X-ray sourcesX-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL Higher...

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

X-Ray sources

Lenny Rivkin, PSI & EPFL

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Curved orbit of electrons in magnetic field

Accelerated charge Electromagnetic radiation

Wavelength continuously tunable !

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

60‘000 users world-wide

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

A larger view

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

The “brightness” of a light source:

Flux, F

FS x Ω

Brightness = constant x _________

Angular divergence, Ω

Source area, S

G. Margaritondo

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Steep rise in brightness

1021

1015

109

1900 1950 2000

Wigglers

Bending magnets

Undulators

Rotating anode

SPring8

ESRF

APS

Bertha Roentgen’s hand(exposure: 20 min)

Moore’s Law for semiconductors

SLSSOLEIL (F)DIAMOND (UK) …

the second waveXFEL

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Higher brightness: more photons on small sample or through a pinhole of ~ λ: coherence

measurements on very small probes (few μm crystals)

small divergence:compact mirrors, optics elementsminimized aberrations

short measurement times

high transverse coherencephase contrast imaging

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Microtomography

Brain blood vessels in a mousewith Alzheimer

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Overbooking of SLS beamlines

0

2

4

6

8

10

Lucia MS PX SIM SIS

2003 2004 2005 2006

Demand for beam time remains high

Industrial use is growing

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Undulators

( )β−= 1emitobs TT22γ

λλ ulight ≈

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Undulator radiation

⎟⎠

⎞⎜⎝

⎛++= 22

2

2 21

2θγ

γλλ Kn

u

Medi

um en

ergy

ring

s

( )un

Kλλ

21 2

21

* +=

λ∗ = 1.5 mm

λ∗ = 2‘500 mm

ESRF

, APS

K-e

dges

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Main R&D directions

o Short period (small gap) undulator developments

o Approaching diffraction limit: very small equilibrium emittance with large rings and damping wigglers

o Detector development complementing source improvements

o Linac based light sources development: ERLs

o Free electron lasers developments

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

In-vacuum undulators / s.c. undulators

Gapsdownto3 mm

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Cryo-cooled undulators

H. Kitamura, SPring-8

Zhentang Zhao PAC07, Albuquerque, New Mexico, June 25, 2007

Third Generation Light Sources in Operation

Zhentang Zhao PAC07, Albuquerque, New Mexico, June 25, 2007

Light SourceEnergy(GeV)

Circumference(m)

Emittance (nm.rad)

Current(mA) Straight Section Status

ESRF 6.0 844.4 3.7 200 32×6.3m Operational(1993)

APS 7.0 1104 3.0 100 40×6.7m Operational(1996)

SPring-8 8.0 1436 2.8 100 44×6.6m, 4×30m Operational(1997)

ALS 1.9 196.8 6.3 400 12×6.7m Operational(1993)

TLS 1.5 120 25 240 6×6m Operational(1993)

ELETTRA 2.0/2.4 259 7 300 12×6.1m Operational(1994)

PLS 2.5 280.56 10.3 200 12×6.8m Operational(1995)

LNLS 1.37 93.2 70 250 6×3m Operational(1997)

MAX-II 1.5 90 9.0 200 10×3.2m Operational(1997)

BESSY-II 1.7 240 6.1 200 8×5.7m, 8×4.9m Operational(1999)

Siberia-II 2.5 124 65 200 12×3m Operational(1999)

NewSUBARU 1.5 118.7 38 500 2×14m, 4×4m Operational(2000)

SLS 2.4-2.7 288 5 400 3×11.7m, 3×7m, 6×4m Operational(2001)

ANKA 2.5 110.4 50 200 4×5.6m, 4×2.2m Operational(2002)

CLS 2.9 170.88 18.1 500 12×5.2m Operational(2003)

SPEAR-3 3.0 234 12 500 2×7.6m,4×4.8m,12×3.1m Operational(2004)

SAGA-LS 1.4 75.6 7.5 300 8×2.93m Operational(2005)

Third Generation Light Sources in Operation

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Main R&D directions

o Short period (small gap) undulator developments

o Approaching diffraction limit: very small equilibrium emittance with large rings and damping wigglers

o Detector development complementing source improvements

o Linac based light sources development: ERLs

o Free electron lasers developments

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

The electron beam “emittance”:

Emittance = S x Ω

Angular divergence, Ω

Source area, S The brightness

depends on the geometry of the source, i.e., on the electron beam emittance

Ring equilibrium emittance

σ0

σ′0

to minimize the blow up due to multiple scattering in the absorber we can focus the beam

σ′ = σ′02 + σ′MS

2 σ′0 >> σ′MS

Theoretical Minimum Emittance lattice

Fmin = 112 15latt

32

0 Fθ ⋅⋅=x

qx J

ECε

Zhentang Zhao PAC07, Albuquerque, New Mexico, June 25, 2007

Third Generation Light Sources

1 2 3 4 5 6 7 8 9

1

10

100

MAX IISAGASAGA

Bessy IITSRF

ALS

CANDLE

PLSKazakhstan

TLS

NewSUBARU

LNLSSiberia II

ANKAIndus II

SESAME

CLS

ELETRRA

SLSSoleil

SPEAR3

ASP

ALBASSRF

DiamondNSLS IITPS

MAX IV

ESRF

PETRA III

APS

Operational Commissioning Construction Planned

Emitt

ance

(nm

.rad)

Energy (GeV)

SPring8

PEP-X

Zhentang Zhao PAC07, Albuquerque, New Mexico, June 25, 2007

New Synchrotron Radiation Facilities

Zhentang Zhao PAC07, Albuquerque, New Mexico, June 25, 2007

New Synchrotron Radiation Facilities

Zhentang Zhao PAC07, Albuquerque, New Mexico, June 25, 2007

New Synchrotron Radiation Facilities

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

FromPEP-II

toPEP-X

Use of damping wigglers as in PETRA III to reach 0.1 nm.rad

Zhentang Zhao PAC07, Albuquerque, New Mexico, June 25, 2007

1 2 3 4 5 6 7 8 9

100

200

300

400

500

600

Operational Commissioning Construction Planned

ELETTRA

SLSPLS

Bessy IITSRF

ALS

CLSIndus II

Kazakhstan

SPEAR3ASP,CANDLE

MAX IV

TPS

Soleil

ANKA

TLS Siberia IINewSUBARU

ALBA

SESAME

SAGA LS

LNLS MAX II

Diamond

SSRF

Circ

umfe

renc

e (m

)

Energy (GeV)

3 4 5 6 7 8 9

1000

1500

2000

25003000

PETRA III

SPring8

APS

ESRFNSLS II

Third Generation Light Sources

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

CERN’s 27 km ‘tunnel with a future’

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Top-up injection: key to stability

TOP-UP INJECTION

TIME

ELEC

TRO

N IN

TEN

SITY

also Trickle Charge cont. Injection at PEP-II, KEKB

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Top-up is key to the source stabilityConstant thermal load on:

• Beam line optics• Accelerator components (BPMs, vacuum chamber…)

Tunnel Temperature [0C] 25 ± 0.03

average Temperatures of the 5 Sectors

25.4

25.3

25.2

25.1

25.0

24.9

24.8

24.7

1 day

0.050average Temperatures of the 5 Sectors

σx

Beamsizes σx σy [µm]

σx

σy

1 day

Vertical emittance εy → 4 pm-rad; coupling εy/εx ~ 0.08%

Beam lifetime ~7h, not relevant! Injection every 1.5 min

1 μm

Diffraction limit @ 1 Å

Damping Rings beam emittances

30

ATFachieved

ILC

ATFDesign

SLC

CLIC DRdesign

CLIC 500 GeVCLIC

3 TeV SLS

NSLS IIscaled

0.001

0.010

0.100

1.000

10.0000.1 1 10 100

Horizontal Emittance (μrad-m)

Vert

ical

Em

ittan

ce (

μra

d-m

)

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

H. Ohkuma, JASRI/SPring-8, EPAC08

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Top up vs. top offWhich definition?

top off vb.

(tr., adv,) to finish or complete, esp. with some decisive action: he topped off the affair by committing suicide.

top up vb. (tr.,adv. ) Brit.

1. to raise the level of (a liquid, powder, etc.) in (a container), usually bringing it to the brim of the container: top up the sugar in those bowls.

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Protein structure

N. Ban et. al.

Part of a Ribosome

Diffraction pattern

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Spectacular growth of structural biology

35’000

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Nobel Prizes in Chemistry to Synchrotron Radiation Work in Protein Crystallography

1997 John E. WalkerStructure of F1-ATPase

2003 Roderick McKinnonStructure of Cellular Ion Channels

2006 Roger D. KronbergStructure of RNA polimerase

Transverse coherence

• High brightness gives coherence

• Wave optics methods for X-rays(all chapters in Born & Wolf)

• Holography

phase contrast imaging

The knee of a spider

J. Gobrecht, SLS-SAC Meeting,11 July 07

Lithographic Performance

MNE 06, Ekinci et al

20 nmHSQ

CALIXARENE

12.5 nm

EIPBN 06, Solak et al

period=35.3 nm (516 Gbit/in2 )

• Worldwide highest resolution in photon-based lithography

• Field size: up to 2x2 mm2 (Achromatic Talbot)

• High throughput: ~10’000x e-beam

• Quality, reproducibility: enabling industrial operation

EIPBN 07, Solak et al

CALIXARENE

Fundamentals:Stable, coherent sourceShort wavelength (13.5 nm)No proximity effect (electron mean free path <1 nm)

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Main R&D directions

o Approaching diffraction limit: very small equilibrium emittance with large rings and damping wigglers

o Short period (small gap) undulator developments

o Detector development complementing source improvements

o Linac based light sources development: ERLs

o Free electron lasers developments

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

X-ray phase contrast imagingusing a shearing interferometer based on microfabricated silicon diffraction gratings

Phase-object example:100µm and 200µm styrene beads

Tomographic phase reconstruction of a spider

Advantages:significantly enhanced contrast compared to conventional "absorption-mode" for light materials

High potential in medical diagnosis and research

C. David, T. Weitkamp

F. Pfeiffer et al., PRL 94, April 2005

User OfficeX-ray Radiography of a fish

conventional Absorption a(+ details c , e, g)

Phase contrast Microscopy b(+ details d, f, h)

(F.Pfeiffer)

User Office

Franz Pfeiffer Coherent X ray

phase contrastabsorption

17.5 keV,synchrotron results

Into the hospital ?

(C.David, F.Pfeiffer)

Franz Pfeiffer – Super-Resolution STXM

Lensless coherent Scanning Microscopy with hard X-rays

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Ultrafast X-ray science

X-ray Free Electron Lasers extend the ultrafast laser techniques to the X-ray domain

„Seeing“ structures evolving with time as phenomena take place

FEMTO: Slicing technique at synchrotrons

Similar technique to reach < 1 fs with XFELs

„If you want to understand function,study structure“

Francis Crick

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

harpo10-27

yocto10-24

milli10-3

micro10-6

nano10-9

pico10-12

femto10-15

atto10-18

zepto10-21

Ultrafast lasers

SynchrotronsLaser plasmas

XFEL’s

Current lasers:

X-ray sources:

Science:Acoustic phonons

Vibrations (Optical phonons) Chemistry and BiochemStrings,

CosmologyParticle Collisions Electron dynamics

Ultrafast Sources and Science

J. Hastings

Laser slicingPioneering ideas and experiments at ALS

Facilities at ALS, BESSYII, SLS

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Dynamics on atomic scale visible with ultra-short X-ray pulses

Phys. Rev. Lett. 99, 174801 (2007)

First optical experiment with atomic resolution:

Amplification and dampingof lattice vibrations

FEMTO

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Main R&D directions

o Approaching diffraction limit: very small equilibrium emittance with large rings and damping wigglers

o Short period (small gap) undulator developments

o Detector development complementing source improvements

o Linac based light sources development: ERLs

o Free electron lasers developments

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Energy Recovery Linac SchematicSingle pass: emittance and energy spread are determined by injector, can be much smaller than in storage ring

Ch. Sinclair, Cornell

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Main R&D directions

o Approaching diffraction limit: very small equilibrium emittance with large rings and damping wigglers

o Short period (small gap) undulator developments

o Detector development complementing source improvements

o Linac based light sources development: ERLs

o Free electron lasers developments

COHERENT EMISSION BY THE ELECTRONS

INCOHERENT EMISSION COHERENT EMISSION

Intensity ∝ N Intensity ∝ N 2

WAVELENGTH

MUCH HIGHER BRIGHTNESS CAN BE REACHED WHEN THE ELECTRONS COOPERATE

INCOHERENT EMISSION COHERENT EMISSION

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

From rings to linear accelerators

o The number of beamlines served simultaneously

o The stability of the rings based sources

o High average brightness

- Fewer beamlines

- Very short pulses, single shot measurements

- High peak brightness

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

European XFELDESY 2013

1 km

JapanSCSS – SPring8 2010

X-FEL facilities

USALCLS – SLAC 2009

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

1035

1025

1015

10 ps 100 fs 1fs

Slicing

ERLs

X-ray FELs atto…

2G rings

3G rings

Peak

Bri

ghtn

ess

Pulse duration

FELs and ERLs COMPLEMENT the Ring sources

H.-D. Nuhn, H. Winick After H.-D. Nuhn, H. Winick

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Structure determination of single molecules before the Coulomb explosion

H. Chapman(2007)

Peak brightness of the FELs

courtesy T. Shintake

X-Ray

~109 103 by e− quality, long undulators

106 by FEL gain

1 Å

photons per phase-space volume per band-width

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Main R&D directions

o Approaching diffraction limit: very small equilibrium emittance with large rings and damping wigglers

o Short period (small gap) undulator developments

o Detector development complementing source improvements

o Linac based light sources development: ERLs

o Free electron lasers developments

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Hybrid-Pixel Technology

Indium bump-bonding technology18um bumps

Si-sensor with pixelated pn-diode structure

CMOS chip technology,

Direct Detection of X-rays

Single Photon Counting

Frame rate ~ 1 kHz

X-rays

Spin-off company from PSIC. Brönnimann, et al

Cutting-edge 2D pixel detectors

Advanced detectors: collaboration with HEP detector groups

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Further reading

X-ray sources, ICFA Seminar, SNAL, October 2008, L. Rivkin, PSI & EPFL

Summary

Strong growth in ring based supply continues

Complementary laser-like X-ray sources for atomic

resolution studies: lots of learning to do

Linac based sources for ultra-fast X-ray science

Detector development is crucial

Sample damage: a problem looking for a solution