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SFB Coherent Control of Quantum Systems UNIVERSITY OF INNSBRUCK IQOQI AUSTRIAN ACADEMY OF SCIENCES Sebastian Diehl IQOQI Innsbruck 3-Body Interactions from 3-Body Loss: 2 Applications Condensed Matter Theory Seminar August 30, 2010 Universitaet Koeln Collaboration: Misha Baranov (Innsbruck) Jake Taylor (NIST) Andrew Daley (Innsbruck) Antonio Privitera (Frankfurt) Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011

3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

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Page 1: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

SFBCoherent Control of Quantum

Systems

UNIVERSITY OF INNSBRUCK

IQOQIAUSTRIAN ACADEMY OF SCIENCES

Sebastian DiehlIQOQI Innsbruck

3-Body Interactions from 3-Body Loss: 2 Applications

Condensed Matter Theory SeminarAugust 30, 2010

Universitaet Koeln

Collaboration:Misha Baranov (Innsbruck) Jake Taylor (NIST)Andrew Daley (Innsbruck) Antonio Privitera (Frankfurt)Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt)Adrian Kantian (Geneva)

Monday, August 29, 2011

Page 2: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Outline

(0) Dissipative generation of a 3-body hardcore interaction

(1) Phase diagram for 3-body hardcore bosons

A. Kantian, M. Dalmonte, SD, W. Hofstetter, P. Zoller, A. J. Daley, Phys. Rev. Lett. 103, 240401 (2009)A. Privitera, I. Titvinidze, SD, A. J. Daley, W. Hofstetter, to be submitted (2010)

(2) 3-component fermions close to a loss resonance

A. J. Daley, J. Taylor, SD, M. Baranov, P. Zoller, Phys. Rev. Lett. 102, 040402 (2009)

• Mechanism and experimental perspectives

• Unique effects of interactions and the constraint

• constrained induced phase separation and superfluid in Lithium systems

0.0 0.5 1.0 1.5 2.08

6

4

2

0

SD, M. Baranov, A. J. Daley, P. Zoller, Phys. Rev. Lett, 104, 165301(2010); SD, M. Baranov, A. J. Daley, P. Zoller , Phys. Rev. B 82, 064509 (2010); Phys. Rev. B 82, 064510 (2010)

Monday, August 29, 2011

Page 3: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Motivation

• 3-body loss processes (-)

• ubiquitous, but typically undesirable• inelastic 3 atom collision• molecule + atom ejected from lattice

• 3-body interactions (+)

• Stabilize bosonic system with attractive interactions• interesting many-body consequences• 3-component fermion system: stabilize atomic color superfluidity

We make use of strong 3-body loss to generate a 3-body

hard-core constraint

iγ3→ γ3

Monday, August 29, 2011

Page 4: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Effective 2-body interactions (Rempe, Duerr, MPQ):

Effective 3-body interactions:

• Observation for 2-body interactions (Feshbach molecules) N. Syassen et al., Science 320, 1329 (2008) J. J. Garcia-Ripoll et al., New J. Phys. 11, 013053 (2009) S. Dürr et al., Phys. Rev. A 79, 023614 (2009)

Related work

Monday, August 29, 2011

Page 5: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

3-body interactions via 3-body loss

A. J. Daley, J. Taylor, SD, M. Baranov, P. Zoller, Phys. Rev. Lett. 102, 040402 (2009)

Monday, August 29, 2011

Page 6: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

!

|0|1

|e

J = |1e|

An analogy: optical pumping

ddt

ρ = −i[H, ρ] + L[ρ]

H =Ω2

(|0e| + |e0|) − ∆|ee|

L[ρ] = Γ

JρJ† − 12(J†Jρ + ρJ†J)

master equation in Lindblad form

with

Γ0→1eff =

Ω2

4∆2 + Γ2Γ

Γ0→1eff ≈ Ω2

4∆2Γ

Γ0→1eff ≈ Ω2

Γ

pumping rate (for )Ω Γ,∆

0 2 4 6 8 10 12 14 16 18 200

0.0025

0.005

0.0075

0.01

Γ/∆0 205 15

Γ0→1eff

Zeno regime: system frozen in |0

• system “freezes” in |0>• leading correction is effective small loss rate 0 -> 1

Γ

Γ0→1eff

large :Γ0→1eff ≈ Ω2/Γ

Monday, August 29, 2011

Page 7: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

0 2 4 6 8 10 12 14 16 18 200

0.0025

0.005

0.0075

0.01

!

|0|1

|e

Analogy to three-body loss

Γ3J

2U

J

!

2U

Γ3

Jdetuning

Rabi frequencydecay rate

onsite interaction energytunnel coupling

0 205 15Γ3/2U

three-body recombination rate

• system “freezes” in subspace with fewer 3 particles per site: 3-body constraint

• stabilizes against particle loss: effective loss rate

Γeff

Γeff

Γeff

Γeff ≈ J2

Γ3

Γeff ≈ J2/Γ3

For , realization of a Bose-Hubbard-Hamiltonian with three-body hard-core constraint on time scales t < 1/Γeff

Γ3 U, J

Monday, August 29, 2011

Page 8: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Physical Realization in Cold Atomic Gases•Estimate loss rate for Cesium close to a zero crossing of the scattering length

(e.g. Naegerl et al.)

• Preparation of the ground state of constrained Hamiltonian: • role of heating effects due to residual particle loss• Approach: Exact numerical time evolution of full Master Equation in 1D;

combine DMRG method with stochastic simulation of ME• Find optimal experimental sequence to avoid heating

|U|

J

γ3

lattice depth

3-body loss can be made the dominant energy scale

Monday, August 29, 2011

Page 9: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Ground State Preparation•Start from Mott ground state in superlattice •Loss causes heating, inhibits reaching ground state

“lucky” trajectory “unlucky” trajectory

“Probabilistic” ground state preparation

Ramp: Superlattice, V/J=30 to V/J=0,

N=M=20

Monday, August 29, 2011

Page 10: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Phase Diagram for Three-Body Hardcore Bosons

microscopic thermodynamic long distance

interactions interactionscondensation

interactionscondensationspin waves

0.0 0.5 1.0 1.5 2.08

6

4

2

0

SD, M. Baranov, A. J. Daley, P. Zoller, Phys. Rev. Lett, 104, 165301(2010); SD, M. Baranov, A. J. Daley, P. Zoller , Phys. Rev. B 82, 064509 (2010); Phys. Rev. B 82, 064510 (2010)

Monday, August 29, 2011

Page 11: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Physics of the constrained Hamiltonian

• The constrained Bose-Hubbard Hamiltonian stabilizes attractive two-body interactions

• Qualitative picture for ground state: Mean Field Theory • homogenous Gutzwiller Ansatz for projected on-site Hilbert space

• Gutzwiller energy

|Ψ = ∏i

|Ψi |Ψi = f0|0+ f1|1+ f2|2

E(rα,φα) = Ur22− JZr2

1

r2

0 +2√

2r2r0 cosΦ+2r22

Φ = φ2 +φ0−2φ1

fα = rαeiφα

PHP =−J ∑i, j

b†ib j +

U

2 ∑i

ni(ni−1) & b†i

3 ≡ 0

U < 0

Monday, August 29, 2011

Page 12: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Mean Field Phase Diagram

• Phase transition reminiscent of Ising (cf Radzihovsky& ʻ03; Stoof, Sachdev& ʻ03):

b = 0, b2 = 0

b = 0, b2 = 0

b ∼ expiθ b2 ∼ exp2iθ

Spontaneous breaking of Z_2 symmetry of the DSF order parameterθ→ θ+π

Uc

Jz=−2

1+n/2+2

n(1−n/2)

critical interaction strength:

210-10

-5

5

0

10

MI

z

• Two symmetry breaking patterns occur:

- Conventional SF

- “Dimer SF”

U/

Monday, August 29, 2011

Page 13: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Beyond Mean Field Phase Diagram• Why?

• Mean Field Theory (MFT) misses out physics at various length scales

Tied to interactions Tied to the constraint

• How?• MFT is a classical field theory • Find a means to requantize this MFT: classical field theory -> quantum field theory

• exact mapping of the constrained Hamiltonian to a coupled boson theory with polynomial interactions• the bosonic operators find natural interpretation in terms of “atoms” and “dimers”

microscopic thermodynamic long distance

n =k3

F3π2 ,T

kld n1/3,T 1/2,ε1/2MεM =− 1

Ma2

“atoms” “dimers”

We have identified several quantitative and qualitative effects:

Monday, August 29, 2011

Page 14: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Implementation of the Hard-Core Constraint

• Introduce operators to parameterize on-site Hilbert space (Auerbach, Altman ʻ98)

t†α,i|vac = |α, α = 0,1,2

• They are not independent:

∑α

t†α,itα,i = 1

• Representation of Hubbard operators:

a†i =√

2t†2,it1,i + t†

1,it0,i

ni = 2t†2,it2,i + t†

1,it1,i|vac

|0

|1|2

t†1,it0,i

Action of operators

a†i

Monday, August 29, 2011

Page 15: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Hkin =−J ∑i, j

t†1,it0,it

†0, j

t1, j +√

2(t†2,it1,it

†0, j

t1, j + t†1,it0,it

†1, j

t2, j)+2t†2,it

†1, j

t1,it2, j

• Hamiltonian:

Hpot =−µ∑i

2t†2,it2,i + t

†1,it1,i +U ∑

i

t†2,it2,i

• Mean field: Gutzwiller energy (classical theory)• interaction: quadratic• hopping: higher order • One phase is redundant: absorb via local gauge transformation

• Role of interaction and hopping reversed• Strong coupling approach facilitated

Implementation of the Hard-Core Constraint

• Properties:

t1,i → exp−iϕ0,i t1,i, t2,i → exp−iϕ0,i t2,it1,i = expiϕ0,i |t0,i|

e.g. t_0 can be chosen real

Monday, August 29, 2011

Page 16: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Implementation of the Hard-Core Constraint• Resolve the relation between t-operators (zero density)

t†1,it0,i = t†

1,i

1− t†

1,it1,i− t†2,it2,i → t†

1,i(1− t†1,it1,i− t†

2,it2,i)

• justification: for projective operators one has from Taylor representation

X2 = X → f (X) = f (0)(1−X)+X f (1) X = 1− t†1,it1,i− t†

2,it2,i

• Now we can interpret the remaining operators as standard bosons:

Hi = |n1i |m2

i , n,m = 0,1,2, ...

Hi = Pi⊕Ui

Pi = |01i |02

i , |11i |02

i , |01i |12

i

• on-site bosonic space

• decompose into physical/unphysical space:

• the Hamiltonian is an involution on P and U:

H = HPP +HUU

• remaining degrees of freedom: “atoms” and “dimers” similarity to Hubbard-Stratonovich transformation

|01i

|11i

|21i

|22i|12

i|02i

“ato

ms”

“dimers”

• correct bosonic enhancement factors on physical subspace √

n = 0,1

Monday, August 29, 2011

Page 17: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

• The partition sum does not mix U and P too:

Z = Tr exp−βH = TrPP exp−βHPP +TrUU exp−βHUU

Implementation of the Hard-Core Constraint

• Usually: Effective Action shares all symmetries of S• Here: symmetry principles are supplemented with a constraint principle

• Legendre transform of the Free energy

• Need to discriminate contributions from U and P: Work with Effective Action

Γ[χ] =−W [J]+Z

JT χ, χ≡ δW [J]δJ

• Has functional integral representation:

W [J] = logZ[J]

Quantum Equation of Motion for J=0

S[χ = (t1, t2)] =Z

dτ∑

i

t†1,i∂τt1,i + t

†2,i∂τt2,i +H[t1, t2]

exp−Γ[χ] =Z

Dδχexp−S[χ+δχ]+Z

JT δχ, J =δΓ[χ]

χ

Monday, August 29, 2011

Page 18: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Condensation and Thermodynamics• Physical vacuum is continuously connected to the finite density case:

Introduce new, expectationless operators by (complex) Euler rotation

b = Rθ Rϕt

t = (t0, t1, t2)T

• Hamiltonian in new coordinates takes form:

H = EGW +HSW +Hint

Mean field: Gutzwiller Energy

Quadratic part: Spin waves (Goldstone for n > 0)

higher order: interactions

microscopic thermodynamic long distance

interactions interactionscondensation

interactionscondensationspin waves

Monday, August 29, 2011

Page 19: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

The requantized Gutzwiller model

Hkin =−J ∑i, j

t†1,i(1−n1,i−n2,i)(1−n1, j −n2, j)t1, j +

√2(t†

2,it1,i(1−n1, j −n2, j)t1, j + t†1,i(1−n1,i−n2,i)t†

1, jt2, j)+2t

†2,it2, jt

†1, j

t1,i

Hkin =−J ∑i, j

t†1,it1, j +

√2(t†

2,it1,it1, j + t†1,it

†1, j

t2, j)

• Hamiltonian to cubic order is of Feshbach type:

Hpot = ∑i

(U−2µ)n2,i−µn1,i

detuning from atom level

(bilocal) dimer splitting into atoms

Dimer energy

two separate atomʼs energy

• quadratic part:

• leading interaction:

detuning

here: detuning

• Compare to standard Feshbach models:

∼ 1/U

∼U

we can expect resonant (strong coupling) phenomenology at weak coupling

Monday, August 29, 2011

Page 20: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Vacuum Problems

• The physics at n=0 and n=2 are closely connected: • “vacuum”: no spontaneous symmetry breaking• low lying excitations:

• n=0: atoms and dimers on the physical vacuum• n=2: holes and di-holes on the fully packed lattice

n=2

n=0

dimer excitation

di-hole excitation

+G (K) = -1d

= +

• Two-body problems can be solved exactly

red blue

Eb/Jz

−U

• Bound state formation:

reproduces Schrödinger Equation: benchmark Square root expansion of constraint fails

di-hole-bound state formation at finite U in 2D0 1 2 3 4 5 6

4

3

2

1

0n = 0 n = 2Eb/Jz

U/Jz

d = 2d = 3

1

an|U |+ bn=

ddq

(2π)d1

−Eb + cn/d

λ(1− cosqeλ)

n = 0 : a0 = 1, b0 = 0, c0 = 2

n = 2 : a2 = 4, b2 = −6 + 3Eb c2 = 4

Monday, August 29, 2011

Page 21: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Beyond Mean Field Phase Diagram

0.0 0.5 1.0 1.5 2.08

6

4

2

0

• Start here!

kld n1/3,T 1/2,ε1/2Mn =

k3F

3π2 ,TεM =− 1Ma2

microscopic thermodynamic long distance

Monday, August 29, 2011

Page 22: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Beyond Mean Field Phase Diagram• Vacuum limit:

• Scattering of a few particles• Requantized Hamiltonian is of Feshbach type

n = 0: Schrödinger Equation reproduced: Benchmark n = 2: finite critical interaction for di-hole bound state in 2D

• low lying excitations:atoms and dimers on the physical vacuum

• low lying excitations:holes and di-holes on the fully packed lattice

kld n1/3,T 1/2,ε1/2Mn =

k3F

3π2 ,TεM =− 1Ma2

microscopic thermodynamic long distance

0.0 0.5 1.0 1.5 2.06

5

4

3

2

1

0

Monday, August 29, 2011

Page 23: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Beyond Mean Field Phase Diagram

kld n1/3,T 1/2,ε1/2Mn =

k3F

3π2 ,TεM =− 1Ma2

microscopic thermodynamic long distance

• Thermodynamic scales: Nonuniversal shifts on the phase border

Quantum fluctuations lead to quantitative deviation from MFT Stronger shifts for small densities: weaker vacuum fluctuations

0.0 0.5 1.0 1.5 2.06

5

4

3

2

1

0Uc = 2πlog 8

√δn

Λ2

−1

Uc = U2

1 + σ |U2|−3

2|U2|δn1/4

Uc = −3 + πlog 4

√δn

Λ2

−1

Uc = U0

1 + 4σδn1/4

Uc = −2(1 + 2√δn).

U0 ≈ −4/3,σ ≈ 0.42

Λ ≈ 5.50, U2 ≈ −11/3

Uc = −4(1 + 2√δn)

Monday, August 29, 2011

Page 24: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Beyond Mean Field Phase Diagram

kld n1/3,T 1/2,ε1/2Mn =

k3F

3π2 ,TεM =− 1Ma2

microscopic thermodynamic long distance

Enhancement of symmetry from Ising quantum critical point near half filling

• Qualitative effects of the constraint and interactions:

0.0 0.5 1.0 1.5 2.08

6

4

2

0

(similar fermions: S.C. Zhang ʼ93)

Monday, August 29, 2011

Page 25: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Symmetry Enhancement in Strong Coupling

• Interpret EFT as a spin 1/2 model in external field:

Isotropic Heisenberg model (half filling n=1):• Emergent symmetry: SO(3) rotations vs. SO(2) sim U(1)• Bicritical point with Neel vector order parameter

λ =v2t

= 1• Leading (second) order perturbation theory:

CDW order

xy plane: superfluid order

• charge density wave and superfluid exactly degenerate• CDW: Translation symmetry breaking

• DSF: Phase symmetry breaking

• physically distinct orders can be freely rotated into each other: “continuous supersolid”

The symmetry enhancement is unique to the 3-body hardcore constraint

with constraint

without constraint

• Perturbative limit U >> J: expect dimer hardcore model

(similar to fermions: S.C. Zhang ʼ93)

Monday, August 29, 2011

Page 26: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

!"# $ $"%

!

&

&

'()*')+,

%! -! .!

%!

-!

!

$

!

%

!

$

%

%! -! .!

$!! $!$$!

$!

&

&

()*/01)+,/01

Signatures of “continuous supersolid”

(1) Second collective (pseudo) Goldstone mode

density profile: Onset of CDW DSF order in textured regions

(2) Use weak superlattice to rotate Neel order parameter

(3) Simulation of 1D experiment in a trap (t-DMRG)

• Proximity to bicritical point governs physics in strong coupling

ω(q) = tz(λεq +1)(1− εq)

1/2

gap

• Next (fourth) order perturbation theory: Superfluid preferred

Second (pseudo) Goldstone mode

Monday, August 29, 2011

Page 27: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

!"# $ $"%

!

&

&

'()*')+,

%! -! .!

%!

-!

!

$

!

%

!

$

%

%! -! .!

$!! $!$$!

$!

&

&

()*/01)+,/01

Signatures of “continuous supersolid”

(1) Second collective (pseudo) Goldstone mode

density profile: Onset of CDW DSF order in textured regions

(2) Use weak superlattice to rotate Neel order parameter

(3) Simulation of 1D experiment in a trap (t-DMRG)

• Proximity to bicritical point governs physics in strong coupling

ω(q) = tz(λεq +1)(1− εq)

1/2

gap

• Next (fourth) order perturbation theory: Superfluid preferred

Second (pseudo) Goldstone mode

Monday, August 29, 2011

Page 28: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

S[ϑ,φ] = SI[φ]+SG[ϑ]+Sint[ϑ,φ]

SI[φ] =Z

∂µφ∂µφ+m2φ2 +λφ4

pure Ising action

pure Goldstone action

coupling term

Interactions persist to arbitrary long wavelength (cf. decoupling SW) : Phase transition is driven first order by coupling of Ising and Goldstone mode

Ising potential landscape: Z_2 symmetry breaking

Frey, Balents; Radzihovsky&

Ising field: Real part of atomic field

Infrared Limit: Nature of the Phase Transition

• Perform the continuum limit and integrate out massive modes:

Sint[ϑ,φ] = iκZ

∂τϑ φ2

κ = 0

• Two near massless modes: Critical atomic field, dimer Goldstone mode• Coleman-Weinberg phenomenon for coupled real fields: Radiatively induced first order PT

Monday, August 29, 2011

Page 29: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

coupling term

Ising Quantum Critical Point around n=1

00

|κ|

n0 1 2

• Plot the Ising-Goldstone coupling:

Sint[ϑ,φ] = iκZ

∂τϑ φ2

Second order quantum critical behavior is a lattice + constraint effect

• Symmetry argument: • dimer compressibility must have zero crossing• Ward identies for time-local gauge invariance and atom-dimer phase locking

must have zero crossing: true quantum critical Ising transition

decoupling

Γ Z

x,τb†

2,i(−g2 µ)b2,i

κ

• Estimate correlation length:

weakly first order, broad near critical domain

Monday, August 29, 2011

Page 31: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Does the loss induced 3-body constraint stabilize the superfluid?

In order to separate processes involving only two dis-tinguishable fermions, we did reference measurements forall possible two-state mixtures by preparing three-component mixtures and removing one component with aresonant laser pulse before ramping to the probe field. Asan example, the result for the mixture of atoms in states j1iand j3i is shown in Fig. 2(b). Away from the Feshbachresonances, all two-component mixtures are stable due toPauli blocking, as a three-body loss process would involveat least two identical fermions. Adding a third distinguish-able fermion allows three-body processes, which can de-crease the stability of the gas. From this, we infer that alldecay observed in Fig. 2(a) for magnetic fields below590 G stems from processes involving atoms in all threespin states.

To get quantitative information about the loss rates wemeasured the decay of the gas over a period of five secondsat several magnetic field values and hence for differenttwo-body scattering lengths. For these measurements, weprepared the three-component mixture as described above,tuned the magnetic field to the value of interest and mea-sured the number and temperature of remaining atoms as afunction of time. As an example, Fig. 3 shows the decaycurve for state j2i at a magnetic field of 300 G. Weobserved that the ratio of particles in the three statesremains one during the whole decay. Therefore, we canassume in the following analysis that all states have equalloss rates that are governed by a three-body process. Theloss of particles can then be described by

_n i! ~r" # $K3ni! ~r"3; (1)

where K3 is the three-body loss coefficient and ni! ~r" de-notes the local, temperature dependent density of atoms perspin state jii. Additionally, we take into account a smallone-body loss with a 1=e-lifetime of about 100 s. From thetwo-component measurements, we infer that we can ne-glect two-body decay processes. To deduce K3 from ourexperimental data, we follow a method described in [29].Loss of atoms occurs predominantly in the center of thetrap where the density is high. The energy taken away by alost particle is thus smaller than the mean energy per

particle when averaging over the whole cloud. This leadsto heating of the sample [see Fig. 3(b)] which requires anumerical treatment of the atom number and temperatureevolution, for which we use the code developed for [29].The model we use describes loss in a thermal gas. ForT=TF % 0:37, minor changes occur due to degeneracy,which we neglect for simplicity. For the analysis of thelifetime curves, we use an effective temperature ( !T inFig. 3) deduced from a Gaussian fit to the density distri-bution after time of flight. If the gas is degenerate, theobtained value !T is slightly higher than the real tempera-ture. As the density in a degenerate Fermi gas is reducedwith respect to a thermal gas of the same temperature, thehigher temperature value compensates to some extent forthe small effects of degeneracy. Hence, we approximateT % !T for our analysis. For most values of K3, this ap-proximation affects only the very first data points, as thetemperature quickly exceeds the Fermi temperature afterinitial loss and heating. The solid line in Fig. 3 shows the fitto the atom number and temperature evolution according tothis model for one decay curve. From such fits, we obtainour values of K3.Figure 4 shows the obtained three-body loss coefficients

for all three species as a function of the magnetic field. Asexpected, K3 reflects the qualitative behavior of the atomnumber in Fig. 2. The relative error of the data points iscaused by the uncertainty in spin balance, difference indetection efficiency for the three states and fitting uncer-tainties. This error can be estimated by the scatter of thefitted values for K3 for different states and is much smallerthan the observed variation of K3. The absolute scale issubject to additional systematic errors in particle numberand trap frequency. AsK3 / N2 !!6, uncertainties of 40% inN and 7% in !! lead to an error of 90% in the absolutescale.Although there is currently no theoretical model which

can quantitatively explain the strong variation of K3 withthe magnetic field, we can qualitatively discuss some as-pects of its behavior. In a naive picture, one can describe athree-body event by elementary two-particle interactionsgoverned by a12, a13, and a23. If two of the three scatteringlengths are close to zero, only two of the three spin states

FIG. 3. Evolution of (a) atom number and (b) temperature ofatoms in state j2i over five seconds at 300 G. !T denotes aneffective temperature deduced from a Gaussian fit to the cloudafter time of flight. Each data point is a mean value of threeindependent measurements taken in random order. The solid lineis a fit to the data, applying the method described in the text.

FIG. 4 (color online). Three-body loss coefficient K3 vs mag-netic field.

PRL 101, 203202 (2008) P HY S I CA L R EV I EW LE T T E R Sweek ending

14 NOVEMBER 2008

203202-3

Trimers Colour superfluid (BCS pairing)

3-Component Fermions on the Lattice

• 3-species Fermi systems• e.g., Lithium-6: Very strong loss features due to Efimov resonance (T. Ottenstein&; O’Hara&)

• Rich many-body physics for attractive isotropic interactions (C. Honerkamp, W. Hofstetter; A. Rapp&)

symmetric

• But small “colour superfluid” domain

• Loss -> Interaction:Onsite Trimers excluded

Monday, August 29, 2011

Page 32: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

The Lithium Case• Strong loss features• 3 components, but no fundamental SU(3) symmetry (strong explicit breaking)

• The interactions are large and attractive, and strongly separated from each other• work with

U1

U2

U3

|1

|2

|3

U3 = −40J, U2 = −20J, U1 = −5J, nα = 1/6

Monday, August 29, 2011

Page 33: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Effective Low Energy Hamiltonian

• Scale separation: full constrained Feshbach Hamiltonian maps to a Fermi-Bose mixture

H = H1F +HBF +H1B

Large fermion-boson repulsion ~ Jz, which originates from the constraint

t1 =2J2

U1

fast fermions

slow bosons

density-density repulsion

|1

|1B = |23

H1F = J

i,j

∇it†1,i∇it1,i

H1B = −t1

i,j

2b†1,ib1,j − m1,im1,i

HBF = Jz

i

n1,jm1,i

• The mapping of constrained to Feshbach-like theory can be leveraged over to fermions

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Page 34: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Constraint Induced Phase Separation

1 ≤ 4π2(d/Ωd)2/dd−2 J

|U1|n2/d−1F

0.35(0.77) for d = 3(2)

• A phase separated state does not feature the strong off diagonal term and is thus energetically favorable

• The system is unstable for typical Li parameters

• Responsible scale uFB = Jz

expect effect to persist for temperatures much larger than bound state condensation temperature

T = O(Jz)O(J2/|U1|)

constraint induced phase separation should be observables in current experiments

“Colour superfluid”Free fermions

• Stability analysis: Canonical energy at low densities in mean field

E(d)(n1,m1) = 4π2Jd

d+ 2

d

Ωd

2/dn2/d+11 + tzm2

1 + 2Jzm1n1

2π, 4π for d = 2, 3

Monday, August 29, 2011

Page 35: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Summary

0.0 0.5 1.0 1.5 2.08

6

4

2

0

• 3-body hard core constraint from strong three-body loss• analogous Quantum Zeno Effect• ground state of constrained system reachable

• Beyond mean field effects in 3-body constrained bosons• based on requantized Gutzwiller theory • existence of Ising QCP• symmetry enhancement leads to “continuous supersolid”

• 3-component fermions with 3-body constraint• fermionic Li is prime candidate loss generated constraint• constraint induced phase separation above T_c• stabilization of atomic “color superfluid” at T=0

Monday, August 29, 2011

Page 36: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Monday, August 29, 2011

Page 37: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Microscopic model: Interactions via Loss• Model: Bosons on the optical lattice with three-body recombination

• Hamiltonian:

• Three-body recombination: loss from lattice to continuum of unbound states

• Modeled by Master Equation

H = −J ∑i, j

b†ib j +

U

2 ∑i

ni(ni −1)

three-body loss rate

dissipative dynamicsunitary dynamics

Monday, August 29, 2011

Page 38: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

He f f = H− iγ3

12 ∑i

(b†i)3

b3i

=J

Jup to double occupancy

triple and higher occupancy

J, U

J, U,

γ3U,J Consider the limit

iγ3

Basic Mechanism: Interactions via Loss

• Rewrite the Master Equation as

Monday, August 29, 2011

Page 39: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Basic Mechanism: Interactions via Loss• Second order Perturbation Theory on Master Equation: Define projector P onto subspace with at most 2 atoms per site (Q=1-P)• Study behavior of the effective Hamiltonian:

Three-body hardcore constraint due to: dynamic suppression of triple onsite occupation (analogous Quantum Zeno Effect)

Γ = 12J2

γ3

Realization of a Hubbard-Hamiltonian with three-body hard-core

constraint on time scales τ = 1/Γ

c j = b2j ∑k| j

bk /√

2

PHP PHQ

QHQQHP

PHP =−J ∑i, j

b†ib j +

U

2 ∑i

ni(ni−1) & b†i

3 ≡ 0

Small decay constant in P subspace:

• The leading real part:

• The perturbative imaginary part:

Monday, August 29, 2011

Page 40: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

ASF - DSF Phase Border

• Result:

Uc

Jz≈ Uc(n = 0)

Jz−

θ|Uc(n = 0)|

2Jzσ, σ≈ 0.53

condensate angle

• Understanding:

(i) low density: coincidence of scales strong shifts, nonanalytic nonuniversal behavior

(ii) maximum density: mismatch of scales, di-hole bound state forms prior to atom criticality mean field like behavior

shifts of the phase border

red d=2

blue d=3

black MFT

- Note: No particle-hole symmetry!

e.g. d=3:

• Goal: Effects of quantum fluctuations on phase border

- dominant fluctuations: associated to bound state formation

- two scales: bound state formation and atom criticality0.0 0.5 1.0 1.5 2.08

6

4

2

0

- strong shifts only observed for low densities

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Page 41: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Constrained Theory for 3-Component Fermions

• Lithium Hamiltonian: species dependent chemical potentials, strongly anisotropic couplings

H = −J

i,j,α

c†i,αcj,α −

α,i

µαni,α +

α,i

Uαni,α+1ni,α+2

• Constraint: No onsite trions

13!αβγc

†αc

†βc

†γ ≡ 0

• The residual states can be parameterized as

empty sites|0i = b†0,i|vac

|αi = t†α,i|vac = c†α,1|0i|αBi = b†α,i|vac = 1

2αβγc†β,ic

†γ,i|0i = |βγi = |α+ 1,α+ 2i

single fermions

“molecules”

U1

U2

U3

|1

|2

|3

Monday, August 29, 2011

Page 42: 3-Body Interactions from 3-Body Loss · Peter Zoller (Innsbruck) Walter Hofstetter (Frankfurt) Adrian Kantian (Geneva) Monday, August 29, 2011. Outline ... Stoof, Sachdev& ʻ03):

Hard-Core Constraint: Summary

• Constrained Model can be mapped on coupled boson theory. This should be seen as a requantization of Gutzwiller mean field theory

• This theory automatically respects constraint: Decoupled physical and unphysical subspaces

• Effective Action path integral quantization favorable: symmetry principles are supplemented with a constraint principle

Monday, August 29, 2011