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Understanding the Influence of Biomass Burning on Tropospheric Ozone through Assimilation of TES data
Jennifer Logan Harvard University
Dylan Jones, Mark ParringtonUniversity of Toronto
Kevin Bowman, Helen Worden, John Worden, Greg OstermanJet Propulsion Laboratory
California Institute of Technology
Impact of Biomass Burning on Tropospheric O3
TES CO, 421 mb: Nov 4-17, 2004 TES O3, 421 mb: Nov 5-17, 2004
GEOS-Chem CO 421 mb: Nov 4-17, 2004 GEOS-Chem O3, 421 mb: Nov 4-17, 2004
Climatological emission inventory in the model underestimates the impact biomass burning on CO and O3 in the southern hemisphere
ppb ppb
Objective: Assess the potential of TES data to improve O3 in the model in a chemical data assimilation framework
Impact of Assimilation on CO and O3 (using a sequential sub-optimal
Kalman filter with TES O3 and CO profile retrievals for Nov. 4-17, 2004)
Change in O3 at 7 km (assim. - without assim.)
24-hr averaged assimilated O3 at 7 km on Nov. 17
(ppb CO)
percent
• Assimilation increases CO throughout the southern hemisphere• Largest increases in O3 (20-50%) are over the Indian Ocean and the
Indonesian/Australian region
(ppb O3)
percent
24-hr averaged assimilated CO at 7 km on Nov. 17
Change in CO at 7 km (assim. - without assim.)
Assimilation of TES O3 for 1 July 2005 - 1 Jan. 2006
Assimilation
Free running model
O3 difference: assimilation - free running model
data gaps
Mean GEOS-Chem O3 at 8 km between 20°S-equator and 180°W-180°E
• In early Sept 2005 the assimilation increases O3 by about 20% in upper troposphere
• During the 2 week data gap in September the analysis reverts to the state of the free running model
Comparison with Ozonesonde Data at La Reunion Island (21°S, 55°E)
12 Oct 2005 17 Oct 2005 28 Oct 2005
2 Nov 2005assimilation
free running model
sonde
• The ozone tropopause in GEOS-Chem is too low in Austral spring 2005 compared to the sonde data
• Assimilation of TES data reduces the bias in the model
Comparison of the O3 Analysis with TES Observations (350 mb)
• During October the assimilation reduces the bias in the model by about a factor of 2
• Despite the reduction in the bias, the residuals for the OmA are still large
Obs minus Forecast
Obs minus Analysis
Comparison of the CO Analysis with TES Observations (350 mb)
• Following the warm-up of the TES optical bench in Dec. 2005, the assimilation significantly reduced the bias in CO in the model
• In contrast to the O3 analysis, the CO OmA residuals are small, reflecting the longer lifetime of CO
Obs minus Forecast
Obs minus AnalysisTES OB warm-up
Assimilation extended through 1 Sept 2006
Latitudinal Dependence of the O3 Analysis Residuals (350 mb)
The assimilation has less impact in summer 2006 because we are propagating the forecast error variance without accounting for forecast error growth by summer 2006 the forecast error is about 15% in the tropics and subtropics, compared to the assumed 50% error in July 2005
Larger OmA residuals in the tropics, reflecting the shorter O3 lifetime and a lower density of TES data
20°S-0°
30°N-60°N
Obs minus Forecast
Obs minus Analysis
Conclusions
•Assimilation of TES O3 data produces a much improved distribution of O3 in the model, which provides greater constraints on model parameters such as the lifetime of NOx a better constraint on the NOx lifetime will result in improved estimates of NOx emissions from lightning and of the export of NOy from continental source regions
•In contrast to the CO analysis, the residuals in the O3 assimilation are large, especially in the tropics, reflecting the shorter lifetime of O3 (and the low density of the TES data) assimilating trace gases that are more chemical active than CO will be a challenge
•A better approach for exploiting the satellite data would be to optimize the model parameters, such as the emissions, using adjoint techniques work is needed to characterize the forecast errors across the range of chemical timescales in the model