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Journal of Luminescence 132 (2012) 1420–1426
Contents lists available at SciVerse ScienceDirect
Journal of Luminescence
0022-23
doi:10.1
n Corr
E-m
journal homepage: www.elsevier.com/locate/jlumin
Density of states in a cylindrical GaAs/AlxGa1�xAs quantum well wire undertilted laser field
Adrian Radu, Ecaterina Cornelia Niculescu n
Department of Physics, ‘‘Politehnica’’ University of Bucharest, 313 Splaiul Independentei, Bucharest, RO 060042, Romania
a r t i c l e i n f o
Article history:
Received 27 November 2011
Received in revised form
4 January 2012
Accepted 6 January 2012Available online 21 January 2012
Keywords:
Quantum well wire
Tilted laser field
Finite element method
Density of states.
13/$ - see front matter & 2012 Elsevier B.V. A
016/j.jlumin.2012.01.020
esponding author.
ail address: [email protected] (E.C. Ni
a b s t r a c t
Within the effective-mass approximation the subband electronic levels and density of states in a
semiconductor quantum well wire under tilted laser field are investigated. The energies and wave
functions are obtained using a finite element method, which accurately takes into account the laser-
dressed confinement potential. The density of states obtained in a Green’s function formalism is
uniformly blueshifted under the laser’s axial field whereas the transverse component induces an
additional non-uniform increase of the subband levels. Our results confirm that the tilted laser field
destroys the cylindrical symmetry of the quantum confinement potential and breaks down the
electronic states’ degeneracy. Axial and transversal effects of the non-resonant laser field on the
density of states compete, bringing the attention to a supplementary degree of freedom for controlling
the optoelectronic properties: the angle between the polarization direction of the laser and the
quantum well wire axis.
& 2012 Elsevier B.V. All rights reserved.
1. Introduction
By the advent of artificial semiconductor structures with sizescomparable to the de Broglie wavelength of electron, newopportunities arise for investigating the intense laser field (ILF)effects on quantum nanostructures. It is proved that the electro-nic transport characteristics and optical properties of low-dimen-sional systems irradiated by ILFs are different from those of a bulksemiconductor, more pronouncedly as the carriers’ confinementis increased by dimensionality reduction [1–14]. Since 1D semi-conductor structures are usable for designing ultrafast electronicdevices, there is a strong motivation to study their response tointense external fields such as lasers. Some theoretical studieshave focused on shallow donor states [13,15–19] and intersub-band transitions [20,21] in QWWs dressed by laser fields polar-ized perpendicularly to the wire axis. By making use of anonperturbative method [13,21], a significant laser-induced shiftof the electronic levels was found, more pronounced for thinnerQWWs. For an ILF linearly polarized along the wire axis recentworks [22–24] have predicted an axial localization effect, whichleads to a transition from one-dimensional to zero-dimensionalbehavior of the density of states (DoS). However, the restrictionon the polarization direction such as being along or perpendicularto the wire axis may not be always experimentally feasible.Moreover, due to the strong optical and magnetic anisotropies
ll rights reserved.
culescu).
induced by ILFs [19,21] the question of an optimal interactionsetup (i.e. the relative orientation between a QWW and an opticalfield, which leads to a maximum interaction) becomes technolo-gically important.
The main objective of our study is to settle on the dependenceof the laser-driven electronic DoS in a cylindrical QWW on thelaser’s tilt angle between two limit cases, the first occurring for alaser radiation linearly polarized along the wire, and the last for apolarization in the QWW’s transverse plane. A proper under-standing of the DoS is important for controlling the opticalproperties related to electrons in semiconductor QWWs. There-fore, besides providing a theoretical framework with which tointerpret polarization-dependent absorption-emission spectra ofQWWs, our results can be used for designing novel electronicdevices in which the DoS tuning plays a significant role.
The paper is organized as follows. Section 2 describes thetheoretical framework. Section 3 presents the influence of the tiltedlaser field on the energy levels and DoS for electrons confined in aGaAs/AlGaAs cylindrical QWW. The possibility of tuning such quan-tities by varying the laser polarization direction and frequency waspointed out. Finally, our conclusions are summarized in Section 4.
2. Theory
2.1. Electron states under tilted laser fields
The physical system we consider is the nanostructure formedby surrounding a long cylindrical wire made up of direct bandgap
A. Radu, E.C. Niculescu / Journal of Luminescence 132 (2012) 1420–1426 1421
semiconductor material (GaAs) by a coaxial layer material with awider bandgap (AlxGa1�xAs) and practically the same latticeconstant (Fig. 1). The QWW is considered to interact with apolarized single-mode laser beam, non-resonant with the energylevels of the electrons in the wire.
The z-axis is chosen along the wire direction. The quasi-monochromatic laser beam is linearly polarized along an s
direction, which makes an angle y with the z-axis. The orthogonaltransverse axis x and y are chosen so that xC(z,s). The hard-wallconfinement potential has the cylindrically symmetric form
VðrÞ ¼0, rA ½0,RÞ
V0, rA ½R,1Þ,
(ð1Þ
where V0 is the conduction-band offset and r¼(x2þy2)1/2 is the
electron’s radial position in the wire.The electrons have a free movement along the wire but in its
transverse plane (x,y) the quantum confinement effect becomesimportant if radius R is comparable to the electron’s Bohr radiusin the bulk semiconductor. We will demonstrate that the laser’stransverse component dresses the energy levels associated withthe lateral confinement, whereas the axial laser field modifies theelectronic energies related to the movement along the wire.
If there is no laser irradiation on the QWW, the electron’senergy levels can be calculated by solving the atemporalSchrodinger equation in cylindrical coordinates
�_2
2mn
1
r@
@rr @
@r
� �þ
1
r2
@2
@j2þ@2
@z2
" #CðrÞþVðrÞCðrÞ ¼ ECðrÞ ð2Þ
The wave functions of the electronic subbands may be set intothe form
Cp,n,kz ðr,j,zÞ ¼Fp,nðr,jÞexpðikzzÞ ¼Rp,nðrÞexpðipjÞexpðikzzÞ,
ð3Þ
where p is an integer and kz ¼ffiffiffiffiffiffiffiffiffiffiffiffiffiffi2mnEz
p=_ is the continuous wave
number in the z direction. Ez is the axial, not quantized, electron’senergy. The radial eigenfunctions Rp,nðrÞ are analytical solutionsof the Bessel equation
r2 @2R
@r2þr @R
@rþ r2 2mn
_2E�VðrÞ� �
�p2
� �R¼ 0 ð4Þ
Fig. 1. Schematic view of a cylindrical GaAs/AlGaAs QWW irradiated by an ILF. R is
the wire’s radius and y is the angle between s, the polarization direction of the
laser and z, the longitudinal axis of the wire.
and have the forms
Rp,nðrÞ ¼Ci
p,nJpðkip,nrÞ, rA ½0,RÞ
Cop,nKpðko
p,nrÞ, rA ½R,1Þ,
8<: ð5Þ
where Jp is the p-order Bessel function, Kp is the modified Besselfunction, ki
p,n ¼ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi2mnEp,n
p=_ and ko
p,n ¼ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi2mnðV0�Ep,nÞ
p=_. Ep,n are
the discrete bound-state energy eigenvalues corresponding to thebottoms of 1D subbands. Coefficients Ci
p,n, Cop,n and energies Ep,n
may be obtained by matching the wave functions given by Eq. (5)and their derivates at the wire boundary and by wave functions’normalization. It should be noticed from Eq. (4) that Ep,n¼E�p,n,which means the states described by eigenfunctions Fpa0,n(r,j)are double-degenerated.
Total subband energies corresponding to the eigenfunctionsCp,n,kz ðr,j,zÞ are given by
Ep,nðkzÞ ¼ Ep,nþEz ð6Þ
Under the tilted laser field described by the vector potentialAðtÞ ¼ ðxsinyþ zcosyÞA0 sinðotÞ the quantum states can beobtained from the time-dependent Schrodinger equation in rec-tangular coordinates
ðp?þ xeAxðtÞÞ2
2mnþðpzþ zeAzðtÞÞ
2
2mnþVð
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffix2þy2
qÞ
" #Cðr,tÞ ¼ i_
@Cðr,tÞ
@t,
ð7Þ
where p? (pz) is the electron momentum perpendicular to (along)the wire axis.
When the vector potential has only an x-component (y¼p/2)Eq. (7) implies that
ðp?þ xeAxðtÞÞ2
2mnþVð
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffix2þy2
qÞ
" #Fðx,y,tÞ ¼ i_
@Fðx,y,tÞ
@tð8Þ
By applying the time-dependent translation x-xþððeA0 sinyÞ=ðmnoÞÞsinðotÞ, one has [25]
p?2
2mnþ ~V ðx,y,tÞ
~Fðx,y,tÞ ¼ i_
@ ~Fðx,y,tÞ
@t, ð9Þ
where ~V ðx,y,tÞ ¼ Vðffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiðxþa0xsinðotÞÞ2þy2
qÞ is the laser-dressed
confinement potential with a0x ¼ ððeA0xÞ=ðmnoÞÞ ¼ ððeA0 sinyÞ=
ðmnoÞÞ denoting the laser parameter in the x-direction. In thehigh-frequency limit [26] the laser-dressed bound states for thetransversal motion are solutions of the time-independentSchrodinger equation
�_2
2mn
@2
@x2þ@2
@y2
!þ ~V aðx,yÞ
" #~Fðx,yÞ ¼ ~E ~Fðx,yÞ, ð10Þ
where ~V aðx,yÞ is the zero-order Fourier component of the dressedpotential energy, i.e. its time average over one period
~V aðx:yÞ ¼o2p
Z 2p=o
0
~V ðx,y,tÞdt ð11Þ
For the particular potential function given by Eq. (1), Eq. (11)may be analytically integrated to the closed form
~V aðx,yÞ ¼V0
p Re Yða0x�x�Re
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiR2�y2
q� �Þarccos
RefffiffiffiffiffiffiffiffiffiffiffiffiffiffiR2�y2
qgþx
a0x
0@
1A
8<:
þYða0xþx�Re
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiR2�y2
q� �Þarccos
RefffiffiffiffiffiffiffiffiffiffiffiffiffiffiR2�y2
qg�x
a0x
0@
1A9=;,
ð12Þ
where Y is the Heaviside unit-step function. This is the firstanalytical form proposed in the literature for the laser-dressed
A. Radu, E.C. Niculescu / Journal of Luminescence 132 (2012) 1420–14261422
confinement potential of a cylindrical QWW, which allows anaccurate calculation of the dressed subband states.
By solving Eq. (10) with a finite element method [27–29], onemay obtain the laser dressed transverse energies ~Ep,n and therelated transverse eigenfunctions ~Fp,nðx,yÞ. The orthogonal states,which degenerate in Fpa0,n(r,j) for a0x¼0 still have x and y asaxis of symmetry, thus their energies and wave functions will bedenoted by ~E
x
p,n, ~Fx
p,nðx,yÞ and ~Ey
p,n, ~Fy
p,nðx,yÞ, respectively.Note that Schrodinger Eq.(8) for the transversal motion is not
affected by the presence of an additional axial componentAzðtÞ ¼ A0cosysinðotÞ of the vecftor potential; thus, the eigenva-lues ~Ep,n and the corresponding eigenfunctions ~Fp,nðx,yÞ obtainedby solving Eq.(10) remain the same. By writing Cðr,tÞ ¼~Fp,nðx,yÞULðz,tÞ [24] in Eq. (7) we obtain two Schrodinger equa-
tions: one related to a motion of electrons perpendicular to thewire axis, which is identical to Eq. (10), and the other for theparallel motion, that is
ðpzþeAzðtÞÞ2
2mnþ ~Ep,n
" #Lðz,tÞ ¼ i_
@Lðz,tÞ
@tð13Þ
Here L(z,t) depends only parametrically on the vector poten-tial component perpendicular to the wire axis, via the energy ~Ep,n.By temporal integration [23,24] of Eq. (13) one finds
Lðz,tÞ ¼Lðz,0Þexp �i ~Ep,nþ_2k2
z
2mnþDEz
!t
_þ2a0zkzsin2 ot
2
� ��DEz
2_osinð2otÞ
" #( ),
ð14Þ
where DEz¼((eA0z)2/(4mn))¼mn((a0zo)/(2))2 is the energy blue-
shift induced by the axial component of the laser field anda0z ¼ ððeA0zÞ=ðm
noÞÞ ¼ ððeA0cosyÞ=ðmnoÞÞ denotes the laser para-meter in the z direction.
Fig. 2. Laser-dressed confinement potential of the cylindrical QWW with R¼75 A.
2.2. Laser-driven density of states
Following the Green’s function approach introduced in[22–24] for quasi-1D electronic systems under ILFs and takinginto account Eq. (14), the retarded propagator (or Green’s func-tion) for non-interacting electrons is written as
Gþ ðp1,n1,kz1; p2,n2,kz2Þ ¼dp1 ,p2
dn1 ,n2dkz1kz2
i_Yðt2�t1Þ
exp i ~Ep,nðkzÞt2�t1
_þ2a0zkz sin2 ot2
2
� ��sin2 ot1
2
� � �
�DEz
2_o sinð2ot2Þ�sin ð2ot1Þ½ �
�ð15Þ
where ~Ep,nðkzÞ ¼~Ep,nþDEzþðð_
2k2z Þ=ð2mnÞÞ.
The laser-driven DoS per unit length in each 1D subband as afunction of electron’s energy can be derived from the imaginarypart of the Green’s function Fourier transform [23,24], so that
dp,nðEÞ ¼Dp,nðEÞ
L¼
gs
2p
ZdðE� ~Ep,nðkzÞÞf 0
2ðkzÞdkz, ð16Þ
where gs¼2 is the spin degeneracy factor and f 0ðkzÞ ¼P
iA2ZJi
ððDEzÞ=ð2_oÞÞJ2iða0zkzÞ, Ji denoting the order i Bessel function. Bymaking use of the Dirac-d function properties, one can obtain [24]the following expression for the overall DoS per unit length
dðEÞ ¼DðEÞ
L¼ gs
ffiffiffiffiffiffiffiffiffiffi2mnp
2p_Xp,n
YðE� ~Ep,n�DEzÞffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiE� ~Ep,n�DEz
q f 02ð
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi2mnðE� ~Ep,n�DEzÞ
q=_Þ
ð17Þ
Due to the term DEz in the denominator and the Y function, anuniform blueshift of the DoS profile as a whole is expected underan axial laser field.
3. Results and discussion
The numerical calculations were performed for a GaAs/Alx-
Ga1�xAs cylindrical QWW with x¼0.3 and R¼75 A. The size ofconsidered GaAs nanostructure is chosen to be slightly smallerthan the electronic Bohr radius in bulk GaAs (ffi100 A). A numberof characteristic features of energy levels are revealed in thisintermediate quantum confinement regime, when the strength ofthe electron-laser field interaction and quantum confinementeffects are comparable.
An isotropic effective mass mn¼(0.0665þ(0.08þ1/300)x)m0
of the electron throughout the nanostructure was assumed (m0
denoting the free electron mass). The conduction-band offsetV0¼228 meV was introduced by taking into account the Miller’srule (V0¼60%DEgapE0.7xþ0.2x2 in eV units). The laser parameteris considered to be a constant a0¼R¼75 A, so that the QWW’sconfinement potential will be significantly modified as the laserpolarization angle y varies from 0 to p/2. In the absence of thelaser filed, there are four bound states in the QWW (the secondand the third being double degenerated): E0,1¼37.22 meV,E1,1¼93.65 meV, E2,1¼164.67 meV and E0,2¼187.96 meV.
3.1. Laser-dressed electronic states
Fig. 2 shows the time-averaged laser dressed confinementpotential given by Eq. (11) for a0x¼75 A (y¼901), when theradiation provokes maximum changes on the potential energy.At high energies the effective potential profile seems to beenlarged along the laser polarization direction, while at thebottom of the well the potential has a sharp profile. The meanwidth of the QWW confinement potential within the y¼0 section,defined as ð2=V0Þ
R V0
0~V a�1ðxþ ,0ÞdV , remains equal with 2R. On the
other hand, the mean width within the x¼0 section has adiminished value with respect to the no-dressing case,ð2=V0Þ
R V0
0~V a�1ð0,yþ ÞdV o2R, because there is no enlargement
in the y direction. These observations clearly suggest a laser-induced strong enhancement of the quantum confinement forlow-energy states.
Fig. 3 illustrates the changes of the transverse probabilitydensity for the electron ground state when rotating the laserfrom axial to transversal polarization. For a0x¼0 (Fig. 3(a))one may observe the angular independence characteristic to
Fig. 3. Cross section of the electron probability density for the ground state, at (a)
y¼0; (b) y¼901.
Fig. 4. Cross section of the electron probability density for the first excited state,
at y¼0 (a) and(c) and y¼901 (b) and (d).
Fig. 5. Cross section of the electron probability density for the second excited
state, at y¼0 (a) and (c) and y¼901 (b) and (d).
Fig. 6. Cross section of the electron probability density for the third excited state,
at (a) y¼0; (b) y¼901.
A. Radu, E.C. Niculescu / Journal of Luminescence 132 (2012) 1420–1426 1423
non-degenerate states and a maximum probability density on thewire axis. This on-axis maximum is enhanced for a0x¼75 A and asignificant blueshift of the ground state energy is observed(Fig. 3(b)).
The probability density of the electron in the first excited stateis presented in Fig. 4. As expected, in the absence of the lasercomponent on the x-axis, there are two orthogonal eigenstateswith the same energy E1,1 (Fig. 4(a) and (c)). For both states theprobability density has an on-axis minimum and two identicalmaxima symmetrically positioned with respect to the wire axis.The ILF breaks down the radial symmetry so that two laserdressed orthogonal states with different energies are obtained(Fig. 4(b) and (d)).
Fig. 5(a) and (c) shows the density of probability for the secondexcited state of the electron, also double-degenerated. For bothorthogonal states the localization probability is zero on the wireaxis and has four equal maximums with equidistant angularseparation. Fig. 5(b) and (d) illustrate the laser-induced degen-eracy breaking with an obvious difference between the orthogo-nal states ~F
x
2,1ðx,yÞ and ~Fy
2,1ðx,yÞ. It’s also apparent fromFig. 5(b) and (d), that the electron wave functions spread in thebarrier regions of the dressed QWW. This later feature is a general
characteristic of low-dimensional structures subjected to non-resonant laser fields [19].
The upper subband state is not degenerated because its wavefunction is also angularly independent (Fig. 6(a)). Two radialmaxima can be observed on the density of probability image,one in the middle of the wire (on-axis maximum) and the otherby the form of a circular ring (near-edge maximum). In hightransverse laser fields (Fig. 6(b)), due to the leakage of the wavefunction into the barrier regions, the probability density isstrongly affected, having two symmetrical large peaks outsidethe wire and another two weaker maxima inside.
Fig. 7 offers a better image of the transverse subband levelsdependence on the in-plane component of the laser parameter.One may observe that, although all the energy levels are blue-shifted, the ground level is the most affected by the field,increasing with more than 60 meV. The effect of the radiation isless pronounced for higher energy levels due to a weakerconfinement in the upper part of the dressed QWW potential. Itis clear from Fig. 7 that large field intensity is needed to induceappreciable changes of the upper-lying states. Indeed, E2,1 levelremains degenerated under relatively high transverse laser
Fig. 7. Transverse subband energy levels versus in-plane laser parameter.
Fig. 8. Energy levels blueshift induced by the axial laser filed, as a function of the
laser frequency.
Fig. 9. Electron DoS versus energy for (a) o/2p¼10 THz; (b) o/2p¼25 THz and
three different orientations of the laser field. Dotted line is for the DoS in the
absence of laser radiation. a,b,c,d represent the ground and the three excited
subbands, respectively. Notations x, y stand for different levels originating from
the same electronic state through laser degeneracy breaking.
A. Radu, E.C. Niculescu / Journal of Luminescence 132 (2012) 1420–14261424
parameter, a0xffiR/2, and for the highest excited state only a slowvariation with growth of a0x is observed. The coalescence of thesubband energy levels with the increase of the transverse laserparameter is a remarkable aspect, which has been also reportedfor square QWs under ILFs [11].
Fig. 8 depicts the energy blueshift induced by the axialcomponent of the laser field as a function of the laser frequency.All levels present a parabolic increase while keeping the sameenergy separation. For relatively small frequency values(o/2po20 THz), the blueshift DEz brought by an axial orientationof the laser field is observed to be less important than the typicalenergy levels increase induced by the same laser in the transverseorientation case (Fig. 7). By maintaining the same laser parameterat higher values of o, one may notice the opposite situation.
3.2. Laser-driven density of states
Accordingly to previous discussion, we calculated the electronDoS for two different values of the laser frequency.Fig. 9(a) presents the results obtained for o/2p¼10 THz, at threedifferent orientations of the laser field. For y¼0 there is only arelatively small and uniform blueshift of all energy levels, inducedby the axial laser field, as compared with the unperturbed DoS. Inaddition, the DoS profile changes from the characteristic shape foran unperturbed QWW to a set of sharp peaks, which is a sign of anincreased confinement due to the axial field effect on the electron[23]. For y¼p/4 the energy blueshift is the combined effect ofboth radiation components. The level splitting, which is apparentfrom this figure results from degeneracy breaking effect producedby the transverse laser component. For y¼p/2, only the
A. Radu, E.C. Niculescu / Journal of Luminescence 132 (2012) 1420–1426 1425
transverse effect remains, the energy spectrum being non-uni-formly blueshifted.
Fig. 9(b) presents the electron DoS for o/2p¼25 THz, at thesame three orientations of the laser field. For y¼0 (axial laserpolarization) there is a large uniform blueshift of the energy levelsand a strong decrease of the DoS profile height. For y¼p/4 theenergy blueshift and the level splitting are the combined effects ofthe axial and transversal laser components. Unlike in Fig. 9(a), theDoS profile is redshifted as compared with y¼0 case. For y¼p/2(transverse laser polarization), there is an even larger redshift ofthe DoS, energies being still blueshifted as compared with theunperturbed DoS profile.
Fig. 10. DoS as a function of the electron energy and the laser field orientation for
(a) o/2p¼10 THz; (b) o/2p¼25 THz.
As a more comprehensive analysis, in Fig. 10(a,b) we presentthe electronic DoS as a function of the energy and the laserpolarization direction. High DoS areas are delimited by singularitylines, where d-N. For a relatively small laser frequency(Fig. 10(a)) the singularity lines are blueshifted by the increase ofthe angle y, starting with a DoS configuration characteristic to theaxial laser (y¼0) and ending up with a configuration typical to thetransverse laser effect (y¼p/2). For higher values of the laserfrequency (Fig. 10(a)) the DoS exhibits a different behavior, thesingularity lines being redshifted by the increase of the angle y.
One may now observe that the question of optimal geometryfor the laser–QWW interaction depends on the electron’s statesinvolved in optical transitions and on the wire size. Since a laserfield polarized along the axis of the wire uniformly shifts thesubband levels (Fig. 9), the intersubband transitions are notaffected. Consequently, geometries with small y values are morelikely to yield efficient tuning of the interband transitions, forwhich there is an uniform and predictable energy blueshift ofððe2A2
0zÞ=ð4ÞÞðð1=mnÞþð1=mn
hhÞÞ, where mn (mn
hh) is the electron(heavy-hole) effective masse. Note that this shift in the jointdensity of states is independent of the quantum wire’s size orshape. One the other hand, at large y values the conductionsubband states are strongly and not uniformly affected by thetransverse laser field (Fig. 10). This effect depends on the sizeand shape of the wire being more pronounced at strongercarrier confinement, i.e. for lowest-lying levels and small R
values. Therefore, the desired energy range for the intersubbandtransitions may be obtained by changing the size and/or compo-sition of the heterostructure as well as the polarizationdirection of the laser field. For GaAs/AlGaAs low-dimensionalstructures the hole states are less sensitive to the transversal laseraction, for two reasons: (i) the mass of the heavy-hole inside theQWW (mn
hh ¼ 0:35m0) is five times larger than the effective massof the electron, so that the laser parameter a0x is five timessmaller for the valence band; (ii) the offset for the heavy-hole isroughly 1.5 times smaller than the conduction band offset, so thatthe THz radiation effect is weakened. Consequently, for thinQWWs in which the electron ground-state subband energy isvery sensitive to the radiation strength, the angle between thepolarization direction of the laser and the wire axis could tune theblueshift of the lowest-energy interband transition (i.e. the band-gap energy).
4. Conclusions
A semiconductor QWW under tilted ILF was investigated in theeffective mass-approximation using a non-perturbative approachand a finite element method. The originality of this work consistsin proposing a new degree of freedom for controlling the electro-nic DoS in 1D nanostructures and the emergent optical proper-ties: the angle between the polarization direction of the laser andthe wire axis. Moreover, an original closed-form expression forthe laser dressed potential of a cylindrical semiconductor QWWwas proposed.
Our results revealed that the effects of the non-resonant laserfield on the electron probability density, reflected in the behaviorof the energy levels, are very dependent on the laser polarizationdirection. An axial laser field induces an uniform blueshift of theenergy levels, which has a parabolic increase with the laserfrequency and is more suitable for interband optical tuning inQWWs. A transverse laser field mostly affects the first conductionsubband level being adequate for tuning the intersubband transi-tions and also the band-gap energy. Any intermediary laserorientation has a combined effect on the energy spectrum andthe DoS, depending on the tilt angle and the frequency.
A. Radu, E.C. Niculescu / Journal of Luminescence 132 (2012) 1420–14261426
Acknowledgment
One of the authors (A.R.) recognizes financial support from theEuropean Social Fund through POSDRU/89/1.5/S/54785 project:‘‘Postdoctoral Program for Advanced Research in the field ofnanomaterials’’.
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