Investigation of the Nocturnal PM Peaks for Evidence of Association with Population Health Risks in Two Border Cities Jessica Gamez1; Donald J. Baca1; Hector A. Olvera1; Nancy Garcia1; Mario Garcia1; Fernando Astorga2; Jose H. Garcia3; Gerardo Mejia4; Kerry Kelly5; JoAnn Lighty5; Wen-Whai Li1,2

1 Department of Civil Engineering, 2 Environmental Science and Engineering, The University of Texas at El Paso; 3 Professional Department (Campus Ciudad Jurez), 4 Centro de Calidad Ambiental (Campus Monterrey), Instituto Tecnolgico y de Estudios Superiores de Monterrey; 5 Institute for Combustion and Energy Studies, University of Utah

AbstractThis paper presents the results of a study characterizing the physical and chemical properties associated with the nocturnal PM10 and PM2.5 spikes that occur in the calm early evening hours (from 6:00 p.m. to 9:00 p.m.) in the two sister border cities (El Paso and Ciudad Juarez) along the U.S.-Mexico border. It represents an ongoing task under a collaborative research effort among several SCERP universities to investigate the nocturnal PM peaks for evidence of association with population health risks.The nocturnal PM peaks previously observed at Sunland Park, New Mexico and several other cities along the U.S.-Mexico border were observed at the two new locations. The evening PM peak was observed to occur under low wind conditions (< 2 m/sec) with a strong correlation with preceding afternoon high to moderate wind conditions. The hourly PM particle count varied from less than 10,000 particles/cm3 in the afternoon to greater than 80,000 particles/cm3 in the evening hours during the study period. The total number of PM particles peaked in the morning as well as in the evening while the mode of the particle size changed from 20 nm to ~100 nm, indicating different PM sources may be responsible for the mass and number concentrations and agglomeration of particles in the atmosphere during the day may possibly plays a role. Larger particles (100 470 nm) were found to associate better than smaller particles (10 100 nm) with PM mass. Wind direction did not have an impact on the PM number concentrations whereas wind speed is negative correlated (although small) to both PM size fractions confirming the occurrence of PM peaks under low wind conditions. Further chemical and statistical analyses are underway.

Statement of Probleminsufficient continuous and time-resolved PM (PM10 and PM2.5) data and meteorological observations for the Ciudad Juarez metropolisincomplete continuous and time-resolved PM (PM10 and PM2.5) data in El Paso to support the development of causal relationship between inhalation exposure and key physiological parameters, such as cardiopulmonary functions and blood chemistry.Insufficient physical characterization of ambient PM

Research ObjectivesCharacterize the temporal and time-resolved PM2.5 and PM10 concentrations;

Identify the sources and locations of the PM evening peaks using the new data and existing data from the Sunland Park study; and

Associate the PM peaks to the concurrently monitored physiological data at two PdN locations

Study LocationsCAMS12ITESM

Experimental SetupInstrumentation (CAMS 12, El Paso)1 TEOM for PM10; 1 TEOM for PM2.51 TSI 3321 APS for Particles between 0.5 and 20 m1 Climet Particle Sizer for Particles between 0.5 and 20 m 1 TSI 3034 SMPS for Particles between 0.01 and 0.5 mSupplementary Meteorological Monitoring of Wind Speed, Wind Direction, Temperature, Pressure, Humidity, and others

Experimental SetupInstrumentation (ITESM, Cd. Juarez)1 TEOM for PM10; 1 TEOM for PM2.51 DATARAM Continuous PM10 Monitors 1 Climet Particle Sizer for Particles between 0.5 and 20 m 1 TSI 3034 SMPS for Particles between 0.01 and 0.5 mA METONE surface meteorological monitoring station for wind speed, wind direction, temperature, and pressure(see presentation of Near-instantaneous impacts of high PM episodes on cardiopulmonary function in healthy adults by H.L.C. Meuzelaar)

Results

PM Concentrations and Wind Speed at CAMS 12

Chart2

1.788165.0425.86

1.2070085.9317.61

1.2517126.8920.63

1.2517124.6314.44

1.4752328.8539.72

1.8328645.0315.63

2.0563847.7630.52

2.3693124.5318.8

1.8328645.4228.72

1.7434566.9238.74

2.7716482.6218.68

2.458722.3214.89

1.788161.6813.59

2.011682.413.35

1.6987523.2914.3

1.2517123.4918.35

1.1623045.838.19

1.9222723.2911.16

1.8328642.663.76

1.02819219.97100.84

1.117620.7782.29

1.29641616.9763.17

1.43052814.6462.62

1.87756814.8358.41

WS m/s

PM2.5

PM10

Time

Mass Concentration (g/m3)

Wind Speed (m/s)

CAMS 12 October 27 2006: PM 10, PM 2.5, and Wind Speed

Data

10/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/0610/27/06

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WS4.002.702.802.803.304.104.605.304.103.906.205.504.004.503.802.802.604.304.102.302.502.903.204.20

WS m/s1.791.211.251.251.481.832.062.371.831.742.772.461.792.011.701.251.161.921.831.031.121.301.431.88

WD3072612792702763303133152782558719250302296842687357289306293315317

PM2.55.045.936.894.638.855.037.764.535.426.922.622.321.682.43.293.495.83.292.6619.9720.7716.9714.6414.83

PM1025.8617.6120.6314.4439.7215.6330.5218.828.7238.7418.6814.8913.5913.3514.318.3538.1911.163.76100.8482.2963.1762.6258.41

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WS2.72.62.42.22.84.32.61.52.433.63.23.43.73.53.32.92.22.51.61.41.71.51.4

WS m/s1.211.161.070.981.251.921.160.671.071.341.611.431.521.651.561.481.300.981.120.720.630.760.670.63

WD3383342963013373463472152081321301161832192372633584227127823232196153

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WD18034434332334833734124104176317272287275284286311284289303303328329330

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WS11.31312.411.312.512.312.713.21212.411.711.111.298.78.87.66.47.98.88.289.18.1

WS m/s5.055.815.545.055.595.505.685.905.365.545.234.965.014.023.893.933.402.863.533.933.673.584.073.62

WD118121121111124116120124105100111110117103988573698689115115104104

PM2.57.316.935.876.497.447.177.18.747.756.56.146.385.676.876.636.236.526.568.18.159.459.148.417.61

PM1040.6735.2128.9131.4528.0131.2127.3344.6337.9332.1532.5632.2928.3726.7324.7722.3123.3622.6228.1526.9328.5629.3221.6919.06

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