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Temperature propagation during cell stacking processes for lithium-ion cells
Gerd Liebig
Oldenburg
October 14-16 2015
Summary
Introduction / Productions processes during battery stack assembly
Modeling Approach
Numerical Model (COMSOL Multiphysics®)
Experimental Study and Simulation Results
Validation
Short-term Thermal Treatment / Laser welding
Conclusions and Outlook
Acknowledgements
21.10.2015 Gerd Liebig / European Comsol Conference 2015 2
21.10.2015 Gerd Liebig / European Comsol Conference 2015 3
Productions processes during battery stack assembly
plasma pretreatment
UV curing
Pretreatment
ultrasonic joining
Laser welding
Welding
Hot gluing
Bonding
Elevated temperatures on the cell surface influences the cell behavior (capacity loss, power fade, safety risks) negatively
hot staking
Modeling approach
21.10.2015 Gerd Liebig / European Comsol Conference 2015 4
Heat Stamp
Jelly Roll
Steel Casing
Pole
Collector
O2
M2
O1
M1
O3
M3
A1
A2
3D cell geometry of the simulated Li-ion cell with thermal sensor spots
Numerical Model (COMSOL Multiphysics®)
21.10.2015 Gerd Liebig / European Comsol Conference 2015 5
Heat transfer equation: heat generation and conduction
𝝆 𝑪𝒑𝝏𝑻
𝝏𝒕= 𝐝𝐢𝐯 𝝀 𝜵𝑻 + 𝑸
Material relationship of heat capacity, heat conductivity and density
𝛌 = 𝛂 𝝆 𝑪𝒑
Boundary conditions represent natural convective cooling with a heat transfer cofficient ℎ and a heat load as a space-homogeneous time dependent temperature function 𝑔
−𝛌 𝛁𝑻 = 𝒉 𝑻 − 𝑻𝒆𝒙𝒕
𝑻 = 𝒈
Comsol Interfaces: “Heat transfer module“ and “CAD Import module“
21.10.2015 Gerd Liebig / European Comsol Conference 2015 6
/ °C
/ °C
Experimental Study and Simulation Results
Temperature distribution [°C] in a prismatic cell at the experimental setting
Thermal stressing with the heat stamp for 60 s at a heat rate of 50 W
21.10.2015 Gerd Liebig / European Comsol Conference 2015 7
Validation
Temperature profiles and simulation errors for the experimental validation
Simulated data vs. Experimental data good agreement
A local peak temperature of 180 °C is reached at the jelly roll
21.10.2015 Gerd Liebig / European Comsol Conference 2015 8
Short-term Thermal Treatment / Laser Welding
Temperature propagation [°C] in the prismatic cell and the Jelly roll
Stress for 4 s at 1500 °C Jelly roll after 4 s
Conclusions and Outlook
A thermo-physical 3D model of a commercial lithium-ion cell was developed and validated.
Temperature distribution inside a lithium-ion cell during battery stackassembly were simulated.
Further studies on various stress scenarios representing battery stack assembly at elevated temperatures will be performed.
21.10.2015 Gerd Liebig / European Comsol Conference 2015 9
21.10.2015 10Gerd Liebig / European Comsol Conference 2015
Acknowledgements
Pamina Bohn
Dr. Lidiya Komsiyska
Dr. Stanislav Vasić