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7/24/2019 Effect of Radiative Heat Transfer on Thermal Ignition
1/6
260
J.THERMOPHYSICS
VOL.3, NO. 3
Effect
of
Radiative Heat Transfer
on
Thermal Ignition
W .W.Yuen*and S. H.Zhu|
University of
California,
Santa Barbara, Santa Barbara,
California
The
effect
of
radiative heat transfer
on
thermal ignition
is
analyzed numerically.
Tw o
specific problems
are
considered. They are 1) the semi-in finite problem in which a large mass of hot burnt gas is suddenly brou ght
into contact with
a
large mass
of
cold unburnt air/fuel mixture,
and 2) the finite-hot-slab
problem
in
which
a finite slab of hot burnt gas is suddenly immersed in a sea of cold unburnt air/fuel mixture. Numerical results
show that
in
both problems
theradiative
emission
and
absorption
by
physical boundaries play essential roles
in
determining the effect of radiation on thermal ignition. In general, radiation is shown to have important effects
on the
ignition delay.
For the finite-hot-slab
problem,
the
minimum slab thickness required
for
ignition
is
also
shown to depend strongly on the radiation effect. Both the optical thickness of the burnt mixture and the
unburnt
mixture
are
important
in
determining
the
actual effect
of
radiation.
Nomenclature
x
b
(t )
a = absorption coefficient,1/m *s(0
B
=
dimensionless parameter,
Eq .
(11
a) #
C
= dimensionless parameter, Eq.(lib)
c
=
specific heat
of
gas, KJ/(Kg-K) *
E
a
=
activation energy,K J / K m o l
E
n
(x) = exponential integral function ^ o
f ( r f ) =
dimensionless temperatureprofile, Eq. ^
(2 1 ) 6/,m
F n,\
c
)
=
function utilizedin Eq. (12)
e
G/(i
=
1,2,3,4,5)
=
parameters defined
by
Eqs. (A3-A7) f
/ / ( /=1,2,3,4)
=
param eters utilized
in
Eqs. (22)
an d
(23)
ft
k - thermal conductivityofgas, W/(m -K)
K
u
= initial optical thick ness of the unbur n t
f t ,
mixture
K
b
= initial
optical
thickness of the burnt
ft>(
r
)
mixture
l
c
=characteristic length defined
by Eq.
&
(3b), m
L =total length of the one-dimensional
* ?
system defined
in
Fig.
1, m
m
=
mass loading
of the
mixture, Kg/m
3
0
M = dimensionless mass loading definedby c
Eq. (10)
M
bu
= mass loading ratio,m
b
/m
u
K
n
= complex index of refractionof particles
K
b - i
N(n)
=function defined
by Eq.
(A10)
*o
q
r
=radiative heat flux, W /m
2
* 2 5
q
r
=
dimensionless rad iative heat
flux
K
L
Q
=
volumetric heat generation rate,
W/m
3
V
Go
= characteristic heat of reaction,
W/m
3
P
R =dimensionless heat generation rate
defined
by Eq. (4) r
R =total dimensionless heat generation
defined by Eq. (5)
T
R
c
=universal gas constant, K J/(Kmo l-K)
T
m,o
S = dimensionless temperature gradient, 0(
T
)
/'(O)
t =t ime,
s
t
c
=characteristic time d efined by Eq. (3a), s Subscripts
T = temperature,
K
u
x =space co ordinate, m b
coordinate
of the
foot
of the
f lame,
m
half-thickness of the f lame, m
dimensionless temperature ratio defined
by
Eq. (9)
dimensionless half-thickness
of
f lame,
=
value
of 6 at
which
dr
m
/d0
= 0
= minimum value of 6 ,-
= activation number,E
a
/R
c
T
b
= dimensionless length defined by Eq. (2)
= dimensionless initial position of the foot
of the
f lame
=
minimum initial slab thickness
fo r
ignition
= d imensionless position of the foot of the
flame
= dimensionless length of the one-dimen-
sional system
= dimensionless variable defined by
Eq. (20)
=
dimensionless time defined
by Eq. (2)
= dimensionless time at which the two
combustion zones are in contact
= optical thickness defined by Eq. (9)
=
optical thickness defined
by Eq.
(A8a)
= optical thickness defined by Eq. (A8b)
= optical thickness defined by Eq. (A8c)
=
optical thickn ess defined by Eq.
(A8d)
= characteristic wavelength, m
= gas
density,
Kg/m
3
= Stefan-Boltzmann constant, W/(m
2
-K
4
)
=
dimensionless temperature defined
by
Eq. (2)
=r(0)
= value of
T
m
at whichdr
m
/d0= 0
=
dimensionless heat generation rate used
in
Eq. (1)
:
properties of theun burnt mixture
properties
of the
burnt mixture
Received
Feb.
9,
1988;
revision received Ju ne
23,
1988.
C opyright
American
Institute of
Aeronautics
and
Astronautics, In c., 1988.
All
rights reserved.
*Professor,
Department
of M echanical and Environmental Engi-
neering. M ember AIAA.
fGraduate Student,
D epartment
of
M echanical
and
Environmental
Engineering.
I.
Introduction
T
HE present work is the second in a series of two papers
that deals with
th e
general
effect of
radiation
on
f lame
propagation and ignition. In the first paper
1
the effect of radi-
ation
on
f lame speed, f lame thickness,
a nd fuel
consumption
7/24/2019 Effect of Radiative Heat Transfer on Thermal Ignition
2/6
JULY
1989
RADIATIVE
THERMAL IGNITION
261
rate
(flame
propagation parameters that are important after
ignition has
occurred)
w as
demonstrated.
The radiative prop-
erties
of the combustion products and the reacting mixture,
together with
the
radiation
from th e
physical boundaries,
were
demon strated to have
significant
effectson theflamepropaga-
tion behavior. The present
work
considers the
effect
of radi-
ative heat transfer on thermal ignition. Tw o specific
one-di-
mensional problems
will
be
analyzed. First,
a large mass of
hot burnt gas is
suddenly
brought into
contact
with
a
large
mass of
coldunbu rnt ai r / fuel mixture.
The
conditions
under
which
ignition occurs
and the
m agnitude
of the
ignitiondelay
will
be determined.Second,aslabof hot bu rnt gas is
suddenly
immersed in a sea of cold unburnt air/fuel
mixture.
Thecrit-
icalconditionsrequired
fo r
ignition will
be
developed. Based
on numerical results
generated
for the two
cases,
th e fund-
amental
effect ofradiation (both fromthe medium and
physi-
ca l
boundaries)
on general
ignition
phenomena
will
be estab-
lished.
In recent years, a number ofworks
2
'
6
have been
reported
dealing
with
the general effect of radiation on thermal igni-
tion. For aone-dimensionalplanar absorbing-emittinghomo-
geneous medium with volumetric Arrhenius
heat
generation,
the critical ignition parameters
(similar
to that derived by
Frank-Kamenetskii
7
in the
no-radiation
case)
f or
thermal
igni-
tiona re
calculated
b y
various
nume rical techniques or approx-
imation procedures. In these analyses, the radiative heating
(or cooling) of the medium b y a hot (cold)wallwas considered
as the major
physical
mechanism leading to
ignition
(extinc-
tion). In manypractical situations,
however,
the combustion
in a
premixed
air/fuel
mixture
is promoted by the use of
sparks or pilot flames.
Ignition
also can be induced by the
simultaneous conductive and radiative heating of the pre-
mixed air/fuel mixture with
a hot
wall
and hot
combustion
products .
Even in an initially
hom ogeneous air/fuel
mixture,
th e heat generation is a function of the
concentration
of the
reacting mixture and temperature. Results from the existing
works
2
'
6
are clearly not
applicable
fo r
such
situations. The
objective
to thepresent
work
is to illustrate the
effect
ofradia-
tion on theseimportant practicalignition problem s.
II . Semi-Infinite
Problem
The
physical
modelisillustratedby Fig. la. A large slab
of
hot combustion products at temperature T
b
is brought into
contact
with a
large slab
of
cold
unburn t
air/fuel mixture
at
temperature
T
u
.
T heobjectiveof the analysis is to determine
conditions under which
the energy
generated
by chemical
reactioni s
sufficient
toovercome thermaldiffusion and ignite
the unburnt
m ixture.
As
discussed
in the previous
work,
1
th e
assumption
of a
semi-infinite
absorbing medium is
accurate
only in the optically thick limit. In order to illustrate the
general
effect of
radiation
for systems
with arbitrary optical
thickness, theanalysismu st include the existence of two black
walls
of temperature
T
u
an d
T
b
in the considered
one-dimen-
sional system as
shown
inFig.
la.
As in the previous
wor k ,
1
the energy an d
species
conserva-
tion
equationcan besimplified
based
on the
Shvab-Zeldovich
transformation and a procedure developed originally by
Spalding
8
to become
2
r
dq
r
(1)
where r, 0, and
f
are dimensionless temperature, time, an d
distance defined
by
T T
(2a)
T
b
-T
u
P ( x ) d x
Pule
(2b)
(2c)
The subscripts
u
an d b stand for propertiesevaluated for the
upstream
unburned
reacting mixtures (T=0) and the down-
stream
burned products ( j =
1), respectively. Note that the
region
0
7/24/2019 Effect of Radiative Heat Transfer on Thermal Ignition
3/6
262 W.
W. Y U E NAND S. H. ZHU
J. THERMOPHYSICS
particles
9
),q
r
can be generatedreadily fromthe solution to the
radiative transfer equation as
u
= C f
L
- fc )
B
r(=2-
K
+
0]
4
E
2
(K - K' ) d K
f
- [T(K') +(3 ]
4
E
2
(
K
f
- K)
d*'
(8)
with
T
b
-T
u
9
d / c
=CM(f) df
an d5, Caredimensionless parameters
given
by
C =a
u
l
c
a
u
=
F n,\
c
)p
u
m
u
(9)
(10)
(lla)
(lib)
(12)
Physically,
small particles in the
reacting
mixture and prod-
ucts are
assumed
to be the prim ary species responsible for the
radiativeabsorption and emission in thedevelopmentofEqs.
(10-12);
m( ) represents the mass loading of the small par-
ticles. The dimensionless parameter
B
represents th eratio of
radiative
flux
to reactive
heat
generation,
while
C stands for
the optical thickness of the system based on the unburned
absorption
coefficient a
u
.
The two
ends
of the
one-dimen-
sional systemare assumed to be bounded byblack boundary
at
temperature
T
u
an d
T
b
,
respectively. The
parameter
F n,
A
c
)
is a function of theoptical constant of the
solid
particles
evaluated at a
characteristic
wavelength X
c
. Th e definition of
various dimensional
parametersa re
given
in the
Nom enclature
section. A more detailed
discussion
of the physical assump-
tions and the
mathematical
development of the
preceding
equationswerepresented in the earlier work.
1
The initialcon-
dition, as represented byFig. la, can bewritten as
7/24/2019 Effect of Radiative Heat Transfer on Thermal Ignition
4/6
JULY 1989
R A D I A T I V E
THERMAL
IGNITION
263
III. Finite-Hot-Slab Problem
The physical model is illustrated by Fig. 3. A slab of hot
combustion products at temperature T
b
and thickness 2x/ is
initially
surrounded by a cold
unburn t
air/fuel mixture at
temperature T
u
o n
both
sides.Becauseof thesymmetryof the
problem,x =0 ischosento be thecenterof theinitialhot slab,
and the
totalthickness
of the medium is taken to be2 L.
Using
the same physical assumptions and definition of
dimensionless
variables as the
semi-infinite
problem,
the dimensionless
ener-
gy
equation isagaingivenbyEq.(1).Because of the change in
coordinate
system
(f is measured
from
the midpoint
between
the two
walls,
an d K
L
no w represents the optical
thickness
from theoriginf= 0 to thewallat
f
=
f
L
) ,
thedimensionless
radiative
heat flux
becomes
K
L
)- E
3
(K
L
- i c ) ]+
[T(K')
+
0]*E
2
(
K
- K ' ) d/c '- [r(/O+
/3]
4
2
(
K
'
- K )
The initial
condition,
as represented by
Fig.
3,
is
0
(17)
(18)
Forcasesinwhichignitionoccurs,the expected temperature
profile
after ignitioni sillustrated
qua litatively
b yFig.4a. The
transient
flame
propagating behavior
is similar to that of the
semi-infinite
problem
as
presented
in the previous
work.
1
For
the extinction
and almost-ignition
case,
the expected
tempera-
ture
profile
is shown
qualitatively
byFig. 4b. The two com-
bustion zones are in contact, and the temperature at
f
= 0 ,
T
m
is
lessthan 1.0.
In the
extinctioncase,r
m
decreases mono-
tonically
toward
zero
after th e
initial
contact. If ignition
occurs, on the other hand, r
m
will
decrease to a minimum
valuegreater
than zero
and,
subsequently,
increase. The
med-
iu m
will eventually
achieve a temperature
profile similar
to
that inFig. 4a, and the flame willpropagate. Sincet he
objec-
tive of thepresent analysis is to determine the minimum slab
thickness required for ignition, the present work willconsider
only th e
flame behavior after
the initial
contact
of the two
combustion
zones.
The integral
method
will
be
used
to
deter-
mine the behavior of r
m
an d
d.
Specifically, assuming
that
the temperature
profile
has the
following
generalized form,
0 < f < 2 6
where
r j
is
given
by
r - s
(19)
(20)
As
demonstrated in Spalding
8
and solutions to the semi-in-
finite
problem,
numerical
predictions
for the
ignition
an d
flame propagat ion
behavior are
insensitive
to the
assumed
dimensionless temperature profile
/(r/).
The same expression
used
in the
previous work
1
is ,
thus, assumed
to be
applicable
in the present
case.
It is
1
(21)
M athematically, Eq.
(21)
is
generated
by the
combination
of
tw o
pieces
of error functions.
Numerical
experiments
show
that
it is an
dequ te
approximation of the temperature pro-
file within
the
combustion zone. Notethat
6, in
addition
to
being the dimensionless thickness of the
combustion
zone, can
also be interpreted as the dimensionless
flame
center for the
present problem. Substituting
Eq.
(21)into
Eq.
(1),
and
inte-
grating
from
0 to
L
an d
from
6 to
& ,
,
a set of two
nonlinear
ordinary
differential
equations can begenerated fo r
6(0)
an d
T
m
(0).
They
are
y
+
7- *IA
-
/
2
(/3
d(r
m
5)
d9
(22)
(23)
with
S
=/'(0) being thedimensionless temperature gradient
atf = 0. Theparameters
/ ,
7
2
,
/
3
,
and7
4
,whichare
related
to
the integral of the dimensionless temperature
profile
and heat
generation
across
the combustion zone, have
been
evaluated in
the previous
wor k .
1
Expressionsforq
r
(d) and
q
r
( L)
are
given
indetailin Appen dix A. TheinitialconditionforEqs.(22)and
(23)
are
r
m
(0
c
)=1.0, 6(0
C
)
=
S
7
(24)
where
0
C
stands fo r the dimensionless time required by the
initial
step-function temperature
profile (a s
shown
in
Fig.
3) to
develop into a
profile
in
which
the two combustion
zones
ar e
in
contact
(as
shown inFig.4b); B
c
an d
< 5 /(notethat
in
general,
6
f
. ft) can be determined from an early time
solution
to
Eq. (1), which is equivalent to the
semi-infinite
case.
As in the semi-infinite
problem,
the important dimension-
less
parameters for thepresent problem ar e B,
C ,
e,
f t ,
f
L
, |8,
and themass loadingratioM
bu
. Physically,theparameter
B
illustrates the
importance
of the radiativeeffect relative to the
chemical
heat
generation
effect. The parameter C is a char-
acteristic
optical thicknessthatalso
represents
the importance
of
th e radiative
effect
compared to the conduction effect.
Again, in
contrast
to
previous
ignition analyses
that
do not
include
th e effect ofradiation, th e size and theoptical
thick-
ness
of the
system(and
the
radiative
emission and
absorption
by
the two cold walls at ft, an d f t , ) play important roles in
determining
th e
effect
of radiation on ignition.
To illustrate the
mathematical
behaviorof T
m
,it isuseful to
expand Eq. (23) and combine with Eq . (22) to yield
(25)
I-28
Fig .
4a Exp ected temperature profile for the finite-slab problem in
which ignition
occurs.
Fig.
4 b
Expected
temperature
profile
for the
finite-slab
problem in
which
possible extinction occurs.
7/24/2019 Effect of Radiative Heat Transfer on Thermal Ignition
5/6
264
1.0
0.8
0.6
0 4
0 2
W. W. YUEN AN D S . H . ZHU J . THERMOPHYSICS
100 r
1rnr
n
r
~
r
n
r
~
r
~ n
r
~
r r
i
r
8
F ig. 5 Schematic representation of the numerical
procedure
used to
determine the minimu m ignition thick ness. (Curve A represents the set
of
points at
which
dr
m
/d 5
=
0.
Curves
i 2 and 3
represent
the
variation
of
r
m
with
6 for
various starting values
of 5. The starting
value
of 5 for curve 1 corresponds approximately to the minimum
ignition thickness.)
Since dd/dd
is
always
positive [as it can be
observed readily
from
Eq. (22), and is also consistent
with
physical expecta-
tion]
, a nd
dT
m
/dO
always
starts
out to be negative at
0
=
d
c
[a s
it
can be
observed
readily from Eq.
(23)],
dr
m
/d6 is
also
negative at 0 =
6
C
.
If ignition
occurs,
T
m
must eventually in-
crease
back
to
1.0.
This
requires
a positive
dr
m
/dd.
A
neces-
sary condition
fo r
ignition
is ,
thus, dr
m
/d d
= 0 .
M athemati-
cally,
the
smallest f /
for which
such condition
can be satisfied
will
have the physical interpretation of a minimum ignition
thickness.
Specifically,
the
following
mathematical
procedure
is used
to determine the minimum thickness
r
quired for
ignition.
For
a
given
set of specified dimensionless
parameters,
a set of
points T
W > O
^o)atwhich
dr
m
/dS
= 0 are
first
determined from
Eq .
(25).
A
typical
set of solutions for
(r
w> 0
,
S o )
are
illustrated
inFig.
5. For
each
set of
r
m
6
0
),Eqs. (22)
a nd
(23)
a re
then
solved
( in
backward
time
step)
to determine the initial value of
6 / [which is identical to 5(0
C
)]at whichr
m
= 1.0.Some typical
solutions
for the (j
mt
d)
history generated
from
Eqs.
(22) and
(23)arealsoshown inFig.5 asillustrations.It can be observed
readily [andalso
can be shown rigorously
from Eqs. (22)
an d
(23)] that as 6
0
increases, the corresponding 6 / approaches
asymptotically to a
constant
6
/> m
.
M athematically,
no
solu-
tions with
6 / m
isdetermined, th e early-time solution can beused
to relate 6 /
> /n
to theminimum
initial
slabthickness f /
> / w
. Numer-
ical results,
however,
showthat in all cases considered in the
present work ,
6 /
> w
isessentiallyidentical to
f/,
m
(i.e., the flame
does
not move very much during the initial diffusion
stage);
6 /
> m
thus can be interpreted as the
minimumhot-slabthickness
required for ignition.
As in the previous work,
1
a
survey
of the physicochemical
dataand typicalflame
temperatures
f or
common hydrocarbon
fuels
10
suggests values of 5.0 and
10.72
foreandB/C,respec-
tively.Num ericaldatafo r
other
values of e (which are of
some
practical
interest in terms of analyzing
different
fuels an d
air/fuel ratios) ar e
presented
elsewhere.
11
Assuming that f
L
=
1500,
th e
minimum ignition
thicknesses for
different
ab -
sorption
coefficients
for the burnt mixture are calculated and
presented in
Fig.
6.The
no-radiation result,
which is
identical
to that generated bySpalding,
8
is presented in the same
figure
for
comparison. The absorption
coefficient
of the
unburnt
mixture
does not appear as a parameter in the
figure
because
it
has
practically
n o
effect
on the minimum
ignition
thickness.
1.0
1.0
0 1
1 0
10
10
I0
3
K
K
Fig .6 Effect of the absorp tion coefficient of the burnt
mixture
on
the minimum
ignition thickness.
The broken line represents the no-
radiation
result.
1 0
0 5
K
U
=O.OI
0 01
0 1
1 0
Fig.
7 Effects of
optical
thicknesses of the
burnt
and unburnt
mixtures on the
ignition
delay for the
finite-slab
problem (the broken
line represents the
no-radiation
results).
Physically,
th e
major
effect of
radiation
on the
minimum
ignition
thickness is to
increase
th e
heat
loss from the initial
burnt mixture to the unburnt mixture an d
cold
wall. As the
optical
thickness of the
burn t
m ixture increases, the radiative
heat loss increases,
and a
larger slab
of
burnt mixture
is re-
quired fo r ignition. The lack of dependence on the optical
property of the unburnt mixture
suggests
that th e
radiative
heattransfer from the hotburn tmixture to thecoldwallis the
dominating cooling
effect controlling ignition.
Another important physical resultassociated wtih th e igni-
tion
process is the
ignition
delay.
Assuming f /
= 50 (which is
greater than the minimum ignition thickness calculated an d
presented in
Fig.
6
and, therefore,
th e
two-combustion zone
does no t meet , an d ignition always occurs), results for the
ignition delay
ar e
plotted
fo r different initial optical
thick-
nesses
K
b
an d
K
u
inFig.7 .Notethat
K
b
an dK
u
ar e
still defined
byEqs. (15)
and (16). Although the
optical
properties of the
unburn t
mixture have
only a small effect on the mini-
mum
ignition thickness,
results in
Fig.
7
show
that
i ts
effect
on
the
ignition
delay is
quite significant. Because
of the increased
preheating
of the
unburn t
mixture by
radiative
absorption,the
ignition delay decreases with
increasing
optical thickness
of
th eunburnt mixtureK
u
.Increasingthe opticalthicknessof the
burn t
mixture,
on the
other
hand,
first increases
an d
then
7/24/2019 Effect of Radiative Heat Transfer on Thermal Ignition
6/6
JULY
1989
RADIATIVE
THERMAL IGNITION
265
decreases th e
ignition
delay. Physically, the increase in the
optical thickness of theburntmixtureleads to two
com peting
effects
on ignition delay.First, it increases the radiative heat
lossfrom the burnt mixtureand,second, it leads to additional
preheatingof the unburnt mixture. For a burnt
mixture
with
small optical
thickness, the
first effect
dominates, and the
ignition
delay thus increases with increasing
optical
thickness
of th e
burnt mixture.
In the limit of an
optically
thick burnt
mixture, the
increase
in
heat
loss caused
by an
increase
in
opti-
cal thickness
is
small compared
to the
total energy radiated
into the unburnt mixture by the burnt
mixture.
The second
effect dominates and leads, therefore, to a reduction in
ignition delay.
IV . Conclusions
An
approximate
analysis is
performed
to
determine
th e
igni-
t ion behavior
of two simple problems: 1) a semi-infinite
one-
dimensional problem in which a slab of hot
burnt
mixture is
brought
into contact with a slab of cold
unburn t
air/fuel
mixture, and 2) a finite-hot-slab problemin which afinite slab
of
hot burntmixtureis surrounded by a cold unburntair /fuel
mixture. Inboth cases, the present work can be considered as
an
extension
of a
previous
work by
Spalding
8
with the inclu-
sion
of the
radiative
heat transfer effect. Th e following
con-
clusions
ar e
generated:
1) In general, the radiation
effect
increases
ignition delay
fo r both
problems,
and for the finite-hot-slab problem it in-
creases
the minimum
thickness required
fo r
ignition. Physi-
cally, this is because of the heat-loss
enhancement
effect of
radiation.
2)
Radiative emission and absorption by physical bound-
ariesplayessential roles indetermining the
effect
ofradiation
on
ignition. Analysesthat assume
semi-infinite medium
with-
out boundary correspond only to cases with
infinite optical
thickness.
Such
analyses
ar e
thus
not useful in illustrating the
general effect ofradiation.
3) For the semi-infinite problem, the ignition delay in-
creases
with
th einitial
optical
thickness of the
burnt
mixture.
The
optical thickness
of the
unburn t
mixture has
only
minor
effect
on ignition delay, except in the limit of an
optically
thick burnt mixture. In the limit of an
optical
thick burnt
mixture
and an optically
thin
unburn t
mixture,
ignition
fails.
4) For the finite-hot-slab problem, the minimum thickness
required for ignition increases with
increasing
absorption
coefficient for the hotburn tgas.T heabsorptioncoefficient of
the unburnt m ixture has
practically
no effect on the
minimum
ignition thickness.
5)
When ignition
occurs in the finite-hot-slab
problem,
th e
ignition delay
depends on
both
the
opticalthickness
of the hot
burnt
gas and of the cold unburnt
mixture.
The ignition delay
decreases withincreasingoptical
thickness
of the unb urnt mix-
ture. For a
fixed
opticalthicknessof the cold
unbu rnt mixture,
increasing the optical thickness of the hot burnt ga s first in -
creases, and then decreases the
ignition
delay.
Appendix
Substituting
Eq.
(19)
intoEq.
(17)
andevaluatingat f
L
and
< ,
one
obtains
K2 8
)- E
3
(
KL
-
K 2 d
) ]
2Bd(G
l
+ G
2
)
=2
(Al)
2Bd(G
3
+G
4
-
G
5
) (A2)
=
\i[l-fW]T
m
+0}
4
E
2
[K
L
+K
b
-
r
, -ri)]N ri)dr
)
(A3)
-i
i
dr ,
-/di)]T
m
1
0
i = \[ T
m
f(ri)
J
0
with
=
C6[l+(M
bu
-
X L
=C[ f
L
+ (M
bu
-
(A4)
(A5)
(A6)
(A7)
(A8a)
(A8b)
(A8c)
(A8d)
where
Physically, K
O
is the optical
thickness
form f= 0 to the
flame
center
f
= 6; K
L
is the optical
thickness
of the half-domain
ranging
from f
= 0 to
f
=
f
L
; K
2d
is the
opticalthickness
of the
flame,
an d
/ ^ - ^ ( r? )stands
for the
opticalthickness from f
= 0
to an
arbitrary
f.
Th e
functions A/0?)
an d
7 V r ? )
ar e
given
by
(A9)
(A10)
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