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Page 1: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with
Page 2: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Division of

Applied nuclear

physics

Scientific Head

Professor Ane Håkansson

Admin. Head of division

Dr. Michael Österlund

Fusion Diagnostics

Professor Göran Ericsson

Nuclear Reaction Research

Professor Stephan Pomp

Total numbers of employees

50

Nuclear Fuel Diagnostics

and Safeguards

Dr. Peter Jansson

Ion Physics

Dr. Daniel Primetzhofer

Internal collaboration with

the Divisions of Materials

Theory and Materials

Physics

Page 3: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Teaching and education

Page 4: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Undergraduate teaching

We are responsible for three education programs:

- “Civilingenjörsprogrammet i energisystem”

- “Högskoleingenjörsprogrammet

i kärnkraftteknik”, KKI

- “Kandidatprogrammet i fysik”

- Contract education

UU provides the nuclear industry with

contract education courses through NANSS.

Teaching objectiveso Provide as many Masters’ Engineering students as possible with

nuclear technology relevant courses. Allow for specialisation in

nuclear engineering.

o Development of the Bachelors’ Engineering programme in nuclear

engineering.

o Provide supervision for students whishing to do a diploma work within

nuclear technology.

o Provide the industry with relevant further education

Teaching and education at UU

Page 5: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Problems

The number of students decreasing (down approx. 10%)

The Nuclear Power Engineering programme, KKI, will most likely be put

on hold.

The shaky funding of nuclear research implies a risk of shortage of

academic teachers leading to a drastically decreased capacity. This is of

national concern:

• It is not unlikely for a political turn regarding nuclear power.

• Regardless of this, nuclear competence will be needed for decades to

come.

Possibilities

• A frustrating fact: The student’s interest for nuclear technology as such

is intact but the don’t consider nuclear sector as an attractive

employer.

• Ongoing work to implement courses within the KKI programme into

the contract education programme by adapting to industrial needs by

modularisation, e-learning (possibly in collaboration with Chalmers

and KTH) etc.

• Ongoing dialogue with the political sphere. There is a clear

understanding of the imminent problem of competence supply.

Teaching and education at UU

Page 6: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Magnus Ahnesjö: Tomographic reconstruction of subchannel void measurements

of nuclear fuel geometries.

Joel Blomberg: Sensitivity study of control rod depletion coefficients.

Daniel Constanda: Control Rod Effect at Partial SCRAM - Upgrade of Plant Model

for Forsmark 2 in BISON After Power Uprate.

Henrik Liljenfeldt: Applying fast calorimetry on a spent nuclear fuel calorimeter.

Tobias Lindström: SPARC fast reactor design Design of two passively safe

metal-fuelled sodium-cooled pool-type small modular fast reactors with

Autonomous Reactivity Control.

Gjertrud Louise Langaas: Measurements of radioactivity in plant and soil

samples taken near a nuclear power plant.

Moa Skan: Analysis of the neutron albedo’s influence on TIP deviations in

Forsmark 1.

Joakim Nordlander: Evaluation of the dimensional stability in the PWR

assemblies in Ringhals.

Sebastian Leo Eile Svanström: Load following with a passive reactor core using

the SPARC design.

Mattias Åkerman: Improved peaking factors with radial enrichment distribution for

PWR fuel assembly.

SKC relevant Diploma Work 2015-

16

Page 7: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with
Page 8: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Fission group

Nuclear

safeguards

Nuclear fuel

diagnostics

Back-end fuel

characterization

Gen IV

systems

Responsible:

Sophie Grape

Responsible:

Peter

Andersson

Responsible:

Peter Jansson

Responsible:

Carl Hellesen

Page 9: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Nuclear Safeguards

• Active and passive interrogation

techniqes for verification of fuel

properties

• Using MVA-techniques to develop

models for verification of spent fuel

properties based on high-

dimensional measured data3He

Pb

W

H2O

SFA

NG

polyethylene

Cd

liner

Page 10: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Nuclear Safeguards Modeling and measurement of Cherenkov light

Presentation tomorrow 10:50 in Uppland

Erik Branger, Uppsala University, Predicting the Cherenkov light intensity of irradiated

nuclear fuel assemblies in wet storage for nuclear safeguards purposes.

• The DCVD is an IAEA-approved

technique for partial defects

verification.

• Partial defects are identified by

measuring Cherenkov-light

intensities that are lower than

predicted.

• Thus, accuracy of predictions is

essential!

Page 11: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Proposal of LOCA rod inspection using gamma tomography was first

presented in SKC symposium in Sigtuna 2015.

Fuel diagnostics

Slide from last

year’s symposium

Results presented

at TOP fuel 2016

Presentation tomorrow 10:30 in Lappland

Peter Andersson, Uppsala University, Nuclear fuel diagnostics within MÅBiL in

collaboration with the Halden Reactor Project

Page 12: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Outer part of

lateral

neutron

shield with

Neutron

channel

[C. JAMMES et al,

Nuclear Engineering

and Design, 2014]

Gen IV reactor systems

Developing detectors for SFR in

colaboration with CEA.

• In-vessel ex-core detectors (Fission

chambers)

• In-core detectors (Self-powered

detectors)

Recent results

- Detectable signature in fission

chambers following withdrawal of outer

control rod

- In-core detectors needed for precise

knowledge of location of perturbations

V. Verma, P. Filliatre, C. Hellesen, S. Jacobsson Svärd, C. Jammes, Neutron flux

monitoring with in-vessel fission chambers to detect an inadvertent control rod

withdrawal in a sodium-cooled fast reactor, Annals of Nuclear Energy, Volume 94,

August 2016, Pages 487-493, ISSN 0306-4549,

http://dx.doi.org/10.1016/j.anucene.2016.04.019.

Page 13: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with
Page 14: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Reaction group

Microscopic

measurements

Nuclear reaction

modeling

Application simulations

and

uncertainty quantificationfeedback

Nuclear Data underpin all of Nuclear

Science and Technology!

Page 15: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Microscopic

measurementsMicroscopic measurements (cross sections and fission yields)

NFS, France (1+1 PhD)• Precision measurements of cross sections, e.g.,

235U(n,f) and 238U(n,f) vs. cross section standards

• Measurement of neutron-induced light-ion production from various targets in the energy range 5 – 200 MeV

IGISOL, Finland (2 PhD)• Measurement of independent fission yields in

thermal and fast neutron spectra

IRMM, Belgium• Measurement of reference cross sections and

neutron emission from fission

partly financed by VR

supported by SSM and

the EU via CHANDA

supported by VR and

the EU via CHANDA

supported SSM and the

EU via CHANDA

Page 16: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Microscopic

measurementsMicroscopic measurements (cross sections and fission yields)

NFS, France (1+1 PhD)• Precision measurements of cross sections, e.g.,

235U(n,f) and 238U(n,f) vs. cross section standards

• Measurement of neutron-induced light-ion production from various targets in the energy range 5 – 200 MeV

IGISOL, Finland (2 PhD)• Measurement of independent fission yields in

thermal and fast neutron spectra

IRMM, Belgium• Measurement of reference cross sections and

neutron emission from fission

Page 17: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Nuclear

reaction

modeling

Nuclear reaction modeling

improved modeling

of fission yields

GEF + TALYS = true from thermal to fast

energy range

(inventory; fuel cycle,…)

+ ISOMERIC YIELD RATIOS…

Page 18: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

TENDL och Total Monte Carlo (TMC)

0.98 1.00 1.02 1.05 1.07

20

40

60

80

100

Experimentell data:kalibrering

e.g. safety parameter

Nuclear data

codes

Experimental data for

calibration

Application

Simulations: reactor

and depletion codes

Result

Page 19: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with
Page 20: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

MÅBiL

Page 21: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Running projects

Chalmers• Aneta Sajdova - ”Accident tolerant Uranium Nitride fuel”

• Kristina Lindgren - ”Ageing of RPV Steel - An Atom Probe Tomography Study”

KTH• Elin Toijer - "Combined experimental and theoretical investigation of

underlying phenomena for irradiation assisted stress corrosion cracking"

Uppsala University• Petter Helgesson - ”Improved nuclear data for material damage applications

in LWR spectra”

• Erki Metsanurk - ”ICEWATER – Irradiation Corrosion Experiment Water”

• Maciej Kaplan - “Amorphous thin films for coatings”

• Peter Andersson - “Nuclear Fuel Diagnostics within MÅBiL in collaboration with the Halden Reactor Project”

MÅBiL

Page 22: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Questions of interest

1. Status: Do the projects fulfill the goals according to plan?

a) Research results

b) Economy

2. Future 1: When are the current projects expected to end?

3. Future 2: In the coming SKC agreement it is, among others, expected a continuous collaboration between the universities:

a) Is MÅBiL the road forward in this respect?

b) Can MÅBiL comprise interdisciplinary research between materials sciences and more classical nuclear technology subjects?

MÅBiL

Page 23: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Questions of interest

Do the projects fulfill the goals according to plan?

Research results.

Overall, all projects have fulfilled the scientific goals so far.

Economy

No project has exceeded the budget.

MÅBiL

Page 24: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

”Accident tolerant Uranium Nitride fuel”

Sol-gel beads with corrosion resistant elements have been manufactured. This kind of material has never before been made and thus it will need extensive characterisation, which is ongoing.

In principle the underpinning idea is that these added elements will migrate to the phase boundaries and there produce a thin layer of protective oxide which will prevent the nitride from reacting. This part will be investigated in detail later in the project.

MÅBiL

Page 25: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Nuclear Fuel Diagnostics within MÅBiL in collaboration with the HaldenReactor Project”

a. Methodology for fuel diagnostics have been developed.

b. New and previous HRP experiment have been analysed.

c. New measuring methods have been developed for studying rod-wise FGR and fuel reallocation within LOCA test rods.

ATF materials have not been studied simply depending on that such materials have not yet been irradiated at HRP. However, the developed methodologies are feasible for studying the ability for ATF to contain volatile fission products.

MÅBiL

Page 26: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

”Ageing of RPV Steel - An Atom Probe Tomography Study”

Application of atom probe tomography (APT) to study clusters/precipitates forming in RPV steels under irradiation. Materials irradiated in Halden (up to 80 years of equivalent dose) have been compared to identical material from surveillance testing. The results show that there are no "late blooming precipitates"; the NiMnSi(Cu) precipitates grow with increasing fluence, but they do not change in nature.

The effect on embrittlement seems to have a weak dependency on flux and the hardness increases linearly with fluence, after a fast increase early in life. Thermal aging has also been studied. It has been found that the welds of the pressurizer becomes embrittled due to the formation of Cu precipitates on dislocations.

MÅBiL

Page 27: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

"Combined experimental and theoretical investigation of underlying phenomena for irradiation assisted stress corrosion cracking"

1. The grain boundary cohesion as function of radiation damage is in the process of being modelled. Elin has studied segregation profiles for phosphorous in a model material (fcc Ni) and is adding Fe, Cr and point defects to describe local chemical effects (in the solid) and interplay with radiation induced defects for the weakening of the grain boundaries.

2. She has also completed a first study of the reactivity in water of 304 stainless steel .

3. The project group has started to make a detailed experimental set up for testing if the effect of chemistry can be isolated from that of radiolysis in the crack tip region (see E. Toijer's presentation).

MÅBiL

Page 28: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

”Improved nuclear data for material damage applications in LWR spectra”

The project has been very successful. Among others, new data for Ni-59 has been obtained and new methods for handling uncertainties in transient calculations connected to uncertainties in nuclear data have been developed, all according to plan. The project’s centre has been shifted somewhat towards structural materials.

In addition to the Ph.D. Student, a postdoc, Augusto Hernadez, funded by UU, is contributing to the project.

MÅBiL

Page 29: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

”ICEWATER – Irradiation Corrosion Experiment Water”

Although in nature ICEWATER is an experimental project, a considerable effort has been put into understanding the theoretical aspects behind IASCC and how would ICEWATER contribute to the existing knowledge.

• Designed and assembled an apparatus capable of heating flowing water at 130 bars of pressure up to 320 °C.

• Performed irradiation experiments in order to assess the buildup of activity in stainless steel foils in order to select the possible ranges of energies and currents for forthcoming experiments.

• Design of a 3-D model of a test cell. With it is possible to stress the sample either with constant or slowly varying load. The next step is to manufacture and assemble the cell in collaboration with Sandvik and KTH.

MÅBiL

Page 30: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

“Amorphous thin films for coatings”

MoSiZr alloys have been studied and to gain knowledge of how the composition affects the crystallisation temperature, which enables further improvement of thermal stability. Crystallisation temperatures of the MoSiZralloys were investigated by heat treatments in vacuum and ex-situ X-ray diffraction and X-ray reflectivity analysis.

The highest thermal stability of the alloys was exhibited by Mo48Si48Zr4, Mo43Si50Zr7, Mo50Si40Zr10 and Mo45Si43Zr12, they remained amorphous after heat treatment at 1073 K. The resulting crystalline phases are Mo3Si, Mo5Si3 and ZrO2. Oxidation of Zr in the alloys is present only when the Zrcontent is ≥10 at%, crystallisation is otherwise mainly driven by formation of Mo3Si.

Further improvement of the thermal stability is possible by introducing new alloying elements at the cost of those that promote crystallisation. Keeping the content of Zr below 10 at% is of great importance to prevent oxidation.

MÅBiL

Page 31: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Questions of interest

Future 1: When are the current projects expected to end?

”Accident tolerant Uranium Nitride fuel”: Lic. Spring 2017, Ph.D. Autumn 2019.

”Ageing of RPV Steel - An Atom Probe Tomography Study”. Ph.D. Spring 2019.

"Combined experimental and theoretical investigation of underlying phenomena for irradiation assisted stress corrosion cracking“: Ph.D. Nov 2019.

”Improved nuclear data for material damage applications in LWR spectra”: Planned dissertation 2018-05-30.

”ICEWATER – Irradiation Corrosion Experiment Water”: Ph.D. 2017.

“Amorphous thin films for coatings”: T.B.D.

Peter Andersson - “Nuclear Fuel Diagnostics within MÅBiL in collaboration with the Halden Reactor Project”: Project ending spring 2017 with a planned continuation.

MÅBiL

Page 32: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Questions of interest

Future 2: In the coming SKC agreement it is, among others, an expectancy on continuous collaboration between the universities: Is MÅBiL the road forward in this respect?

MÅBiL is the first of its kind. Collaboration all over the scope (sometimes more, sometimes less). Generally seems to work adequately but we can do better in a MÅBiLII so the answer is “yes”.

MÅBiL has been a valuable stepping stone for creating international collaborations e.g. within IAEA CRP inom Primary Radiation Damage Cross Sections.

Within all projects, various methodologies have been developed that would give MÅBiLII a flying start. This forms another rationale for continuing the idea of MÅBiL.

MÅBiL

Page 33: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Questions of interest

Future 2: In the coming SKC agreement it is, among others, an expectancy on continuous collaboration between the universities: Can MÅBiLII comprise interdisciplinary research between materials sciences and more classical nuclear technology subjects?

MÅBiL tries to address this issue to some extent. But only parts of reactor physics, nuclear chemistry, safety & security, … are involved explicitly.

On the other hand, there is collaboration between for example Chalmers and UU in reactor relevant research. How to take care of such collaborations?

MÅBiL

Page 34: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with

Issues

All projects are not adequately funded implying either part-time working Ph.D. students and/or supervision paid by faculty money, which leads to delays. In addition:

• ”Accident tolerant Uranium Nitride fuel”

On-going discussion with Westinghouse regarding patenting of results => risk for additional delay.

• “Amorphous thin films for coatings”

The project is recently manned with a new student, waiting for a go/no go decision.

• The requirement that all publications shall pass the industrial partners prior to publishing has obviously not reached all project leaders. We must do better here.

• The work with quarterly reports is put on top of exponentially increased volume of administrative duties => less time for thoughts and supervision.

MÅBiL

Page 35: Division of Applied nuclear - KTH · Joakim Nordlander: Evaluation of the dimensional stability in the PWR assemblies in Ringhals. Sebastian Leo Eile Svanström: Load following with