

2.976-002

E.25

TABLE E.2.e. Fiision Products (Isotopic), g/gU, at 15 MWd/kgM


H 3Lt 6LI 7SE 9Bt 10

C 14ZN 66ZN 67GA '71GE *72GE 73GE 74AS 75GE 76SE 76SE 77SE 78SE 79OR 79SE 80KR 80BR 81KR 81SE 82KR 82KR 83CR 84KR 85RB 85KR 86SR 86RS 87SR 87SR 88

Y 89SR 90

Y 9CZR 90ZR 91ZR 92ZR 93NB 93NO 93PZR 94NO 94Mo 95ZR 96NO 96MO 97Mo 98TC 98TC 99

1.435-008 1.283-OC81.246-010 1.246-OlC4.613-012 4.613-0128.887-012 e.887-0125.S29-011 5.92S-0111.197-011 1.197-0111.816-014 1.816-0147.586-016 7.586-0163.E52-013 3.852-0139.897-009 9.897-OC92.129-008 2.129-0084.495-008 4.495-OCe9.566-008 9.566-0CC2.!69-007 2.369-OC71.270-009 1.270-0094.85-0071.107-0062.756-0063.357-0106.266-0069.C8S4-0111.C47-0056.335-0121.606-0052.474-0072.269-0055.150-0056.C63-0065.279-0059.236-0059.459-0081.188-0047.577-0101.707-0042.234-0042.C62-0045.171-0086.451-0052.E66-0043.C69-0043.438-0044.989-0101.276-0093.464-0042.963-0103.624-0043.718-0047.317-0063.450-0043.761-0041.383-0093.721-004

4.98 5-OC71.IC7-OC62.756-0063.945-01Cf.26d-OCd9.084-0111.047-0056.335-0121 .6C6-OC52.474-0072.269-OC55.15C-OC55.328-0065.352-0059.234-OC59.459-0C1 .188-0047.577-01E1 .7C7-OC42.234-OC41 .966-OC44.931-0087.41C-0052.866-0043.069-0043.438-OC46.527-O11.433-0093.464-0042.963-01C3.624-0043.718-0047.317-OC63.650-0043.761-0041 .383-0093.721-004

E. 26

1.147-008 1.0Z5-OC81.246-CIO 1.246-0104.613-012 4.613-0128.887-012 8.887-0125.929-Ci1 S.929-0111.197-011 1.196-0111.816-C14 1.816-0147.586-016 7.58; `63.852-C13 3.852-. 39.897-C09 9.897-OC92.129-COB 2.129-0084.495-008 4.495-0089.566-C08 9.566-0082.369-C07 2.369-0071.270-009 1.270-0094.985-007 4.985-0071.107-C06 1.107-0062.756-006 2.756-OC64.533-010 5.122-0106.266-006 6.266-OC69.084-011 9.084-0111.047-005 1.047-0056.335-012 6.335-0121.606-005 1.606-0052.474-007 2.474-0C72.269-005 2.269-0055.150-005 5.150-OC54.682-006 4.114-OC65.417-005 5.474-0059.236-005 9.236-OC59.459-008 9.459-0081.188-004 1.188-0047.577-010 7.577-0101.707-004 1.707-OC42.234-004 2.234-OC41.875-004 1.788-0044.701-008 4.483-0088.324-005 9.196-0052.866-004 2.866-0043.069-004 3.069-0043.438-004 3.438-0048.218-010 1.005-0091.576-009 1.705-0093.464-004 3.464-0042.962-010 2.962-0103.624-004 3.624-0043.718-004 3.718-0047.317-006 7.317-0063.650-004 3.650-0043.761-004 3.761-0041.383-009 1.383-0093.721-004 3.721-004

J

'-'4

TABLE E.2.e. (Contd)


RU 99MOiOORU100RUIOIRU102RH102RHI 03RU104PD1 04PD105RU1o6RH106PD106P0107A6107P0108A6108PCD108A6109CD109PDlOAGIIOPCD110CDi1CD112CD113CDI13P1IN113CD114SN114IN11SSN115CD116SN116SN117SN118SN1 19SN119VSN120SN121SEi21SN122TE122SN123S8123TE123SN124TE124SE125TEI 25TEI 25P.SN126

1.367-008 1.6C9-OCE 1.851-0084.221-004 4.221-004 4.221-0042.C98-005 2.0se-005 2.098-0053.537-004 3.537-OC4 3.537-0043.342-004 3.342-004 3.342-0042.160-011 1.339-011 8.304-C122.423-004 2.423-OC4 2.423-0042.223-004 2.223-004 2.223-0045.C91-005 5.091-005 5.C91-0051.584-004 1.584-004 1.584-0046.348-008 1.6C5-OCC 4.C56-0095.967-014 1.5CE-014 3.812-0151.254-004 1.254-OC4 1.254-0047.550-005 7.95G-005 7.950-C059.348-011 1.1G4-01C 1.274-0105o380-005 5.38C-005 5.380-COS3.745-013 3.7C4-013 3.664-0137.274-011 7.274-011 7.274-G113.C82-005 3.082-005 3.082-0051.S16-016 6.435-017 2.161-C171.785-005 1.785-005 1.785-0056.644-012 8.759-013 1.155-0136.218-006 6.218-006 6.218-0061.C40-005 1.04C-OC5 1.040-0056.525-006 6.525-006 6.525-0061.315-007 1.315-007 1.315-0076.C59-008 5.51C-OOt 5.CIO-0084.201-008 4.75C-OCt 5.249-C089.454-006 9.454-OC6 9.454-0062.357-010 2.357-01C 2.357-0101.896-006 1.896-00t 1.896-C061.456-007 1.456-OC7 1.456-0073.724-006 3.724-006 3.724-0062.406-006 2.4C6-006 2.406-0063.782-006 3.782-O06 3.782-0063.E15-006 3.815-OC6 3.815-0063.793-006 3.793-006 3.793-0067.C27-013 8.899-014 1.127-0143.E75-006 3.875-OC6 3.875-0061.242-009 1.2C8-009 1.175-0093.916-006 3.916-OCt 3.916-0064.280-006 4.28C-006 4.280-0061.243-007 1.243-007 1.243-0076.107-016 1.212-017 2.404-0194.769-006 4.769-006 4.769-0061.111-009 1.111-009 1.111-0095.799-006 5.799-006 5.799-0069.196-008 S.196-OC 9.196-0085.171-007 3.135-007 1.901-0077.886-006 8.092-0C6 8.218-0067.233-009 4.386-OC9 2.659-0091.211-005 1.211-005 1.211-005

E.27

2.093-0084.221-0042.098-0053.537-0043.342-0045 .148-0122.423-0042.223-OC45.09 1-0051.584-0041.025-0099.636-0161.254-0047.950-0G51.444-0105.380-0053.624-0137.274-0113.082-0057.256-0181.785-0051 .522-0146.218-0061.040-OC56.525-OC61.315-0074. 556-0085.703-0089.454-0062.357-0101.896-0061.456-0073.724-0062.406-0063.782-0063.81 5-0063.793-0061.427-0153.875-0061.142-0093.916-0064.280-0061.243-0074.776-0214.769-0061.111-0095.799-0069.196-0081.152-0078.293-0061.612-0091.211-005



a8126Sb126TE126TE127P1127

TE128XE128I129

XE129TE130XE13CXE131XE1323A132C S133XE134CS134BA1 34CS1353A135XE136BA136CS137SAl 37YA137BA138LA138LA139CE140PRI41CE142ND142ND143CE144PR144PRI44PND144ND145ND146P14146SM146PI147SM147ND148S148SM149ND150SM150EUi50SM151EU151SMI 52

5.756-0134.376-0152.848-0075.441-0172.458-0054.863-0056.117-0078.C89-0051.719-0091.570-0042.t02-0062.313-0044.450-0044.162-0105.538-0046.t84-0049.875-0073.t44-0052.2 21-0042.d95-0089.630-0046.313-0064.'02-0041.282-0046.5 81-0115. 6 5-0043.327-0095.i28-0045.5 99-0045.203-0045.197-0045.554-0064.!42-0042.398-0081.C13-0125.C62-0155.4 38-0043.314-0042.S56-0045.916-0101.930-0097.2 21-0061.335-0041.681-0045.610-0051.862-0067.778-0051.113-0041 .C68-0138.296-0066.780-0076.626-005

5.756-013 5.756-0134.376-015 4.376-0152.849-OC7 2.851-0075.228-019 5.019-G212.458-005 2.458-C054.863-OC5 4.863-0056.117-007 6.117-0078.089-O05 8.C89-0051.726-OC9 1.734-C091.57C-OC4 1.570-C042.6C2-006 2.602-C062.313-OC4 2.313-C044.45C-0C4 4.450-0044.162-010 4.162-C105.538-004 5.538-C046.684-OC4 6.684-0045.041-OC7 2.574-0073.692-OCS 3.717-C052.221-OC4 2.221-C042.7C9-008 2.722-C089.63C-OC4 9.630-C046.313-OC6 6.313-C064.1C8-004 3.922-0041.476-004 1.662-0046.284-011 6.COO-C115.865-004 5.865-0043.327-OC9 3.327-0095.628-OC4 5.628-0045.599-OC4 5.599-C045.2C3-004 5.203-0045.197-OC4 5.197-0045.554-006 5.554-0064.342-OC4 4.342-0044.039-0C9 6.803-0101.7C5-013 .2.872-C148.525-016 1.436-C165.438-OC4 5.438-C043.314-OC4 3.314-0042.956-004 2.956-0044.598-01C 3.574-0101.979-005 2.017-0094.257-006 2.510-C061.365-004 1.382-0041.681-004 1.681-0045.610-005 5.610-0051.862-00 1.862-0067.778-005 7.778-0051.113-004 1.113-0041.027-013 9.884-0148.169-OC6 8.C44-006

5.755-0134.376-0152.853-0073.940-0232.458-0054.863-0056.117-0078.089-OC51.741-0091 .570-0042. 602-0062. 31 3-0044.450-0044.162-0105.538-0046.684-OC41.314-0073.729-OC52. 221-0042.735-OC89.630-OC46. 313-00 63.745-0041.839-0045.729-0115.865-OC43.327-OC95.628-OC45. 599-0045.203-0045.197-0045.554-0064. 342-0041.146-0104.838-0152.418-0175. 438-0043.314-0042.956-0042.778-0102.046-0091.479-OC61.392-0041.681-0045.610-0051 .862-0067.778-0051.113-0049.511-0147.921-006

8.048-00? 9.297-007 1.053-0066.626-OC5 6.627-005 6.627-005

E.28

; I TABLE E.2.e. (Contd)


EU15260152EU1S36D1 53SM1 54EU1 546D154EV1556D1556D1566D1 57GC158T8 1596D160DY160DY161DY162DY163DY164N0165H0166FER166ER167ER168TM169ERI 70YB 170TMt71Y8171YB172SUMTOT

TOTAL

2.360-008 2.131-001 1.925-008 1.738-OCe1.763-008 1.826-OE 1.E84-008 1.936-OC8-3.S82-005 3.982-OG5 3.S82-005 3.982-0051.791-013 2.211-014 2.728-015 3.367-0161.479-005 1.479-OCS 1.479-005 1.479-OC54.11S-006 3.503-00t 2.981-06 2.537-0065.99-006 6.312-006 6.833-006 7.277-0061.C22-006 7.730-007 5.845-007 4.419-0073.159-006 3.4G8-006 3.597-006 3.739-0061.391-005 1.391-005 1.391-005 1.391-0054.561-008 4.561-00e 4.561-008 4.561-0085.601-006 5.6C1-OG6 5.601-C06 5.601-OC69.232-007 9.232-OC? 9.232-007 9.232-0074.S509-007 4.SC9-007 4.509-007 4.509-0075.607-008 5.607-008 5.607-008 5.607-0081.704-007 1.7C4-007 1.704-007 1.704-0071.334-0078.117-0081.483-0083.495-0081.881-0101.C51-0081.546-0092.120-0098.139-0121.606-0151.225-012

8.£71-0164.C79-0145.619-0161.547-002

1.*547-002

1.334-007 1.334-007 1.334-0078.117-008 8.117-008 8.117-0081.483-00C3.495-OC01.878-01C1 .051-Oc01 .546-0C92.12C-OC98.139-0121.8Cd-0151.225-0123.338-0164.114-0145.619-011.547-002

1.547-OC2

1.483-C08 1.483-0083.495-008 3.495-OC81.876-010 1.874-0101.051-C08 1.051-0081.546-009 1.546-0092.120-009 2.120-0098.139-012 8.139-0121.806-CIS 1.806-0151.225-012 1.225-0121.621-016 7.876-0174.131-C14 4.140-0145.619-016 5.619-0161.547-002 1.547-002

1.547-002 1.547-002

E.29

TABLE E.2.f. fission Products (Elemental). g/gU, at 15 MWd/kgl4

IC YEARS 12 YEARS 14 YEARS 16 YEARS'S4

HLI3EC

ZNGAGEASSE9RKRR3SR

yZRNB8MOTCRURHPDAGCD-INSNS3TE

IXECS3ALACEPRNDPMSMEUGDTBD YH0ERT MYBSUMTOT

1.435-0081.292-0106.817-0111.197-0111.892-0143.852-0133.130-0079.566-0082.t69-0051 .C47-0051.729-0041.716-0043.770-0042.235-0041.720-0032.C71-0091.5 33-0033.721-0049.313-0042.423-0044.858-0043.C82-0053.e51-0051.938-0064.C01-0059.202-0062.140-0041.C55-0042.311-0031.207-0037.575-0045.628-004I.C80-0035.203-0041.856-0037.221-0063.S21-0044.5 66-0052.888-0059.232-0074.5 59-0073. 514-0081.418-0088.140-0121.266-0121.547-002

1.283-0081 .292-O1C6.817-0111.197-0111.892-0143.85 2-0133.13C-0079.566-0082.6e9-OC51.047-OC51.721-0041.724-OC43. 67 4-0042.235-OC41.73C-OC32 .382-0091.533-0033.721-OC49.313-OC42.423-OC44.859-0043.082-OCs3.6 51-0051.943-O04.OC1-0058 .999-0062.142-OC41.055-0042.311-OC31 .187-OC37.774-OC45.628-0041 .0eC-0035.2C3-004I .856-OC34.257-OC63.95C-OC44.492-0052.974-OC59.232-0074.559-0073.514-0081. 41 8-0088.14C-0121.266-0121.547-0C2

1.147-COS1.292-0106. 817-0111.197-0111.892-C143.852-C 133.130-0079.566-0082.669-CO51.C47-CO51.715-0041.730-CO43.52-Co42.235-0041.739-0032.694-C091.533-0033.721-0049.312-0042.423-CO44.859-CO43.082-CO53.650-C051.948-0064.001-0058. 875-0062.143-0041.055-C042.311-C031.168-0037.962-0045.628-0041.C80-0035.203-0041.856-G032.510-0063.966-0044.433-0053.045-0059.232-0074.559-0073.514-COB1.418-0088.139-C121.266-0121.547-002

1.025-0081.292-0106.817-0111.196-0111.892-0143.352-0133.130-0079.566-0082.669-0051.047-OC51 .709-OC41.736-OC43.495-0042.235-0041.747-0033.005-0091.533-0033.721-0049.312-OC42.423-OC44.859-0043.082-OC53.650-0051.953-0064.001-0058.800-OC62.144-OC41.055-0042. 311-0031.151-0038.140-0045.628-0041 .080-OC35.203-0041.856-0031.480-OC63.975-0044.387-0053.104-0059.232-OC74.559-0073. 51 4-0081.418-0088.139-0121.266-0121.547-002

TOTAL 1.547-002 1.547-002 1.547-002 1.547-002

E.30

TABLE E2.g. Fission Products (Isotopic), C/gU, at 15 MWd/kgM

10 YEARS 12 YEARS 14 YEARS 16 -YEARS

BE .1-C 14

SE 79KR 81KR 85RE 87SR 90Y 90

ZR 93NO 93rNB 94rC 98TC 99RHI02RU106RH106P0107A6108A6108PA6109PCD109AGIOAG110FCD113PSN1I19FSN121rSN123TE123FSB125TE125VSN126S8126S8126FTE 27TE127f1129

CS134CS135CS137BAl 37MCE142CE144PR144PR144HN0144PH146SH146PM14?SM147EU150SM151

1.386-004 1.239-0041.325-012 1.325-0125.339-011 5.337-0111.S21-007 1.921-0071.333-013 1.333-0132.'80-003 2.0S1-031.C40-011 1.04C-0112.814-002 2.683-002:2.e15-002 2.684-0028.t42-0073.607-0075.553-0111.203-0126.310-0062.f12-0082.125-0042.125-0044.C90-0088.f90-0139.764-01 24.550-0134.550-0134.200-0103.158-0081.314-0053.148-0097.344-0085.C21-0129.423-0165.342-0041.303-0043.4 39-0074.E14-0083.4 39-007S.C29-0135.134-0131.429-0081 .278-0032 .5 59-0073.744-0023.541-0021.248-0117.653-0057.653-0059.184-0076.4 36-0162.35-0076.7 54-0146.697-0033.C35-0127.071-0122.183-004

e .642-pC74.053-OC75.553-0111.2G3-0126.31C-OCt1.61S-OC85.371-0055.371-0054.09C-OCe6.596-0139.65 8-0121.662-0131.662-0135.5 36-0114.162-0091.1S5-0053.987-01C7.143-OCE9.962-0141. 39 7-0173.23E-OC4?.9C4-0C53.431-0074.814-0083.438-0074.832-0154.933-0151. 429-0086.525-OC42.S59-0073.575-0023.382-OC21.248-0111 .289-OCS1.289-0051.547-0076 .4 36-0162.048-0076.925-0143.948-0033.102-0126.8C4-0122.150-004

E.31

1.107-0041.325-Cl 25.336-C111.921-0071.333-0131.838-003I C40-0112.558-0022.559-0028.642-C074.456-CO?5.552-C111.203-0126.310-C061.004-0081.358-0051.3 58-OC54.C90-0088.502-C139.5 53-0125.581-C145. 581-0147.298-0125.487-0101.087-0055.C48-0116.948-0081.976-0151.297-0191.963-0044.791-0053.438-0074.814-0083.438-0074.643-Cl74.736-0171.429-CO83.331-G042. 5 59-0073.413-0023.229-0021.248-0112.171-0062.171-0062.605-0086.436-0161. 592-0077.057-0142.327-0033.142-0126. 547-0122.117-004

9.895-OC 51. 325-0125.335-0111.921-0071.333-0131.615-OC31.040-0112.439-0C22.440-OC28.642-OC74.820-0075.552-0111.203-0126.31C-0066.225-0093.431-0063.431-0064.09C-008E.410-0139.449-0121.874-0141.874-0149.620-0137.233-0119.884-0066.392-0126.757-0083.927-017

.0001.190-OC42.905-0053.438-0074.814-0083.438-0074.457-0193.717-0191.429-0081.701-0042.559-0073.259-0023.083-0021.248-0113.656-0073.656-0074.388-0096.436-0161.237-0077.160-0141.372-0033.166-0126'.299-0122.085-004

-1

TABLE E.2.g. Contd)


EU152 4.C83-C06 3.687-OCd 3.330-006 3.007-006GD153 6.!19-010 7.7SS-011 9.625-012 1.188-012EU154 1.111-003 9.459-OC 8.C50-004 6.852-004EU155 4.756-004 3.596-OC4 2.719-004 2.056-004i01O6 3.376-010 3.373-01C 3.369-010 3.365-010T?171 .7.485-013 3.636-013 1.766-013 8o579-014SUMTC 1.427-001 1.321-OCI 1.238-001 1.167-001

TOTAL 1.427-001 1.321-OCI 1.238-001 1.167-001

E.32

TABLE E.2.h. Fission Products (Elemental), C/gyl, at 15 MWd/kgM,


H - 1.386-004 1.23S-004 1.107-004BE 1.325-0t-2 1.325-012 1.325-012-C 5.339-011 5.337-011 5.336-011

SE 1.S21-007 1.921-OC7 1.S21-CO7KR -2.380-003 2.091-OC3 1.838-003RE 1.C40-011 1.04C-011 1 .C40-011SR 2.814-002 2.683-002 2.558-002Y 2.15-002 2.684-OC2 2.559-CO2

ZR 8.642-007 E.642-007 8.642-007NS 3.608-007 4.054-007 4.456-007TC 6.310-006 6.31G-006 6.310-006RU 2.125-004 5.371-005 1.358-COSRH 2.125-004 5.372-05 1.359-005PD 4.C90-008 4.09C-OCE 4.C90-008A6 3.201-008 4.229-OCS ,.665-C10CD 1.314-005 1.195-OC5 1.C87-005-S N 4.204-007 4.157-OC7 4.134-CO7se 5.346-004 3.242-004 1.967-004TE 1.303-004 7.9C4-005 4.791-005I - 14297008 1.429,-OCe 1.429-'008

Cs 3.871-002 3.640-OC2 3.446-002BA 3.S41-002 3.382-002 3.229-002CE 7.653-005 1.289-005 2.171-006PR 7.745-005 1.3C4-OC5 2.197-006NO 6.436-016 6.436-016 6.436-016PM 6.f97-003 3.948-003 2.328-003SM 2.183-004 2.15C-OC4 2.117-004EU 1.591-003 1.3C9-OC3 1.C40-003GD 6.319-010 7.799-011 9.625-012HO 3.376-010 3.373-01C 3.369-010TM 7.485-013 3.636-013 1.766-C13SUNTOT 1.427-001 1.321-OCI 1.238-001

9.895-0051.325-0125.335-0111.921-0071.615-OC31.040-0112.439-0022.440-OC28.642-0074.820-0076.310-0063.431-0063.438-OC64.090-0088.360-0119.884-OC64.114-0071 .194-0042.905-0051.429-OC83.276-0023.083-0023.656-0073.700-0076.436-0161.372-0032.085-0048.938-O41.188-0123.365-0108.579-0141.167-OC1

TOTAL 1.427-001 1.321-OC1 1.238-001 1.167-001

E.33

TABLE E.2.i. Neutron Source (Alpha-n), Neutrons/sec-gU, at 15 MWd/kgM

I1C YEARS 12 YEARS 14 YEARS 16 YEARS

PU238PU239PU24CAN241CM242C14243CM244

-4.217-001 4.151-01 4.087-0011.'64-001 1.964-OCI 1.964-COI2.C48-001 2.042-OCi 2.043-COI7.838-001 8.892-001 9.844-C013.441-003 3.413-003 3.382-0032.C99-003 1.9SS-OC3 1.905-0036.298-002 5.834-002 5.404-002

4.023-0011.964-0012.047-0011.070+0003. 351-0031.814-0035.006-002

TABLE E.2.j. Neutron Source (Spontaneous fission),Neutrons/sec-gU, at 15 MWd/kgM


U238 1.222-002 1.222-OC2 1.222-002 1.222-002PU238 6.877-002 6.770-OC2 6.664-002 6.561-002PU240 1.C80.000 1.080+oCC 1.C79+000 1.079+000PU242 1.631-001 1.631-OCI 1.631-COI 1.631-001CM242 1.469-002 1.656-OC2 1.641-CO2 1.626-OG2CM244 7.5834000 7.024+0CC 6.506+COO 6.027+000C1246 8.509-003 8.9C6-003 8.904-03 8.901-O3

"S0

'-I0

E.34

TABLE E.3.

Subtable

E.3.a

E.3.b

E.3.c

E.3.d

E.3.e

E.3.f

E.3.g

E.3.h

E.3.1

E. 3.


Species-Units



Actinides (Isotopic), Ci/gU E.39

Actinides (Elemental), Ci/gU E.41

Fission Products (Isotopic), g/gU E.42


Fission Products (Isotopic), Ci/gU E.47


Neutron Source (Alpha-n), Neutrons/sec-gU E.50

Neutron Source (Spontaneous fission), Neutrons/sec-gU E.50

U

E.35



HE 4P8207PE208PB212RA224RA226AC227TH228TM229TH23CG TH231TH232TH234PA231PA233U232U233U234U235U236U237U238NP235NP236NP237NP238NP239PV236PU238PU239PU240PU241PU242PU244AM241AM242PAM242AM243CM242CM243CM244CM245CM246CM247CM248CF249SF250SUMTOT

4.121-007 4.592-OC?1.73e-015 2.669-0152.C00-011 2.7CC-0116oC27-015 6.416-0155.257-014 5.5S6-0143.C27-015 4.772-0151.398-014 1.846-0141.C22-011 1.085-0117.898-014 8.795-014

;8.431-011 1.141-01C4.160-014 -4.16C-0148.-745-Cld 1.027-OCS1.392-011 1.392-0111 227-0107.817-0124.346-0109.641-0104.S48-0061.C23-0022.18-0031.33-0119.588-0012.994-0151.E40-0102.301-0049.199-0142.136-0113.710-0115.C68-0054.71.8-0031.604-0035.275-0041 .87-0043.E41-0093.489-0044.906-0075.E69-0122.485-0051.188-0098.530-0082.E76-0061.102-0077.895-0094.492-0111.358-012

1.425-01C7.857-01 24.4C2-O1C1.1 19-OC95.729-0Cf1 .023-OC22.618-0C31.483-0119.588-OCI8 .33e-0161 .84C-01C2. 31 3-0049.115-0142 .13 5-0112.281-0114.989-OCS4.718-003I .6C}-0034.791-OC41.987-0043 .841-0093.961-OC44. 862-0075.815-0122.485-0051.178-0098.125-002.664-OCt1.1C2-0077. 893-0094.492-0111.358-012

5.C83-C073.877-C153.431-Cl 16.616-Cl 55.771-C147.C80-C152.347-C141.1 19-Cu19.825-C141.481-Clo4.1 60-0141.179-CC91 .392- CI11.624-C1O7.S02-0124.403-C101.274-C096.498-0061.C23-0022.619-0031.347-Cll9.588-0012. 3 22-0161.840-C102.3 26-0049.032-0142.135-0111.403-0114.9 11-0054.717-003t .603-C034.351-0041.987-0043.841-0094.387-0044.817-0075.763-C122.4 84-0051 .167-0097..739-0082.468-C061.102-0077.891-0094.492-C111.358-0129.952-0153.544-0129.794-001

5.590-OC75. 391-0154. 178-0116.699-0155.843-0141.003-0142.897-0141.133-0111.099-0131.865-0104. 161-0141 .332-OC91.392-0111.822-0107. 951-0124.372-O1C1.431-OC97.2 56-0C61.023-OC22.619-OC31.224-0119.588-0016.466-0171.840-0102.341-0048.950-0142.134-0118.626-0124.835-0054.717-OC31.603-0033.952-0041 .987-0043.841-0094.772-0044.774-0075. 710-012?.484-0051.157-0097.372-0082.286-0061.102-0077.888-0094.492-0111.358-0129.913-0153.819-0129.794-001

1.C03-014 9.991-0152.932-012 3.249-0129.794-001 9.794-001

TOTAL 9.794-001 9.794-001 9.794-001 9.794-001

E.37

-

TABLE E.3.b. Actinides (Elemental), g/gU, at 20 MWd/kgM

IC YEARS 12 YEARS 1 YEARS 16 YEARS 'Sd

NESFPaRAACTMPA

UNPPUAMCMC FSUNTOT

4.121-0072.S32-0122.COO-C115.562-0141.398-0149.f30-0101.305-0109. 717-0012.301-0047.C98-0033.742-0043.C81-0061.144-0149.7 94-001

4. 52-0073.249-0122.7CC-0116.076-0141.84t-0141 .lee-oCs1.5C4-O1C9.717-OCI2.313-OC47.049-OC3*.21 4-OC42.865-OCd1.131-0145.754-OCI

5.C83-0073.544-C123.432-C116.483-C 142.347-C141.353-0091.703-CIO9.717-0012. 326-C04?.CO4-0034.640-CO42.665-C61.118-0149.794-CO

5.590-0073. 819-0124.179-0116.850-0142.897-0141 .544-OC91.902-0109.717-OCl2.341-0046.963-OC35.025-OC42.479-0061.107-0149.794-OCI

TOTAL 9.794-001 9.794-001 9.794-001 9.794-001

E.38

TABLE E.3.c. Actinides (Isotopic) C/gUl, at 20 MWd/kgM

TL207TIL208TL209PE209PB210P9211PE212PB214812106I21 1SI212el213BI214P0210P0211 P0212P0213P0214P021SP0216P0218AT217RN219RN220RN222FR221FR223RA223RA224RA225RA226AC225AC227TH227TH228TH229TH230TH231TH232TH234PA231PA233PA234PPA234U232U233U234U235U236U237U238U240

IC YEARS 12 YEARS 14 YEARS

1.C09-012 1.334-012 1.696-0123.C1O-C09 3.2C4-005 3.304-0093.31-016 4.043-01f 4.516-0161.681-014 1.872-014 2.091-C144.484-016 .513-016 9.624-0161.C12-012 1.338-012 1.701-0128.378-009 e.918-OCS 9.196-G092.594-015 4.71S-015 7.02-0154.466-016 6.516-016 9.'628-0161.C12-012 1.338-012 1.701-0128.378-009 8.91e-009.9.196-'0091.681-014 1.872-014 2.C91-C142.994-0154.719-015 7.002-0154.486-016 5.86C-016 8.626-0162.833-015 3.747-015 4.764-C155.367-009 5.714-OCS 5.'892-CO91.644-014 1.831-014 2.046-0142.593-015 4.718-015 7.COO-0151.C12-012 1.338-012 1.701-C126.378-009 8.918-005 9.196-C092.994-015 4.72C-015 7.003-0151.081-014 1.872-014 2.C91-0141.C12-012 1.338-012 1.701-0128.378-009 6.918-OC9 9.196-0092.S94-015 4.72C-015 7.003-0151.681-014 1.872-014'2.091-0141.396-014'1.844-01442.344-0141.C12-012 1.33e-012 1.701-0128.'78-009 8.918-OC9 9196-0091.C81-014'1.872-014 2.091-0142.994-015 4.72C-015 i.003-0151.681-014 1.872-014 2.091-0141.CI1-012 1.336-012 1.698-012

16 YEARS

2.094-0123.346-0095.052-0162.339-0141.411-01 52.100-0129.311-OC99.915 5-01 51.411-0152.100-0129.311-Ot92.339-0149.91 -01'51.268-0155.880-0155.966-092.288-0149.913-0152.100-0129.311-0099.917-0152.339-0142.100-0129.311-0099.917-,0152.339-0142.893-0142. 100-0129.311-0092.339-0149.917-01s2.339-0142.096-0122.071-0129.288-0092.339-0143.765-0122.213-0081.461-0163.225-0078.611-0121.651-0073.225-0074.192-0109.361-0091.386-0114.535-0082.213-0081.695-0079.992-0073.225-0076.807-014

9. 77-0138.377-0091.81-0141.703-0122. 213-0089.595-0173.225-00?5.798-0121.t23-0073.2 25-0074.192-0109.305-0099.336-0123.C93-0082.213-0081.695-0071.334-0063.225-0076.807-014

1.32C-0128.896-0091.872-0142.303-0122.213-0081.127-0163.225-0076.735-0121.631-0073.225-0074.192-01C9.425-0091.084-0113.581-0082.213-0081.695-0071.211-0063.225-0076.807-014

E. 39

1.678-0129.174-0092.C91-0142.991-0122.213-0081.294-0163.225-0077.673-0121.641-0073.225-C074 .192-C109.428-0091.234-0114. 062-0082.213-0081 .695-0071.100-0063. 225-0076.807-014


10.YEARS 12 YEARS 14 YEARS 16 YEARS

NP235NP236NP237NP238NP239NP240P-PU236PU238PU239PU240PU241PU242PU243PU244AM241AM242PAM242AM243CM242CM243CM244CM245C 1246CP247CM248-BK249CF249CF250CF251CF252SUMT0t

4.203-0122.4 25-0121.d23-0072.385-0084.S56-0066.807-0141 .72-0088.680-0042.534-0043.56-0045.437-0027.590-0074.169-0156.116-0141.198-0034.770-0064.746-0064.556-0063.929-0064.4C5-0062.328-0041.894-0082.426-0094.169-0155.777-0155.374-0154.110-0141.C05-0137.491-0166.538-0155.736-002

i .17C-0122.425-0121.631-0072.363-0084.95 5-0066.8C7-0141.213-0088 544-0042 .934-0043.655-OC44.938-0027.59C-0074.169-0156.816-0141 .36C-0034.727-0C64.7C3-0064.955-63.894-OC64.1S6-OCt2 .157-0041.893-0082.425-0094.169-0155.777-0151.1C5-0154.095-0149.042-0147.679-0163.866-0155.25C-OC2

3. 2 59-0132.4 25-0 121.641-0072.342-0084.9 54-C066. 807-0147.456-C098.411-0042.934-0043.655-C044.485-C027.590-0074.169-0 156.816-0141.506-0034.684-0064.660-0064.9 54-0063.861-C063.997-0061.998-0041.893-0082.4 25-0094.169-0155.777-0152.270-0164.079-Cl48,133-0147. 667-0162.286-0154.808-002

9.075-0142.425-0121 .651-OC72.321-OC84.953-0066.807-0144.585-0098.280-0042.933-0043.655-OC44.073-OC27.590-0074.169-0156.816-0141.638-OC34.641-OC64.618-OC64.953-OC63.826-OC63.807-0061.850-0041.893-0082.424-0094.169-0155.777-0154.668-0174.063-0147.315-0147.655-0161.351-0154.407-002

TOTAL. 5.736-002 5.25C-002 4.808-002 4.407-002

E.40

TABLE E3.d. Actinides (Elemental), Ci/gU, at 20 MWd/kgM

- 10 YEARS 12 YEARS 14 YEARS 16 YEARS

TL 3.CI1-009Pe 8.379-00981 8.379-009PO 1.375-008AT 1.681-014RN 8.379-009FR 3.C77-014RA 8.379-009AC 1.C28-012

3.530-007PA 4.E52-007

-U 1.E88-006NP 5. 42-006PU 5.590-002AM 1.212-003CM 2.412-004BK 5.374-015CF 1. 489-013SUMTOT 5.736-002

TOTAL ' 5.736-002

3.2C6-OC9 3.306-009e.919-009 9.198-C098.919-OC9 9.198-0091.463-008 1.509-0081.872-014 2.091-0148.91S-OS 9.198-0093.715-014 4.435-0148.919-09 9.198-0091.355-012 1.719-0123.535-007 3.538-0074.66C-007, '4.870-0071.771-006 1.664-0065.142-006 5.142-C065.089-002 4.635-0021.374-003 1.521-0032.238-004 2.076-C041.1C5-015 2.270-0161.360-013 1.252-0135.25G-002 4.808-002

3. 348-0099.313-0099.313-0091.528-0082.339-0149.313-0095.231-0149.313-0092.120-0123.539-0074 880-OC71.568-0065.141-0064.222-OC21.653-0031 .927-OC44.668-0171.159-0134.407-002

4.407-OC25.250-002 4.808-002

.1.

E .41

TABLE E.3.e. Fission Products (Isotopic), g/gU, at 20 MWd/kgM

IC YEARS 12 YEARS 14 YEARS 16 YEARS'S

LlLIBEI EC

ZNZNGAGEGEGEASGESESESESEaRSEKRSRKRSEKRKRKRKRR3KRSRRBSRSR

YSRYZRZRZRZRNSNBZRNBMOZRM0MoMOTCTC

3679

1C1466677172737475767677787979808C818182828384858586868787a8899090909192939393P949495969697989899

1.S60-008 1.752-OCe1.425-C1O 1.425-OIC6.139-012 6.139-0121.182-011 1.182-0117.888-011 7.88e-0111.'93-011 1.593-0112.282-014 2.282-0149.492-016 9.492-0165.!45-013 5.345-0131.'57-008 1.357-0082.845-008 2.845-008

-6.C13-008 6.013-0081.262-007 1.262-OC?3.C98-007 3.098-OC?2.252-009 2.252-0096.456-007 6.456-OC71.472-006 1.472-OC63.623-006 3.623-0064.419-010 5.192-01C8.217-006 8.217-OC61.'29-010 1.32S-01C1.357-005 1.357-OCS1.C68-011 1.068-0112.C81-005 2.081-OC54.215-007 4.215-OC?2.798-005 2.798-0056.758-005 6.758-OC57.774-006 6.831-0066.758-005 6.852-0051.179-004 1.179-0041.435-007 1.635-OC71.515-004 1.515-0041.285-009 1.285-OC92.174-004 2.174-004

1.566-008 1.400-OC81.425-010 1.425-0106.139-012 6.139-0121.182-011 1.182-0117.888-011 7.888-0111.592-C11 1.592-0112.282-014 2.282-0149.492-C16 9.492-0165.345-C13 5.345-0131.357-008 1.357-0082.845-008 2.845-0086.C13-008 6.013-0081.262-007 1.262-0073.098-CO7 3.098-0072.252-009 2.252-0096.456-007 6.456-0071.472-006 1.472-0063.623-C06 3.623-0065.965-010 6.738-0108.217-C06 8.217-OC61.329-C1O 1.329-0101.357-CO5 1.357-0051.068-011 1.068-0112.081-COS 2.081-0054.215-007 4.215-0072.798-CO5 2.798-0054.758-005 6.758-OC56.003-006 5.274-0066.935-005 7.008-0051.179-004 1.179-0041.635-007 1.635-0071.515-004 1.515-0041.285-009 1.285-0092.174-004 2.174-0042.840-004 2.840-0042.385-004 2.274-0045.980-008 5.702-0081.G61-C04 1.172-0043.664-004 3.664-0043.951-C04 3.951-0044.447-004 4.447-0041.066-009 1.302-0092.C40-009 2.206-0094.525-004 4.525-0044.431-010 4.431-0104.713-004 4.713-0044.886-004 4.886-0041.310-005 1.310-0054.827-004 4.827-0045.003-004 5.003-0042.490-009 2.490-0094.863-004 4.862-004

2.140-0042.6 23-0046. 77-0088.225-0053.664-0043.551-0044.447-0046.477-0101.652-0094.5 25-0044 .432-0104.713-0044.886-0041.310-0054.827-0045.C03-0042.490-0094. 8 63-004

2.84C-OC42.501-0046.271-0029 .445-OCS3.664-OC43.951-0044.447-0048.468-01 1.856-0094*525-0044.431-010

.713-0044.886-0041 .31C-0054.827-0045.OC3-0042.490-0094.863-004

E.42


IC.YEARS 12 YEARS 14 YEARS 16 YEARS

RU 99M0100MORIOO-RU 100RUoRU102RH102RHI103RUI04PD104

iPD105RU106RH106PD106PD107AG107P0108A61098CD108A6 109CD109PD110AGIIOFColicCDIIIC0112CDI13CD113co113CD114SN114IN115SN115CD 1 6SN116SNI 6SN117SNIISN119SN 1F.

,SN121FS9121SN122TE122SN123SB123TE123SN124TE124S9125TE125TE125F.SN126

1.7e7-a08 2.1C3-OCE5.3S-004 5.635-0043.772-005 3.772-0054.722-004 4.722-OC44.!67-004 4.567-OC43.S01-011 2.419-0113.157-004 3.157-0043.170-004 3.17C-OC49.179-005 9.179-OCS2.271-004 2.271-0049.647-008 2.438-OCE9.C67-014 2.292-0141.941-004 1.942-OC41.224-004 1.224-OC4

2.420-C085.635-C043.772-0054.722-C044.567-C041.500-0113.157-C043.170-C049.179-CO52.271-C046.163-C95.793-Cl51.942-0041.224-C04

1.438-010 1.6S9-01C 1.960-ClO8.371-005 £.371-005 8.371-0055.190-013 5.826-013 5.763-0131.504-010 1.5C4-OIC 1.504-C1O4.02-005 4.6C2-OC5 4.602-0055.214-016 1.751-016 5.879-0172.751-005 2.751-OC5 2.751-0051.365-011 1.799-012 2.371-C131.283-005 1.283-OC5 1.283-COS1.562-005 1.562-OCS 1.562-0059.548-006 S.548-OC6 9.548-C061.399-007 1.39-007 1.399-0078.577-008 8.163-008 7.423-0086.190-008 7.0C3-008 7.743-0081.343-005 1.343-OCS 1.343-0054.541-010 4.541-01C 4.541-0102.117-006 2.117-006 2.117-0062.C00-007 2.OCC-OC? 2.000-C075.111-W006 5.111-006 5.111-0063.846-006 3.846-006 3.846-0065.182--006 .5.182-006 5.182-C065.224-006 5.224-006 5.224-0065.201-006 5.2G1-006 5.201-0061.C04-012 1.271-013 1.610-0145.307-006 5.3C7-OCi 5.307-C061.791-009 1.742-009 1.695-009-5.299-006 5.299-006 5.299-0065.852-006 5.852-006 5.852-0062.281-007 2.281-OC7 2.281-0078.421-016 1.671-017 3.315-0196473-006 6.473-006 6.473-0062.487-009 2.487-009 2.487-0097.909-006 7.9C9-006 7.909-0061.93-007 1.693-007 1.693-0077.196-007 4.362-007 2.645-0071.C95-005 1.124-005 1.141-0051.C07-008 6.103-009 3.700-0091.679-005 1.679-905 1.679-005

E.43

2.736-OC£5.635-0043.772-OCS4.722-OC44.567-OC49. 297-0123.151-0C43.170-0049.179-OC52.271-0041 .558-OC91.464-0151.942-OC41. 224-0042. 222-0108.371-O55.700-0131.504-0104.602-0051.974-0172.751-0053.126-0141.283-OC51 .562-0059.548-0061.399-0076.750-0088.415-0081.343-0054.541-0102.117-OC62.000-0075.111-0063.846-0065.182-0065.224-0065.201-0062.03.8-0155.307-0061.648-0095.299-0065.852-0062.281-0076.585-0216.473-0062*487-0097.909-0061.693-0071.603-0071.152-0052.243-0091.679-005



S8126S8126PTE126 'TE127P1127

TE128XE1291129

XE129TE130XE130XE131XE1328A132CS133XE134CS1348A134CS135SAl 35XSI36BA136CS137SA 1373At 37P9A138LA138LA139CE140PRI41CE142ri142NDt43CE144PR144PR144PND144ND145ND146P146SM1446P1147SF147N0148SM148SP149ND150SM150'EUlSOS151EU151SF152

7.S78-013 7.978-0136.C66-015 .066-0154.203-007 4.2C5-OC77.677-017 7.37d-0I93.412-005 3.412-OCS6.e82-005 6.682-OC51.157-006 1.157-OCE1.102-004 1.1C2-OC44.258-009 4.267-OC92.137-004 2.137-OC44.797-006 4.797-0062.938-004 2.932-oC46.170-004 6.17C-0047.465-010 7.465-O1C7.198-004 7.198-OC48.f90-004 8.890-0041.726-006 8.813-OC76.365-005 6.45C-OC52.459-004 2.459-OC46.352-008 6.367-OCE1.'42-003 1.342-O39.532-006 9.532-O065.744-004 5.484-0041.712-004 1.971-OC48.787-011 8.391-0117.748-004 7.748-OC43.954-009 3.954-0097.427-004 7.427-0047.440-004 7.44C-OC46.852-004 6.852-OC46.855-004 6.855-0041.C02-005 1.OC2-0055.372-004 5.372-OC43.123-008 5.26C-OC91.319-012 2.221-0136.592-015 1.11C-0157.452-004 7.452-OC44.275-004 4.275-0043.S92-004 3.992-0049.731-010 7.563-OIC3.186-009 3.266-OC98.305-006 4.896-0061.539-004 1.573-0042.240-004 2.24C-OC48.698-005 8.698-OCS2.C47-006 2.047-0061.C61-004 1.061-0041.501-004 1.5CI-0041.231-013 1.185-0139.149-006 9.0C9-0067,434-007 8.832-0078.621-005 8.621-005

7.978-Ct36.C66-C1S4.207-0077.C82-C213.412-COS6.6t2-C051.157-CO61.102-CC44.277-C092.137-0044.797-C062.938-0046.1 70-0047.465-C107.198-0048.8 90-0044.499-C076.493-0052.459-0046. 382-C081.342-C039.532-0065.237-C042.219-0048.012-C117.748-0043.954-0097.427-CO47.440-C046.852-0046.855-0041.002-0055.372-0048.858-0103.740-0141.870-0167.453-0044.275-0043.992-0045.878-0103.328-0092.886-0061.593-0042.240-0048.698-0052.047-0061.061-0041.501-0041.140-0138.871-0061.021-0068.622-005

7.978-0136.066-0154.210-OC77.149-02 33.412-OC56.682-OC51.157-0061.102-OC44.287-oC92.137-0044.797-0062.938-O46.170-OC47. 46 5-0107.198-OC48.890-0C42.297-OC76.515-OC52.459-OC46.396-0081.342-0039.532-0065.000-0042.455-0047.650-0117.748-0043.954-0097.427-0047.440-oC46.852-0046.855-0041.002-0055.372-0041.492-0106.300-0153.149-0177.453-0044.275-0043.992-0044.568-0103.*377-0091.702-0061.605-0042.240-0048.698-0052.047-0061.061-0041.501-0041.097-0138.735-0061.157-0068.622-005

E. 44



EUIS26D152EU153GD153S P154EU154GD154.EU15560155.6D156GDI57GD158T81596D160DY160DY161DY162DY163DY164M1C165H0166PER166ER167ER168TM169ER17aYE170TM171Y8171YB172SUMTOT

TOTAL

2.159-0081.4 26-0085.946-0052.434-0132.139-0057.4 83-006I-.C35-0051 .620-0064.88-0062.466-0055.933-0088.934-0061.428-0066.S88-0071.111-0072.488-0072.C68-0071.385-0072.255-0086.181-0084.331-0101.870-0081 .92-0093.722-0091681-0115.f26-0153.03-0122.947-0151.735-0133.256-0152.C61-002

2.C61-002

1.950-OCe 1.761-0081.684-008 1.737-0085.946-OCS S.946-0053.0C4-014 3.?07-C152.139-005 2.139-CO5d.369-OC 5.421-C061.147-OC5 1.242-0051.225-006 9.262-0075. 383-0062.466-OC55.933-OCE8.934-0061.428-0066.988-OC71.111-0072.488-O72.068-0071.385-0072.255-OC06.1e1-0084.326-OlC1.87C-00E1 .992-oC93.722-OC91.861-0115.626-0153.8G3-0121.431-0151.75G-0133.256-0152.061-OC2

2.061-002

5.681-0062.466-0055.933-0088.9 34-0061.428-0o66.988-0071.111-0072.488-C072.068-0071.385-C002.255-0086.181-0084.321-0101.870-0081.992-0093.722-0091.861-0115.626-0153.803-0126.953-0161.758-0133.256-Q152.061-C02

2.C61-002

I.*590-0081 .784-OC85.946-0054. 575-0162.139-0054.614-0061.322-0057.003-0075.907-0062.466-0055.933-0088.934-0061 .428-OC66.988-0071.111-0072.488-0072.068-0071.385-0072.255-008t.181-0084.316-0101.870-0081.992-0093.722-0091. 861-0115.626-0153.803-0123.378-0161.761-0133.256-0152.061-OC2

2.061-002

E.45

TABLE E.3.f. Fission Products (Elemental), g/gU, at 20 MWd/kgM

IC YEARS 12 YEARS 14 EARS 16 YEARS

HLIBECZNGAGEASSEBRKRRaSR

-ZRNBMOTCRURHPDAGCDINSNS.B-TFI

XECSBALACEPRNDPMSMEUGD

DYHOERTMYBSUNTOT

1 .60-0081.486-0109.C70-0111.593-0112.378-0145.145-0134.120-0071.s62-0073.477-0051.358-0052.216-0042.190-0044.798-0042.E41-0042.230-0032.743-0092.C31-0034.E63-0041.284-0033.157-0047.466-0044.602-0055.678-0052.179-0065.552-0051.249-0052.923-0041.443-0043.148-0031.542-0031.C19-0037.427-0041.429-003

1.752-0011 .486-OIC9.07C-0111.593-0112.378-0145.345-0134.12C-0071 .262-0073.477-OC51.358-0052.2C7-OC42.2CC-OC44.676-0042.841-0042.242-OC33.146-OC92.031-OC34.863-0041.284-0033.157-OC47.467-0044.6C2-0055.677-0052.187-OC65. 552-0051.221-OCS2.926-OCA1.443-0043 .148-0031.515-OC31.046-OC37. 427-0041.429-OC

1.566-C081.486-0109.070-0111.592-0112.378-0145.345-0134.1 20-0071. 262-0073.477-0051.358-C052.1 99-0042.208-C044.5 60-0042. 8 41-0042.253-0033.549-C092.031-Co34.863-CO41.284-0033.1 57-0047.467-0044.602-0055.676-0052.195-0065.5 52-0051.204-0052.927-C041.443-0043.148-0031.490-0031.C71-C037.427-0041.429-C036.852-C042.449-OC32.887-0065.149-0046.684-0055.247-0051.428-0067.277-0076.224-0082.442-0081.861-0113.982-0122.061-002

1.400-OC81.486-0109.070-0111.592-0112.378-0145.345-0134.120-0071.262-0073.477-0051.358-0052.191-0042.215-OC44.449-OC42.841-0042.264-0033.951-OC92.031-0034.863-0041.284-0033.157-0047.467-0044.602-0055.675-0052.202-0065.552-0051.193-OC52.928-OQ41 .443-0043.148-0031.466-OC31.095-0037.427-0041.429-OC36.852-0042.449-0031.702-0065.160-0046.595-0055.350-0051 .428-OC67.277-0076.224-0082.442-0081.861-0113.983-0122.061-002

'S

6.852-004 6.852-OC42.449-003 2.449-0038.306-006 4.897-006S.C98-004 5.13C-OC46.933-005 6.796-0054.971-005 5.122-0051.428-006 1.422-OC7.277-007 7.277-0076.224-008 6.224-0082.442-008 2.442-0081.E62-011 1.861-0113.980-012 3.982-0122.C61-002 2.061-002

TOTAL 2.C61-002 2.061-002 2.061-002 2.061-002'-4

E.46

TABLE E.3.g. Fission Products (Isotopic), Ci/gU, at 20 MWd/kgM


H 3BE 10C 14

SE 79KR 81KR 85Re 87SR 90

Y .90ZR 93NB 93NB 94TC 98TC 99RHI02RU106RH106PD107AG1OSA6108A6109CD109AGIIOAGI1'CD113PSN19PSNI21ISN123TE123PS8125TE1251'SN126SB126SB126TE127TE127,1129

CS134CS135CS137BA137,CE142CE144PR144PR1440ND144PM146SM146PK14751147EU1505151

1.893-004 1.692-0041.763-012 1.763-0127.103-011 7.IC1-01I2.525-007 2.525-OC72.246-013 2.246-0133.CS1-003 2.681-OC31.326-011 1.326-0113.579-002 3.413-OC23.580-002 3.413-0021.118-006 1.11t-0044.71-007 5.247-0078.306-011 E.3C6-0112.164-012 2.164-0128.247-006 8.247-0064.717-008 2.924-OCE3.229-004 6.162-0053.229-004 6.162-OC56.299-008 6.299-0081.367-012 1.352-0121.536-011 1.519-0111.347-012 4.522-0131.347-012 4.522-0138.d25-010 1.137-01C6.485-008 8.548-OC91.947-005 1.771-0054.497-009 5.695-01C1.C60-007 1.031-0076.924-012 1.374-0132.440-015 3.541-0177.433-004 4.5C6-0041.814-004 1.1CC-OC44.766-007 4.766-0C76.673-008 6.673-OC84.766-007 4.766-0077.C96-013 6.818-0157.244-013 6.96C-0151.S45-008 1.945-O02.235-003 1.141-OC32.832-007 2.832-0074.998-002 4.773-OC24.728-002 4.515-O21.446-011 1.644-0119.966-005 1.678-OC59.S66-005 1.679-OC51.196-006 2.014-0078.819-016 8.820-0164.334-007 3.368-0071.115-013 1.143-0137.702-003 4.54C-0033.499-012 3.577-0128.153-012 7.845-0122.408-004 2.371-004

E.47

1.512-0041.763-0127.100-0112.525-CO2.246-0132. 356-0031.326-C113.2 54-0023. 2 55-0021.118-0065.768-0078.305-C112.164-0128.247-0061.813-0082.063-0052.063-0056.299-0081.337-0121.503-0111.518-0131.518-0131 .4 99-0111.127-0091.610-G057.211-0111.002-0072.725-C155.681-C192.732-0046.667-0054.766-0076.673-0084.766-0076.5 50-0176.6 82-0171.945-0085.E24-0042.832-0074.557-0024.311-CO21.646-0112.827-0062.827-0063.392-0088.820-0162.618-0071.165-0132.677-0033.623-0127.549-0122.335-004

1.351-0041.763-0127.098-0112.525-OCi2.246-0132.070-OC31.326-0113.103-OC23.103-0021.118-0066.238-OC7E.305-0112 .164-0128.247-0061.124-0085.214-OC65.215-OC66.299-0081.323-0121.486-0115.099-0145.099-0141.976-0121.485-0101.464-0059.131-0129.749-0085.415-017

.0001.656-0044.042-OC54.766-0076.672-0084.766-0076.606-0196.746-0191 .945-OCS2.973-0042.832-0074.351-0024.116-0021.646-0114.761-0074.761-0075.714-0098.820-0162.035-0071.182-0131.578-0033.650-0127.264-0122.299-004

4

TABLE E.3.g. Contd)


EU152 3.735-006 3.373-006 3.046-006 2.751-0066D153 8.587-010 1.06C-O1C 1.308-011 1.614-012EU154 2.C21-003 1.72C-OC3 1.464-003 1.246-003EU155 7.538-004 5.6ss-O04 4.309-004 3.259-OC4H0166P 7.776-010 7.767-01C 7.758-010 7.749-010TH171 3.210-012 1.559-012 7.574-013 3.679-013SUNTOT 1.869-001 1.73C-OC1 1.621-001 1.529-001

TOTAL 1.E69-001 1.73C-OCI 1.621-001 1.529-001

E.48

TABLE E.3.h. Fission Products (Elemental), C/gU, at 20.MWd/kgM


ff 1.893-004 1.692-004 1.512-004 1.351-0C4BE 1,763-012 1.763-012 1.763-012 1.763-012C 7.103-011 7.101-011 7.100-C1 7.098-011

SE 2.525-007 2.525-007 2.525-007 2.525-007KR 39C51-003 2.681-003 2.356-003 2.070-003RB 1.326-011 1.326-011 1.326-C1I 1.326-011SR 3.579-002 3.413-002 3.254-002 3.103-OC2Y 3.580-002 3.413-002 3.255-002 3.103-002

ZR 1.118-006 1.118-OCt 1.118-006 1.118-006NS 4.f71-007 5.248-OC7 5.769-CO? 6.239-007TC 8.247-006-8.247-0C6 8.247-006 8.247-006RU 3.229-004 E.162-OC5 2.C63-005 5.214-006RH 3.229-004 8.165-005 2.065-CO5 5.226-006PD 6.299-008 6.299-0C 6.299-008 6.299-008AG 6.573-008 e.679-OC9 1.158-009 1.667-010CD 1.547-005 1.771-OC5 1.610-005 1.464-005SN 5.871-007 5.8C2-0C7 5.769-007 5.741-007Se. 7.439-004 4.512-OC4 2.737-004 1.662-OC4TE' 1.814-004 1.1CC-04 6.667-005 4.042-OCSI - 1.945-008 1.945-00e 1.945-CO 1.945-008-

CS 5.222-002 4.887-OC2 4.615-02 4.381-002BA 4.728-002 4.515-OC2 4.311-C02 4.116-OC2CE 9.S66-005 1.678-005 2.827-C06 4.761-007PR 1.C09-004 1.699-005 2.861-006 4.819-007NO 8.819-016 8.82C-016 8.820-C16 8.820-016PM 7.702-003 4.541-003 2.677-C03 1.578-OC3SM 2.408-004 2.371-04 2.335-C04 2.299-004EU 2.778-003 2.293-003 1.898-003 1.574-003GD 8.587-010 1.06C-01C 1.308-011 1.614-012Ho 7.776-010 7.767-01C 7.758-010 7.749-010TM 3.210-012 1.559-012 7.574-013 3.679-013SUMTOT 1.E69-001 1.73C-OC1 1.621-001 1.529-001

t

TOTAL 1.E69-001 1.73C-001 1.621-001 1.529-001

E.49

TABLE E.3.i. Neutron Source (Alpha-n), Neutrons/sec-gU, at 20 MWd/kgM


PU238PU239PU24CAM241AM243CM242CM243C10244

8.258-001 6.129-OCI 8.COZ-COI 7.878-0012.137-001 2.137-OCI 2.137-CO 2.137-0012.770-001 2.77C-OC1 2.769-COI 2.769-0011.1494000 1.3C4+OCC 1.445+000 1.571+OCO4.228-003 4.227-0C3 4.226-C03 4.226-0035.274-003 5.23C-OC3 5.183-003 5.136-0035.865-003 5.5E6-OC3 5.321-003 5.068-0032.E57-001 2.4e1-OC1 2.280-COI 2.112-OCI

TABLE E.3.J. Neutron Source (Spontaneous fission),Neutrons/sec-gU, at 20 MWd/kgM


PU238PU240PU242C4244CM246

1.347-001 1.326-OCI 1.305-001 1.285-0011.4604000 1.46C+OOC 1.460*000 1.460+0003.349-001 3.349-001 3.349-001 3.349-0013.199+001 2.963+0C1 2.745+CO1 2.542+OC17.C26-002 7.024-OC2 7.C22-C02 7.020-002

'S

E.50

TABLE E.4.

Subtable

E.4.a

E.4.b

E.4.c

E.4.d

E.4.e

E.4.f

E.4*g

E.4.h

E.4.i

E.4.J

Radionuclide Inventories at 25 MWd/kgM as a Function ofDecay Time

Species - Units

Actinides (Isotopic), g/gU

Actinides (Elemental), g/gU

Actinides (Isotopic), Ci/gU

Actinides (Elemental), Ci/gU

Fission Products (Isotopic), g/gU

Fission Products (Elemental), g/gU

Fission Products (Isotopic), Ci/gU

Fission Products (Elemental), Ci/gU

Neutron Source (Alpha-n), neutrons/sec-U

Neutron Source (Spontaneous fission), neutrons/sec-gU

E.53

E.54

E.55

E.57

E.58

E.62

E.63

E.65

E.66

E.66

E.51


lC YEARS 12 YEARS 1 YEARS 16 YEARS

HE 4P6207PB208PE212RA224RA226AC227TH228TH229TH230TH231TH232TH234PA231PA233U232-U233U234U235U236U237U238

NP235NP236NP237NP238NP239PU236PU238PU239PU240PU241PU242PU244AM241AM242MAM242AM243CM242C1243CM244CM245CM246CM247CM248CF249CF250CF251SF250SUNTOl

6.595-007 7.291-OC7 8.005-0071*344-015 2.067-015 3.002-0153.240-011 4.385-011 5.583-0119.E53-015 1.05C-014 1.C84-C148.595-014 9.161-014 9.454-0144.439-015 7.1G6-015 1.C67-0141.C82-014 1.42S-0141.670-011 1.776-0111.257-013 1.371-0131.281-010 1.752-O1C3.230-014 3.23C-0149.£68-010 1.158-OCS1.366-011 1.386-0119.505-011 1.105-01C1.C48-011 1.053-0117.119-010 7.214-01G1.225-009 1.433-OC97.E13-006 9.1C2-0C67.944-003 7.944-OC32.943-003 2.943-0032.C95-011 1.9C2-0119.545-001 9.545-OCI4.50-015 1.295-0152.703-010 2.7C3-OIC3.C87-004 3.1C2-0041.173-013 1.162-0134.415-011 4.614-0116.179-011 3.8CC-Ol8.361-005 8.23C-OC54.918-003 4.918-0C31.S61-003 1.961-0036.765-004 6.144-0043.362-004 3.362-0041.125-008 1.125-004.451-004 5.057-0046.256-007 6.2CO-0077.484-012 7.416-0125.370-005 5.369-00c1.515-009 1.502-OC91.749-007 1.666-0078.306-006 7.694-0063.836-007 3.835-0073.686-008 3.685-0082.728-010 2.72E-O1C1.C87-011 1.087-0119.685-014 9.649-0141.C06-014 9.052-0155.969-015 5.96C-0157.227-012 8.1C5-0129.742-001 9.742-001

1.817-0141.833-C111.503-C132.295-CdO3.2 30-0141.329-C091 .386-C 111 .259-C101.C59-C117:219-C101 .642-0091.037-0057.944-0032.944-0031.728-0119.545-0013.606-C162.703-C103.118-0041.152-0134.fj3-C112.337-C118.1 02-0054.917-0031.961-0035.580-0043.362-0041.125-0085.604-0046.143-0077.349-C125.368-0051.489-0091.587-0077.127-0063.834-0073.684-008'2.728-0101.087-0119.611-0148.141-0155.951-0158.922-0129.742-001

8.738-OC74 .175-0156.807-0111.098-0149.577-0141.5 25-0142.244-0141.856-0111.654-0132.907-0103.230-0141 .501-0091.386-0111.413-0101.065-0117.169-0101.851-0091.162-0057.945-OC32.944-OC31.569-0119.545-0011.004-0162.703-0103.137-0041.141-0134.612-0111.437-0117.975-0054.917-OC31.962-0035.068-0043.362-0041.125-OOE6.097-0046.087-0077.282-0125.367-0051.475-0091.511-0076.602-0C63.834-0073.683-0082.728-0101.087-0119.574-0147.323-0155.942-0159. 680-0129 .742-001

TOTAL 9.742-001 9.742-001 9.742-001 9.742-001

E. 53

TABLE E.4.b. Actinides (Elemental), g/gU, at 25 4Wd/kgti


HES'Ps131RAAC -TN1PA

UNPPUAMCMCFSUMTO

TOTAL

6595-0077.227-0123.241-0111.C48-0159.C41-0141.C82-0141.146-0091.C55-0109.654-0013.C87-0047.S75-0034.S95-0048.903-0061.131-0139.742-001

7.2S1-OC?8.1C5-0124.31?-0111.133-015S.874-0141 .429-0141 .365-OC91.21C-O1C9.654-OCI3.IC2-0047. 91 2-0035.6CC-0C48.283-OCU1.116-0139.742-OCI

8.C05-CO7 8.738-0078.922-C12 9.680-0125.585-011 6.809-0111.189-015 1.230-0151.C52-013 1.111-0131.818-C14 2.244-0141.591-009 1.824-0091.365-C10 1.519-0109.654-C01 9.654-0013.118-C04 3.137-0047.854-C03 7.801-OC36.147-C04 6.640-0047.708-C06 7.175-0061.103-013 1.090-0139.742-001 9.742-OCI

9.742-001 .742-OCI 9.742-001 9.742-OCIN*1.0

'-4

'-

-

E.54

TABLE E.4.c. Actinides (Isotopic)i C/gU, at 25 MWd/kgM


TL207TL208TL209P8209P8210P6211P8212P921481210BI211BI21281213BI214P0210P0211P0212P0213P0214P0215P0216P0218AT217RN219RN220RN222FR221FR223RA223RA224RA225RA226AC225AC227TH227TH228TH229T 2303i231TH232TH234PA231PA233PA234FPA234U232U233U234U235U236U237U238U240

7.£07-013 1.033-012 1.314-0124.921-009 5.245-00 5.413-0095.777-016 6.3C3-01 6.911-C162.674-014 2.916-014 3.200-0147.300-016 1.026-015 1.489-0157.129-013 1.036-012 1.317-Cl21.370-008 1.46C-OCE 1.507-0084.390-015 7.028-015 1.055-C147.302-016 1.027-015 1.490-0157.E29-013 1.036-012-1.317-C121.370-008 1.4dC-0ce 1.507-0082.674-014 2.918-014 3.200-C144.390-015 7.028-015 1.055-0147.302-016 9.297-016 1.340-0152.192-015 2.9C1-015 3.689-0158.775-009 9.353-OC9 9.652-C09.2.d17-014 2.855-014 3.130-0144.389-015 7.02d-015 1.C55-C147.129-013 1.036-012 1.317-Cl21.370-008 1.46C-OC8 1.507-COt4.391-015 7.029-015 1.055-0142.674-014 2.918-014 3.200-0147.129-013 1.036-012 1.317-0121.370-00& 1.46C-OCE 1.507-0084.391-015 7.029-015 1.G55-C142.674-014 2.91e-014 3.200-0141.C80-014 1.427-014 1.815-014

1.622-0125.483-0097.602-0163.519-0142.167-0151.627-0121.526-OC81.508-0142.168-0151.627-0121.526-OC83.519-0141.508-0141.950-0154.554-0159.778-0093.443-0141.508-0141*627-0121,526-0081.508-0143.519-0141.627-0121.526-OC81.508-0143.519-0142.241-0141.627-0121.526-OCS3.519-0141.508-0143.519-0141.624-0121.604-0121.522-0083.519-0145.871-0121.718-0081.647-0163.210-OC76.676-0122.212-0073.210-OC74.174-0101.535-0081.793-0117.264-00C81.718-0081.905-0071.281-0063.210-0071.994-013

7.e29-0131.3 70-0082.6 74-0144.391-0152.74-0147.627-0137.721-0131.370-0082.74-0142.5 86-0121.718-0081.C83-0163.210-0074.491-0122.177-0073.210-0074.174-0101.524-0081.187-0114.684-0081.718-0081.S05-0071.710-0063.210-0071.S94-013

1.036-0121.460-OC02.918-0147.029-0152. 918-0141.034-0121.022-0121.456-0062.918-0143. 53 8-0121.718-00e1.271-0163.21C-OC75. 21 9-0122.187-0073.21C-0074.174-01C1.545-00e1.386-011S .69C-001.718-0061.9CS-0071 .553-OC03.21C-0071.994-013

1.317-0121.507-0083.200-C141.C55-0143. 200-0141.315-0121.299-Cl?1.503-0083.199-0144.634-C121.718-0081.459-0163.210-0075.947-0122.1 99-C073.210-0074.174-C101.546-COB1.5 90-0116.483-0081.718-0081.905-0071.411-CO63.210-0071.994-013

E. 55



NP235NP236NP237NP238NP239NP24OPPU236PU238PU239PU240PU241PU242PU243PU244AM241AM242PAP242AM43C 242CM243CN244CM245CP246;M247CM2489K249C F 249CF250CF251CF252-SU4TOT

6.526-012 1.817-0123.562-012 3.562-0122.177-007 2.17-OC73.C41-0081.C71-0051.994-0133.285-0081.432-0033.C58-0044.470-0046.973-0021.284-CO62.532-Cl41.997-0131.528-0036.C83-0066.C52-006I.C71-005S.C11-0069.C31-CO66.723-0046.588-0081.133-0082.532-0144.t25-0145.224-0143.S69-0131.101-0129.471-015I.C61-0137.416-002

3.014-OC81.071-0051.994-0132.02C-OCI1.41C-OC33.058-OC4.471-OC46.333-OC21.284-CCt2.532-0141.997-01'1 .736-0036.027-0065.997-OC61 .071-OC54.969-oc8.6C3-OC66.227-OC4d .587-0081.132-0082. 53 2-0144.625-0141.074-0143.954-0139.899-0139.457-0156. 275-0146.79C-OC2

5.061-C133.5 62-0122.199-CO72.986-0081 .C7O-C051.994-0131.242-CO81.3 88-0033.C58-0044.471-C045.751-C021.284-0062.532-Cl41.997-0131.924-C035.973-C065.943-0061. C70-0054.924-C068.194-C065. 7 69-0046.586-C081.132-C082.532-C144.625-C142.206-Ci53.9 39-0138.904-0139.442-0153.710-0146.221-C02

1.409-0133.562-0122. 212-0072.959-OC81.070-0051.994-0137.638-OC91.366-0033.058-0044.471-OC45.223-OC21 .284-0062.532-0141.997-0132.093-OC35.918-OC65.889-oc61.070-OC54.879-0067.805-OC65.343-OC46.585-0081.132-OC82.532-0144.625-0144.535-0163.924-0138.009-0139.428-0152.194-0145.703-OC2

TOTAL 7.416-002 6.79C-002 6.221-002 5.703-002

a

E .56

TABLE .4.d. Actinides (Elemental),.Ci/gU, at 25 MWd/kgM


Tt

IPo

ATR'NFRRAACTNPA. uNP -PUAMCmBKCFSUMTOT

* 4.522-0t9 5.246-00;1.370-008 1.4fC-00e1.370-008 1:46C-0CE-2.247-008 2.395-00E2.474-014 2.918-0141.370-008 1.46C-00E3.755-014 4.345-0141.370-008 1.46C-00e8.C95-013 1.063-012-3.519-007 3.52£-OC?5.391-007 5.4C2-0C72.303-006 2.155-0061.C96-005 1.096-OC57.191-002 6.549-OC21.551-003 1.759-OC36.864-004 6.364-OC45.224-014 1.074-0141.13-012 1.458-0127.416-002 6.79C-0C2

5.414-0091.507-C081.507-C082.472-0083.200-C141.507-C085.014-C141.507-0081.347-0123.533-C075.414-C 072.C20-CO61.C95-C055.966-0021.947-C035.900-0042.206-C151.331-0126.221-002

5.485-0091 .526-OC81. 526-0C82.504-0083. 519-0141 .526-OCe5.760-0141.526-0081.659-0123.534-0C75.427-0C71 .898-OC61.095-OC55.435-OG22.116-OC35.471-OG44.535-0161.225-012S.703-OC2

TOTAL 7.416-002 h.7SC-0C2 6.221-C02 5.iO3-oc2. . . .

, .

* f :

- 8 ' - 0.:0 , . ,

s : . . ; .-

. , .

. .

.. . ..

:

I I I

I

i i

. ,

.

.

. ;. ,

. . . . .

. . ..

:

.. .

.

. i

E.57



HLILIBEBEC

ZhZNGAGEGEGE.ASGESESESESEBRSEKR

K RSEKRKRKRKRR1

.KRSRRBSRSRY

SRY

ZRZRZRZRNB8NB8ZRN3m40ZR

No740TCTC

36-79

1 C1466677172737475767677787979808C8181828283848585868637878899090909192939393"949495969697989899

2.502-C081 .531-01 07.6 60-0121 .475-0119.142-0111.988-0112.700-0141.117-0156.876-G131.739-0083.563-0087. 5 43-0081.562-0073.E04-0073.5 20-0097. 41-0071.834-0064.4 66-0065.452-0101 .C1G-CO51.7 77-0101.51-0051.615-0112. 5 33-0056.371-0073.233-0058.335-0059.3 70-0068.132-0051.415-0042.5 08-0071.815-0042.CIO-0092.603-0043.3 95-0043.137-0047.866-0089.162-0054.A04-0044.781-0045.403-0047.196-0102.C09-0095.551-0046.C08-0105.750-0046.C 26-0042.C65-0055.986-0046.239-0043.S42-0095.953-004

2.236-OCE1.531-01C7 .66C-01 21.4.75-0119.842-0111.9E7-0112 .7CC-0141.17-015t.876-0131 .739-OCI3.563-OC877.543-OCI1.562-0073.8C4-OC73.52C-OCS7.841-0071 .834-0064.466-0066.4c-51C1.O1C-0051 .777-01C1 .651-OC51.615-0112.533-OCS6.371-OC73.233-OC58.335-0052.234-OCE8 .246-OCS1.415-0C42.58C-OC71.815-0042.OIC-0092.6C3-OC43.395-0042.991-OC47.5CC-0081.132-OC44.4C4-0044.781-0045.403-0041.032-0092.256-0095.551-0046.0C7-01C5 .750-0C46.026-0042.065-OCS5.986-0046.239-0043.942-OC95.953-004

1.999-C08 1.787-0ca1.531-C10 1.531-0107.660-C12 7.660-01214475-C11 1.475-0119.242-C11 9.842-0111.987-Ci1 1.986-0112.700-C14 2.700-0141.117-015 1.117-0156.876-C13 6.876-0131.739-C08 1.739-O003.563-C08 3.563-OC87.543-C08 7.543-0081.562-C07 1.562-OC?3.804-C07 3.804-OC73.520-C09 3.520-0097.841-007 7.841-OC71.834-C06 1.834-OC64.466-C06 4.466-0067.358-CIO 8.311-0101.010-005 1.010-0051.777-010 1.777-0101.651-C05 1.651-0051.615-011 1.615-0112.533-0O5 2.533-0056.371-007 6.371-0073.233-005 3.233-0058.335-005 8.335-0057.235-C06 6.357-OC68.346-005 8.434-0051.415-C04 1.415-0042.508-007 2.508-0071.815-C04 1.815-0042.C10-009 2.010-0092.603-004 2.603-OC43.395-C04 3.395-0042.852-004 2.719-0047.151-008 6.819-0081.271-004 1.404-0044.404-004 4.404-0044.781-004 4.781-0045.403-G04 5.403-OC41.298-009 1.585-0092.480-009 2.682-0095.551-004 5.551-0046.007-C10 6.007-010S.750-C04 5.750-0046.026-004 6.026-0042.065-005 2.065-0055.986-004 5.986-0046.239-004 6.239-0043.942-009 3.942-0095.953-004 5.953-004

E. 58



RU 99

RU100RU101RU1 02Rm1 02RH103RU104PD104P0105RU106RH1 06PD106PD107

PD108AGIOSP

CDI 09

PD110AGIO9F

CDII

CC112CD113C1 13F.IN113

CD116SN114

SN115SN118SN116

S117

SNII6 SNII19

SN119KSN120SNIZI!, So1 21SN122rE122 aSN123SB1 23TEl 23SN124TE124SE125TE125TEI25FSN126

2.188-008 2.575-00e 2.963-0087.C48-004 7.048-004 7.048-0045.963-005 5.963-OC5 5.963-CO55.SC2-004 5.9C2-004 5.902-C045.E40-004 5.840-004 5.840-C046.149-011 3.813-011 2.364-0113.827-004 3.827-004 3.827-0044.194-004 4.194-OC4 4.194-0041.446-004 1.446-0C4 1.446-C043.COO-004 3.OCC-004 3.000-0041.340-007 3.388-00a 8.564-C091.260-013 3.115-014 8.050-C152.749-004 2.75C-004 2.750-0041.715-004 1.715-004 1.715-CO42.C13-010 2.379-01C 2.745-0101.182-004 1.182-OC4 1.182-0048.336-013 .246-013 8.156-C13

3.350-0087.048-0045.963-0055.902-oc45.84 0-0041 .466-01 13. 827-0044.194-0C41.446-0043. 000-0042.165-OC92.035-0152.750-oc41 .715-0043.111-0101.182-0048.068-013

2.f45-010 2.645-01C 2.645-C10 2.645-0106.2 35-0051.131-0153.169-0052.372-0112.252-0052.162-0051.298-0051.475-0071.241-0078.517-0081.775-0057.661-0102.266-0062.570-0076.565-0065.468-006:6.46-0o66.696-0066.673-0061. 339-0126.102-0062.377-0096.706-0067.4 87-0063. 6 79-0071.081-0158.219-0064.641-0091.CO9-0052.746-007

t.235-05 6.235-0053.798-01 1.275-0163.869-oc5 3.869-COS3.127-012 4.122-C132.252-OC5 2.252-0052.162-OC5 2.162-0051.29E-005 1.298-CO51.475-O? 1.475-0071.129-OC7 1.026-0079.641-008 i.066-0071.775-005 1.775-0057.661-01C 7.661-0102.266-0C6 2.266-C062.570-OC7 2.570-0076.565-O6 6.565-0065.468-00d 5.468-0066.646-006 6.646-0066.696-006 6.696-0066.673-006 6.673-0061.696-013 2.147-0146.8C2-006 6.802-0062.312-009 2.248-0096.7C6-OC6 6.706-0067.487-006 7.487-0063.679-OC? 3.679-0072.146-017 4.257-C19E.219-OC6 8.219-0064.641-009 4.641-CO91.0C9-005 1.009-0052.746-007 2.746-007

f.235-OC54. 283-0173.869-0055.434-0142.252-0052.162-0051.298-0051.475-0079.334-0081.159-0071.775-0057.661-0102.266-0062.570-0076. 565-0065.468-0066.646-0066.696-0C66.673-0062.719-0156.802-0062.187-0096. 706-0067.487-0063.679-oc78.442-0218.219-0064.641-0091.009-0052.746-0072.076-0071.489-0052.905-oc92.168-005

9.319-007 -5.65c-007 3.425-0071.416-005 1.453-005 1.475-005

-1.303-008 7.9C4-009 4.792-0092.168-005 2.168-005 2.168-005

E. 59



SB126S8126'TE126TE127P1127

TE128XE128I129

XE129TE130XE130XE131XE1323A132CS133XE134CS134BA1334CS135SAl 35XE136BA 136CS137BA1 37BA137MSA138LA138LA139CE140PR1 41CE142ND142N0143CE144PR144PR144PND144ND1 45ND146P1146Sf146PM1147SM147ND148Sf148SM149ND15CSf450EU150SM151EU151SM152

1.C30-C127.131-0155.737-0071.C02-0164.400-0058.559-0051.913-0061.397-0048.797-0092.717-0047.763-0063.4 88-0047.S96-0041.177-C098.761-C041.109-0032.647-0069.765-0052.644-0041.248-0071.731-0031.308-0057.188-0042.142-0041.100-0109.607-0044.397-0099.197-0049.280-0048.461-0048.485-0041.590-0056.2 28-0043.121-0081 613-0128.C66-0159.565-0045.171-0045.C60-0041 .411-0094.627-0099.C02-0061.670-0042.101-0041.197-0042.2 58-0061.354-0041.891-0041.363-013l.CO1-0058.106-0071.C39-004

1.03C-0127.83C-0155.74C-OG7S.63C-0194.4CC-OC58.559-OCS1.913-OCt1.357-0048.81C-OCS2.717-OC47.763-0063.488-OC47.996-OC41.177-008.761-OC4I .1C9-0C31 .351-OC69.894-OC52.644-OC41 .25C-0071.731-0031.3C8-OC56.863-OC42.467-0041 .0SC-o1 C9.aC7-OC44.397-OS9.197-OC49.20C-OC48.461-OC48.485-OC41,.SSG-OCS6.228-OC46. 436-0092. 717-0131.358-0159.566-OC45.171-0045.06C-O041.097-0094.743-0095.3C7-0061 .7C7-OC42.8G1-0041.197-0042.258-OC61.354-OC41.891-0041. 311-0139.857-O009.637-0071.039-004

1.030-012 1.030-0127.830-015 7.830-0155.743-007 5.746-OC79.245-021 9.333-0234.400-005 4.400-OC58.559-C05 8.559-OC51.913-006 1.913-OC61.397-004 1.397-OC48.822-009 8.835-OC92.717-C04 2.717-0C47.763-006 7.763-0063.488-C04 3.488-OC47.996-CO4 7.996-0041.177-009 1.177-0098.761-004 8.761-0041.109-003 1.109-0036.898-O07 3.522-0079.961-C05 9.994-0052.644-004 2.644-OC41.251-C07 1.253-0071.731-003 1.731-0031.308-COS 1.308-OCS6.553-004 6.257-0042.776-004 3.072-OC41.03-010 9.573-0119.607-004 9.6C7-0044.397-009 4.397-0099.197-004 9.197-0049.280-C04 9.280-0048.461-004 8.461-0048.485-004 8.485-0041.590-005 1.590-OC56.228-004 6.228-OC41.084-009 1.826-0104.577-014 7.708-0152.288-C16 3.853-0179.566-004 9.566-0045.171-004 5.171-0045.C60-004 5.060-0048.524-010 6.625-0104.833-009 4.904-0093.129-006 1.844-0061.728-004 1.741-OC42.801-004 2.801-0041.197-004 1.197-0042.258-006 2.258-0061.354-004 1.354-0041.891-004 1.891-0041.262-013 1.214-0139.707-CG6 9.558-OC61.114-006 1.263-OC61.039-004 1.039-004

E.60



EU152GDISZEU1 536D153SM154EU154GD154EU1556D155GD156GD157GD158TB159GD160DY.16CDY161DY162DY163DY164HC16510166FER166ER167ER16tTM169ER 70YSITOTMI71Y8171Y8172SUMTOI

TOTAL,

1 .43-008-1.466-0088.C09-0052.$ 66-0132.869-0051.163-005i.f10-0052.386-0067.336-0064.t31-0057.708-0081.319-0052.C15-0069.E58-0071.83-007.3.353-0072.S03-0072.125-0073.241-0089.548-0088.571-0103.C84-0082.509-0095.37-0093.541-0111.365-0149.194 0129.216-0155.390-0131.294-0142.574-002

'2.574-002

1.754-0081.518-OC8e sOc-'OCS3.661-0142.869-0059.899-OC61 .783-OC51.8C4-OOE7.918-OCe4.031-OCS7.7CE-OC81.319-OCS2.015-OCE9.858-OC71 .883-OC73.353-OC72.9C3-0072.125-OC73.241-00E9.94E-0088.561-01C3. 084 -0082.5CS-0095.837-OC93.541-0111.365-0149.194-0124.477-0155.437-0131.294-0142.574-OC2

2. S74-002

1.*584-0081.566-0088.C09-OO54.518-0152.869-0058.4 25-0061 .930-COS1.364-0068.358-0064.C31-C057.?08-C081. 319-C052.C15-C069.858-CO71.683-C073.353-C072.903-C072.125-0073. 2 41-0089.948-0088.5 51-0103.084-0082.509-0095.837-0093.541-0111.365-0149.194-0122.175-0155.460-0131.294-0142.574-002

2.574-002

1.431-OC81.608-008e.009-OC55.576-0162.869-OC57.171-OC62.056-0051.032-0068.690-OC64.031-0057.708-0C81.319-0052.01 5-0069.858-OC71.883-OC73.353-OC72.903-0072.125-0073.241-0089.948-OCS8. 542-0103.084-0082.509-OC95.837-OC93. 541-0111.365-0149.194-0121.056-0155.471-013.1.294-0142.574-002

2.574-002

..

. . .

. .

. .

, .. .

.

:

.:

I

E.61



HLIBE

CZNGAGEASSEBRKR

SRY

ZRNB8

TCRURHPDAGCDINSNS3TEIXECSBALACE.PRNDPpS14EU

TaDYHOERTMY3SUMTOT

2.S02-0081.07-0101.132-0101.988-0112.813-0146.8 76-0135.C89-0071.'62-0074.252-CO51.51-0052.672-0042.629-0045.743-0043.396-0042.715-0033.399-0092.523-0035.953-0041.653-0033.e27-0041.C48-0036.235-0058.171-0052.351-0067.180-0051.586-0053.726-0041.837-0043.998-0031.e62-0031.286-0039.197-0041.776-0038.461-0043.C34-0039.C03-0066.207-0049.494-0057.801-0052..C15-0061.C59-006I.C03-0073.18-0083.542-0119.746-0122.574-002

2.236-OCE 1.999-0081.6C7-01C 1.607-CIO1.132-01C 1.132-C01.987-011 1.987-0112.813-014 2.613-C14t.876-013 6.876-C135.085-0C7 5.C89-CO71.562-007 1.562-C074.252-OC5 4.252-0051.651-005 1.651-C052.6CC-OC4 2.650-0042.64C-OC4 2.650-C045.597-OC4 5.458-CO43.396-004 3.396-CO42.73C-003 2.744-C033.889-0C9 4.378-C092.523-00 2.523-0035.953-004 5.953-0041.653-OC3 1.653-0033.827-OC4 3.827-C041.048-OC3 1.C48-0036.235-OC5 6.235-0058.17C-OC5 8.169-0052.363-006 2.373-C067.IOC-OC5 7.180-0051.549-OCS 1.527-0053.73C-004 3.732-C041.837-004 1.837-0043.998-003 3.998-0031.828-OC3 1.797-0031.319-OC3 1.351-C039.197-004 9.197-CO61.776-003 1.776-0038.461-OC4 8.461-C043.034-OC3 3.034-C035.3CI-006 3.129-0066.242-OC 6.262-0049.278-O5 9.101-0058.033-005 8.224-0052.015-OC 2.C15-0061.059-OCe 1.C59-0061.0C3-OC7 1.C03-0073.918-00! 3.918-0083.541-011 3.541-0119.751-012 9.753-0122.574-OG2 2.574-002

1 .787-OC81.607-0101.132-0101.986-0112.813-0146.876-0135.089-OC71 .562-OC74.252-OC51.651-OC52.641-OC42.659-OC45.325-OC43.396-O42.757-OC34.868-od92. 523-0035. 953-0041.653-0033.827-OC41.048-OC36.235-0058.168-0052.382-0067.180-0051.513-0053.734-OC41.837-0043.998-0031.767-0031 .381-0C39.197-0041.776-OC38.461-OC43.034-0031 .845-O66.274-0048.957-0058.383-0052.015-0061.059-0061.003-0073.919-0083.541-0119.754-0122.574-002

TOTAL 2.574-002 2.574-002 2.574-C02 2.574-002

E.62

'-4

TABLE E.4.g. Fission Products (Isotopic), Ci/gU, at 25 MWd/kgM

- ICI YEARS 12 YEARS 14 YEARS 16 YEARS

H 3-BE- 10C 14

SE 79KR, 81KR -85Re 87SR 90

Y.90ZR 93NB 93PNB 94rC 98TC 99RH102RU106RH106PD107AG108AGIO8P!A6109PC D109AGI 10AG1 1OCD113PSNI 19VSN121SN123TE123VSB125TEI 2SSN126Se126SB126TE127TEI27P1129

CS134CS135CS137BAI 37VCE142CE144PR144PR144PND144PM1146SM1146PH1147SM147EU150SM151

2.416-004 2.159-OC4 1.930-004 1.725-0042.200-012 2.200-012 2.200-012 2.200-0128.E62-011Ve.86C-011 8.858-011 8.856-0113*112-007 3.112-OC7 3.112-C07 3.112-OC?3.399-013 3.399-013 3399-013 3.399-013-3.78-003 3.232-oC3-2.840-003 2.495-OC31.589-0114.280-002-4.281-0021.356-0065.f60-0071.126-0103.426-0121.ClO-Q057.435-0084.487-0044.487-0048.E26-0081.535-0122.174-0112.S22-0122.922-0121.499-0091.127-0072.693-0055.599-0091.406-0078.892-012S.C74-0159.f27-0042.349-0046.153-0078.f14-0086.153-0079. 263-0139.4 57-0132.4 67-0083.4 26-0033.C46-0076.2 55-0025.S17-0022.C37-0111.219-0041.219-0041.463-0061.132-0156.285-0071.619-0138.348-0033.796-0129.C27-0122.635-004

1.589-01 14.081-OC24.082-OC?I .358-00t6.380-0071.126-01C3.426-0121 .01C-0C54.610-OC81.134-OC41.134-0C48.826-0081.914-0122.15C-0119.811-0139.811-0131.977-01C1.466-0082.449-OCS7.597-01C1.367-0071.764-0137.379-0175.836-0041.424-004i.153-OC7e.614-OCS6.153-0078.9CC-0159.08 7-0152.467-OE1.749-0033.046-0075.97!-OC25.65C-OC22.037-0112.034-0052.054-OC52.445-0071.132-0154.885-0071.66G-0134.921-0033.88G-0128.6E6-0122.594-004

1.589-C11 1.589-0113.892-C02 3.711-OC23.892-C02 3.712-0C21.358-006 1.358-OC67.C12-007 7.583-OC71.126-C1O 1.126-01C3.426-C12 3.426-0121.C1O-005 1.010-0052.858-008 1.772-OC82.867-CO5 7.246-0062.867-005 7.246-OC68.826-008 8.826-0081.893-012 1.872-0122.127-011 2.104-0113.294-013 1.106-0133.294-013 1.106-0132.605-C11 3.435-0121.959-C09 2.582-0102.227-005 2.025-OS9.619-011 1.218-0111.330-CC7 1.293-0073.500-015 6.941-0171.C43-018 .0003.538-004 2.145-0048.o34-C05 5.234-0056.153-C07 6.153-0078.614-008 8.614-OC86.153-007 6.153-0078.551-017 8.624-0198.724-017 8.807-0192.467-008 2.467-OC88.929-004 4.558-OC43.046-007 3.046-0075.703-C02 5.445-0025.395-002 5.151-0022.037-011 2.037-0113.459-006 5.826-0073.459-006 5.826-0074.151-008 6.991-0091.132-015 1.132-0153.797-007 2.951-0071.691-C13 1.716-0132.901-003 1.710-0033.929-012 3.959-0128.358-012 8.042-0122.555-004 2.516-004

E. 63

YABLE E.4. . 1Contd)


EUI 52GD1 53EU1 54EU155H0166PTM 71SUMTOT

TOTAL

3.361-006 3.035-OC61.C46-009 1.292-01C3.141-003 2.673-OC31.1 10-003 E.395-OC41.539-009 1.537-OC91.C04-011 4.877-0122.299-001 2.121-OC1

2.299-C01 i.12E-OCI

2.74 1-C061.594-0112.275-C036.348-0041.535-0092. 369-01 21 .994-001

1 .994-COI

2.475-0061.967-0121 .936-0034.800-0041 .534-0091.151-012I .880-OCI

1.880-OCI

-I

E.64

JTABLE E.4.h. Fission Products (Elemental), Ci/gU, at 25 MWd/kgM


H24 1 6s416-004 2.159-OC4 1.930-004 1.725-0049E 2.200-012 2.2CC-012 2.200-012 2.200-012C 8.862-011-E.86C-011 8.858-011 8.856-o1

SE 3.112-007 3.112-OC7 3.112-007 3.112-007KR - 3078-003 3.232-003 2.840-C03 2.495-0C3'R - 1.589-011 1.589-011 1.589-C11 1.589-011SR -4.280-002 4.081-002 3.892-002 3.711-OC2Y 4.281-002 4.082-002 3.892-002 3.712-002

ZR 1.358-006 1.35E-OCE 1.358-006 1.358-006NO 5.681-007 6.381-OC? 7.C14-C07 7.584-007TC 1.CIO-005 1.O1C-005 1.G10-C05 1.010-OC5RU '4.487-004 1.134-OC4 2.867-CO5 7.246-006RH 4.488-004 1.135-OC4 2.869-C05 7.264-006PO 8.826-008 8.826-OC8 8.826-COB 8.826-oCeAG 1.143'007.1.5C8-OC8 2.C09-C09 2.847-010CD -. 693-005 2.449-005 2.227-CO5 2.025-005SN ; 7.419-007 7.528-007 7.483-CO7 7.446-007Se 9.634-004 5.843-OC4 3.545-04 2.152-OC4TE 2.249-004 1.424-OC4 8.634-CO5 5.234-OC5I 2.467-008 2.467-00e 2.467-008 2.467-008

Cs 6.598-002 i.148-OC2 5.792-002 5.491-OC2BA 5.517-002 5.65C-OC2 5.395-002 5.151-OC2CE 1.219-004 2.054-005 3.459-006 5.826-007PR 1.234-004 2.07$-OC5 3.501-006 5.896-007ND 1.132-015 1.132-015 1.132-015 1.132-015PM 8.349-003 4.922-003 2.902-C03.1.711-003SM 2.635-004 2.594-004 2.555-C04 2.516-004EU 4.254-003 3.516-003 2.913-003 2.419-0036 1.C46-009 1.292-01C 1.594-011 1.967-012HO 1.539-009 1.537-OS 1.535-CO9 1.534-009TM 1.C04-011 4.877-012 2.369-012 1.151-012SUMTOT 2.299-001 2.128-001 1.994-001 1.880-001

TOTAL 2.299-001 2.12E-001 1.994-001 1.880-001

E.65

TABLE E.4.i. Neutron Source (Alpha-n), neutrons/sec-gU, at 25 MWd/kgM

IC YEARS 12 YEARS 14 YEARS 16 YEARS w

PU238 1.362'000 1.341+0CC 1.320+COO 1.300+000PU239 2.228-001 2.227-OC1 2.227-001 2.227-001PU240 3.387-001 3.382-OC1 3.388-001 3.388-001AP241 1.466+000 1.e65+OCC 1.845+000 2.008+000AM243 9.136-003 9.134-OC! 9.132-003 9.130-003 w

CM242 6.727-003 6.67C-OC3o.610-C03 6.550-003CI243 1.202-002 1.145-OC2 1.G91-C02 1.039-OC2C1244 7.672-001 7.1C7-OG1 6.583-COl 6.098-001

TABLE E.4.J. Neutron Source (Spontaneous fission), neutrons/sec-gU,at 25 MWd/kgM

iC YEARS 12 YEARS 14 YEARS 16 YEARS

PU238 2.222-001 2.187-OCI 2.153-CO 2.119-001PU240 1.786+000 1.786+0CC 1.786+000 1.786+000PU242 5.468-001 5.668-001 5.668-001 5.668-001C4244 9.237*001 2.556+001 7.926+CO1 7.342+OC1CM246 3.280-001 3.27S-OCi 3.279-COl 3.278-001

E .66

TABLE E.5. Radionuclide Inventories at 30 MWd/kgM as a Function of Decay Time

Subtable Species - Units

E.5.a Actinides (Isotopic), g/gU E.69

E.5.b Actinides (Elemental), g/gU E.70

E.5.c Actinides (Isotopic), C/gU E.71

E.5.d Actinides (Elemental), Ci/gU E.73

E.5.e Fission Products (Isotopic), g/gU E.74

E.5.f Fission Products (Elemental), g/gU E.78

E.5.g Fission Products (Isotopic), Ci/gU E.79

E.5.h Fission Products (Elemental), Ci/gU E.81

E.5.i Neutron Source (Alpha-n), neutrons/sec-gU E.82

E.5.j Neutron Source (Spontaneous fission), neutrons/sec-U E.82

E.67



HE 4P8207P8208PB21281212RA224RA226AC227T228TH229TH230TH231TN232TH234PA231PA233U232U233U234U235U236U237U238

NP235NP236NP237NP238NP239PU236PU238PU239PU240PU241PU242PU244AF1241AP242PAM242AM243CM242CM243CM244CM245C1246CM247C248CF249CF250CF251CF252SF250SUNTOT

9.714-007 1.07C-OC6 1.170-C061.C29-015 1.58C-015 2.295-015'4.785-011 6.487-011 8.268-0111.464-014 1.561-014 1612-C141.388-015 1.481-015 1.529-0151.277-013 1.362-013'1.406-0136.C91-015 5.852-015 1.490-0148.260-015 1.051-014 1.388-0142.481-011'2.64C-011 2'.726-C111.889-013 2.028-013 2.189-C131.799-010 2.478-01C 3.263-0102.468-014 2.448-014 2.468-C14'1.C70-009 1.255-OCS 1.440-C091.379-011 1.375-011 1.379-0117.257-011 8.435-011 9.612-C111.315-011 1.32C-011 1.327-C111.C5S-009 1.073-OCS 1.C74-C091.478-009 1.739-OC9 2.000-0091.124-005 1.315-OC5 1.502-COS6.C70-003 6.07C-OC3 6.C70-C033.177-003 3.177-003 3.178-CO32.419-011 2.197-011 1.995-Cl19.501-001 S.5C1-OC1 9.501-0016.534-015 1.819-015 5.067-0163.f20-010 3.62C-01C 3.620-0103.870-004 3.888-OC4 3.907-0041.313-013 1.3C1-013 1.289-0138.312-011 8.31C-011 8.308-0119.292-011 5.714-011 3.514-C111.234-004 1.215-OC4 1.196-C045.C47-003 5.047-003 5.046-0032.303-003 2.3C4-OC3 2.305-0037.E13-004 7.096-004 6.445-0044.548-004 4.948-004 4.S48-C042.652-008 2.652-008 2.652-0085.116-004 5.816-004 6.447-0047.C03-007 6.939-007 6.876-0078.377-012 8.3C1-012 8.226-0129.71-005 S.67G-005 9.668-0051.96-009 1.681-005 1.666-0092.987-007 2.845-OC7 2.710-C071.S21-005 1.78C-005 1.648-0051.C23-006 1.023-06 1.023-0061.262-007 1.262-07 1.262-0071.161-009 1.161-009 1.161-0095.855-011' 5.855-011 5.855-0116.C37-013 6.015-013 5.991-0136.191-014 6.198-014 5.575-0144.453-014 4.446-014 4.439-0141.866-015 1.103-015 6.523-0161.534-011 1.734-011 1.920-0119.091-001 9.691-001 9.691-001

1.271-0063.190-0151.009-0101.634-0141.550-0151 .425-0132.143-0141.713-0142.762-0112.372-0134.152-01C2.468-0141 .625-OC91.379-0111.079-0101 .334-0111 .06?-OC92.263-0091. 686-0056.07C-OC33.178-OC31.812-011S.501-OCI1.411-0163.620-0103.928-OC41.278-0138. 307-0112.161-0111.177-OC45.046-0032.306-OC35. 853-0044.948-0042.652-0087.017-0046.814-O78.151-0129.666-0051.651-OC92.581-0071.527-0051.022-0061 .261-OC71.161-0095.855-0115.968-0135.014-0144.432-0143.857-0162.092-0119.691-001r _ _

E.69


10 YEARS 12 YEARS 14 YEARS 16 YEARS "S0

HESFPe9IRAACTPA

UPPUA Poc pCFSUMTCT

9.714-0071.534-0114.786-0111.568-0151.338-0138.i61-0151.286-0098. 5 72-0119.593-0013.e70-0048.750-0036.C90-0042.C66-0057.190-0139.t91-001

1.07C-OCe1 .734-0116.4E2-O1 11.695-0151 .461-0131 .092-0141 .543-0C99.755-0119.593-OCI3.882-OC42.677-OC36.79C-OC41 .923-0057 .09C-0139 .691 -001

1.170-0061.920-C118.270-C111.779-CI51.556-C131.388-C141.807-C09I .C94-C1O9.593-C0l3.SC7-CC48.610-CC37.421-004t .791-COS6.999-C139.691-001

1.271-OC62.092-0111 .009-01C1. 839-0151.640-0131.714-0142.081-OC91.212-0109.593-OC13.928-OC48.550-OC37.991-0041 .668-OC56.916-0139.691-OC1

TCTAL 9.f91-001 9.6S1-OCI 9.891-COl 9.691-OCI

'S

E.70

JS



TL207TL208TL209PB2G9P5210PE211PE212PE214BI2106121181 212BI213d1214P0210PC21 1P0212P0213P0214P0215P0216P0218AT217RN219RN220RN222FR221FR223RA223RA224RA225RA226AC225AC227TH227TH228TH229TH230TH231TH232TH234PA231PA233PA234PPA234U232U233U234U235U236U237U238U240

5.962-013 7.889-013-1.C03-CI27.310-009 7.798-OCS 8.C52-C098.d8 5-0164.C21-0141. 120-0155.578-0132.C35-008*6.C24-0151.121-0155.578-C132.C35-00B4.C21-0146.C24-01 51.121-01511.474-0151.304-0083.934-0146.C22-0155.S78-0132.C35-0086.C25-0154.C21-0145.578-0132.C35-0086.C25-0154. C21-01.48. 249-0155.S78-0132.C35-0084.C21-0146.C25-0154.C21-0145.577-0135.896-0132.C35-0084.C21-0143.632-0121.313-0081.174-0163.195-0073.429-0122.729-0073.195-0074.154-0102.267-0081.432-0117.C29-0081.313-0082.C56-0071.S75-0063.195-0074.699-013

9.322-01d4.316-0141.522-01 57.911-0132.17C-OCe9.743-01 51.523-0157.911-0132.17C-OCE4.316-0149. 74 3-0151-. 39C-01 S2.215-01'I .391-OCE4.222-0149.741-015-7.911-0132.17C-OCE9. 74 5-0154.316-0147 .911-01 32.17C-OCe9.745-0154.316-0141 .090-01 47.911-0132.17G-OC84 .316-0149.745-0154.316-01 47.898-0137.802-0132.16 5-0Ce4 .316-0145.0C5-0121.31 3-OC81 .377-0163.195-OC73.986-0122.742-0073.195-0074.154-01C2.299-00e1.684-0118.218-00e1.31 3-00e2.056-0071 .794-0063.195-0074.699-013

E. 71

1.C06-C154.6 58-C142.161-C151.006-Cl 22.241-CC81.474-C 142.162-C 151 .C06-C122.241-CC84.653-C141.474-C141.953-C152.817-C1 5

;1.4 36-C084. 5 57-01 41. 474-C141.006-C122.241-COS1.4 74-0 144.658-0141 .C06-C122.241-COB1.474-C144.658-0141.386-C141 006-Cl22.241-0084.658-C141.474-C144.658-0141.004-0129.922-C132.235-C084.658-0146. 590-0121.313-C081.579-C163.195-0074.542-0122.755-0073.1 95-0074.1 54-CIO2.301-0081.9 37-0119.388-0081.313-0082.057-0071. 6 29-0063.195-0074.699-013

1. 239-012E.159-OC91.090-0155.04e-0143.107-0151.242-0122.271-OC82.119-0143.1C8-0151.242-0122.271-0CE5.048-0142.119-0142.803-0153 .478-01 51.455-OC84. 939-0142.119-0141.242-0122.271-OC82.120-0145.048-0141.242-0122.271-0082.120-0145.048-0141.711-0141.242-0122.271-OC85.048-0142.120-0145.048-0141.240-0121. 225-0122.265-OC85.048-0148.384-0121.313-0081.782-0163.195-0075.098-0122. 770-0073.195-OC74.154-0102.28 5-0082.191-0111.054-0071.313-0082.057-0071.480-0063.195-0074.699-013



NP235NP236NP237NP238NP239NP240PPU236PU238PU239PU240PU241PU242PU243PU244AP241AM2421AM242AM243CM242CM243CM244CO245CM246CM247CM248BX249CF249CF250CF251CF252SU!T07

9.170-0124.771-0122.7 29-0073.404-0081.S29-0054.099-0134.S39-0082.114-0033. 139-CO45.250-0048.C53-0021 .90-0061 .C78-0134.7 05-0131.757-0036.809-0066.775-0061.S29-0055. 1-0061.S42-0051.555-0031.7 5 7-0073.879-008I C78-0132.490-0133.280-0132.474-0127.536-0127.C65-014t.C04-0128.87-002

2 .554-0124.771-0122.742-OC7-. 374-0C81 .928-OC54. 699-0133.037-OCe2.081 -0033.138-0045.252-OC47.313-OC21.89C-OCd1.078-0134.7C5-0131.9S7-0036.747-0066. 713-0061 .928-OC55.562-OCe1 .469-OC51 .44C-OC31 .757-OC73.878-Oe1.078-0132.4SC-0136.74C-0142.465-0126.778-0127.054-0145.935-0137.957-OCZ

7.111-013 1.980-0134.771-Cl2 4.771-0122.755-007 2.77C-0073.343-C08 3.313-OC81.928-C05 1.928-OC54.699-013 4.699-0131.868-008 1.149-0082.048-C03 2.016-0033.138-C04 3.138-OC45.254-004 5.256-OC46.642-CO2 6.033-OC21.890-C06 1.890-OC61.C78-C13 1.078-0134.705-013 4.705-0132.214-003 2.409-OC36.686-C06 6.625-OC66.652-006 6.592-OC61.928-005 1.928-0055.511-006 5.461-OC61.399-C05 1.333-OC51.334-C03 1.236-OC31.756-007 1.756-OC731077-08 3.876-0081.078-C13 1.078-0132.490-013 2.490-0131.385-014 2.847-0152.455-012 2.446-0126-.097-Cl2 5.484-0127.C43-C14 7.032-0143.509-013 2.075-0137.293-002 6.690-002

TOTAL 8.487-002 7.957-OC2 7.293-C02 .690-002

.,

'-w

E. 72

TABLE E.5.d. Actinides (Elemental), C/gU, at 30 MWd/kgM

IC YEARS 12 YEARS 14 YEARS. 16 YEARS

TL 7.311-009 7.799-OCS 8.C53-C09PE 2.C35-008 2.17C-OC 2.241-0088I 2.C35-008 2.17C-00e 2.241-008P0 3.338-008 3.561-00C 3.677-008AT 4.C21-014 4.316-014 4.658-014RN 2.C35-008 2.17C-00 2.241-008FR 4.146-014 5.4G5-014 6.C44-014RA 2.C35-008 2.17C-0C 2.241-COAC 6.380-013 6.33C-013 1.C51-C12TH 3.530-007 3.543-0C7 3.550-007PA 5.929-007 5.941-007 5.955-007U 2.407-006 2.438-OCd 2.285-C06

NP 1.559-005 1.959-OC5 1.S59-C05PU 8.348-002 7.6C6-0C2 6.931-CC2AM 1.790-003 2.03C-0C3 2.246-C03CM 1.576-003 1.461-OC3 1.354-003SK 3.280-013 6.740-014 1.385-014CF 1.108-011 9.9E7-012 8.973-C12SUMNOT 8.687-002 7.957-0C2 7.293-C02

TOTAL 8.e87-002 7.957-OC2 7.293-C02

8.160-OC92.271-0082.271-0083.726-oC85.048-0142.271-0086.759-0142.271-oC81.290-0123.553-0075.970-0072.147-OC61.959-OC56.318-OC22.442-OC31.255-0032.847-0158.207-0126.690-aC2

6.690-002

i 11

.~ ~E 73



HLILIBeBE

CZNZNGAGEGEGEASGESESESESEBRSEKRBRKRSEKRKRKRKRRSKRSRRSSRSR

YSR

YZRZRZRZRNBN3ZRNBNoZRMONoMOTCTC

3679

101466677172737475767677787979-sO8C81818282838485858686878788899090909192939393P949495969697989899

3.C58-0081.579-0109.176-0121.766-0111.179-0102.381-0113.C77-0141.265-0158.4 32-0132.137-0084.283-0089.C91-0081.8 57-0074.492-0075.C84-0099.148-0072.194-0065.2 89-0066.459-0101.193-0052.243-0101.928-0052.286-0112.965-0058.533-0073.5 85-0059.891-0051 .C87-0059.419-0051.435-0043.5 72-0072.C95-0042.S87-CO93.CC2-0043.908-0043.12-0049.C57-0081.138-004S.C95-0045.568-0046.314-0049.254-0102.350-0096.549-0047.456-0106.740-0047.141-0043.C09-0057.130-0047.470-0045.761-0096.990-004

2.733-OC81.579-OIC9.176-0121 .766-0111.179-O1C2.38C-0113.077-0141.265-0158.432-0132.137-0084.283-0019.091-OCE1.857-0074.492-0075. 084-0099.148-0072.194-OC65.2e9-OCd7.588-Ol1.193-OC52.243-O1C1.928-OC52.28f-0112.965-OC58 .933-OC73.585-0059.891-OC59.553-00f9.551-OCS1 .635-OC43.572-0072.095-OC42.987-0093.0G2-OC43.9Ce-0C43.444-0048.636-OC1 3C6-OC45.095-0045.568-OC46.314-OC41.2C9-0092.639-0096.549-OC47.655-O1C6.74C-0047.141-0043.0C9-OC57.130-0047.47C-0045.7 61-0096.99G-004

E. 74

2.443-C081 .579-C1O9.176-C121.766-Ct11.179-0102.380-a113.C77-0141.265-0158.432-0132.137-0084.283-0089.C91-CO1 .857-0074.492-0075.084-C099.148-0072.194-C065.288-0068.716-C101.193-0052.243-0101.928-0052.286-0112.965-C058.933-0073. 585-0059.891-COS8.394-0069.667-0051 .635-0043.572-0072.G95-0042.987-C093.C02-C043.908-0043.284-0048.234-COS1.467-0045.095-0045.5 68-0046.314-0041.5 20-0092.900-0096.549-0047.655-0106.740-0047.141-0043.009-0057.130-0047.470-0045.761-0096.990-004

2.183-0081.579-0109.176-0121.766-0111.179-0102.379-0113.077-0141.265-0158.432-0132.137-0084.283-0089.091-OC81.857-0074.492-0075.084-0099.148-OC72.194-0065.288-OC69.845-0101.193-0C52.243-0101.928-0052.286-0112.965-OC58.933-OC73.585-OC59.891-OC57.376-0069.768-0051 .635-OC43.572-OC72.095-OC42.987-OC93.002-0043.908-OC43.131-0047.852-0081.619-0045.095-0045.568-0046.314-0041 .856-0093.135-0096.549-0047.654-0106.740-0047.141-0043.009-0057.130-0047.470-0045.761-0096.990-004

'S0



RU 99M0100RU10RU101RU102RHI02RHI03RU104PD104PD105RU 106RHI06PD106P107'A6107PD108AGI 08PCD108A6109C0109PD110AGIIOPCDO10CDIi1C0112CD1 13CD1 3IN1 3CDil4SN114INISSN115CD116SN116SN117SN118SN119SN1 19 PSKI 20SN1 21PSIB1 21SKI 22TE1 22SN123SB123TE1 23SN1124TE1245B125TE125TE125PSN1126

2.569-008 3.024-OC 3.479-0088.460-004 8.460-OC4 1.460-0048.704-005 8.7C4-OC5 8.704-GO57.C75-004 7.075-OC4 7.C75-0047.155-004 7.155-OC4 7.155-0048.509-011 5.523-011 3.424-C114.422-004 4.422-OC4 4.422-CO45.280-004 5.28C-OC4 5.280-C042.C93-004 2.093-004 2.093-0043.755-004 3.755-OC4 3.755-C041.751-007 4.427-OCE 1.119-C081.646-013 4.161-014 1.C52-0143.666-004 3.66e-004 3.668-0042.255-004 2.255-004 2.255-0042.644-010 3.129-OIC 3.607-0101.562-004 1.562-004 1.562-C041.105-012 1.093-012 1.G81-0124.204-010 4.2C4-01C 4.204-C107.S05-005 7.9C5-005 7.905-0052.133-015 7.163-016 2.405-0165.112-005 5.112-OC5 5.112-0053.723-011 4.9C8-012 6.470-0133.568-005 3.56e-005 3.568-0052.132-005 2.832-005 2.832-0051.481-005 1.681-005 1.681-0051.523-007 1.523-007 1.523-0071.f41-007 1.492-007 1.357-0071.121-007 1.269-OC7 1.404-0072.236-005 2.236-005 2.236-0051.192-009 1.152-009 1.192-0092.365-006 2.365-OC6 2.365-C063.164-007 3.164-OC7 3.164-C078.C83-006 8.083-006 8.083-0067.246-006 7.246-006 7.246-0068.170-006 8.17C-OC6 8.170-006.8.229-006 8.229-006 8.229-0068.207-006 .2C7-OC6 8.207-0061.713-012 2.169-013 2.746-0148.359-006 8. 359-OCU 8.359-0062.990-009 2.908-OC9 2.828-0098.131-006 6.131-O00 8.132-0069.183-006 9.183-OC6 9.183-0065.476-007 5.476-007 5.476-0071.331-015 2.641-017 5.240-C199.S99-006.9.999-O06 9.999-0067,.742-009 7.742-009 7.742-0091.234-005 1.234-005 1.234-0054.117-007, 4.117-007 4.117-0071.153-006 6.991-007 4.238-0071.749-005 1.795-005 1.823-005

-1.613-008,9.781-009 5.929-0092.674-005 2.674-005 2.674-005

3.933-0C8,8.460-OC48.704-OC57.075-0047.155-0042.123-0114.422-OC45.280-OC42.093-0043.755-OC42.829-OC92. 659-0153.668-O42.255-OC44.088-0101.562-0041.070-0124.204-0107.905-0058.077-0175.112-0058. 529-0143.568-0052.832-0051.681-OC51.523-OC71.234-OC71.527-0072.236-OC51.192-OC92.365-OC63.164-0078.083-0067.246-0068.170-0068.229-OC68.207-0063.478-0158.359-0062.751-0098.132-OC69.183-0065.476-0071.039-0209. 999-0067.742-0091.234-OC54.117-0072.569-0071.840-0053.595-0092.674-005

E. 75


IC YEARS 12 YEARS 14 YEARS 16 YEARS'Sd

S5126SB1 26PTE1267E127P

1127TE128XE1281129

XE129TE130XE130XE131XEt323A132CS133XE134CS1348AI 34CS1353A1 35XE136SA1 36CS137SA1 37SAl 37PBA138LA1 38LA139CE140PRI 41CE142ND1 42ND143CE144PR144PRI 44PND144ND1 45ND 46PM146SM1146PM1I47S14147N0148SM148S149ND1SOS150EU15CSM1 518U151SM152

1.271-'0129.460-0157.460-0071.247-0165.409-0051 .C48-0042.504-0061.693-0041.617-0083.306-0041.158-0053. S 60-0049.527-0041.714-0091 .C22-0031.329-0033.740-0061.381-0042.813-0042.187-0072.125-0031.96-0058.33-0042. 57 2-0041.321-0101.144-0034.687-0091.C94-0031.112-0031 .C03-003.C09-003

2.3 32-0056.534-0044.498-0081.199-0129.494-0151.179-0036.C07-0046.165-0041.894-0096. 210-0099.3 97-0061.742-0043.362-0041.5 31-0042.474-0061.653-0042.288-0041.481-0131 .C79-0058.716-0071. 197-004

1 .271-0125.66C-0157.444-0C71.1se-01e5.4CS-OC51.048-OC42.9C4-OCd1.693-OC41 .619-OCe3.3C6-OC41.158-0053.96C-0049.927-0041 .714-0091.022-OC31.329-OC01.91C-OO01.359-0C42.813-OC42.1e8-0072.125-OC31.696-OC58.243-OC42.96 2-0041 .241-01C1.144-OC34.687-OC91.094-OC31 .112-OC31 .0C3-OC3l.OCS-OC32.332-OC56.934-OC47. 575-0093.199-0131.59S-0151.179-OC36.OC7-O046.165-OC41 .472-OC96.366-009.5 4G-006

1.781-OC43.362-0041.531-0042.474-OC61.653-OC42.288-OC41.425-0131.062-0051.037-0061.1S7-OC4

1.271-C129.660-C 157.467-G071.151-C205.409-0051 .C48-0042.9 04-C061.693-C041.6 20-0083.306-0041.158-0053.960-0049.927-C041.714-C091.C22-C031.329-0039.749-C071.409-C042.813-0042.190-0072.1 25-C031 .696-CO57.871-C043.334-C041.204-0101.144-0034.6 87-0091 .C94-C031.112-0031.003-0031 .CO9-C032.332-COS6.9 34-0041. 276-0095.387-0142.693-0161.179-C036.C07-0046.165-0041.144-0096.487-C093.266-C061.803-0043.362-0041.5 31-0042.474-0061.653-0042.288-0041.371-0131.046-0051.199-0061.197-004

1.271-0129.660-0157.471-OC?1.161-0225.409-OC51.048-OC42.904-0061 .693-OC41.622-0083.30o-OC41 .158-OC53.960-0049.927-0041.714-OC91.022-OC31 .329-OC34.977-0071.413-OC42.813-0042.192-0072.125-0031 .696-0057. 515-0043.690-OC41.15C-0101.144-0034.687-OC91.094-O31.112-0031.003-0031 .009-OC32.332-OC56.934-0042.1 49-0109. 074-0154.536-0171.179-0036.007-0046.165-0048.893-0106.582-0091 .925-OC61.817-0043.362-0041.531-0042.474-0061.653-0042.288-0041.319-0131.030-0051.359-0061.197-004

E. 76



EU1526D152

1.752-008 1.592-008 1.429-COS 1.290-OCt131 8-008 1.365-006 1.408-008 1.447-OCS

EU153 1.C08-004 1.0C8-004GD153 =3.434-013 4.239-014SM1S4 3.d61-005 3.661-005EU154 1.634-005-1.391-O05GD154 2.263-005 2.5C6-005EU155 3.282-006 2.482-0066D155 1.C07-005 1.087-OCSGD156 6.189-005 6.189-OC5GD157 9.590-008 9.9sC-OCe6D158 1.860-OO5 1.86C-OC5TE159 2.473-006 2.673-OC66D160 1.305-006 1.3C5-0C6DY160 2.191-007 2.891-OC?DY161 4.291-007 4.291-OC7DY162 .3.E23-007 3.823-007DY163 3.C35-007 3.035-OC7DY164 4-.458-008 4.458-OCEH0165 1.509-007 1.5C9-OC7H0166P 1.545-009 1.543-009ER166 4.852-008 4.852-008ER167 3.160-009 3.16C-OC9ER168 8.17-009 £.617-OC9TM169 6.C48-011 6.048-011ER170 2.E40-014 2.84C-014Y107- 1.907-011 1.9C7-011TM171 2.376-014 1.154-014Y8171 1.379-012 1.391-012Y8172, 4.C71-014 4.071-014SUMTOT 3.C86-002 3.086-002

TOTAL 3.C86-002 3.086-002

1.008-0045.231-0153.661-C051.184-C052.71 3-COS1.877-0061.148-C056.1 89-CO59.S90-0081.6 60-CO52.673-C061 .305-0062.891-C074.291-CC73.6823-0073.C35-CC74.4 58-C081.509-0071. 541-0094.852-0083.160-0098.617-0096.048-0112.840-C141.907-0115.606-01 51.397-0124.C71-C143.086-002

3.C86-002

1.008-0046.456-0163.661-OC5I .008-0152.890-0051.419-0C61.194-0056.189-0059.990-0081 .860-0C52.673-OC61 .305-0C62.891-0074. 291-0073.823-0073.035-OC?4.458-OC81.509-0071.540-0094.852-OCS3.160-OC98.617-0096.048-0112.840-0141.907-0112.723-0151.400-0124.071-0143.086-002

3.086-OC2

. . .~~~~~~~~~~~~~~~~

I .

E. 77



HLIBEC

ZNGAGEASSEaRKRRBSRT

ZRN3M0TCRURHPDAGCDINSNS3TE

IXECSBALACEPRNDPpSMEUGDTBDYHOERTMY3SUMTOT

3.C58-008 2.733-OC81.671-010 1.671-01C1.355-010 1.355-01C2.381-011 2.38C-0113.206-014 3.2C6-0148.432-013 8.432-0136.C43-007 6.043-OC71.e57-007 1.857-OC?4.S99-005 4.99-OCS1.S28-005 1.928-OC53.100-004 3.087-OC43.C37-004 3.05C-OC46.17-004 6.45C-OC43.509-004 3.9C9-0043.181-003 3.197-OC34.C41-009 4.613-OCS3.C1O-003 3.01C-OC'6.590-004 f.99C-0C42.C38-003 2.038-OC34.422-004 4.422-OC41.384-003 1.384-OC37.505-005 7.9C5-OCS1.116-004 1.116-OC42.477-006 2.492-OC68.880-005 e.8WC-OC51.528-005 1.883-OC54.547-004 4.552-0042.234-004 2.234-OC44.f58-003 4.858-OC32.171-C03 2.13C-OC31.557-003 1.598-0031.C94-003 1.094-OC32.121-003'2.121-OC31.C03-003 1.0C3-OC33.t14-003 3.614-OC39.399-006 5.541-OCd7.256-004 7.2S3-OC41.213-004 1.183-0041.146-004 1.179-004.2.673-006 2.673-OC61.449-006 1.449-0061.524-007 1.524-OC76.C29-008 6.029-0086.C50-011 6.049-0112.C49-011 2.051-0113.C86-002 3.0E6-002

2.44-3-0081.671-0101. 3 55-0102.380-G113.206-Cl48.432-C136. 0 43-C 071.857-C074.999-C051.9 28-0053.075-0043.C61-C46.289-C043.909-C043.213-C035.185-C093.C10-0036.990-0042.C38-C034.4 22-0041.384-C037.S05-G051.115-0042.505-0068.679-C051.855-C054.554-0042.234-0044.858-0032.C92-0031.636-0031 .C94-Co32.121-0031.003-0033.614-C033.267-CO67. 314-0041.157-0041 .205-0042.673-0061.449-C061.524-0076.C30-C086.048-Cl I2.C51-0113.086-C02

2.183-OC81.671-0101.355-0102.379-0113.206-0148.432-0136.043-0071.857-0074.999-OC51.928-0053.065-0043.072-OC46.137-OC43.9C9-0043.229-0035.757-0093.010-OC36.990-0042.038-OC34.422-OC41.384-O037.905-OC51.115-0C42.518-0C68.879-OC51.839-0054.556-OC42. 234-0044.858-0032.056-OC31.672-0031.094-0032.121-0031.003-0033.614-0031.926-0067.326-0041.137-0041.227-OC42.673-0061.449-0061.524-0076.030-0086.048-0112.051-0113.086-002

TOTAL 3.C86-002 3.086-OC2 3.C86-002 3.086-002

E. 78

TABLE E.5.g. Fission Products (Isotopic), C/gU, at 30 MWd/kgM

I IC YEARS 12 YEARS 14 YEARS 16 YEARS

1 3BE 10C 14

SE 79KR 81-KR 85RS 87SR 90Y 90

ZR 93NE 93MNE 94TC 98TC 99RH102RU106RH106PD107AG1OAG108PA6109PCD109AGIIOAGICPCD113PSNI119PSN121SN123TE123FS8125TEl25FSN1126S8126s81261TE127TEI 27F1129

CS134CS135CS137BA137MCE142CE144PR144PR144MND144PH146SM146PM147SM147EUISOSMI 51

:-

2.S52-004 2.638-OC4 2.358-004;2.108-0042. 35-012 2.635-012 2.635-012 2.635-012*1.C62-C10 1.061-01C 1.C61-C10 1.061-010-3.486:007 3.686-007 3.686-C07 3.685-0074.E10-013 4.81C-013 4.810-013 4.810-0134.267-003 3.745-OC3 3.295-C03 2.895-OC31.34-011 1.834-011 1.834-011 1.834-0114.S28-002 4.699-OC2 4.481-C02 4.273-OC24.S30-002 4.7C1-OC2 4.482-002 4.274-OC21.587-006 1.587-OCt 1.587-C06 1.587-OC66.444-007 7.461-0C0 8.199-007 8.866-0071.435-010 1.435-01C 1.435-010 1.435-0105.C07-012 5.0C7-012 5.C07-C12 5.007-0121.185-COS 1.185-OC5 1.185-005 1.185-OC51.C77-007 6.678-00e 4.140-008 2.567-OC85.E63-004 1.482-004 3.746-CC5 9.468-0065.863-004 1.482-OC4 3.746-COS 9.468-OC61.161-C07 1.161-OC7 1.161-C07 1.161-OC?2.5o5-012 2.537-012 2.509-C12 2.482-0122.881-011 2.85C-011 2.819-C11 2.789-0115.510-012 1.85C-012 6.213-013 2.086-0135.510-012 1.85C-012 6.213-C13 2.086-0132.353-009 3.1C2-OIC 4.C90-C1I 5.391-0121.770-007 2.333-OCE 3.C75-C09 4.053-0103.560-005 3.237-005 2.S44-C05 2.677-O57.474-009 9.717-01C 1.230-C10 1.558-0111.768-007 1.72C-007 1.673-007 1.627-OC71.C95-011 2.172-013 4.309-015 8.546-0179.'90-015 1.366-016 1.930-018 6.108-0201.191-003 7.221-OC4 4.378-C04 2.654-0042.906-004 1.762-OC4 1.C68-004 6.477-OC57.590-007 7.59C-007 7.590-007 7.590-0071.C63-007 1.063-007 1.G63-007 1.063-0077.590-007 7.59C-OC7 7.590-007 7.59C-OC71.153-012 l.lC8-014 1.064-016 1.073-0181.177-012 1.131-014 1.086-016 1.096-0182.990-008 2.99C-OCE 2.990-008 2.990-0084.142-003 2.472-OC3 1.262-003 6.442-0043.240-007 3.24C-OG7 3.240-CO7 3.240-0077.512-002 7.173-002 6.849-002 6.540-0027.107-002 6.766-002 6.479-002 6.187-0022.422-011 2.422-011 2.422-011 2.422-0111.435-004 2.418-OC5 4.072-006 6.858-0071.435-004 2.418-005 4.072-006 6.858-0071.723-006 2.9C1-007 4.886-008 8.229-0091.'95-015 1.395-015 1.395-Ci5 1.395-0158.437-007 6.557-007 5.096-007 3.961-0072.173-013 2.228-013 2.270-013 2.303-0138.715-003 5.138-003 3.029-C03 1.786-0033.560-012 4.048-012 4.100-012 4.130-0129.608-012 9.438-012 9.081-012 8.738-0122.139-004 2.796-004 2.753-004 2.711-004

E.79

TABLE E.5.g. (Contd)


EU152 3.C31-006 2.737-006 2.472-C06 2.232-0066D153 l.212-009 1.495-O1C 1.845-011 2.278-012EU154 4.413-003 3.756-OC3 3.197-C03 2.721-003EU155 1.527-003 1.155-OC3 8.732-004 6.602-OC410166P 2.774-009 2.771-OCS 2.767-C09 2.764-009TP171 2.588-011 1.257-011 6.107-012 2.966-012SUNTC 2.721-001 2.517-OC1 2.353-COl 2.223-OCI

TOTAL 2.721-001 2.517-OCI 2.358-C01 2.223-001

E.80

1-S



HECSEKRRESR

YZRNBTCRURHPDAGCDSNSeTEI

CSBACEPRNDP14S MEUGDHOT OTSUNTOT

2.5S2-0042.35-0121.C62-0103.f86-0074.267-0031.834-0114. 28-0024.S 30-0021.587-0066.f45-0071. 185-0055.863-C045.864tO041.161-0071.793-0073.560-0059.436-0071.192-0032.906-0042.990-0087.S96-0027.107-0021.435-0041.453-0041.395-0158.716-0032.839-0045.543-0031.212-0092.774-0092.588-0112.721-001

2.638-OC4 2.358-C04 2.108-OC42.635-012 2.635-Cl2 2.635-0121.061-01C 1.G61-010 1.061-0103.666-OC7 3.486-C07 3.685-OC73.749-OC3 3.295-003 2.895-0031.834-011 1.834-C11 1.834-0114.699-002 4.481-02 4.273-OC24.7C1-OC2 4.482-C02 4.274-OC21 587-OC7.462-OC71.185-OC51.4E2-OC41 .43-OC41.161-OC72.367-OCE3.237-OC59.32C-OC77.23C-OC41.762-0042.99C-OCe7.42C-0C26. 78 6-0022.41E-0052.447-OCS1.395-0155.138-0032.796-O44.913-OC31 .495-01C2.771-OCS1.257-0112.517-OC1

1.587-C06 1.587-0068.201-C07 8.867-OC71.185-CO5 1.185-OCS3.746-CO5 9.468-OC63.750-C05 9.493-0061.161-007 1.161-0073.147-C09 4.413-0102.544-005 2.677-OC59.264-CC7 9.218-OC74.386-004 2.663-0041.068-004 6.477-OC52.990-008 2.99C-OCE6.975-C02 6.604-0026.479-002 6.187-OC24.072-006 6.858-0074.121-006 6.940-0071.395-C15 1.395-0153.029-003 1.786-OC32.753-004 2.711-OC44.C72-003 3.3e3-oC31.845-C11 2.278-0122.767-009 2.764-0096.107-012 2.966-0122.358-C01 2.223-OC1

TOTAL 2.7 21-001 2.517-001 2.358-001 2.223-001

E.81

TABLE E.5.i. Neutrun Source (Alpha-n), neutrons/sec-gU,,at 30 MWd/kgM


PU238PU239PU24CAM241AM4243C1242CM243C4244

2.C1100D2.286-0013.5 78-0011 . 85+0001.e45-0027.5 32-0032.C54-0021.774+000

1.98C+OCC 1.949+COO 1.918+0002.216-OC1 2.286-001 2.286-OCI3.98C-001 3.981-CO 3.982-0011.915+OCC 2.1234C00 2.311+0001.645-002 1.645-C02 1.645-0027.466-OC3 7.399-003 7.331-OC31.956-OC2 1.863-002 .1.775-OC21.644+0CC 1.523+C00 1.410+000

TABLE E.5.j. Neutron Sourceat 30 MWd/kgM

(Spontaneous fission), neutrons/sec-gU,


PU238PU240PU242CM244CM246

3. 2 79-0012.C97?*008.341-C012.136.0021 .123+000

3.228-OCI 3.178-C01 3.128-OCI2.092+0CC 2.C99+000 2.099+OCOE.341-OC1 8.341-C01 .341-OCI1.979+0C2 1833+C02 1.698+0C21.123+000 1.123+COO 1.122+000

�.d

IJ

E.82

TABLE E.6. Radionuclide Inventories at 35 MWd/kgM as a Function of Decay Time

Subtable Species - Units

E.6.a Actinides (Isotopic), g/gU E.85

E.6.b Actinides (Elemental), g/gU E.86

E.6.c Actinides (Isotopic), C/gU E.87

E.6.d Actinides (Elemental), Ci/gU E.89

E.6.e Fission Products (Isotopic), g/gU E.90

E.6.f Fission Products (Elemental), g/gU E.94

E.6.g Fission Products (Isotopic), Ci/gU E.95

E.6.h Fission Products (Elemental), Ci/gU E.97

E.6.i Neutron Source (Alpha-n), neutrons/sec-g/U E.98

E.6.j Neutron Source (Spontaneous fission), neutrons/sec-gU E.98

E. 83


10 YEARS 12 YEARS 14 YEARS 16 YARS

HE 4P8208PE212E1212RA224RA226AC227TH228TH229TH230TH231TM232TH234PA231PA233U232U233U234U235U236U237U238NP235NP236NP237NP238NP239PU236PU238PU239PU240PU241PU242PU244AM241AM242PAM242AM243CM242CM243CR244CM245CM246CR247CM248CF249CF250CF251CF252SF250SUMTOT

1.358-006 1.496-OCt 1.634-0066.!98-011 &.956-011 1.143-0102.C27-014 2.164-014 2.235-C141.923-015 2.053-015 2.120-C1S1.768-013 1.88E-013 1.950-0137.536-015 1.293-014 1.967-C146.248-015 8.254-015 1.C49-0143.437-0113.659-011 3.780-Cll

-Z .702-013 2.863-013 3.'C51-C132.382-010 3.298-OIC 4.358-C101.E64-014 1.864-014 1.864-C141.126-009 1.319-OC9 1.513-C091.373-011 1'.373-011 1.373-Cil5.485-011 6.374-011 7.263-C111.575-011 1.581-011 1.589-0111.468-009 1.489-OC9 1.490-C091.721-009 2.032-OCS 2.345-C091.513-005 1.773-OCS 2.C29-C054.584-003 4.5E4-OC3 4.585-0033.327-003 3.328-003 3.328-0032.747-011 2.495-011 2.266-0119.454-001 9.454-001 9.454-0018.553-015 2.382-015 6.633-0164.549-010 4.549-01C 4.549-0104.637-004 4.656-OC4 4.678-0041.374-013 1.361-013 1.349-0131.337-010 1.337-01C 1.336-0101.298-010 7.983-011 4.909-0111.688-004 1.661-OC4 1.635-G045.118-003 5.118-003 5.118-0032.555-003 2.557-003 2.559-0038.E72-004 8.05E-OC4 7.318-CO46.d90-004 i.69C-OC4 6.690-0045.380-008 5.38C-008 5.380-0085.772-004 6.546-OC4 7.284-0047.326'007 7.26C-OC7 7.194-0078.764-012 8.68,4-012 8.605-0121.556-004 1.555-OC4 1.555-0041.775-009 1.759-009 1.743-0094.502-007 4.289-OC7 4.C85-0073.782-005 3.5C3-005 3.245-0052.252-006 2.252-C 2.252-0063.468-007 3.467-007 3.466-0073.845-009 3.845-009 3.845-0092.380-010 2.38C-01C 2.380-0102.759-012 2.749-012 2.738-0123.386-013 3.045-013 .2.739-0132.333-013 2.33C-013 2.326-0131.206-014 7.128-015 4.214-C152.879-011 3.27C-011 3.634-0119.f40-001 9.64C-001 9.640-001

1.772-OC61 .395-01C2.265-0142.149-0151.976-0132.840-0141.295-0143. 830-0113.267-0135.559-0101.864-0141 .707-0C91.373-0118.152-0111.597-0111.480-0092.660-0092.281-OCS4.585-0033. 329-0032.058-0119.454-0011.847-0164.549-0104.702-OC41.337-0131.336-0103.019-0111.610-0045.118-0032.561-0036.646-0046.690-0045.380-0087.931-0047.128-0078.527-0121.555-OC41.727-0093.891-0073.006-0052.251-OC63.465-0073.845-0092.380-0102.728-0122.463-0132.322-0132.492-0153.971-0119.640-001

TOTAL 9. 40-001 S.64C-OG1

E. 85

9.640-001 9.640-001



HESFPa3IRAACTNPA

UNPPU

CMCFSUMTOT

1.358-0062.879-0116.f00-0 12.190-0151.848-0136.249-0151.412-0097.C59-0119.534-C014.37-0049. 398-0037.335-0044.C88-CG53. 3 43-0129.d4G-C01

1.4;f-OCU3.27C-0118.958-0112.368-0152.017-0138.255-0151 .7CC-OC97.9S5-0119.534-OC14.656-OC4S.316-OC!e.129-OC43.8C7-0C53.294-0129 .64C-OC1

1.634-C06 1.772-0063.634-C11 3.971-0111.143-C1O 1.395-0102.486-C15 2.569-0152.147-C13 2.26C-0131.C49-C14 1.295-0142.COO-CQ9 2.315-0098.852-C1 9.749-0119.534-CO 9.534-OC14.678-C04 4.702-OC49.241-003 9.173-OC38.846-C04 9.493-0043.546-C05 3.305-0053.249-012 3.209-0129.640-C01 9.640-001

TOTAL 9.d40-001 .64C-OC1 9.640-C01 9.640-OC1

E.86



TL207TL208-TL209PB209PE210P8211P9212P8214BI210BI211'BI212E12138I214P0210PC211P0212P0213P0214P0215-P0216P0218AT217RN219RN22CRN222FR221.FR223RA223RA224RA225RA226AC225AC227TH227TH228TH229TH230TH231TH232TH234PA231PA233PA234PPA234V232U233U234U235U236U237U238U240

4.510-013 5.96t-0131.C13-008 1.081-0081.242-015 1.316-0155.749-014 6.093-0141.637-015 2.153-0154.522-013 5.982-0132.818-008 3.0C8-00E7.£48-015 1.279-0141.638-015 2.154-0154.522-013 5.982-0132.f18-008 3.0Ce-0085.749-014 6.093-0147.E48-015 1.279-0141.638-015-1.981-0151.266-O15 1.675-0151.E06-008'1.927-OCE5.25-014 5.961-0147.E47-015 1.27&-0144.522-013 5.982-0132.f18-008 3.OC-OCE7.E50-015 1.279-0145.749-014 6.093-0144.522-013 5.982-0132.818-008 3.0C8-OCE-7.f5O-015 1.279-0145.749-014-6.093-0146.240-015 £.242-0154.522-013 5.982-0132.E18-008 3.OC8-0085.749-014 6.093-014

7.585-C13I .1 16-0081.403-0156.494-C 142.985-C157.606-0133.107-0081.945-C142.987-CI57. 606-0133.1 07-CO6.494-0141.945-Cl42.712-C152.130-0151 .991-C086.353-C141.944-C147.606-C133.107-COB1.945-014-6.494-0147.606-0 133.107-C081.945-C146.494-0141 .C48-C147.606-C133.107-0086.494-C14

9.363-0131.131-OC81.502-0156.95 2-0144.228-0159.390-0133.149-0082.808-0144.229-0159.390-0133.149-0086.952-0142. 808-0143.827-0152.629-0152.017-OC86.801-0142.808-0149.390-0133.149-OE2.809-0146. 952-0149.390-0133.149-0082.809-0146.952-0141.293-0149.390-0133.1'49-0086.952-0142.809-0146.952-0149.373-0139.26C-0133.141-0086.952-0141.123-0119.915-0091.872-0163.180-0073.852-0123.316-O73.180-0074.134-0103.169-0082.576-0111.426-OC79.915-0C92.154-0071.680-0063.180-0079.533-013

7.E50-0155. 749-0144. 521-0134.460-0132.818-0085. 7 49-0144.810-0129.913-0091.2 35-0163.180-0072.5 92-0123.270-0073.180-0074 .134-0103.143-0081.666-0119.45'9-0089.S13-0092.153-0072.243-0063.180-0079.533-013

1.279-014 1.945-C146.093-014 6.494-0145.972-013 7.593-0135.9CC-01 7.501-C133.OCl-OC8 3.C99-0086.093-014 6.494-0144.66C-012 8.800-0129.913-OC9 9.914-0091.447-01f 1.660-0163.18C-007 3.180-0073.012-012 3.432-0123.284-007 3.299-C073.180-OC? 3.180-0074.134-01C 4.134-0103.187-OOE 3.191-0081.968-011 2.271-0111.1C9-OC7 1.269-CC79.913-OC9 9.914-0092.154-007 2.154-0072.037-006 1.850-0063.1EC-OC7 3.180-C079.533-013 9.533-013

E.87


1C YEARS 12 YEARS 14 YEARS 16 YEARS .

NP235NP236NP237NP238NP239NP24CPPU236PU238PU239PU24CPU241PU242PU243PU244AF241AI0242AM242AP243CM242CM243CP244CM245Cr246Cr4247CM248BK249CF249CF250CF251CF252SUMTOT

1.200-011 3.343-0125.S95-012 5.995-012'3.270-CO? 3.2f4-OC?3.562-008 3.529-OCE3.102-005 3.1C2-0C59.533-013 9.533-0136.901-008 4.244-OCE2.891-003 2.845-OC33.183-004 3.183-OC45.824-0049.144-0022.55!-0063.569-0139.'45-0131.S82-0037.123-0067.C87-0063.102-0055.872-0062.325-0053.C61-0033.E69-0071.C66-0073.569-0131 .C12-C121.509-0121.131-0113. 7 03-0113.702-0136.486-0121 C04-001

5.829-004I.3C5-OC22.555-OCe3.569-0139.545-0132.255-OC}7.058-OCt7.023-0C43.1C2-0055 .819-0062.215-OC52.836-0033.868-OC?1.O6-OC73.56 9-0131.012-0123.1C2-0131.127-0113.33C-0113.696-0133.835-0129.199-OC2

9.309-C135.995-C123.299-C073.497-C083.101-C059.533-C132.610-C082.201-C033.183-CO45.834-C047.542-C022.555-C063.569-C139.545-C132.501-0036.994-0066.959-CC63.101-COS5.766-0062.110-0052.627-C033.868-C071.C65-C073.569-C131.012-Cl26.3 75-0141.122-C112.995-C1I3.690-Cl32.267-G128. 436-002

2. 592-0135.995-0123.316-OC73.465-0083.101-OC59. 533-0131 .605-OCS2.757-OC33.182-00.45.838-OC46.850-OC2Z.555-OC63. 569-0139.545-0132.723-OC36.931-OC66.896-OC63.101-OC55.713-OC62.009-0C52.433-0C33.867-OC71.065-OC73.569-0131.012-0121.310-0141.118-0112.694-0113.685-0131.341-0127.742-OC2

"Sd

'-S

TOTAL 1.C04-001 9.199-OC2 8.436-002 7.742-O2

E.88

TABLE E.6.d. Actinides (Elemental), C/gU, at 35 MWd/kgM


TLPB9'PoATRNF RRAACTNPA

UNPPUAMCMBKCFSUMTOT

TOTAL

1.C13-008 1.081-O0E2.818-008 3.0CE-00t2.E18-COB 3.0C8-OCE4.f24-008 4.935-OCE5.749-014 6.093-0142.818-008 3.0CE-OCE6.373-014 6.917-0142.18-008 3.0CE-OCE5.C97-013 6.5e2-0133.561-007 3.575-OC76.454-007 f.46E-OC72.S12-006 2.723-OC63.139-005 3.13e-OC59.523-002 E.679-OC22.C27-003 2.3CC-OC33.C91-003 2.864-0031.509-012 3.1C2-0135.519-011 4.877-0111.C04-001 9.199-OC2

.C04-001 S.19-OC2

1..116-0083.1 07-0083.107-008S.C97-0086.494-0143.107-COB7.541-0143.107-C088.243-Ct33.589-CC76.483-C072.5 52-0063.1 38-0057.913-CO22.546-G032.654-C036.375-0144.381-Ci18.436-002

1.131-0083.149-OC83.149-OCE5.166-0086.952-0143.149-OC88.245-0143.149-0081.007-0123.593-OC76.500-OC72.398-0063.137-0057.216-OC22.768-OC32.459-OC31 .31C-0143.983-0117.742-002

8.436-002 7.742-OC2

E. 89



HLIL IBEBE-C

ZNZNGAGEGEGEASGESESESESEBRSEKRaRKRSEKRKRKRRR3K RS RRBSRSRY

SRY

ZRZRZRZRN9N3ZRN3MOZRMOMO

TCTC

3679

10146667717273747576767778797.9808081818282838485858686878788899090909192939393,949495969697989899

3.f26-0081.587-0101.C69-0112.C56-0111.373-0102.773-0113.416-0141.396-0151 .CO1-0122.549-0085.CO4-C081.C66-0072.147-0075.163-0076.S49-0091.C38-0062.552-0066.C91-0067.442-0101.371-0052.724-0102.191-0053.C92-0113.378-0051.188-0063.E60-0051.143-0041.228-0051.C62-0041.840-0044.832-0072.'54-0044.277-0093.372-0044.380-0044.C50-0041.C16-0071.280-0045.740-0046.314-0047.181-0041.C56-0092.74-0097.519-0049.359-0107.f82-0048.233-0044.150-0058.257-0048.497-0047.961-0097.970-004

3.241-0081 .587-OIC1.069-0112 .056-0111 .373-01C2. 77 2-0113.416-0141 .394-0151.OC1-0122.549-OCE5 .0C4-0081.066-OC72.147-OC75.163-OC76 .949-OC91 .038-OCe2.552-OC66.09 1-0Ce8.742-O1C1.371-OC52.724-01C2.191-0053.092-0113.378-OC51 .188-0Cf3.86C-OC51.14 3-0041.079-OCS1 .077-OC41.84C-OC44.832-OC72.354-OC44. 277-0093.372-OC44.38C-OC43.862-0049.6e4-0081.468-0045.74C-OC46.314-OC47.181-OC41 .378-0093.OC3-0097.519-0049.358-01C7.682-OC48.233-OC44.15C-0058.257-OC48.697-OC47.961-0097.97C-OC4

2.897-0081.587-0101.C69-C112.C56-C111.373-C102.771-0113.416-C141.396-015.C01-C12

2.549-C085.C04-008I .66-0072.147-0075.163-0076.9 49-0091 .C38-CO62.552-C066.C91-C061.C04-G091.371-0052.724-C102.191-CO53.C92-C 113.378-CO51.188-0063.860-CO51.143-0049.484-C061.C90-C041 .840-0044.832-0072.354-C044.277-C093.372-C044.380-CO43.682-C049.233-0081.648-C045.7 40-0046.314-0047.181-0041.732-0093.300-C097.519-C049.3 57-0107.682-C048.2 33-0044.1 50-0058.2 57-0048.697-0047.961-0097.970-004

2.589-0081.587-0101.069-0112.056-0111.373-0102.771-0113.416-0141.396-0151.001-0122.549-008S.004-OC1 .066-OC?2.147-0075.163-OC?6.949-OC91.038-0062. 552-0066.091-0061.134-OC91 .371-OC52.724-0102.191-0053.092-0113.378-OC51.1 8s-oC63.860-OC51.143-0048.334-OC61.102-0041 .84C-0044.832-0072.354-0044.277-OC93. 372-0044.380-0043.511-0048.804-0081.819-OC45.740-0046.314-0047.181-0042.114-OC93.568-OC97.519-0049.357-0107.682-0048.233-0044.150-0058.257-0048.697-0047.961-0097.970-004

'-40

E. 90



RU 99M010RU 100RUIOlRU102RH102RHI03RU104PD104PD105RU106RH106PD106PDIO7AG107PD108AGIOS8CD108AG109CD109PDioAGIIOFCDIIOCD111CD112C0113CD113PIN113CDI14SN114IN115SN115C0116SN116S N117SNI ISNI19SN119VSh120SN121PS8121SN122TE122SN123S6123TE123SN124TE124Se125TE125-TE125PSN126

2.529-008 3.446-OCe 3.967-C08 4.4e6-OC89.f68-004 9.8d8-OC4 9868-C04 9.868-0041.201-004 1.2Cl-004 1.201-004 1.201-0048.238-004 8.23E-OC4 8.238-C04 8.238-0C48.512-004 8.512-OC4 8.512-004 8.512-OC41.216-010 7.536-011 4.673-C1i 2.897-0114.S44-004 4.944-004 4.944-C04 4.944-0046.426-004 6.426-004 6.426-C04 6.426-0042.E54-004 2.854-004 2.854-004 2.854-OC44.525-004 4.525-004 4.525-004 4.525-OC42.198-007 5.555-008 1.404-008 3.549-0092.C66-013 5.221-014 1.320-C14 3.336-0154.i95-004 4.697-OC4 4.697-C04 4.698-0042.E41-004 2.41-OC4 2.841-004 2.841-0043.328-010 3.934-01C 4.540-C10 5.146-0101.d74-004 1.974-OC4 1.974-C04 1.974-0C4,1.403-012 1.388-012 1.373-012 1.358-0126.221-010 6.221-01C 6.221-010 6.221-0109.588-005 5.5ef-005 9.588-CO5 9.588-OCS3.t42-015 1.223-015 4.107-C16 1.379-0166.474-005 6.474-005 6.474-005 6.474-0055.432-011 7.161-012 9.439-013 1.244-0135.263-005'5.263-005 5.263-005 5.263-0053.573-005 3.573-05 3.573-005 3.573-0052.103-005 2.1C3-005 2.103-CO5 2.103-0051.571-007 1.571-OC7 1.571-CO7 1.571-OC72.103-007 1.913-OC7 1.739-007' 1.582-OC71.430-007 1.62C-OC7 1.793-007 1.951-0072.727-005 2.727-OC5 2.727-005 2.727-OC51.753-009 1.753-009 1.753-009 1.753-OC9-2.437-006 2.437-OCt 2.437-006 2.437-0063.780-007 3.78C-OC7 3.780-CO7 3.780-OC79.663-006 9.661-OC6 9.663-C06 9.663-OC69.156-006 9.156-OC6 9.156-006 9.156-0069.754-006 9.754-006 9.754-006 9.754-0069.123-006 9.823-O00 9.823-G06 9.823-OC69.901-006 9.8C1-006 9.801,-C06 9.801-0062.128-012 2.695-013 3.412-C14 4.321-0159.s76-006 5.97f-0Cf 9.976-C06 9.976-0C63.-f28-OO9 3.529-OC9 3.432-009 3.339-0099.569-006 9.569-OCt 9.570-006 9.570-0061.C94-005 1.094-005 1.C94-005 1.094-0057.700-007 7.7CC-OC? 7.700-C07 7.700-0071.591-015 3.157-017 6.263-019 1.242-0201.181-005 1.1e1-oo5 1.181-005 1.181-0051.196-008 1.196-006 1.196-008 1.196-0081.465-005 1.465-005 1.465-005 1.465-005S.842-007'5.842-007 5.842-007 5.842-0071.383-006 8.383-007 5.082-007 3.081-0072.C95-00,5 2.1SC-005 2.183-005 2.204-0051.S34-008 1.173-00e 7.110-009 4.310-0093.198-005 3.19E-OC5 3.197-005 3e197-005

E.91



S8 26

T91 26TE127PI127

TE128XE128

I129XE 129TEI 3CXE130XE131XE1323Al 32CS133XE134CS1343A134CS135BA1 35XE136BA1 36CS1373A1378A137P3A 381A1 38LA139CE140PRI41CE142ND 42ND1 43CEl44PR144PR144PND144ND 45ND146PM146

PM 47SM147N0148SM1148S14149ND 150SM150EUlsoS14151EU151SM152

1.519-0121.155-0149.383-0071.'03-0166.4 35-0051.245-C044.154-0061.S87-0042. 3 5-0083.S06-0041. 31-0054.358-0041.196-0032.359-0091.158-0031.548-0034.; 89-0061.844-0042.591-0043.530-0072.g25-0032.121-0051.C08-0033.C03-0041.542-0101.326-0034.840-0091.265-0031.297-0031.157-0031.167-0033.234-0057.488-0045.154-0082.176-0121.C88-0141.410-0036.781-0047.306-0042.410-0097.889-0099.581-0061.772-0043.S24-0041.E60-0042.709-0061.S60-0042.687-0041.588-0131.157-0059.335-007

1.519-0121.155-0149.388-0071 .444-01e6.435-OC51.245-O44.154-0061 .987-0042.736-OCE3.9Cf-OC41 .631-OC54. 35 -0041.196-OC32.359-OC91 .158-OC31.548-OC32.547-OCE1.868-0042.991-OC43.532-OC72.525-OC32.121-0059.622-OC43.458-0041 .472-01C1.326-OC34.84C-OC9I .265-OC31 .297-OC3I .157-OC31.167-OC33.234-0057..48-OC48.68C-OC93.665-0131.832-0151 .41C-OC36.781-OG47.306-0041 .873-OCS8.0a8-OC95.649-0061.811-0043.924-OC41.860-0042.709-0061.96C-OC42.687-OC41 .528-0131. 140-0051.11-O0

1.519-012 1.519-0121.155-014 1.155-0149.392-CO? 9.397-OC71.388-020 1.401-0226.435-C05 6.435-0051.245-C04 1.245-O044.154-006 4.154-OC61.987-004 1.987-0042.738-008 2.740-OC83.906-004 3.906-OC41.631-005 1.631-0054.358-004 4.358-0041.196-C03 1.196-OC32.359-009 2.359-OC91.158-003 1.158-0031.548-C03 1.548-OC31.300-C06 6.638-OC71.881-004 1.887-0042.991-C04 2.991-OC43.533-007 3.535-OC72.525-C03 2.525-o032.121-05 2.121-0059.188-004 8.773-OC43.892-C04 4.307-0041.406-010 1.342-0101.326-003 1.326-OC34.840-C09 4.840-OC91.265-003 1.265-OC31.297-003 1.297-0031.157-003 1.157-0031.167-003 1.167-0033.234-CO5 3.234-OC57.488-004 7.488-OC41.462-C09 2.462-0106.173-014 1.040-0143.C86-016 5.197-0171.410-C03 1.410-OC36.781-004 6.781-OC47.306-C04 7.306-0041.456-009 1.132-0098.242-C09 8.362-0093.330-006 1.963-0061.835-C04 1.848-0043.924-004 3.924-0041.860-004 1.860-0042.709-006 2.709-0061.960-004 1.960-0042.687-004 2.687-0041.470-013 1.415-0131.122-0OS 1.105-O0S1.285-006 1.456-0061.336-004 1.336-0041.336-004 1.336-004

E. 92



EU152 1.587-008 1.433-OCe 1.294-008 1.169-0C86D152 1.186-008 1.229-OCE 1.268-008 1.303-OC8EU153 1.209-004 1.2C9-OC4 1.209-C04 1.209-OC46D153 3.845-013 4.746-014 5.857-015 7.228-016SM154 4.514-005 4.514-005 4.514-005 4.514-005EU154 -2.135-005'1.817-005 1.547-005 1.317-OC56D154 2.S60-005 3.278-005 3.548-C05 3.779-OC5EU155 4.268-0063.227-006 2.440-006 1.845-OC66D155 1.308-005 1.412-OC5 1.491-005 1.550-OC560156 9.C44-005 5.044-OCS 9.044-005 9.044-0056D157 1.302-007 1.3C2-OC7 1.302-CO7 1.302-007G6158 2.551-005 2.551-005 2.551-005 2.551-005TB159 3.405-006 3.405-004 3.405-006 3.405-0C66D160 1.655-006 1.655-006 1.655-C06 1.655-006DY100 4.141-007 4.141-OC7 4.141-007 4.141-OC7DY161 5.330-007 5.330-007 5.330-007 5.330-007DY162 4. 826-0C7 4.826-007 4.826-OC7DY163 4.118-007 4.11e-OC7 4.118-C07 4.118-0070Y164 5.522-008 5.922-OE 5.922-COB 5.922-008H0165 2.190-007 2.19C-007 2.190-C07 2.190-007H0166t 2.607-009 2.6C4-OCS 2.601-009 2.598-OC9ER166 7.386-008 7.386-OC 7.387-008 7.387-008ER167 4.C39-009 4.039-009 4.C39-C09 4.039-009ER168 ,1.230-008 1.23C-OCE 1.230-C08 1.230-OCETM169 9.t45-011 9.645-011 9.645-011 9.645-011ER170 5.333-014 5.333-014 5.333-C14 5.333-014Y8170 3.568-011 3.568-011 3.568-011 3.568-011TMI71 5.368-014 2.6C7-014 1.267-C14 6.153-015Y8171 3.C89-012 3.117-012 3.130-012 3.137-012YE172 1.C89-013 1.0E9-013 1.C89-013 1.089-013SUMTOT 3.596-002 3.596-002 3.598-002 3.598-002

TOTAL 3.598-002 3.596-OC2 3.598-002 3.598-002

:

E.93

TABLE E.6.f. tT.sion Products (Elemental), g/gU, at 35 MWd/kgM

1C YEARS 12 EARS 14 YEARS 16 YEARS

NLIBE

CZNGAGEASSE3RKRRaSRY

ZRNS140 TCRURHPDAGCDINSNSaTE

IXECSaALACEPRNDPMSMEU6DT8DYNOERTMYBSUMTOT

3.c26-008i.e 94-0101.*5t79-0102.773-0113.559-0141.CO1-0126.985-0072.147-0075.718-0052.191-C053.5 03-0043.416-0047.426-0044.381-C043.27-0034.t66-0093.492-0037.s70-0042o438-0034.544-0041.754-0039.588-0051.467-00422.580-0061.C65-0042.276-0055.383-0042.e31-0045.725-0032.470-0031.832-0031.265-0032.465-0031.157-0034.188-0039.584-0068.249-0041.475-0041.404-0043.405-0061. S 91.-0062.216-0079.C20-0089.451-0113.888-0113.598-002

3.241-0081 .694-O1C1.579-01C2. 77 2-0113.559-0141 .OC1-0126 .5-OC?2.147-OC75.718-O52.191-OC3.488-OC43.431-OC47.238-OC44.38 1-OC43.646-OC35.317-OCS3.492-OC37.97C-OC42.438-0C34.944-OC41.754-OC39.588-OC51 .467-OC42.559-oe1 .065-OC42.222-OCS5.3e9-0042.631-OC45.725-0032.422-OCI1.8aC-OC31 .265-OC32.465-OC31.157-OC34 .188-OC35.65G-OC8.286-O41 .434-OC41.646-OC43. 4C5-0061 .9C1-OCt2.216-OC79.021-OCa9.64 8-0113.891-0113.598-002

2.e97-0081.694-C101.579-0102. 771-0113.559-C141.C01-Cl26.985-C072.147-0075.718-0052.191-C053.475-GQ43.444-C047.C58-0044.381-C043.664-C035.967-C093.492-C037.9 70-0042.4 38-0034.944-G041.754-C039.588-0051.467-C042.616-C06I.C65-0042.189-0055.392-C042.631-0045.725-0032.377-C031.925-C031.265-0032.465-C031.157-0034.188-0033.331-C068.308-C041.401-0041.681-0043.405-0061. 9 01-0062.216-0079.021-0089.647-C113.892-C113.5 98-002

2. 589-0081.694-0101,579-0102.771-0113. 5 59-0141.001-0126. 985-0072.147-OC75.718-0052.191-0C53.464-OC43.456-OC46.887-0044. 381-0043.681-0036.618-0093.492-OC37.970-oC42.438-OC34.944-OC41.754-OC39.588-OC51.466-OC42.632-OC61.065-OC42.169-0055.394-OC42.631-O'5.725-0032.335-0031.967-0031 .265-OC32. 465-0031.157-0034.188-OC31.964-0068.319-0041 .374-OC41.710-0043.405-0061.901-0062.216-OC79.021-0089.646-0113.893-0113.598-OC2

"S0

TOTAL 3.598-002 3.558-OC2 3.598-002 3.598-OC2

E. 94

TABLE E.6.g. Fission Products Isotopic), C/gU, at 35 MWd/kgM


h 3 3.501-004BE 10 3.C69-012CA 4 1.236-010

SE 79 4.245-007KR 81 6.505-013KR 85 4.621-003Re 87 2.C61-011SR 90 5.526-002Y 90 5.528-002

ZR 93 1.805-006NE 93P 7.562-007NE 94 1.754-010TC 98 6.520-012TC 99 1.352-005RH102 1.470-007RU1O6 7.356-004RH106 7.356-004PD107 1.462-007A6108 3.256-012AG108 3.f58-011AG109V 9.407-012CD109 9.407-012AGIO 3.434-009AG110 2.582-007CD113P 4.563-005SN119P 9.534-009SN121P 2.146-007SN123 1.308-011TE123P 1.597-014S8125 1.428-003TE125P 3.485-004SN126 9.C75-007S8126 1.271-007S8126P 9.C75-007TE127 1.389-012TE127P 1.418-012

I129 3.509-008CS134 6.458-003CS135 3.445-007CS137 8.770-002BA137M 8.296-002CE142 2.E02-011CE144 1.645-004PR144 1.645-004PRI44P 1.574-006ND144 1.668-015PM146 1.C73-006S?146 2.761-013PM147 8.E86-003SM147 4.G29-012EU150 1.C52-011SM151 3.C46-004

3.129-OC43.069-0121.236-01G4.245-0076 .5C50134.237-OC32.061-0115 .269-0025.271-OC21 .8C5-oC8.49 1-OC71.754-01C6.92C-0121.352-OC59.112-OCS1.859-OC41.85S-0041.462-0073.22C-0123.618-0113.159-0123 .159-0124.526-O1C3.4C3-OCe4.149-OCSI .2C7-0092.0e7-OC72.596-0132.323-0168.659-OC42.113-OC49.075-OC?1.271-0079.075-0071.335-0141.363-0143.5C9-OC83.297-0033.445-0078.374-OC27.921-0022.8G2-0112.77C-OG52.77G-OC53.324-OC71.668-0158.343-0072.83C-0135.238-0034.118-0121.012-0112.999-004

2.797-C04 2.500-OC43.069-012 3.069-0121.236-010 1.235-0104.245-007 4.245-OC76.505-013 6.505-013'3.723-003 3.271-0032.C61-011 2.061-0115.C24-002 4.791-OC25.C26-C02 4.792-0021.805-006 1.805-0069.330-C07 1.009-0061.754-010 1.754-0106.920-012 6.920-0121.352-005 1.352-0055.650-008 3.503-OCe4.700-005 1.188-OC54.700-005 1.188-OCS1.462-007 1.462-OC73.185-C12 3.151-0123.579-011 3.540-0111.C61-012 3.562-0131.C61-012 3.562-0135.966-011 7.865-0124.406-C09 5.913-01C3.773-CO5 3.431-0C51.529-010 1.936-0112.030-007 1.975-0075.150-015 1.021-0163.400-018 1.076-0195.249-004 3.182-0041.281-004 7.767-0059.C75-007 9.075-0071.271-007 1.271-0079.075-007 9.075-0071.283-016 1.294-0181.309-G16 1.322-0183.509-008 3.509-0081.683-003 8.593-0043.445-007 3.445-0077.995-002 7.634-OC27.564-002 7.222-OC22.802-011 2.802-0114.666-006 7.858-0074.666-C06 7.858-0075.599-008 9.430-0091.668-015 1.668-0156.484-007 5.040-0072.884-013 2.926-0133.088-003 1.821-0034.171-012 4.202-0129.739-012 9.371-0122.953-004 2.908-004

E. 95

TABLE E.6.g. Contd)


EU1S2 2.745-006 2.479-OCt 2.239-C06 2.022-OC6GD153 1.357-009 1.674-01C 2.066-CII 2.550-012EU154 5.766-003 4.9CE-OC3 4.177-C03 3.555-OC3EU155 1.586-003 1.5C1-OC3 1.135-C03 8.584-OC4H0166P 4.f81-009 4.676-OC9 4.671-C09 4.665-009TM171 5.847-011 2.840-011 1.380-C11 6.702-012 '

SUMTOT 3.134-001 2.857-OC1 2.713-C01 2.558-001

TCTAL 3.134-001 2.897-OCI 2.713-C01 2.558-001

.~~~~~~~~~~~~~~~~~~~~~~~'

E.96


IC YEARS 12 YEARS

HeE

C ' -

SEKRRESR

YZRNETCRURHPDAGCDSNseTE

I.CSBACEPRNDPMSMEUGDHOTMSUMTOT

3.501-0043.C69-0121.236-0104.45-0074.E 21-0032.C61-0115.S26-0025.S 28-0021 .105-0067.564-0071.352-0057.156-0047.358-0041.462-0072.616-0074.563-0054.132-0061.429-0033.485-C043.509-0089.415-0028.296-0021.645-0041.665-0041.668-0158.E87-0033.C46-0047.754-0031.357-0094.681-0095.147-0113.134-001

3.129-OC43.069-0121 .236-01C4.24 5-0074.237-OC32.061-0115 .269-OC5.271-OC21.8C5-00dE.453-O71.352-0051.859-OC41 .86C-OC41.462-OC73.45 3-OCE4.149-OC51 .117-08.67C-OC42.113-O43.5C9-0088.7C3-0027.921-O22.77C-0052.8C3-0051.668-0155.239-O32.999-OC46.412-0031.674-01C4.676-OCS2.84C-0112.897-001

14 YEARS 16 YEARS

2.797-C04 2.500-0043.C69-C12 3.069-0121.236-010 1.235-0104.245-CO 4.245-0073.723-003 3.271-0032.C61-C1 2.061-0115.C24-002 4.791-OC2S.C26-002 4.792-0021.805-C06 1.805-OC69.332-C07 1.009-OC61.352-CO5 1.352-OC54.700-005 1.188-0054.706-005 1.191-OC51.462-C07 1.462-0074.586-009 6.381-01C3.773-C05 3.431-0051.111-C06 1.105-OC65.260-004 3.193-OC41.281-C04 7.767-0053.509-008 3.509-OC88.164-002 7.72C-OC27.564-002 7.222-OC24.666-006 7.858-0074.722-006 7.952-0071.668-G15 1.668-0153.C89-C03 1.821-OC32.953-004 2.908-0045.315-003 4.416-0032.066-011 2.550-0124.t71-009 4.665-0091.380-C11 6.702-0122.713-001 2.558-001

TOTAL 3.134-001 2.8S7-OC1 2.713-001 2.558-001

E.97

TABLE E.6.i. Neutron Source (Alpha-n), neutrons/sec-gl, at 35 MWd/kgM

IC YEARS 12 YEARS 14 YEARS 16 YEARS 'SO

PU238PU239PU240AM241AM243CP243CM244

2.7504000 2.7C7+OCC 2.665+000 2.623+0CO2.318-001 2.318-OCI 2.318-301 2.318-OCI4.413-001 4.417-01 4.420-CC1 4.423-0011.a01o000 2.162+OCC 2.399+COO 2.612+OCO2.647-002 2.646-OC2 2.646-C02 2.645-0023.C6-002 2.949-OC2 2.809-C02 2.675-0023.4934000 3.236+00C 2.997+C00 2.776+000

TABLE E.6.j. Neutron Source (Spontaneous fission), neutrons/sec-gU,at 35 MWd/kgM


PU238PU24CPU242CM244CM246

4.485-001 4.415-OCI 4.346-CO1 4.278-0012.326+000 2.328+0CC 2.330+C00 2.332+0001.1284000 1128+0CC 1.128+C00 1.128+OCO4.206+002 3.896+002 3609+C02 3.343+0C23.C874000 3.086+0CC 3.C85+000 3.084+0C0

E. 98

APPENDIX F

RADIOISOTOPES DETERMINED DURING BURNUP ANALYSES

TABLE F.1. R

Isotope

UraniumUV g/g oxide234U, wt.%

235U, wt.%

236U, wt.%

238U, wt.%

adioisotopes Determined During Burnup Analyses

N-9C-D N-9C-J N-9B-D N-9B-N N-9B-S

0.8497

0.013

0.572

0.353

0.84300.014

0.733

0.335

99.063 98.919

PlutoniumPu, g/g oxide238pu, wt.%239Pu, wt.%240Pu, wt.%241Pu, wt.%242pu, wt.%

Neodymium

Nd, atoms x 1015g oxide

143Nd/148Nd

144Nd/ 148 Nd145Nd/148Nd

146Nd/148Nd

1SONd/148Nd

0.00767

1.700

54.760

27.625

9.019

6.897

0.00773

1.475

58.869

25.500

8.818

5.339

1.184

2.055

3.619

1.811

1.843

0.487

1.109

2.208

3.497

1.841

1.829

0.485

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