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Stelios Tzortzakis Science Program, Texas A&M University at Qatar Institute of Electronic Structure and Laser, FORTH & University of Crete, Greece University of Crete

Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

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Page 1: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Stelios Tzortzakis

Science Program, Texas A&M University at Qatar

Institute of Electronic Structure and Laser, FORTH

& University of Crete, Greece

University of Crete

Page 2: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Introduction

o Intense laser beams – Solitons – Filaments and Complex spatio-

temporal wave packets

o Sculpted Exotic beams for tamed waves

Advanced materials engineering

o Large volume high resolution photo-polymerization

Silicon Photonics

o Direct laser writing of photonic circuits in the bulk of silicon –

merging optics and electronics under the same platform

Teaser: Passive radiative cooling

o Improving the performance of photovoltaics

Page 3: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Dynamic equilibrium in space and time between Kerr effect and ionization

Ker

r ef

fect

ion

izat

ion

Page 4: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

'' 2

2

2,

2 2

E i k EE i N E

z k t

2 22 2

2 2 2

0 2 0 0

0

2 2 2

0

: ,

1

12

12

1

Kerr Plasma MPA

t

Kerr

Plasma C

KKMPA

at

where N E T N E N TN E

N E ik n a E ik n a R t E d

N

N E E

T it

2 2 2K

K at

i

at U

0

0

0 0

2 20 0

:

1

:1

K at K

K

K

MPI K

i

C

C C

K

Cross Section for Multi Photon Ionization

with rate W I

Ufor K photons

kCross Section for Inverse Bremsstrahlung

n

Unidirectional Pulse PropagationEquation (UPPE)

Page 5: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

APL 93, 041120 (2008); PRA 84, 053809 (2011)

Page 6: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams
Page 7: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Phys. Rev. Lett. 105, 253901 (2010)

Airy3

light bullet

Page 8: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Opt. Lett. 36, 1842 (2011)

Exciting candidates for a variety of applications, as in bio-medicine, laser nanosurgery and optical lithography (e.g. photopolymerization)

Page 9: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams
Page 10: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

❖ 3D Writing of complex Micro- & Nano-structures but limited in volume, typically

100 μm - height

I. Sakellari et. al, ACSNano, 6, 3, 2302–2311 , 2012

[*]

Page 11: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

w: width of the primary Airy ring

r0: radius of the primary Airy ring

sam

ple

Typical phase mask

0 10 20 30

0,0

0,5

1,0

Inte

nsi

ty (

no

rm)

Z(mm)

Ring-Airy propagation dynamics

800nm,160fs, 50Hz

Intensity profileat the FT plane 100μm

100μm

Page 12: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

By adjusting the w and/or r0 parameters of the primary ring, using the appropriate phasemask, the focus position can be manipulated in real time with the SLM.

Intensity profiles of ring-Airy beams as capturedby the CCD at the FT plane

0 10 20 30 40

0,0

0,5

1,0

Threshold Line

Inte

nsi

ty (

norm

)

Z(mm)

Experimental intensity distributions (normalized values) of the ring-Airy beams along the propagation axis

Page 13: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Focal voxel aspect Ratio comparative curves

• In an MPP application the polymerization takes place only at areas where the intensity is high enough.

• We used the 80% of the peak intensity distribution as a threshold.

• The ring Airy beams keep the voxel aspect ratio almost invariant !

• The voxel aspect ratio for Bessel beams is increasing as the beam focus is pushed further away.

Focus Aspect Ratio: 𝐿𝑜𝑛𝑔𝑖𝑡𝑢𝑑𝑖𝑛𝑎𝑙 𝑠𝑖𝑧𝑒 𝑜𝑓 𝐹𝑜𝑐𝑢𝑠

𝐹𝑜𝑐𝑢𝑠 𝐷𝑖𝑎𝑚𝑒𝑡𝑒𝑟Focal volume

FWHM

Spotsize

Optica 3, 525-530 (2016)

Page 14: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Optica 3, 525-530 (2016)

Page 15: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Aspect ratio ~20000μ𝑚

4𝜇𝑚BurjKhalifa, Dubai

Page 16: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams
Page 17: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

“Laser Matter Interactions: from fundamental studies to innovative laser processing”

• Advanced knowledge on propagation and laser materials interaction (metals, semiconductors and dielectrics), I <1019 W/cm2

• Development of new photonic processes• New materials, new features• …….

▪ Higher synergy between IESL - LP3 and their organizations▪ Access to complementary equipment▪ Increased international visibility▪ Strengthening of AMU & FORTH’s relations within the Mediterranean

region

Coordinators: Mark Sentis (LP3) & Stelios Tzortzakis (IESL)

Page 18: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

The road from this…

Page 19: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

To this…The 50 Gbps

Si Photonics Link

Page 20: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Experimental holographic setup

Excellent agreement between our simulations and experimental results

Page 21: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Excellent agreement between our simulations and experimental results

The problem is projected to a stretched space-time one such that it

becomes paraxial!

Page 22: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Two-photon absorption and defocusing in plasma lead to the depletion of thepulse energy on the way to focus.

To date all attempts to modify the bulk of Si using femtosecond pulses have failed! Why?

Page 23: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

Induce permanent index modification in the bulk of Si using extreme localization

of light in space and time.

Took 20 years to reach this milestone from the time of the first demonstration

in the bulk of glasses!

Nat. Commun. 8, 773 (2017)

Page 24: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams
Page 25: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

▪ Radiative cooling: Dissipate excess

heat into remote heat sinks via thermal

radiation.

▪ Materials: Combination of natural and

artificial materials, like metamaterials.

▪ Application in photovoltaic cells:

reduced temperature of operation,

resulting in higher performance and

longer lifetimes.

▪ A joint research project between

FORTH and Texas A&M University,

funded by Qatar Foundation.

Page 26: Femtosecond Driven Radiation Sources and Applications · Introduction o Intense laser beams –Solitons –Filaments and Complex spatio- temporal wave packets o Sculpted Exotic beams

UNIS group:

V. Fedorov

T. Koulouklidis

M. Manousidaki

D. Mansour

Ch. Daskalaki

M. Loulakis

D. Papazoglou

Collaborators:

Farsari / Manousidaki, FORTH

Kafesaki / Perrakis, FORTH

Grojo / Chanal, Univ. of Marseille

Zacharakis / Di Batista, FORTH

A. Couairon, Ecole Polytechnique

D. Christodoulides, CREOL

Moloney / Kolesik, Arizona

X.-C. Zhang, RochesterFunding

University of Crete