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Spatiotemporal Patterns of Urban Trace Gases and Pollutants Observed with a Light Rail Vehicle Platform in Salt Lake City, UT Logan E. Mitchell 1,* , Erik Crosman 1 , Ben Fasoli 1 , Luke Leclair-Marzolf 1 , Alexander Jacques 1 , John Horel 1 , John C. Lin 1 , David R. Bowling 2 , James R. Ehleringer 2 1 Department of Atmospheric Sciences, University of Utah, Salt Lake City, UT; 2 Department of Biology, University of Utah, Salt Lake City, UT * Corresponding author. E-mail address: [email protected] Operates on the Utah Transit Authority (UTA) TRAX light rail system: Red Line: traverses the entire Salt Lake Valley (northeast to southwest, including a symmetric elevation profile) at hourly intervals. Green Line: runs from the SLC airport to West Valley with two legs perpendicular to the dominant north-south transport providing plume characterization opportunities. 2. Experimental Setup 3. Greenhouse Gases 5. Particulate Matter 4. Ozone 7. Salt Lake Valley Measurement Programs (a) TRAX light rail network (http://meso1.chpc.utah.edu/mesotrax/ ) (b) 5-station, urban CO 2 network (http://co2.utah.edu ) (c) MesoWest (http://mesowest.utah.edu/ ) (d) Utah Dept. of Environmental Quality (http://air.utah.gov/ ) (e) RACCOON mountaintop observatory (http://www.eol.ucar.edu/homes/stephens/RACCOON/ ) We gratefully acknowledge technical & logistic support from UTA TRAX & Siemens (Teresa Jessen, Elijah Jackson, Tal Brooks, & the rest of UTA TRAX staff) as well as Ryan Bares, and Will Howard. Funding provided by the GCSC & federal & state agencies. 1. Introduction Urban environments are characterized by both spatial complexity and temporal variability, each of which present challenges for measurement strategies aimed at constraining estimates of greenhouse gas emissions and air quality. To address these challenges we initiated a project in December 2014 to measure trace species (CO 2 , CH 4 , O 3 , and Particulate Matter) by way of a light rail vehicle (Utah Transit Authority) whose fixed route traverses the entire Salt Lake Valley in Utah on an hourly basis through commercial, residential, suburban, and rural typologies. Light rail vehicles offer three advantages as a measurement platform: the absence of in situ fossil fuel emissions, repeated transects across urban typologies that provides both spatial and temporal information, and relatively low operating costs. We present initial results of the spatiotemporal patterns of greenhouse gases and pollutants across the Salt Lake Valley from the first year of operations. Carbon Dioxide Elevated mixing ratios observed in the urban core where rail line is in the middle of traffic and along the whole urban corridor. Lower CO 2 on the urban periphery. Local enhancement of CO 2 along every road. Diel profile shows influence of convective mixing during the day and stable boundary layer at night. Methane Plumes associated with natural gas power plants, landfills, and a brick factory. Intermittent plumes visible during discrete times of day. Morning profile shows influence of stable nighttime boundary layer in northern part of valley (points 0-100 on Red Line). Seasonal Averages Highest mixing ratios on the valley benches, lowest along the urban corridor. Local depletions due to NOx scavenging associated with higher traffic. Valley benches & suburbs are exposed to higher mean summertime O 3 than central urban corridor. Afternoon vs. Nighttime Exposure O 3 is highest in the afternoon and is uniformly distributed due to convective mixing. At night & in the early morning the prominent spatial pattern between valley benches & urban corridor is evident. Low urban corridor O 3 suggests that O 3 is destroyed nocturnally by NOx, particularly in the nighttime boundary layer. Health implications: do mean values or peak values cause greatest health impacts? Spatial pattern of health impacts could inform this question. Frequent wintertime atmospheric inversions trap pollutants and lead to exceedances of National Ambient Air Quality Standards. Excellent correlation during these episodes between rail-mounted instruments and DAQ measurements (~2 km away). Spatial pattern is opposite that of O 3 . Strong influence of topography. Do the intraurban spatial patterns of health impacts track the spatial pattern of PM 2.5 ? 6. Conclusions & Future Directions. We used a light-rail platform to observe and characterize patterns of GHGs and air pollutants. There are large, abrupt intra-urban gradients associated with sources and sinks. Future Directions: Measures CO 2 , CH 4 , PM 2.5 , and O 3 . Dec 2014 to present. > 1500 transects on the Red Line > 1300 transects on the Green Line. Sensors and sampling on roof. Expanded PM 2.5 observations to a second rail car in January 2016. Upcoming Possibilities: Expand this setup to additional rail cars to increase spatial & temporal coverage. Additional trace gas species that could be added include: (a) NOx (NO 2 and N 2 O) would assist in closing the ozone budget, (b) ethane (C 2 H 6 ) would provide a distinction between biogenic & fossil CH 4 sources, and (c) radon ( 222 Rn) would constrain local atmospheric mixing. Dec 2014 – Nov 2015 Hours: 0400-2400 Dec 2014 – Nov 2015 Hours: 0400-2400 Jan 8, 2015 – Jan 12, 2015 Hours: 0400-2400 May 2015 – Sept 2015 Hours: 0400-2400 Inverse modeling of GHGs Integrate mobile platforms. Uncertainty using stationary sites vs. mobile vs. both. Use multiple species to leverage divergent emission patterns. Intra-urban relationships Pollutants and health. Co-benefits of GHG and pollutant mitigation policies. Socio-institution relationships. Expansion Other cities. Low cost sensors. Electric buses. Real Time TRAX Data: 0 10 20 30 40 50 60 70 80 0 10 20 30 40 50 60 70 80 Hawthorne PM2.5 Other instrument PM2.5 R 2 = 0.91942 y = 1.2861x + -4.0007 Slope 95% CI: 1.25-1.32 R 2 = 0.87775 y = 0.36903x + 0.048924 Slope 95% CI: 0.36-0.37 E-Sampler GRIMM 1-1 line North South North South North South Univ of Utah Downtown I-15 freeway Daybreak

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Page 1: Spatiotemporal Patterns of Urban Trace Gases and ......Spatiotemporal Patterns of Urban Trace Gases and Pollutants Observed with a Light Rail Vehicle Platform in Salt Lake City, UT

Spatiotemporal Patterns of Urban Trace Gases and Pollutants Observed with a Light

Rail Vehicle Platform in Salt Lake City, UT

Logan E. Mitchell1,*, Erik Crosman1, Ben Fasoli1, Luke Leclair-Marzolf1, Alexander Jacques1, John Horel1, John C. Lin1, David R. Bowling2, James R. Ehleringer2

1 Department of Atmospheric Sciences, University of Utah, Salt Lake City, UT; 2 Department of Biology, University of Utah, Salt Lake City, UT* Corresponding author. E-mail address: [email protected]

• Operates on the Utah Transit Authority (UTA)

TRAX light rail system:

• Red Line: traverses the entire Salt Lake Valley

(northeast to southwest, including a symmetric

elevation profile) at hourly intervals.

• Green Line: runs from the SLC airport to West

Valley with two legs perpendicular to the

dominant north-south transport providing plume

characterization opportunities.

2. Experimental Setup

3. Greenhouse Gases 5. Particulate Matter

4. Ozone

7. Salt Lake Valley Measurement Programs(a) TRAX light rail network

(http://meso1.chpc.utah.edu/mesotrax/)

(b) 5-station, urban CO2 network (http://co2.utah.edu)

(c) MesoWest (http://mesowest.utah.edu/)

(d) Utah Dept. of Environmental Quality (http://air.utah.gov/)

(e) RACCOON mountaintop observatory

(http://www.eol.ucar.edu/homes/stephens/RACCOON/)

We gratefully acknowledge technical & logistic support from UTA

TRAX & Siemens (Teresa Jessen, Elijah Jackson, Tal Brooks, & the

rest of UTA TRAX staff) as well as Ryan Bares, and Will Howard.

Funding provided by the GCSC & federal & state agencies.

1. Introduction

Urban environments are characterized by both spatial complexity and temporal variability, each

of which present challenges for measurement strategies aimed at constraining estimates of

greenhouse gas emissions and air quality. To address these challenges we initiated a project in

December 2014 to measure trace species (CO2, CH4, O3, and Particulate Matter) by way of a light

rail vehicle (Utah Transit Authority) whose fixed route traverses the entire Salt Lake Valley in

Utah on an hourly basis through commercial, residential, suburban, and rural typologies. Light

rail vehicles offer three advantages as a measurement platform: the absence of in situ fossil fuel

emissions, repeated transects across urban typologies that provides both spatial and temporal

information, and relatively low operating costs. We present initial results of the spatiotemporal

patterns of greenhouse gases and pollutants across the Salt Lake Valley from the first year of

operations.

Carbon Dioxide

• Elevated mixing ratios observed in the urban core

where rail line is in the middle of traffic and along

the whole urban corridor.

• Lower CO2 on the urban periphery.

• Local enhancement of CO2 along every road.

• Diel profile shows influence of convective mixing

during the day and stable boundary layer at night.

Methane

• Plumes associated with natural gas power plants,

landfills, and a brick factory.

• Intermittent plumes visible during discrete times

of day.

• Morning profile shows influence of stable

nighttime boundary layer in northern part of

valley (points 0-100 on Red Line).

Seasonal Averages

• Highest mixing ratios on the valley benches, lowest

along the urban corridor.

• Local depletions due to NOx scavenging associated with

higher traffic.

• Valley benches & suburbs are exposed to higher mean

summertime O3 than central urban corridor.

Afternoon vs. Nighttime Exposure

• O3 is highest in the afternoon and is uniformly

distributed due to convective mixing.

• At night & in the early morning the prominent spatial

pattern between valley benches & urban corridor is

evident.

• Low urban corridor O3 suggests that O3 is destroyed

nocturnally by NOx, particularly in the nighttime

boundary layer.

• Health implications: do mean values or peak values

cause greatest health impacts? Spatial pattern of

health impacts could inform this question.

• Frequent wintertime atmospheric inversions trap

pollutants and lead to exceedances of National

Ambient Air Quality Standards.

• Excellent correlation during these episodes

between rail-mounted instruments and DAQ

measurements (~2 km away).

• Spatial pattern is opposite that of O3.

• Strong influence of topography.

• Do the intraurban spatial patterns of health

impacts track the spatial pattern of PM2.5?

6. Conclusions & Future Directions.

We used a light-rail platform to observe and characterize

patterns of GHGs and air pollutants.

There are large, abrupt intra-urban gradients associated with

sources and sinks.

Future Directions:

• Measures CO2, CH4, PM2.5, and O3.

• Dec 2014 to present.

• > 1500 transects on the Red Line

• > 1300 transects on the Green Line.

• Sensors and sampling on roof.

• Expanded PM2.5 observations to a second rail car

in January 2016.

• Upcoming Possibilities:

• Expand this setup to additional rail cars to

increase spatial & temporal coverage.

• Additional trace gas species that could be

added include: (a) NOx (NO2 and N2O) would

assist in closing the ozone budget, (b) ethane

(C2H6) would provide a distinction between

biogenic & fossil CH4 sources, and (c) radon

(222Rn) would constrain local atmospheric

mixing.

Dec 2014 – Nov 2015Hours: 0400-2400

Dec 2014 – Nov 2015Hours: 0400-2400

Jan 8, 2015 – Jan 12, 2015Hours: 0400-2400

May 2015 – Sept 2015Hours: 0400-2400

Inverse modeling of GHGs

Integrate mobile platforms.

Uncertainty using stationary sites vs. mobile vs. both.

Use multiple species to leverage divergent emission patterns.

Intra-urban relationships

Pollutants and health.

Co-benefits of GHG and pollutant mitigation policies.

Socio-institution relationships.

Expansion

Other cities.

Low cost sensors.

Electric buses.

Real Time

TRAX Data:

0 10 20 30 40 50 60 70 800

10

20

30

40

50

60

70

80

Hawthorne PM2.5

Oth

er

instr

um

ent

PM

2.5

R2 = 0.91942

y = 1.2861x + -4.0007

Slope 95% CI: 1.25-1.32

R2 = 0.87775

y = 0.36903x + 0.048924

Slope 95% CI: 0.36-0.37

E-Sampler

GRIMM

1-1 line

North South North South

North South

Un

ivo

f U

tah

Do

wn

tow

n

I-1

5 f

reew

ay

Day

bre

ak