The Physics of the Nonlinear Optics of Plasmas at Relativistic Intensities for Short-Pulse Lasers.pdf

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    1942 IEEE JOURNAL OF QUANTUM ELECTRONICS, VOL. 33, NO. 11, NOVEMBER 1997

    The Physics of the Nonlinear Optics of Plasmas atRelativistic Intensities for Short-Pulse Lasers

    W. B. Mori

    (Invited Paper)

    AbstractThe nonlinear optics of plasmas at relativistic inten-sities are analyzed using only the physically intuitive processes oflongitudinal bunching of laser energy, transverse focusing of laserenergy, and photon acceleration, together with the assumptionof conservation of photons, i.e., the classical action. All that isrequired are the well-known formula for the phase and groupvelocity of light in plasma, and the effects of the ponderomotiveforce on the dielectric function. This formalism is useful when thedielectric function of the plasma is almost constant in the frameof the light wave. This is the case for Raman forward scattering(RFS), envelope self-modulation (SM), relativistic self-focusing(SF), and relativistic self-phase modulation (SPM). In the past,the growth rates for RFS and SPM have been derived in termsof wavewave interactions. Here we rederive all of the aforemen-tioned processes in terms of longitudinal bunching, transversefocusing, and photon acceleration. As a result, the physicalmechanisms behind each are made clear and the relationshipbetween RFS and envelope SM is made explicitly clear. Thisallows a single differential equation to be obtained which couplesRFS and SM, so that the relative importance between eachprocess can now be predicted for given experimental conditions.

    I. INTRODUCTION

    T

    HE nonlinear optics of plasmas was developed exten-

    sively in the early 1970s [1][4]. This development

    resulted in the identification of numerous so-called para-metric instabilities. Among these were Raman and Brillouin

    scattering, so-named because of their close connection to

    the processes which occur in unionized gases [5]. In these

    original analyses [1][4], the instabilities were formulated in

    terms of wavewave interactions and the ponderomotive force.

    Using this formalism, general dispersion relations were derived

    which can in principle be used to describe the evolution

    of arbitrary noise sources. These dispersion relations also

    described the well-known filamentation/self-focusing [4], [5],

    [7][9] and self-phase modulational instabilities [1][4], [9].

    Mechanisms which occur only when the laser oscillates the

    electrons at relativistic velocities were also identified in the

    early work by Max et al. [4]. However, the relativistic analyses

    were confined to the weakly relativistic limit. Almost all of the

    early work was undertaken because of its importance to laser

    Manuscript received August 22, 1996; revised July 1, 1997. This work wassupported by DOE under Grant DE-FG0392ER40727, LLNL under ContractB291465 and Contract B335241, and the National Science Foundation underGrant DMS-9722121.

    The author is with the Department of Electrical Engineering and theDepartment of Physics and Astronomy, University of California of LosAngeles, Los Angeles, CA 90095 USA.

    Publisher Item Identifier S 0018-9197(97)07828-7.

    fusion which utilized lasers with relatively long pulse lengths

    and modest intensities.

    With the advent of short-pulse laser technology [10], new

    applications [11][13] have evolved and the relevant insta-

    bilities of the lasers in plasmas has changed. As a result,

    there has been a large amount of new work in the field of

    the nonlinear optics of plasmas at relativistic intensities. For

    short-pulse lasers, the nonlinear optics of plasmas involves

    only electron motion because the ions are immobile during

    the transit time of the laser. This significantly limits thenumber of instabilities which can occur. The most important

    instabilities for short-pulse lasers are Raman forward scattering

    (RFS) [14][30], relativistic self-focusing (SF)[4], [31][33],

    and relativistic self-phase modulation (SPM) [4], [27]. Each

    of these instabilities can be described conventionally in terms

    of wavewave interactions [1][4], [18], [19], [23][27]. In

    each case, an incident electromagnetic wave at frequency

    decays into two forward moving electromagnetic sidebands at

    frequencies (the Stokes wave) and (the anti-

    Stokes wave). The frequency corresponds to modulations

    to the index of refraction. In RFS, , where is

    the plasma frequency, and an electrostatic plasma wave is

    generated. This instability is important because the phasevelocity of the plasma wave is nearly the speed of light. This

    allows the plasma wave to accelerate electrons to relativistic

    energies [11][13]. In filamentation and SPM, , and

    the modulation at is caused by relativistic mass corrections

    to the electrons motion.

    Recently, the importance of RFS type instabilities for short

    pulses was clearly demonstrated in fluid simulations [18][22].

    In these simulations, finite-width pulses were found to break

    apart axially into beamlets separated in time by roughly

    . Associated with this breakup was the generation of

    a large amplitude plasma wave. This clearly indicates the

    occurrence of some form of RFS. In explaining these results,

    one group developed a theory which described an envelope

    self-modulation for finite-width pulses [28], [29], and the other

    used a conventional Raman wavewave analysis [18], [19].

    The physical mechanism for the envelope self-modulation

    (SM) is as follows [13], [22], [28], [29]. First, the laser

    pulse creates a plasma wave wake noise source. Next, the

    density compressions and rarefactions of the plasma wave

    wake transversely focus and defocus laser energy. As a result,

    the laser spot size and hence intensity are modulated at nearly

    the plasma frequency and at nearly the wavenumber

    00189197/97$10.00 1997 IEEE

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    MORI: THE PHYSICS OF THE NONLINEAR OPTICS OF PLASMAS FOR SHORT-PULSE LASERS 1943

    . The ponderomotive force of the intensity modulation

    then excites a larger wake and the process feeds back on

    itself. Importantly, no mention is made of the light wave

    decaying into other light waves. It was subsequently shown

    that the differential equation and growth rate for this envelope

    SM are the same as those for RFS at small forward angles,

    [23][26]. It was also shown that the above

    physical picture is complicated by the fact that the intensity

    modulations and the density modulations are not resonantly in

    phase [23], [24] and that the envelope analysis cannot describe

    RFS in the exact or near forward direction,

    [23][26]. RFS in the near forward direction (very small

    angles) is distinct from SM by the phase relation between

    the density and intensity modulations. We will henceforth use

    RFS0 to mean scattering into the near forward direction. It has

    also been pointed out [23], [24], [34], [35] that plasma waves

    produced by RFS0 can also cause transverse focusing even

    when so-called SM has not occurred. In spite of all this new

    work to identify the various regimes of RFS, there is still some

    confusion and disagreement as to how RFS and envelope self-

    modulation are related and which mechanisms are importantfor given experimental conditions.

    In this paper, we present a formalism which hopefully

    removes some confusion. We analyze RFS0, envelope self-

    modulation (SM), self-focusing (SF), and self-phase modula-

    tion (SPM) all from the same set of physical phenomena. We

    do not use the concepts of Stokes and anti-Stokes waves, rather

    we calculate the modulation in laser intensity in terms of the

    physically intuitive phenomena of longitudinal bunching of

    laser energy, transverse focusing of laser energy, and photon

    acceleration [36], [37]. Each of these phenomena arise when

    modulations in the index refraction appear stationary in the

    light waves frame, i.e., the index of refraction has a relativistic

    phase velocity. The local index of refraction determines thelasers group and phase velocity. Longitudinal bunching (LB)

    is caused by longitudinal variations in the group velocity,

    transverse focusing (TF) is caused by transverse variations

    in the phase velocity, and photon acceleration (PA) is the

    change in local frequency caused by longitudinal variations

    in the phase velocity. Recall that both SF and envelope SM

    are typically explained in terms of transverse focusing of

    laser energy. We calculate the overall change in the waves

    amplitude from all of these effects, by assuming that photon

    number, i.e., action is conserved [1][4], [38]. An equation is

    then derived which relates the amplitude modulations to the

    modulations of the index of refraction. By combining these

    equations, we recover the exact growth rates for RFS0, SM, SFand SPM. Therefore, it is possible to precisely identify which

    phenomena causes which instability. In addition, because

    direct comparison between each phenomenon is now possible,

    we may now determine which instability is most important

    for given experimental conditions. We will argue that in all

    existing experiments [39][42] one-dimensional (1-D) and

    higher dimensional (2-D and/or 3-D) effects of RFS0 are more

    important than SM. In future experiments, in which shorter

    pulse lasers and lower plasma densities are used, then SM may

    dominate. Incidentally, these same physical phenemona can be

    applied to instabilities in other media so long as the index of

    refraction appears stationary in the light waves frame, i.e., the

    Stokes and anti-Stokes waves are both important.

    II. PHYSICAL PHENOMENA

    In this section, we begin by stating the basic assumptionsof this formalism and then describe how the waves amplitude

    can be changed by modulations to the index of refraction.

    A. Assumptions

    In an unmagnetized plasma, the index of refraction of a

    linearly polarized light wave is where

    , is the plasma density, and

    is the normalized vector potential of the incident laser,

    . A useful formula is 0.85 10 (W/cm ) ( m)

    where is the laser intensity and is the laser wavelength;

    is commonly referred to as . It is clear that the

    index of refraction can be altered by either modulating the

    plasma density, the laser amplitude, or the laser frequency. In

    this paper, we consider only small modulations and weakly

    relativistic pumps. Therefore, the index of refraction can beexpanded as

    (1)

    where is the normalized density perturbation, and

    represents averaging over the fast laser oscillations. In general,

    , so an expression for is

    (2)

    and an expression for is [43], [44]

    (3)

    Therefore, it is clear that both and can be modulated

    through changes in either density, laser intensity, or frequency.

    Note that when the relativistic term is included [43],

    [44].

    In addition, we assume that within a local volume the

    photon number, i.e., the classical action, is conserved. The

    conservation of the classical action in laser-plasma instabiliteshas been discussed extensively in the literature [1][4], [38],

    [45]; however, for completeness, we provide a derivation inAppendix A. Conservation of action can be stated as

    constant (4)

    where represents averaging over the fast oscillations, is

    the spot size, and is some initial longitudinal extent. The

    lasers vector potential can therefore be modulated by only

    three ways:

    1) modulate longitudinal bunching;

    2) modulate transverse focusing;

    3) modulate photon acceleration.

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    MORI: THE PHYSICS OF THE NONLINEAR OPTICS OF PLASMAS FOR SHORT-PULSE LASERS 1945

    Fig. 2. A physical picture for photon acceleration.

    III. GROWTH RATES

    In this section, we consider specific modulations to andand derive the growth rates for each instability.

    A. Raman Forward Scattering

    In order to derive growth rates, we need to identify how the

    index of refraction is being modulated. In the 1-D limit, the

    laser intensity can only be modulated from either longitudinal

    bunching or photon acceleration. This is illustrated in Fig. 3.

    Therefore, can be written as

    (17)

    and evolves in time as

    (18)

    Substituting (9) and (16) into (18) gives

    (19)

    In RFS0, the modulations to , i.e., and , are solelythe result of modulations to . Therefore, from (2) and (3)

    we can rewrite (18) as

    (20)

    It is of interest to note that longitudinal bunching and photon

    acceleration contribute equally to the modulation of . We

    define and

    where depends slowly with both and , to obtain

    (21)

    Therefore, in RFS0 the modulations to are out of

    phase with the density response, . In order to derive

    a growth rate, we need an equation which describes how

    Fig. 3. A physical picture for RFS0. RSF0 is due to equal amounts oflongitudinal bunching and photon acceleration.

    modulations to cause density perturbations. This is well

    known to be a harmonic oscillator equation of the form [1][4]

    (22)

    where the right-hand side is the divergence of the ponderomo-

    tive force. In the speed of light variables, this becomes

    (23)

    which can be rewritten as

    (24)

    where

    and depends slowly on . In reducing (23) to (24), we are

    not considering the strongly coupled (others call it the short-

    pulse) regime of RFS0 [13], [18], [19], [23][26], [28][30],

    because we are interested in the portions of the pulse with themost -foldings. Combining (24) with (21) gives

    (25)

    where . This is identical to [25, eq. (10)]

    which was obtained from the conventional wavewave anal-

    ysis using Stokes and anti-Stokes sidebands. It describes

    the so-called four-wave resonant regime. Therefore, we have

    shown that in RFS0 the density modulations of the plasma

    wave are out of phase with , and the perturbations

    to are caused equally by longitudinal bunching and photon

    acceleration. The longitudinal bunching is caused by the

    changes to . Note that the changes to from photon

    acceleration also change but these modulations do not have

    the correct phase to be reinforced.

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    1946 IEEE JOURNAL OF QUANTUM ELECTRONICS, VOL. 33, NO. 11, NOVEMBER 1997

    Fig. 4. The physical picture for relativistic SPM, which is photon accelera-tion followed by longitudinal energy bunching.

    Equation (24) can be solved in closed form for specified

    boundary and initial conditions [23][26]. Here, we simply

    give its asymptotic solution which is

    (26)

    As noted earlier, this growth corresponds to four-wave res-

    onant RFS0 and more research is required to obtain the

    four-wave nonresonant growth of RFS0 using these simple

    physical pictures.

    B. Relativistic Self-Phase Modulation

    In relativistic self-phase modulation, the index of refraction

    is modified by the relativistic term in (2). This leads

    to a modulation in from photon acceleration. However,unlike RFS0, the modulation to which results from this

    does not have the correct phase to reinforce the original

    perturbations of . Instead the modulation of causes

    to vary, causing energy to bunch longitudinally. This is

    illustrated in Fig. 4. This is a two-step process and this is why

    SPM has a lower growth rate than RFS.

    To calculate the growth rate, we first write the change in

    from only longitudinal bunching,

    Therefore, evolves in time as

    (27a)

    Substituting (9) into (27a) gives

    (27b)

    Assuming that the changes in are due to the term in

    (3) results in

    (28)

    where we have substituted .

    Differentiating (28) with respect to time leads to

    (29)

    The evolution of with time is given by (16) provided

    that the modulations in phase velocity are the result of the

    relativistic term in (2). This results in

    (30)

    which upon substitution into (29) gives

    (31)

    If then

    grows in time as

    (32)

    Thus, it would appear that grows exponentially intime with a growth rate which increases indefinitely

    with . Note that if this is times smaller

    than the RFS0 growth rate. In reality, there is a term which

    balances this growth for large . To understand this, we must,

    for the moment, realize that the intensity modulation can be

    represented as the superposition of a pump at frequency and

    two sidebands at . The two sidebands cannot both be

    exactly resonant because the linear dispersion relation of light

    is quadratic, i.e., . Therefore the beat pattern of

    is not stationary in the light waves frame, but appears

    to have a real frequency. A real frequency term would appear

    on the right-hand side of (32) but with the opposite sign.To calculate the effective frequency, we assume that is

    of the form

    (33)

    where and. We assume the s are the

    same, and that to obtain

    (34)

    Using a trigonometric identity, this can be rewritten as

    (35)

    Using the definitions for the s gives

    (36a)

    and

    (36b)

    Therefore, consists of a beat pattern moving at the

    speed of light times a temporal oscillation which means that in

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    MORI: THE PHYSICS OF THE NONLINEAR OPTICS OF PLASMAS FOR SHORT-PULSE LASERS 1947

    the speed of light frame, oscillates at . Since

    is the same for both the Stokes and anti-Stokes waves, we

    can Taylor expand about to find

    (37a)

    and

    (37b)

    Therefore, dispersion leads to

    (38)

    Since in the absence of any growth must oscillate at this

    frequency, we can add

    (39)

    to the right-hand side of (32) to obtain the final equation for

    relativistic SPM

    (40)

    Therefore, the threshold for instability is and

    the maximum growth rate is

    (41)

    and it occurs for

    These results are in agreement with [4]. Therefore, the

    physical picture of SPM is as follows. It requires first for the

    frequency, i.e., the phase, of the wave to be modulated and

    second for the laser energy to bunch longitudinally because

    of the group velocity modulations associated with the changes

    in . It is due to the relativistic corrections to , not to .

    This physical picture was given qualitatively in [4]. Note that

    the other mechanisms which modulate the laser amplitude do

    not have the correct phase to be reinforced. In particular, the

    relativistic terms in do not lead to an instability, but rather

    to group velocity steepening.

    C. Relativistic Self-Focusing

    In the next two sections, we consider the effects of trans-

    verse focusing. We begin with relativistic self-focusing and

    show that our physical arguments for deriving an equation for

    the evolution of the spot size yield the exact SF equation.

    We start from (12) and assume that varies only from the

    relativistic term in (2) to get

    (42)

    This is not the whole story since is the absence of variations

    the spot size increases because of diffraction. Therefore, we

    need to add the diffractive term on the right-hand side of (42).

    The diffractive term in SF is analogous to the dispersion term

    in SPM. The evolution of the spot size from diffraction for a

    Gaussian beam is well known to be [5]

    (43)

    where is the Rayleigh or diffraction time,

    is the laser wavelength, and is the spot size

    at the focus. In Section II-C, we considered nearly planar

    wavefronts, i.e., regions near the focus. Near the focus, (43)

    can be differentiated twice to get

    (44)

    Adding this term to the right-hand side of (42) yields

    (45)

    Therefore, self-focusing occurs if the term in brackets is

    negative. The threshold condition for SF is therefore

    (46)

    This is identical to the result obtained from more formal and

    more complicated derivations using source-dependent expan-

    sions [48], [49] or variational techniques [50]. We emphasize

    that in the derivation presented in Section II-C the position of

    the outer position of the wavefront was somewhat arbitrarily

    assumed to be one spot size away from the axis. The more

    rigorous derivations must therefore be done at least once.The threshold condition is in terms of the product ,

    which is proportional to the laser power. Therefore, (46) can

    be viewed as a power threshold condition where

    the critical power is [31]

    GW (47)

    Note that if only transverse focusing occurs that is a

    constant, i.e., the laser power is conserved.

    D. Envelope SM (Laser Sausaging)

    Transverse focusing can also be caused if the index ofrefraction is varied by the density pertubation term in (12).

    In this case, (12) reduces to

    (48)

    Note that if is negative, focusing occurs while, if

    is positive, defocusing occurs. In order to couple the evolution

    of the spot size to that of the density pertubation, we need to

    relate to . From (5)

    (49)

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    1948 IEEE JOURNAL OF QUANTUM ELECTRONICS, VOL. 33, NO. 11, NOVEMBER 1997

    from which it follows

    (50)

    Equation (50) combined with (23) completely describes enve-

    lope SM, and as before we are not considering the strongly

    coupled regime. Using the same definitions as before for the

    field envelopes gives

    (51a)

    (51b)

    Combining (51a) and (51b) gives a single equation for :

    (52)

    We rewrite the right-hand side in terms of and to get

    (53)

    This is identical to the equation obtained by differentiating [28,

    eq. (4)] with respect to , which was derived using the source-

    dependent expansion method. This differential equation has no

    closed form solution. However, using saddle point integration

    techniques, the asymptotic form for the solution can be shownto be [23][26], [28], [29]

    (54)

    Before proceding, there are several points to make. First,appears in the differential equation because of the

    choice for normalizing the parameters; the relativistic SF terms

    have been neglected. We will comment more on this shortly.

    Second, an identical differential equation and hence asymptotic

    solution was derived using a conventional wavewave RFS

    analysis [23], [24] for scattering angles of .

    Therefore, the scattered light is not in the direct forwarddirection but is at well-defined angles. This results in the

    generation of higher order Gaussian modes. Third, in SM,

    only transverse focusing and defocusing occurs. The intensity

    modulations arise from reductions and increases in the spot

    size, so sometimes SM is referred to as laser sausaging

    due its analogy with an electron beam instability. Fourth,the asympotic solution also has an imaginary part to the

    phase, which means that the density pertubation and intensity

    modulations are not out of phase [23], [24], and the phase

    velocity of the plasma wave gradually decreases in time [25],

    [26]. The decrease in phase velocity means that SM is less

    likely to generate ultrarelativistic electrons. Last, transverse

    focusing is not equivalent to SM, it can also occur during

    RFS0. Since in RFS0, and are still out of

    phase, transverse focusing leads to contour shapes in which

    one-half is narrow and the other half is wide. These shapes

    have been refered to as inverse D shapes [24], [34], [35]. This

    Fig. 5. The effects of TF from RFS0 without SM. If n and p

    are = 2 outof phase and the wave is moving to the right, then intensity contours becomeinverse D-shaped, so a signature of transverse focusing in RFS0 is inverseD-shaped contours.

    is shown in Fig. 5, and such shapes cannot be generated inthe SM process.

    Envelope SM is directly related to RFS in the so-called

    four-wave nonresonant regime and is distinct from RFS0.

    The term nonresonant refers to the fact that because of the

    extra phase shift, the plasma wave does not oscillate

    at exactly . The difference between four-wave nonresonant

    RFS0 and SM lies in which term dominates in the mismatch

    quantity of [23], [24], i.e., if then RFS

    dominates. Similar conclusions were independently reached by

    Andreev et al. [25], [26]. In the nonresonant regime of RFS,

    multiple cascading is less likely to occur [25], [26], [34], [35],

    [51]. Therefore, an experimental diagnostic of RFS0 is the

    observation of strong multiple cascading.In the original SM paper by Esarey et al. [28], [29], it

    was indicated that relativistic SF was critical to envelope SM.

    They stated that needed to be larger than roughly 1/2

    (depending on the sharpness of the rise time) in order for

    strong SM to occur. We believe this to depend on the parameter

    space under consideration. In the preceding analysis and in the

    conventional wavewave analyses [23][26], the relativistic

    SF terms have been neglected. This assumption is valid so long

    as the spot size changes little from SF or diffraction before the

    instability saturates. In particular, it is obvious from (53) that

    for any given value of a pulse length can be chosen such

    that SM (or RFS0) can still occur within a Rayleigh time. In

    PIC simulations, beam breakup is observed even for0.5 [51][53].

    The SF and diffraction terms can easily be included by

    combining (45) and (48) to get

    (55)

    Combining (54) with (49) now gives

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    MORI: THE PHYSICS OF THE NONLINEAR OPTICS OF PLASMAS FOR SHORT-PULSE LASERS 1949

    If a matched beam is assumed, i.e., , or equivalently

    a preformed channel is used [20], [21], then the equations

    given earlier in this section are still valid. The physical

    mechanism of the instability is not due to relativistic SF,

    but rather is completely due to transverse focusing in plasma

    waves. The inequality, , can be important if

    relativistic guiding is required to increase the interaction length

    beyond several Rayleigh lengths.

    IV. COMPARISON BETWEEN RFSAND ENVELOPE SELF-MODULATION

    In the previous section, we carefully described the differ-

    ences between longitudinal bunching (LB), photon accelera-

    tion (PA), and transverse focusing (TF). We also showed that

    when these processes are caused by plasma waves, they lead

    to RFS0 and SM. In this section, we make detailed compar-

    ison between the relative importance of the 1-D phenomena

    (LB and PA) and the 2-D phenomenon (TF), with particular

    emphasis given to discerning which processes dominate for

    given experimental conditions.

    For simplicity, we begin by assuming a constant amplitudeplasma wave and compare the relative contributions to

    from 1-D and 2-D effects. This simple exercise is very illus-

    trative and it has direct implications to beat wave excitation of

    plasma waves where the plasma wave amplitude changes little

    in . Focusing in constant amplitude plasma waves is related

    to cascade focusing [54]. If is constant in at a value

    , then (21) and (50) can be integrated in to give

    (56a)

    and

    (56b)

    It is immediately clear that grows as while

    grows as . The reason is that TF is a two-step

    process which requires the wavefronts to first curve before

    energy can be focused. Therefore, the 1-D effects always

    dominate early in time while transverse focusing dominates

    late in time. In terms of the magnitudes of (note the

    phases are different), the transition occurs when

    (57)

    For tenuous plasmas, i.e., , this is typically a

    small number. In beatwave excitation, is generally so

    low, and the interaction time so large that TF almost alwaysdominates. From (56b), 100% modulations to occur

    within a Rayleigh length from TF when is near unity.

    This could have deleterious consequences to the multiple pulse

    excitation process [55][58] since it requires accurate phase

    relationships to be maintained between each subsequent pulse.

    On the other hand, in single-frequency experiments, the

    RFS0 instability may have saturated before the transition to

    the TF dominated regime occurs. In this case SM, which is

    entirely the result of TF, may not occur. We reiterate that TF

    can occur in RFS0. The signature for the SM regime is not

    that TF occurs, but that the phase shift between and

    be , and that TF dominates. To be more precise,

    we next derive a differential equation which couples both the

    1-D and 2-D effects and then calculate its asymptotic response.

    This equation does not include the nonresonant regime of

    RFS0, which is reasonable if , i.e., small

    [23], [26].If this inequality is not satisfied, then RFS0 always

    dominates.

    We start by defining , where

    the subscript stands for total. Therefore,

    (58)

    and we substitute (21) and (50) into the right-hand side to get

    (59)

    Substituting the earlier definitions for and and (24)

    into (59) gives

    (60)

    where we have defined and . Note that

    if (no TF) we recover (25) while if (no LB

    or PA) we recover (52).

    Equation (60) cannot be solved exactly. However, we can

    calculate its asymptotic behavior from stationary phase argu-

    ments. We assume solutions of the form for

    and obtain the dispersion relation

    (61)

    The stationary phase conditions are

    (62a)

    and

    (62b)

    The solutions to (62b) can be seperated into two regimes

    depending on whether the parameter is large

    or small compared to unity. In the small limit

    (63)

    Substituting (63) and (62a) into the phase factor

    leads to the asymptotic behavior

    (64)

    In the opposite limit where is small,

    (65)

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    MORI: THE PHYSICS OF THE NONLINEAR OPTICS OF PLASMAS FOR SHORT-PULSE LASERS 1951

    electrons because the phase velocity of the plasma wave it

    generates has a spatio-temporal-dependent phase velocity.

    We close this section with a few comments. First, this

    analysis is only stricly valid for and for times before

    saturation occurs. In some of these experiments, ,

    and this can lower the growth rate [23][26]. Second, the

    asymptotic solutions have restrictions. The front part of the

    pulse, i.e., smaller values of , makes a transition to SM

    earlier than the back of the pulse. This will obviously effect

    how the back of the pulse evolves. The asymptotic solutions

    given here only include the stationary phase part. Saddle point

    integration provides other factors to the asymptotic solutions.

    Third, the theory assumes diffraction-limited beams, while

    the beam quality varies from experiment. Last, the time of

    saturation and the transverse profile depends on the noise

    source. There have already been several types of noise sources

    which have been identified [22], [25], [26], [34], [35], [38],

    [51][53]. Therefore, to understand current experiments, PIC

    simulations [34], [35], [51][53] are required. These indicate

    that RFS0 plays an important role and that the dominant

    saturation mechanism is wavebreaking. It is worthwhile tonote that some of these PIC simulations were carried out

    before many of the above experiments and that many of theirpredictions have been born out in the subsequent experiments.

    VI. SUMMARY AND FUTURE WORK

    In this paper, we have given simple physical pictures

    for the nonlinear optics of plasmas at relativistic intensities.

    Here, relativistic refers to either the electrons oscillating at

    relativistic energies or the plasma dielectric function having

    a relativistic phase velocity. In particular, Raman forward

    scattering (RFS0), envelope self-modulation (SM), relativis-

    tic self-focusing/filamentation (SF), and relativistic self-phasemodulation (SPM) were analyzed. The analyses used only the

    concepts of longitudinal bunching (LB), transverse focusing

    (TF), and photon acceleration (PA), together with the as-

    sumption of conservation of photons, i.e., the classical action.

    Using just these concepts and the well-known phase and group

    velocity of light, the growth rates for RFS0, SM, SF, and SPM

    were rederived.

    Direct comparison between each instability is now possible

    because they were derived from the same set of physical

    phenomenon (although the derivations are not rigorous). It wasshown that RFS0 is caused by equal amounts of LB and PA

    (both are 1-D effects). On the other hand, SPM is caused by

    PA followed by LB. It is therefore a two-step process so ithas a lower growth rate than RFS0. It was also shown that

    SF is caused by TF from relativistic mass corrections to the

    light waves phase velocity. Finally, SM is the result of TF

    in a nonresonant plasma wave. Importantly, it was shown

    that TF in RFS0 generated plasma waves is not the same as

    SM. A comparison between RFS0 and SM showed that in

    self-trapped electron experiments RFS0 plays a key role. This

    could change in future experiments.

    We close with a few remarks regarding future work. This

    analysis is only strictly valid in the weakly relativistic limit,

    . Based on the success of this weakly relativistic

    analysis, it seems worthwhile to try and extend it to the fully

    relativistic limit, . This will require precise knowledge

    of the fully nonlinear phase and group velocities of light in

    plasmas. To date we have not made a successful treatment

    for . Another area to investigate is the role of photon

    acceleration during SPM. In particular, a modulation to

    could lead to a from PA, which in turn could lead to

    further modulations to from PA. This two-step process

    was neglected in Section II-B, but it may be important. Still

    another area for future research is implementing hosing and the

    nonresonant regime of RFS0 into these physical pictures. Last,

    we point out that this analysis not only allows one to rederive

    known growth rates, it also makes it possible to identify new

    processes and to properly analyze old problems. For example,

    it is possible for SF to occur because of transverse variations

    to caused by PA [61], and the phenomenon of resonant

    relativistic self-focusing [33] can be coupled to SM [62].

    Note Added in Proof: The field of nonlinear optics of plas-

    mas is still developing rapidly, as illustrated by the numerous

    experimental results on electron acceleration which have been

    obtained since the original submission data, e.g., [63][65].

    APPENDIX A

    LOCAL ACTION CONSERVATION

    In this paper, we have assumed that the action, i.e., photon

    number, is conserved locally. In this appendix, we derive alocal conservation law for the action using similar reasoning

    as others when they derived a global conservation law [38],

    [45]. We begin with the basic quasi-static equation for the

    normalized vector potential

    (A1)

    where and are the speed of light frame

    variables defined in the paper. Next, we assume to be of the

    form to obtain the envelope equation

    (A2)

    We next define the operator

    and take the linear combination of (A2)

    to get

    (A3)

    To obtain a global conservation law, (A3) can be integrated

    over all space, i.e., ; but to obtain the more powerful

    local conservation law, we need to rewrite several terms in

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    1952 IEEE JOURNAL OF QUANTUM ELECTRONICS, VOL. 33, NO. 11, NOVEMBER 1997

    terms of complete derivatives. The first two terms of (A3) can

    be combined as

    (A4)

    which can be rewritten as

    (A5)

    The third term of (A3) can also be rewritten as a complete

    derivative

    (A6)

    Recombining (A5) and (A6) gives a local conservation law in

    the coordinates

    (A7)

    Integrating (A7) over and gives the global conservation

    law

    (A8)

    The term in brackets can be identified as the action by

    rewriting ; substituting this form for

    into the term in brackets in (A8) gives

    (A9)

    which is times the action, , since is the

    instantaneous frequency.

    A local conservation of law of a quantity, , has the generic

    form

    (A10)

    where is the flux of and is the flow velocity of .

    Therefore, we can interpret

    (A11)

    and

    (A12)

    Note, to lowest order the velocity of the action is equal to

    the group velocity of light, so in the speed of light frame

    and . Using these

    definitions, it is straightforward to verify that interpretations

    (A11) and (A12) are correct.

    In conclusion, in this Appendix, we have derived the local

    conservation law

    (A13)

    and have given arguments that it is a conservation law for theaction.

    ACKNOWLEDGMENT

    The author acknowledges useful discussions with K.-C.

    Tzeng and Dr. T. Katsouleas, Dr. C. D. Decker, Dr. C. Joshi,

    Dr. J. M. Dawson, Dr. E. Esarey, and Dr. G. Shvets.

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